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Molecular Ferroelastic Induced by Mono-/Double-Protonation Strategy

Chinese Journal of Chemistry 2024年第15期42卷 1706-1712页

作者： Jia-Qi Luo Meng-Meng Lun Qiang-Qiang Jia zhi-jie wang Hai-Feng Lu Yi Zhang Da-Wei Fu Institute for Science and Applications of Molecular Ferroelectrics Key Laboratory of the Ministry of Education for Advanced Catalysis MaterialsZhejiang Normal UniversityJinhuaZhejiang 321004China Ordered Matter Science Research Center Jiangsu Key Laboratory for Science and Applications of Molecular FerroelectricsSoutheast UniversityNanjingJiangsu 211189China

Molecular ferroelastics with the natural features of mechanical flexibility and switchable spontaneous strain have attracted widespread attention in the scientific community due to their potential applications in tunable gratings,flexible memorizers,strain sensors,and intelligent ***,most designs of molecular ferroelastics remain in the stage of blind exploration,posing a challenge to achieve a functional ferroelastic more ***,we have successfully obtained a molecular ferroelastic,[Me_(2)NH(CH_(2))_(2)NH_(3)](ReO_(4))_(2)(Me_(2)NH(CH_(2))_(2)NH_(3)=N,N-dimethylethylenediammonium),under the guidance of the mono-/double-protonation ***_double-protonated[Me_(2)NH(CH_(2))_(2)NH_(3)](ReO_(4))_(2) undergoes a paraelastic-ferroelastic phase transition with the Aizu notation of 2/mFi at 322 ***,the theoretical calculation and experimental measurement simultaneously show that[Me_(2)NH(CH_(2))_(2)NH_(3)](ReO_(4))_(2) possesses good mechanical flexibility,because its elastic modulus(E)of 8.26 GPa and hardness(H)of 0.45 GPa are smaller than the average values of organic crystals(E of 12.05 GPa and H of 0.5 GPa),which makes it promising to apply in wearable pressure sensors,implantable medical sensors,high-precision tuners,*** work further enriches the molecular ferroelastic family and demonstrates that mono-/double-protonation is one of the effective molecular modification strategies for designing ferroelastics.

关键词： Molecular crystal Ferroelastic Mono-/double-protonation Mechanical flexibility Phase transition Crystal engineering Computational chemistry Molecular dynamics

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Beurling Type Theorem on the Hilbert Space Generated by a Positive Sequence

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Acta Mathematica Sinica,English Series 2019年第9期35卷 1511-1519页

作者： Chang Hui WU zhi jie wang Tao YU School of Mathematical Sciences Dalian University of Technology Dalian 116024 P. R. China Department of Mathematics Physics and Information Engineering Jiaxing University Jiaxing 314001 P. R. China

Let H^2(γ) be the Hilbert space over the bidisk D^2 generated by a positive sequence γ={γnm}n,m≥0. In this paper, we prove that the Beurling type theorem holds for the shift operator on H^2(γ) with γ={γnm}n,m≥0 satisfying certain series of inequalities. As a corollary, we give several applications to a class of classical analytic reproducing kernel Hilbert spaces over the bidisk D^2.

关键词： Beurling type theorem invariant subspace wandering subspace

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High Expression of ERCC1 Is a Poor Prognostic Factor in Chinese Patients with Non-small Cell Lung Cancer Receiving Cisplatin-based Therapy

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Chinese Journal of Cancer Research 2010年第4期22卷 296-302页

作者： Qing-zhi Guo jie wang Hua Bai Tong-tong An Meina Wu Jun Zhao Lu Yang Jian-chun Duan Yu-yan wang zhi-jie wang Key laboratory of Carcinogenesis and Translational Research （Ministry of Education） Department of Medical Oncology Peking University Cancer Hospital ＆ Institute Beijing 100142 China

Objective： to determine the role of excision repair cross-complementing group 1 gene （ERCC1） and ribonucleotide reductase subunit M1 （RRM1） expression in predicting response and survival in Chinese patients with advanced stage non-small cell lung cancer （NSCLC） treated with platinum-based chemotherapy. Methods： Formalin-fixed, paraffin-embedded biopsy tissues were retrospectively obtained from 160 advanced NSCLC patients. mRNA expression levels of ERCC1 and RRM1 were determined by real-time PCR. Results： Associations between mRNA expression level of ERCC1 and RRM1 and clinic-pathologic parameters were analyzed. One handred and forty two （88.75%） specimens were successfully amplified. mRNA expression level of ERCC1 and RRM1 was negatively associated with tumor response. ERCC1 expression levels ranged from 0.01 to 78.79 [median 0.63, mean 4.25 and standard deviation （SD） 9.23] and RRM1 from 0.00 to 30.91 （median 0.63, mean 0.87 and SD 3.36）. By adopting cut-off values according to median expression levels, we found that MST in patients with low ERCC1 mRNA levels was significantly longer in overall population than in patients with higher levels （18.63 versus 13.69 months, log-rank 5.73, P=0.017）, but we did not found the survival benefit of the patients with low expression level of RRM1. （19.07 versus 14.88, log-rank 1.66, P=0.197）. Further, in the multivariable Cox regression model analysis we found that low level of ERCC1 expression, the presence of weight loss and target therapy, were significant prognostic factors for survival. Conclusion： ERCC1 expression is associated with patients’ survival in Chinese advanced NSCLC patients treated with platinum-based regimen and may serve as a biomarker in predicting tumor response and clinical outcome in the patient population.

关键词： ERCC1 RRM1 NSCLC Platinum-based chemotherapy mRNA Realtime PCR

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Application of DC component to select fault branch in arc suppression coil grounding system

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Journal of Coal Science & Engineering(China) 2013年第3期19卷 396-401页

作者： zhi-jie wang Yan-Wen wang School of Mechanical Electrical and Information Engineering China University of Mining and Technology (Beijing) Beijing 100083 China

When single phase earth fault occurs in the arc suppression coil grounding system, the amplitude of the transient capacitance current is high and decays fast, but the attenuation of the transient inductance current is much slower. This paper analyses the DC component of fault branch, and has found it is much bigger than that of the normal branches in transient state. All the simulation results obtained from three compensation types, different fault time and different wave cycles show that the DC component of fault branch is much higher than that of those normal branches. These results verify the effectiveness of taking the DC component as the method of fault line selection in the arc suppression coil grounding system.

关键词： DC component arc suppression coil fault line selection transient state

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Enhanced memristor performance via coupling effect of oxygen vacancy and ferroelectric polarization

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Journal of Materials Science & Technology 2024年第4期171卷 139-146页

作者： zhi Yun Yue zhi Dong Zhang Zhan jie wang Shenyang National Laboratory for Materials Science Institute of Metal ResearchChinese Academy of SciencesShenyang 110016China School of Materials Science and Engineering University of Science and Technology of ChinaShenyang 110016China School of Materials Science and Engineering Shenyang University of TechnologyShenyang 110870China

As a new type of nonvolatile memory,the resistive memristor has broad application prospects in in-formation storage and neural computing based on its excellent resistive switching(RS)*** present,it is still a great challenge to improve both ferroelectric polarization and leakage current to achieve a high RS on/offratio of ferroelectric ***,epitaxial Pb(Zr_(0.40)Ti_(0.60))O_(3)(PZT)thin films with low content Ca doping were deposited on the Nb:SrTiO_(3)substrate to prepare PCZT/NSTO het-erostructures and their RS behaviors were *** research findings show that compared with pure PZT film,the ferroelectric polarization of 1-mol%-Ca-doped PZT film is slightly improved,while the leak-age current is increased by three orders of ***,the RS on/offratio reaches 2.5×10^(5),about three orders of magnitude higher than pure PZT *** theoretical analysis reveals that the RS behavior of PCZT/NSTO heterostructures is controlled by the PCZT/NSTO interfacial barrier and the space charge-limited current *** results demonstrate that the ferroelectricity and electricity of ferroelectric thin films can be improved simultaneously by doping low-content Ca ions to increase the RS performance,which provides a good reference for the development of high-performance ferroelectric memristor devices.

关键词： Ferroelectric memristor Ca-doped PZT Ferroelectric polarization Oxygen vacancies Resistive switching

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Effect of temperature on the demography of Galerucella birmanica （Coleoptera： Chrysomelidae）

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Insect Science 2008年第4期15卷 375-380页

作者： Fu-Shan Zheng Yu-Zhou Du zhi-jie wang Jia-Jun Xu Institute of Applied Entomology Yangzhou University Yangzhou Jiangsu Province Laiwu Vocational Technology Institute Laiwu Shandong Province China

Studies on the effect of temperature on the development of the water chestnut beetle, Galerucella birmanica Jacoby were carried out in the laboratory at seven different temperatures： 16 ℃, 19 ℃, 22 ℃, 25 ℃, 28 ℃, 31 ℃ and 34 ℃. The developmental time decreased with increase in temperature. The developmental time at 16 ℃, 19℃, 22 ℃, 25 ℃, 28 ℃, 31 ℃ and 34 ℃ was 96.60, 80.68, 58.96, 43.48, 35.03, 30.08 and 28.02 days for the period from egg hatching to adult emergence, respectively. The developmental threshold estimated for a generation by linear regression was 10.36℃. The fecundity per female at 22 ℃, 25 ℃, 28 ℃, 31 ℃ and 34 ℃ was 102.3, 134.5, 141.2, 130.1 and 116.2 eggs, respectively. Oviposition period ranged from 15.6 days at 22 ℃ to 8.6 days at 34 ℃. Hatchability of eggs was highest at 31 ℃ with 76.9% and lowest at 34 ℃ with 57.1%. The highest generation survival rate was 65.3% at 31 ℃, and the intrinsic rate of natural increase （rm） for G. birmanica was the highest at 34 ℃.

关键词： demography developmental threshold fecundity Galerucella birmanicaJacoby longevity survivorship temperature

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TIME-DOMAIN RESPONSES OF IMMERSING TUNNEL ELEMENT UNDER WAVE ACTIONS

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Journal of Hydrodynamics 2009年第6期21卷 739-749页

作者： CHEN zhi-jie wang Yong-xue wang Guo-yu HOU Yong State Key Laboratory of Coastal and Offshore Engineering Dalian University of Technology Dalian 116024 China CCCC-FHDI Engineering Co. Ltd Guangzhou 510230 China

The time domain responses of the tunnel element under wave actions during its immersion are investigated based on the linear wave diffraction theory. The integral equation is derived by using the time-domain Green function that satisfies the free water surface condition in the finite water depth, and is solved by the boundary element method. The motion equations of the tunnel element are solved by the fourth order Runge-Kutta method. A comparison between the computed and measured results reveals that the numerical model can effectively simulate the motion responses of the tunnel element and the cable tensions when the motions of the tunnel element are within some limit. Taking the tunnel element of 100 m in length, 15 m in width and 10 m in height as an example, the computational results of the motion responses of the tunnel element and the cable tensions in different immersing depths are obtained under different incident wave conditions.

关键词： Immersed tunnel time-domain response cable tension boundary element method

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CATIRI:An Efficient Method for Content-and-Text Based Image Retrieval

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Journal of Computer Science & Technology 2019年第2期34卷 287-304页

作者： Mengqi Zeng Bin Yao zhi-jie wang Yanyan Shen Feifei Li Jianfeng Zhang Hao Lin Minyi Guo Department of Computer Science and Engineering Shanghai Jiao Tong University Shanghai 200240 China School of Data and Computer Science Sun Yat-sen University Guangzhou 510006 China Guangdong Key Laboratory of Big Data Analysis and Processing Guangzhou 510006 China National Engineering Laboratory for Big Data Analysis and Applications Beijing 100871 China School of Computing University of Utah Salt Lake City 84112 U.S.A. Alibaba Group Hangzhou 311121 China

The combination of visual and textual information in image retrieval remarkably alleviates the semantic gap of traditional image retrieval methods,and thus it has attracted much attention *** retrieval based on such a combination is usually called the content-and-text based image retrieval(CTBIR).Nevertheless,existing studies in CTBIR mainly make efforts on improving the retrieval *** the best of our knowledge,little attention has been focused on how to enhance the retrieval ***,image data is widespread and expanding rapidly in our daily ***,it is important and interesting to investigate the retrieval *** this end,this paper presents an efficient image retrieval method named CATIRI(content-and-text based image retrieval using indexing).CATIRI follows a three-phase solution framework that develops a new indexing structure called *** MHIM-tree seamlessly integrates several elements including Manhattan Hashing,Inverted index,and *** use our MHIM-tree wisely in the query,we present a set of important metrics and reveal their inherent *** on them,we develop a top-k query algorithm for *** results based on benchmark image datasets demonstrate that CATIRI outperforms the competitors by an order of magnitude.

关键词： image retrieval text-and-visual feature indexing top-k

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Immediate Versus Delayed Treatment with EGFR Tyrosine Kinase Inhibitors after First-line Therapy in Advanced Non-small-cell Lung Cancer

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Chinese Journal of Cancer Research 2011年第2期23卷 112-117页

作者： zhi-jie wang Tong-tong An Tony Mok Lu Yang Hua Bai Jun Zhao Jian-chun Duan Mei-na Wu Yu-yan wang Ping-ping Li Hong Sun Ping Yang jie wang Key Laboratory of Carcinogenesis and Translational Research （Ministry of Education） Department of Thoracic Medical Oncology Department of Integrative Medicine Peking University School of Oncology Beijing Cancer Hospital ＆ Institute Beijing China Department of Clinical Oncology Chinese University of Hong Kong Hong Kong China Department of Oncology General Hospital of Navy Beijing China

Objective： To analyze the outcomes of patients who received TKI immediately after the first-line without progression as maintenance treatment （immediate group） vs. those received delayed treatment upon disease progression as second-line therapy （delayed group）. Methods： The study included 159 no-small-cell lung cancer （NSCLC） patients who received gefitinib or erlotinib as maintenance treatment in the immediate group （85 patients） or as second-line therapy in the delayed group （74 patients）. The primary end point was progression-free survival （PFS）. EGFR mutation status was detected using denaturing high-performance liquid chromatography （DHPLC）. Results： PFS was 17.3 and 16.4 months in the immediate and delayed groups, respectively （hazard ratio [HR], 0.99; 95% Confidence Interval [CI]： 0.69-1.42; P=0.947）. In a subgroup analysis that included only patients with EGFR mutation, however, PFS was significantly longer in the immediate group than in the delayed group （HR, 0.48; 95% CI： 0.27-0.85; P=0.012）. In patients with wild type EGFR, the risk for disease progression was comparable between the two groups （HR, 1.23; 95% CI： 0.61-2.51; P=0.564）. No significant difference was demonstrated between the immediate and delayed group in terms of the overall survival （OS）（26.1 months vs. 21.6 months, respectively; HR=0.53; 95% CI： 0.27 to 1.06; P=0.072）. There was also no difference in the incidence of adverse events between the two groups. Conclusions： EGFR TKI maintenance improves PFS in patients with EGFR mutation. Prospectively designed clinical studies that compare TKI immediate vs. delayed treatment after first-line chemotherapy upon disease progression are needed.

关键词： EGFR tyrosine kinase inhibitor Maintenance therapy Non-small-cell lung cancer

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NFT Security Matrix:Towards Modeling NFT Ecosystem Threat

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Computer Modeling in Engineering & Sciences 2024年第6期139卷 3255-3285页

作者： Peng Liao Chaoge Liu jie Yin zhi wang Xiang Cui Key Laboratory of Trustworthy Distributed Computing and Service Beijing University of Posts and TelecommunicationsBeijing100876China Zhongguancun Laboratory Beijing100094China Institute of Information Engineering Chinese Academy of SciencesBeijing100085China

Digital assets have boomed over the past few years with the emergence of Non-fungible Tokens(NFTs).To be specific,the total trading volume of digital assets reached an astounding$55.5 billion in ***,numerous security concerns have been raised by the rapid expansion of the NFT *** holders are exposed to a plethora of scams and traps,putting their digital assets at risk of being ***,academic research on NFT security is scarce,and the security issues have aroused rare *** this study,the NFT ecological process is comprehensively *** process falls into five different stages encompassing the entire lifecycle of ***,the security issues regarding the respective stage are elaborated and analyzed in depth.A matrix model is proposed as a novel contribution to the categorization of NFT security *** data are collected from social networks,the Ethereum blockchain,and NFT markets to substantiate our claims regarding the severity of security concerns in the NFT *** this comprehensive dataset,nine key NFT security issues are identified from the matrix model and then subjected to qualitative and quantitative *** study aims to shed light on the severity of NFT ecosystem security *** findings stress the need for increased attention and proactive measures to safeguard the NFT ecosystem.

关键词： Non-fungible token blockchain cyber security

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