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Rare Metals 2024年第10期43卷 5082-5094页

作者： Jing-Yu Zhou zhi-cheng han Shu Zhao Tao Yang Da-Zhou Yan Hai-Jun Yu Institute of Advanced Battery Materials and Devices College of Materials Science and EngineeringBeijing University of Technology Key Laboratory of Advanced Functional Materials Ministry of EducationBeijing University of Technology China ENFI Engineering Corporation National Engineering Research Center of Silicon-Based Materials Manufacturing Technology

The pursuit of highly active oxygen evolution reaction （OER） catalysts,especially those free of noble metals,is a focal point in fuel cell *** extensive density functional theory calculations,this study designed and evaluated the activity and stability of singleatom catalysts （SACs） composed of 3d,4d and 5d transition metals supported on tungsten-based MXene for OER *** highlighted the exceptional OER performance of Ni@W2CO2,Rh@W2CO2and Pt@W2CO2,displaying remarkably low overpotentials The catalytic activity of TM@W2CO2SACs exhibited a robust correlation with surface properties,particularly the d-band center index and surface work *** Ni@W2CO2,Rh@W2CO2and Pt@W2CO2emerged as promising candidates for OER and oxygen reduction reaction （ORR） bifunctional catalysis,while Pt@W2CO2and Rh@ W2CO2showed high potential for OER and hydrogen evolution reaction （HER） bifunctional catalysis The effectiveness of tungsten-based MXene as a substrate for non-noble-metal SACs marks a breakthrough in OER catalyst design,driving advancements towards sustainable energy solutions and addressing critical challenges in energy conversion and storage.

关键词： Density functional theory MXene Non-noble metal Oxygen evolution reaction Single-atom catalysts

Mixed Dead-time Effect Suppression Strategy for Modular Multilevel Converters

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CSEE Journal of Power and Energy Systems 2024年第3期10卷 1075-1084页

作者： zhi Geng Minxiao han School of Electrical and Electronic Engineering North China Electric Power UniversityBeijing 102206China IEEE

Dead time is necessary for the coupled power switches to prevent shoot-through,especially in the modular multilevel converters(MMCs)with a large number of power *** paper proposes a dead-time effect suppression strategy for MMCs with nearest level *** operational principles of MMCs are first *** to the operational features of MMCs,the method that removes a switching signal from the coupled switches and the reduced switching frequency voltage balancing algorithms(RSFVBAs)are mixed in the proposed *** the intervals that are furthest away from the zerocrossing points(ZCP)of arm currents,the single switching signal method can completely eliminate the dead-time effect(DTE).Alternatively,the DTE is suppressed by the RSFVBA in intervals that are close to the *** the combination of the two methods,the dependence of the DTE suppression method on currents is reduced and the influences of ZCP are also released without degrading the normal operation performance of ***,the output performance of MMCs is improved and the voltage stress on the arm inductor dramatically ***,the validation of the method is verified by the simulation results with the professional tool Matlab/Simulink.

关键词： Dead-time effect modular multilevel converters switching frequency voltage balancing algorithm

Prediction and Output Estimation of Pattern Moving in Non-Newtonian Mechanical Systems Based on Probability Density Evolution

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Computer Modeling in Engineering & Sciences 2024年第4期139卷 515-536页

作者： cheng han Zhengguang Xu School of Automation and Electrical Engineering University of Science and Technology BeijingBeijing100083China Key Laboratory of Knowledge Automation for Industrial Processes University of Science and Technology BeijingBeijing100083China

A prediction framework based on the evolution of pattern motion probability density is proposed for the output prediction and estimation problem of non-Newtonian mechanical systems,assuming that the system satisfies the generalized Lipschitz *** a complex nonlinear system primarily governed by statistical laws rather than Newtonian mechanics,the output of non-Newtonian mechanics systems is difficult to describe through deterministic variables such as state variables,which poses difficulties in predicting and estimating the system’s *** this article,the temporal variation of the system is described by constructing pattern category variables,which are non-deterministic *** pattern category variables have statistical attributes but not operational attributes,operational attributes are assigned to them by posterior probability density,and a method for analyzing their motion laws using probability density evolution is ***,a data-driven form of pattern motion probabilistic density evolution prediction method is designed by combining pseudo partial derivative(PPD),achieving prediction of the probability density satisfying the system’s output *** on this,the final prediction estimation of the system’s output value is realized by minimum variance unbiased ***,a corresponding PPD estimation algorithm is designed using an extended state observer(ESO)to estimate the parameters to be estimated in the proposed prediction *** effectiveness of the parameter estimation algorithm and prediction method is demonstrated through theoretical analysis,and the accuracy of the algorithm is verified by two numerical simulation examples.

关键词： Non-newtonian mechanical systems prediction and estimation pattern moving probability density evolution pseudo partial derivative

Clinical features and possible pathogenesis of multiple evanescent white dot syndrome with different retinal diseases and events:a narrative review

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International Journal of Ophthalmology(English edition) 2024年第3期17卷 583-595页

作者： Chun-Li Chen Yi-Zhe cheng zhi-han Zhang Ge Wang Xiao-Yan Peng Department of Ophthalmology Beijing Tongren HospitalCapital Medical UniversityBeijing 100730China Beijing Ophthalmology and Visual Science Key Laboratory Beijing 100730China State Key Laboratory of Ophthalmology Zhongshan Ophthalmic CenterSun Yat-sen UniversityGuangzhou 510600Guangdong ProvinceChina

●Multiple evanescent white dot syndrome(MEWDS)is a rare fundus disease,characterized by acute vision loss and visual field *** previous studies have explained the possible pathogenesis and clinical features of primary ***,as the number of reported cases increases,secondary MEWDS occurs in other related retinal diseases and injuries,exhibiting some special *** associated retinal diseases include multifocal choroiditis/punctate inner choroidopathy(MFC/PIC),acute zonal occult outer retinopathy,best vitelliform macular dystrophy,pseudoxanthoma elasticum,and ocular *** related retinal injury is laser photocoagulation,surgery,and *** primary MEWDS often have a self-limiting course,secondary MEWDS may require treatment in some cases,according to the severity of concomitant diseases and ***,MEWDS secondary to MFC/PIC that is prone to forming choroidal neovascularization and focal choroidal excavation,needs positive treatment with *** possible underlying pathogenesis of secondary MEWDS is the exposure of choroidal antigen after the disruption of Bruch’s *** MEWDS-related features in secondary MEWDS are still evanescent under most *** prognosis and treatment depend on the severity of *** studies propose that the etiology is associated with immune factors,including viral infection,inflammation in choroid and Bruch’s membrane,and antigen exposure caused by retinal and/or choroidal *** pathogenic studies should be conducted in the *** diagnosis for secondary MEWDS could benefit patients in aspects of management and prognosis.

关键词： multiple evanescent white dot syndrome punctate inner choroidopathy multifocal choroiditis secondary multiple evanescent white dot syndrome

Topology of charged AdS black hole in restricted phase space

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Chinese Physics C 2024年第9期48卷 291-299页

作者： han Wang Yun-zhi Du College of Mathematics and Statistics Shanxi Datong UniversityDatong 037009China Department of Physics Shanxi Datong UniversityDatong 037009China Institute of Theoretical Physics Shanxi Datong UniversityDatong 037009China

The local topological properties of black hole systems can be expressed through winding numbers as *** date,AdS black hole thermodynamics are often depicted by the dual parameters of(T,S),(P,V),(Φ,Q) in the extended phase space,while there have been several studies on the black hole thermodynamics in the restricted phase *** this paper,we analyze the topological properties of charged AdS black holes in the restricted phase space under the higher-dimension and higher-order curvature gravity *** results show that the topological number of the charged black hole in the same canonical ensembles is a constant and is independent of the concrete dual thermodynamical ***,the topological number in the grand canonical ensemble is different from that in the canonical ensemble for the same black hole ***,these results are independent of dimension d and highe st order k of the Lanczos-Lovelock densities.

关键词： topology phase transition black hole

An unexpected approach to enhance specific surface area and mesopore amount of polyaniline by Zn doping

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Rare Metals 2024年第9期43卷 4585-4594页

作者： zhi-Da Zhu Yu-Zhe han Xiao-Bi Jing School of Mechanical Engineering Yangzhou UniversityYangzhou 225127China School of Chemistry and Chemical Engineering Yangzhou UniversityYangzhou 225002China

Poly-p-anisidine could be easily fabricated via the oxidative polymerization reaction of p-anisidine using H_(2)O_(2)as the green *** was unexpectedly found that zinc doping could significantly improve the adsorption ability of the material versus heavy metals such as Pb,Cu,Pd,Ag and *** of nitrogen adsorption–desorption experiments demonstrated that Zn doping could enhance the specific surface area and mesopore amount of the prepared material,which might facilitate its absorption to *** work not only provides a novel material for the treatment of heavy metal-polluted water but also leads to a nice mesoporous catalyst support for environment protection and organic synthesis,*** Zn-doped poly-panisidine can be employed as the catalyst support to prepare Cu@PANI-OMe/Zn or Pd@PANI-OMe/Zn for the oxidative degradation reaction of phenol or Suzuki–Miyaura coupling reactions,*** discloses a new strategy for fabricating the mesoporous polyaniline materials with profound application potential.

关键词： Surfaces Porous materials Rare metal concentration Adsorption Catalysis

Wettability regulation from superhydrophilic to superhydrophobic via nanosecond laser ablation

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Science China(Technological Sciences) 2024年第6期67卷 1829-1841页

作者： CHEN zhi WU zhicheng ZhanG GuoJun LI DongHui han FengLin State Key Laboratory of Precision Manufacturing for Extreme Service Performance College of Mechanical and Electrical EngineeringCentral South UniversityChangsha410083China Guangdong Provincial Key Laboratory of Manufacturing Equipment Digitization Guangdong HUST Industrial Technology Research InstituteDongguan523808China China Harzone Industry Corp. Ltd.Wuhan430299China

Metal surfaces play a crucial role in numerous applications,from self-cleaning and anti-icing to anti-fogging and oil-water *** regulation of their wettability is essential to enhance their performance in these *** paper proposes a multi-state regulation method for metal surface wettability,leveraging nanosecond laser *** creating non-uniform microstructures on a metal surface,the contact area between the solid and liquid phases can be increased,resulting in the attainment of superhydrophilic properties(contact angle(CA),ranging from 4.6°to 8.5°).Conversely,the construction of uniform microstructures leads to a decreased solid-liquid contact area,thereby rendering the metal surface hydrophilic(CA=12.2°–53°).Furthermore,through heat treatment on a surface with uniform microstructures,organic matter adsorption can be promoted while simultaneously reducing surface *** process results in the metal surface acquiring hydrophobic properties(CA=92.1°–133.5°),facilitated by the“air cushion effect.”Building on the hydrophobic surface,stearic acid modification can further reduce surface energy,ultimately bestowing the metal surface with superhydrophobic properties(CA=150.1°–152.7°,and sliding angle=3.8°).Performance testing has validated the durability and self-cleaning effectiveness of the fabricated superhydrophobic surface while also highlighting the excellent anti-fog performance of the superhydrophilic *** findings strongly indicate the immense potential of these surfaces in various engineering applications.

关键词： nanosecond laser ablation surface wettability superhydrophobic superhydrophilic

Information manifold and fault detection of multi-agent systems

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Chinese Journal of Aeronautics 2024年第10期37卷 410-423页

作者： Ruotong QU Bin JIANG Yuehua cheng Xiaodong han College of Automation Engineering Nanjing University of Aeronautics and AstronauticsNanjing 210016China China Academy of Space Technology Beijing 100098China

With the increase of the number of agents in multi-agent systems and the rapid increase of the complexity of the overall structure of the system,the fault detection and diagnosis work has brought great *** have carried out considerable research work on fault detection and diagnosis of multi-agent systems,but there is no research on fault state estimation and diagnosis based on the information and state of the whole multi-agent *** on the global perspective of information geometry theory,this paper presents two new physical quantities of the information manifold of multi-agent systems,as Lagrangian and energy–momentum tensor,to express the state of the overall information of multi-agent systems,and to characterize the energy state and development trend of *** this paper,two new physical parameters are introduced into the research of multi-agent fault detection and diagnosis,and the fault state and trend of multi-agent system are evaluated from the global perspective,which provides more comprehensive theoretical support for designing more scientific and reasonable fault diagnosis and fault recovery *** of the application example confirms the competitive performance of the proposed method.

关键词： Multi-Agent Systems(MASs) Fault information manifold Lagrangian Fault detection Energy-momentum Tensor

Safety and efficacy of a programmed cell death 1 inhibitor combined with oxaliplatin plus S-1 in patients with Borrmann large type III and IV gastric cancers

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World Journal of Gastrointestinal Oncology 2024年第4期16卷 1281-1295页

作者： Zhe-han Bao Can Hu Yan-Qiang Zhang Peng-cheng Yu Yi Wang zhi-Yuan Xu Huan-Ying Fu Xiang-Dong cheng Department of Interventional Radiology Zhejiang Cancer HospitalHangzhou 310004Zhejiang ProvinceChina Department of Gastric Surgery Zhejiang Cancer HospitalHangzhou 310022Zhejiang ProvinceChina Department of Colonic Surgery Jinhua Central HospitalJinhua 321000Zhejiang ProvinceChina Department of Breast Surgery Lin’an People’s HospitalHangzhou 311300Zhejiang ProvinceChina

BACKGROUND Gastric cancer(GC)is the fifth most common and the fourth most lethal malignant tumour in the *** patients are already in the advanced stage when they are diagnosed,which also leads to poor overall *** effect of posto-perative adjuvant chemotherapy for advanced GC is unsatisfactory with a high rate of distant metastasis and local *** To investigate the safety and efficacy of a programmed cell death 1(PD-1)inhibitor combined with oxaliplatin and S-1(SOX)in the treatment of Borrmann large type III and IV *** A retrospective analysis(IRB-2022-371)was performed on 89 patients with Borrmann large type III and IV GCs who received neoadjuvant therapy(NAT)from January 2020 to December *** to the different neoadjuvant treatment regimens,the patients were divided into the SOX group(61 patients)and the PD-1+SOX(P-SOX)group(28 patients).RESULTS The pathological response(tumor regression grade 0/1)in the P-SOX group was significantly higher than that in the SOX group(42.86%vs 18.03%,P=0.013).The incidence of ypN0 in the P-SOX group was higher than that in the SOX group(39.29%vs 19.67%,P=0.05).The use of PD-1 inhibitors was an independent factor affecting tumor regression ***,the use of PD-1 did not increase postoperative complications or the adverse effects of *** A PD-1 inhibitor combined with SOX could significantly improve the rate of tumour regression during NAT for patients with Borrmann large type III and IV GCs.

关键词： Neoadjuvant therapy Immunotherapy Gastric cancer Borrmann type Tumor regression grade

Reactor field reconstruction from sparse and movable sensors using Voronoi tessellation-assisted convolutional neural networks

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Nuclear Science and Techniques 2024年第5期35卷 173-185页

作者： He-Lin Gong han Li Dunhui Xiao Sibo cheng Paris Elite Institute of Technology Shanghai Jiao Tong UniversityShanghai 200240China School of Mathematical Sciences Tongji UniversityShanghai 200092China Department of Computing Data Science InstituteImperial College LondonLondon SW72AZUK

The aging of operational reactors leads to increased mechanical vibrations in the reactor *** vibration of the incore sensors near their nominal locations is a new problem for neutronic field *** field-reconstruction methods fail to handle spatially moving *** this study,we propose a Voronoi tessellation technique in combination with convolutional neural networks to handle this *** from movable in-core sensors were projected onto the same global field structure using Voronoi tessellation,holding the magnitude and location information of the *** convolutional neural networks were used to learn maps from observations to the global *** proposed method reconstructed multi-physics fields(including fast flux,thermal flux,and power rate)using observations from a single field(such as thermal flux).Numerical tests based on the IAEA benchmark demonstrated the potential of the proposed method in practical engineering applications,particularly within an amplitude of 5 cm around the nominal locations,which led to average relative errors below 5% and 10% in the L_(2) and L_(∞)norms,respectively.

关键词： Voronoi tessellation Field reconstruction Nuclear reactors Reactor physics On-line monitoring