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Structural and functional design of geopolymer adsorbents:a review

Tungsten 2024年第1期6卷 48-76页

作者： Hai-Ze Jin chen-Xi Qiu Yan-Song Li Bao Liu Jun-Yi Liu Qiao chen Xue-Feng Lu Cui-Xia Li Qi-Kun Wang School of Materials Science and Engineering Lanzhou University of TechnologyLanzhou 730050China State Key Laboratory of Advanced Processing and Recycling of Non-Ferrous Metals Lanzhou 730050China Shenyang Nonferrous Metals Research Institute Co. LTDShenyang 110000China Automotive Engineering Research Institute Jiangsu UniversityZhenjiang 212013China School of Materials Science and Engineering Jingdezhen Ceramic UniversityJingdezhen 333403China

The water pollution derived from the discharge of heavy metals,antibiotics,dyes and surfactants wastewater,*** seriously affected human survival and ecological *** an efficient and low-cost physical wastewater treatment process,the adsorption is a continuous hot spot in related scientific research and *** are non-crystal or semi-crystalline materials with high-efficiency adsorption performance due to the alkali metal ions that balance the electronegative aluminosilicate skeleton can be efficiently replaced by other cations in the aqueous *** related studies of different application conditions,service objects and morphological differences of geopolymer adsorbents based on structure-function design have been in-depth exploration and *** review aims to summarize the research progres s of the structure-function design based on the geopolymerization mechanism and kinetics and service *** overview of service characteristics and progress of geopolymers in the wastewater treatment field(e.g.,dyes,heavy metals,radionuclides,surfactants,antibiotics,ammonium,phosphorus,nitrogen and CO_(2),etc.)are systematically *** the evolution and development of morphological differences and the relationship of structure-function design of geopolymer adsorbents were compared and ***,the challenge worth overcoming,the trends worth considering and perspectives worth developing are highlighted.

关键词： Geopolymer Wastewater Adsorption Structure-function design Application

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3名日本女子乒乓球世界冠军运动员的技战术分析

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首都体育学院学报 2019年第4期31卷 345-352页

作者：周世杰罗棽月刘超陈振江首都体育学院北京100191 北京体育大学北京100084 北京市通州区官园小学北京101100 中国乒乓球协会国家乒乓球队北京100061

运用文献资料法、录像观察法、三段指标分析法及数理统计法,对3名日本女子乒乓球运动员的技战术进行分析,为中国乒乓球女队运动员备战2020年东京奥运会提供参考。结果:伊藤美诚发球旋转强、速度快、落点变化多,第3板的衔接较快,具有一... 详细信息

运用文献资料法、录像观察法、三段指标分析法及数理统计法,对3名日本女子乒乓球运动员的技战术进行分析,为中国乒乓球女队运动员备战2020年东京奥运会提供参考。结果:伊藤美诚发球旋转强、速度快、落点变化多,第3板的衔接较快,具有一定的威胁,但是失误较多;接发球技术很全面,能够在比赛中灵活使用,但稳定性欠佳;相持中的正手拍和反手弹是其主要得分技术。石川佳纯技术全面,手感细腻,比赛经验丰富,但力量小,击球得分一般;发球变化较多,能给对手的接发球轮制造一定的难度,发球后的衔接比较流畅,击球较为合理,失误少;接发球以控制性技术为主,落点较为单一,威胁较小,第4板中防守技术使用较多;相持段中落点意识突出,衔接较快。平野美宇的技战术特点是击球速度快,上手果断,落点变化多;反手技术十分强势,但正手有明显弱点;发球轮中,逆旋球的威胁较大,第3板进攻意识较强,但稳定性欠佳;接发球技术较为全面,但因为主动进攻的意识不强,所以在接抢轮显得较为被动;相持段主动变线的意识较强,但是命中率不高。

关键词：日本女子乒乓球世界冠军技战术分析

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野大麦–内生真菌共生体作为生态草的潜力浅析

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草业科学 2021年第9期38卷 1715-1725页

作者：翟纡润陈振江魏学凯陈泰祥段廷玉李春杰兰州大学草地农业科技学院甘肃兰州730020

草地作为陆地生态系统的重要组成部分,草地生态环境与国家生态安全息息相关。我国的草地退化问题日益严重,草地面积和产草量正在逐年减少,不仅影响了经济发展,同时还引发了水土流失、荒漠化等多种环境问题。目前迫切需要具有抗逆性强、... 详细信息

草地作为陆地生态系统的重要组成部分,草地生态环境与国家生态安全息息相关。我国的草地退化问题日益严重,草地面积和产草量正在逐年减少,不仅影响了经济发展,同时还引发了水土流失、荒漠化等多种环境问题。目前迫切需要具有抗逆性强、适应性广等特点的优良生态草种,坚持自然恢复为主的方针,来改善草地退化现状,积极应对环境变化。野大麦(Hordeum brevisubulatum)广泛分布在我国盐碱化草甸上,其产量高,品质好,根系发达,抗旱耐寒、耐瘠薄、耐盐碱,内生真菌侵染后野大麦的抗性和适应性得到了进一步的提高。除放牧、刈割、青贮、加工草粉或调制干草外,在低湿地建立栽培草地或改良盐渍化土壤等方面颇有前途。本研究从野大麦优良特性、利用价值以及内生真菌对宿主野大麦生长、抗性和竞争力的影响3个方面进行综述,分析了野大麦–内生真菌作为生态草种的潜力,以期为野大麦–内生真菌共生体的深入研究和合理利用提供参考。

关键词：野大麦内生真菌生态草抗性改善环境栽培草地生态建设

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Target Detection Algorithm in Foggy Scenes Based on Dual Subnets

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Computers, Materials & Continua 2024年第2期78卷 1915-1931页

作者： Yuecheng Yu Liming Cai Anqi Ning Jinlong Shi Xudong chen Shixin Huang School of Computer Science Jiangsu University of Science and TechnologyZhenjiang212100China Information Department China Merchants Heavy IndustryNantong226116China

Under the influence of air humidity,dust,aerosols,etc.,in real scenes,haze presents an uneven *** this way,the image quality and contrast will *** this case,It is difficult to detect the target in the image by the universal detection ***,a dual subnet based on multi-task collaborative training(DSMCT)is proposed in this ***,in the training phase,the Gated Context Aggregation Network(GCANet)is used as the supervisory network of YOLOX to promote the extraction of clean information in foggy *** the test phase,only the YOLOX branch needs to be activated to ensure the detection speed of the ***,the deformable convolution module is used to improve GCANet to enhance the model’s ability to capture details of non-homogeneous ***,the Coordinate Attention mechanism is introduced into the Vision Transformer and the backbone network of YOLOX is *** this way,the feature extraction ability of the network for deep-level information can be *** experimental results on artificial fog data set FOG_VOC and real fog data set RTTS show that the map value of DSMCT reached 86.56%and 62.39%,respectively,which was 2.27%and 4.41%higher than the current most advanced detection *** DSMCT network has high practicality and effectiveness for target detection in real foggy scenes.

关键词： Target detection fog target detection YOLOX twin network multi-task learning

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Blocking the PD-1 signal transduction by occupying the phosphorylated ITSM recognition site of SHP-2

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Science China Life Sciences 2024年

作者： Wenjie Li Wenyi Mei Hewei Jiang Jie Wang Xiaoli Li Lina Quan Yanyan Diao Yanni Ma Sisi Fan Zhuwei Xie Mengdie Gong Huan Zhu Dewen Bi Feng Zhang Lei Ma Jian Zhang Yufeng Gao Aris Paschalidis Honghuang Lin Fangfang Liu Kangdong Liu Mingliang Ye zhenjiang Zhao Yajun Duan Zhuo chen Yufang Xu Weilie Xiao Shengce Tao Lili Zhu Honglin Li Innovation Center for AI and Drug Discovery East China Normal University Shanghai Key Laboratory of New Drug Design School of PharmacyEast China University of Science&Technology Shanghai Center for Systems Biomedicine Key Laboratory of Systems Biomedicine (Ministry of Education)Shanghai Jiao Tong University Lingang Laboratory Key Laboratory of Medicinal Chemistry for Natural Resource Ministry of EducationYunnan Characteristic Plant Extraction LaboratoryYunnan Provincial Center for Research&Development of Natural ProductsState Key Laboratory for Conservation and Utilization of Bio-Resources in YunnanSchool of Pharmacy and School of Chemical Science and TechnologyYunnan University CAS Key Laboratory of Separation Sciences for Analytical Chemistry National Chromatographic R&A CenterDalian Institute of Chemical PhysicsChinese Academy of Sciences Department of Cardiology The First Affiliated Hospital of USTCDivision of Life Sciences and MedicineUniversity of Science and Technology of China Department of Infectious Diseases The First Affiliated Hospital of Anhui Medical University Department of Medicine University of Massachusetts Chan Medical School Department of Pathophysiology School of Basic Medical SciencesAcademy of Medical ScienceCollege of MedicineZhengzhou University

Targeting the PD-1/PD-L1 axis with small-molecular inhibitors is a promising approach for immunotherapy. Here, we identify a natural pentacyclic triterpenoid, Pygenic Acid A(PA), as a PD-1 signaling inhibitor. PA exerts anti-tumor activity in hPD-1 knock-in C57BL/6 mice and enhances effector functions of T cells to promote immune responses by disrupting the PD-1 signaling transduction. Furthermore, we identify SHP-2 as the direct molecular target of PA for inhibiting the PD-1 signaling transduction. Subsequently, mechanistic studies suggest that PA binds to a new druggable site in the phosphorylated PD-1 ITSM recognition site of SHP-2, inhibiting the recruitment of SHP-2 by PD-1. Taken together, our findings demonstrate that PA has a potential application in cancer immunotherapy and occupying the phosphorylated ITSM recognition site of SHP-2 may serve as an alternative strategy to develop PD-1 signaling inhibitors. In addition, our success in target recognition provides a paradigm of target identification and confirmation for natural products.

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Controllable CPL response driven by achiral UV-photosensitive dichroic dye through cholesteric liquid crystals

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Science China Chemistry 2024年第4期67卷 1250-1255页

作者： Yihan chen Yang Li Hang Li Lulu Li Yiwu Quan Yixiang cheng State Key Laboratory of Analytical Chemistry for Life Science School of Chemistry and Chemical EngineeringNanjing UniversityNanjing 210023China Key Laboratory of High-Performance Polymer Material and Technology of Ministry of Education School of Chemistry and Chemical EngineeringNanjing UniversityNanjing 210023China School of Environmental and Chemical Engineering Jiangsu University of Science and TechnologyZhenjiang 212003China

Versatile stimuli-responsive circularly polarized luminescent(CPL)materials have potential applications in information storage,security encryption,and intelligent *** this study,the Z/E isomerization of ultraviolet(UV)-photosensitive achiralα-cyanostilbene derivative was used as an achiral dichroic dye(Switch)to drive the controllable CPL-active response in cholesteric liquid crystals(CLCs).Under irradiation by 365 nm UV light,the resulting CLCs-Z-Switch underwent a Z-to-E configuration isomerization as CLCs-E-Switch,accompanied by a decrease in its dichroic order parameter(SFvalue)from 0.15to *** the quantum yield(QY)of CLCs-E-Switch increased from 8.1%(CLCs-Z-Switch)to 16.8%,the corresponding glumvalues of CPL emission decreased from+0.55/-0.57 to+0.37/-0.39 due to a decrease in the order of helical arrangement of E-Switch in E7 *** study enables photosensitive CLCs-Switch to be applied for optical information storage devices.

关键词： circularly polarized luminescent photosensitive dichroic dye cholesteric liquid crystals chiral induction

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Analysis and Optimization of Transient Mode Switching Behavior for Power Split Hybrid Electric Vehicle with Clutch Collaboration

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Automotive Innovation 2024年第1期7卷 150-165页

作者： Dehua Shi Sheng Liu Yujie Shen Shaohua Wang Chaochun Yuan Long chen Automotive Engineering Research Institute Jiangsu UniversityZhenjiang 212013China Jiangsu Province Engineering Research Center of Electric Drive System and Intelligent Control for Alternative Vehicles Zhenjiang 212013China

The power split hybrid electric vehicle(HEV)adopts a power coupling configuration featuring dual planetary gearsets and multiple clutches,enabling diverse operational modes through clutch engagement and *** multi-clutch configuration usually involves the collaboration of two clutches during the transient mode switching process,thereby substantially elevating control *** study focuses on power split HEVs that integrate multi-clutch mechanisms and investigates how different clutch collaboration manners impact the characteristics of transient mode *** powertrain model for the power-split HEV is established utilizing matrix-based *** the formulation of clutch torque curves and clutch collaboration models,this research systematically explores the effects of clutch engagement timing and the duration of clutch slipping state on transient mode switching *** upon this analysis,an optimization problem for control parameters pertaining to the two collaborative clutches is *** simulated annealing algorithm is employed to optimize these control *** results demonstrate that the clutch collaboration manners have a great influence on the transient mode switching *** with the pre-calibrated benchmark and the optimal solution derived by the genetic algorithm,the maximal longitudinal jerk and clutch slipping work during the transient mode switching process is reduced obviously with the optimal control parameters derived by the simulated annealing *** study provides valuable insights for the dynamic coordinated control of the power-split HEVs featuring complex clutch collaboration mechanisms.

关键词： Power split hybrid electric vehicle Transient mode switching Clutch collaboration Simulated annealing Powertrain model

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Strong metal-support interaction between AuPd nanoparticles and oxygen-rich defect ZrO_(2) for enhanced catalytic 5-hydroxymethylfurfural oxidation

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Chinese Chemical Letters 2024年第2期35卷 507-511页

作者： Yunlei Zhang Yiran Liu Wen Guan Mengxue Cao Yao chen Pengwei Huo Institute of Green Chemistry and Chemical Technology School of Chemistry and Chemical EngineeringJiangsu UniversityZhenjiang 212013China School of the Environment and Safety Jiangsu UniversityZhenjiang 212013China

The unique properties of metal oxide surfaces,crystal surfaces and defects play vital roles in biomass upgrading *** this work,hierarchical porous bowl-shaped ZrO_(2)(HB-ZrO_(2))with mixed crystal phase was designed and employed as the support for loading AuPd bimetal with different proportions to synthesize AuPd/HB-ZrO_(2) *** effects of surface chemistry,oxygen defects,bimetal interaction and metal-support interaction of AuPd/HB-ZrO_(2) on catalytic performance for the selective oxidation of 5-hydroxymethylfurfural(HMF)to 2,5-furandicarboxylic acid(FDCA)were systematically *** Au 2 Pd1/HB-ZrO_(2) catalyst afforded a satisfactory FDCA yield of 99.9%from HMF oxidation using O_(2) as the oxidant in water,accompanied with an excellent FDCA productivity at 97.6 mmol g^(−1) h^(−1).This work offers fresh insights into rationally designing efficient catalysts with oxygen-rich defects for the catalytic upgrading of biomass platform chemicals.

关键词： 5-Hydroxymethylfurfural oxidation 2,5-Furandicarboxylic acid Oxygen-rich defect ZrO_(2) AuPd bimetal Bowl-shaped structure

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南四湖富营养化状况分析与评价

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当代化工研究 2023年第5期 46-49页

作者：王贤姜晓宇纪杰善孔舒陈振江济宁学院工程学院山东273155 济宁水文中心山东272019 济南市水文中心山东250013

本研究在对南四湖2021年1—12月南阳、独山、二级湖闸上、微山岛、韩庄闸5个监测站点浮游藻类和水环境质量监测的基础上,对其富营养化状况进行了分析与评价。结果表明,南四湖优势种群主要为绿藻门和硅藻门,全年藻细胞密度的波动范围在3.... 详细信息

本研究在对南四湖2021年1—12月南阳、独山、二级湖闸上、微山岛、韩庄闸5个监测站点浮游藻类和水环境质量监测的基础上,对其富营养化状况进行了分析与评价。结果表明,南四湖优势种群主要为绿藻门和硅藻门,全年藻细胞密度的波动范围在3.5~490×10^(4)个/L,未超过藻细胞浓度限值,全年没有发生水华事件。综合分析高锰酸盐指数、总磷、总氮、叶绿素a和透明度等指标,独山、二级湖闸上、韩庄闸闸上水质类别均为Ⅲ类,南阳站和微山岛站水质类别为Ⅳ类,主要污染物为总磷,超地表水Ⅲ类标准10.82和7.08倍。2021年南四湖营养化等级为轻度富营养。南四湖整体水域生态系统较稳定,水环境良好,本研究可为南四湖资源保护、南水北调东线工程建设及可持续发展提供依据。

关键词：南四湖富营养化浮游藻类水环境质量

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Multifunctional AlPO_(4)reconstructed LiMn_(2)O_(4)surface for electrochemical lithium extraction from brine

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Journal of Energy Chemistry 2024年第2期89卷 410-421,I0010页

作者： Jun Gu Linlin chen Xiaowei Li Guiling Luo Linjing Fan Yanhong Chao Haiyan Ji Wenshuai Zhu School of Materials Science and Engineering Jiangsu UniversityZhenjiang 212013JiangsuChina School of Chemistry and Chemical Engineering Jiangsu UniversityZhenjiang 212013JiangsuChina College of Science State Key Laboratory of Heavy Oil ProcessingChina University of Petroleum-BeijingBeijing 102249China School of the Environment and Safety Engineering Jiangsu UniversityZhenjiang 212013JiangsuChina

LiMn_(2)O_(4)(LMO)electrochemical lithium-ion pump has gained widespread attention due to its green,high efficiency,and low energy consumption in selectively extracting lithium from ***,collapse of crystal structure and loss of lithium extraction capacity caused by Mn dissolution loss limits its industrialized ***,a multifunctional coating was developed by depositing amorphous AlPO_(4)on the surface of LMO using sol-gel *** characterization and electrochemical performance test provided insights into the mechanism of Li^(+)embedment and de-embedment and revealed that multifunctional AlPO_(4)can reconstruct the physical and chemical state of LMO surface to improve the interface hydrophilicity,promote the transport of Li^(+),strengthen cycle ***,after 20 cycles,the capacity retention rate of 0.5AP-LMO reached 93.6%with only 0.147%Mn dissolution *** average Li^(+)release capacity of 0.5AP-LMO//Ag system in simulated brine is 28.77 mg/(g h),which is 90.4%higher than ***,even in the more complex Zabuye real brine,0.5AP-LMO//Ag can still maintain excellent lithium extraction *** results indicate that the 0.5AP-LMO//Ag lithium-ion pump shows promising potential as a Li^(+)selective extraction system.

关键词： LiMn_(2)O_(4) Multifunctional AlPO_(4)coating Li^(+)embedment and de-embedment mechanism Stability Hydrophilicity Various solution

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