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Controlling reversible complexation-mediated polymerization(RCMP)via deep eutectic solvents:fast kinetics,narrow molecular weight distribution and mechanistic insights

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Science China Chemistry 2024年第8期67卷 2728-2736页

作者： Xin Fu Zhen Lu Shen Li zheng-Hong luo Lin-Xi Hou Department of Materials-Oriented Chemical Engineering College of Chemical EngineeringFuzhou UniversityFuzhou 350116China Department of Chemical Engineering School of Chemistry and Chemical EngineeringState Key Laboratory of Metal Matrix CompositesShanghai Jiao Tong UniversityShanghai 200030China Chemical Engineering Zhicheng College of Fuzhou UniversityFuzhou 350116China Qingyuan Innovation Laboratory Quanzhou 362801China

The exploitation of new green polymerization avenues for the effective synthesis of polymers by reversible-deactivation radical polymerization plays a critical role in pursuing the development of polymeric *** this work,serials of deep eutectic solvents(DES)with intermolecular-hydrogen-bonding interaction were constructed as catalysts and medium for actuating reversible complexation-mediated polymerization(RCMP)for the first time,yielding methacrylate polymers with high monomer conversion and narrow dispersion molecular weight in both water and oil *** mechanism and elementary reaction of RCMP were explored deeply,revealing that the complexation of initiator with DES to generate radicals was a ratecontrolling step and intermolecular-hydrogen-bond was primary factor to influence polymerization ***,the insights of density functional theory calculations revealed that negative electrostatic potential ensured nucleophilic *** investigation demonstrated the considerable potential of DES for RCMP,which is anticipated for other polymerization applications as a novel medium mode.

关键词： deep eutectic solvent reversible complexation-mediated polymerization intermolecular hydrogen bonding density functional theory elementary reaction steps

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Solid-state non-volatile memories based on vdW heterostructure-based vertical-transport ferroelectric field-effect transistors

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Science China(Information Sciences) 2024年第6期67卷 198-206页

作者： Qiyu YANG zheng-Dong luo Fei XIAO Junpeng ZHANG Dawei ZHANG Dongxin TAN Xuetao GAN Yan LIU Zhufei CHU Yinshui XIA Genquan HAN Hangzhou Institute of Technology Xidian University State Key Discipline Laboratory of Wide Band Gap Semiconductor Technology School of MicroelectronicsXidian University School of Artificial Intelligence Xidian University School of Materials Science and Engineering University of New South Wales (UNSW) Sydney ARC Centre of Excellence in Future Low-Energy Electronics Technologies (FLEET) University of New South Wales (UNSW) Sydney Key Laboratory of Light Field Manipulation and Information Acquisition Ministry of Industry and Information Technologyand Shaanxi Key Laboratory of Optical Information TechnologySchool of Physical Science and TechnologyNorthwestern Polytechnical University Faculty of Electrical Engineering and Computer Science Ningbo University

Driven by the explosive development of data-centric computation applications, it is becoming urgent to develop in-memory computing devices that are beyond the von Neumann architecture with an arrangement of separated logic and memory components. The transistor-type solid-state non-volatile memories,such as ferroelectric field-effect transistors(Fe FETs), have long been regarded as a competitive candidate for future in-memory computing architectures. However, the density scaling towards high-density arrays would require advanced Fe FETs with reduced footprints, which remains a great challenge so far. Here, a vertical-transport(VT) Fe FET that flips the charge transport channel perpendicular to the substrate plane is proposed, in which a ferroelectric gate and a van der Waals(vd W) heterojunction channel are vertically integrated, effectively reducing the device footprints. The proposed VT-Fe FET shows not only the robust binary non-volatile memory states but also several key synaptic functionalities at the device level. An artificial neural network with supervised learning was simulated based on the device conductance switching properties,showing excellent classification accuracy for the MNIST handwritten digits. These findings suggest that the proposed VT-Fe FET could offer a new solution for future non-volatile memories as well as more advanced neuromorphic systems.

关键词： vdW heterostructure non-volatile memory vertical-transport transistor ferroelectric field-effect transistor memristive devices

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Effects of Helicobacter pylori and Moluodan on the Wnt/β-catenin signaling pathway in mice with precancerous gastric cancer lesions

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World Journal of Gastrointestinal Oncology 2024年第3期16卷 979-990页

作者： Yi-Mei Wang zheng-Wei luo Yu-Lin Shu Xiu Zhou Lin-Qing Wang Chun-Hong Liang Chao-Qun Wu Chang-Ping Li Department of Gastroenterology The Affiliated Hospital of Southwest Medical UniversityLuzhou 646000Sichuan ProvinceChina

BACKGROUND Helicobacter pylori(***)is the primary risk factor for gastric cancer(GC),the Wnt/β-Catenin signaling pathway is closely linked to *** has a high mortality rate and treatment cost,and there are no drugs to prevent the progression of gastric precancerous lesions to ***,it is necessary to find a novel drug that is inexpensive and preventive to against *** To explore the effects of *** and Moluodan on the Wnt/β-Catenin signaling pathway and precancerous lesions of GC(PLGC).METHODS Mice were divided into the control,N-methyl-N-nitrosourea(MNU),***+MNU,and Moluodan *** first created an *** infection model in the ***+MNU and Moluodan groups.A PLGC model was created in the remaining three groups except for the control *** was fed to mice in the Moloudan group ad *** general condition of mice were observed during the whole experiment *** tissues of mice were grossly and microscopically *** quantitative real-time PCR(qRT-PCR)and Western blotting analysis,the expression of relevant genes were *** Mice in the ***+MNU group showed the worst performance in general condition,gastric tissue visual and microscopic observation,followed by the MNU group,Moluodan group and the control ***-PCR and Western blotting analysis were used to detect the expression of relevant genes,the results showed that the ***+MNU group had the highest expression,followed by the MNU group,Moluodan group and the control *** *** can activate the Wnt/β-catenin signaling pathway,thereby facilitating the development and progression of *** suppressed the activation of the Wnt/β-catenin signaling pathway,thereby decreasing the progression of PLGC.

关键词： Helicobacter pylori Gastric cancer Wnt/β-catenin signaling pathway Moluodan

Application of Fusobacterium nucleatum as a biomarker in gastrointestinal malignancies

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World Journal of Gastrointestinal Oncology 2024年第6期16卷 2271-2283页

作者： Long-Chen Yu Ya-Ping Li Yue-Ming Xin Mai Mao Ya-Xin Pan Yi-Xuan Qu zheng-Dong luo Yi Zhang Xin Zhang Department of Clinical Laboratory Qilu Hospital of Shandong UniversityShandong Engineering Research Center of Biomarker and Artificial Intelligence ApplicationJinan 250012Shandong ProvinceChina

The morbidity and mortality of gastrointestinal(GI)malignancies are among the highest in the world,posing a serious threat to human *** of the insidious onset of the cancer,it is difficult for patients to be diagnosed at an early stage,and it rapidly progresses to an advanced stage,resulting in poor treatment and *** nucleatum(***)is a gram-negative,sporefree anaerobic bacterium that primarily colonizes the oral cavity and is implicated in the development of colorectal,esophageal,gastric,and pancreatic cancers via various intricate *** development in novel research suggests that *** may function as a biomarker in GI *** the abundance of *** in stool,saliva,and serum samples of patients may aid in the diagnosis,risk assessment,and prognosis monitoring of GI *** editorial systematically describes the biological roles and mechanisms of *** in GI malignancies focusing on the application of *** as a biomarker in the diagnosis and prognosis of GI malignancies to promote the clinical translation of *** and GI tumors-related research.

关键词： Gastrointestinal malignancies Fusobacterium nucleatum Biomarker Diagnosis Prognosis

Effects of Curcumin on Neuroinflammation and the Nrf2/HO-1 Pathway in Rat Brains Following Gas Explosion

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Biomedical and Environmental Sciences 2024年第8期37卷 943-947页

作者： Xinwen Dong Yaguang Su zheng luo Lyufei Deng Xiaofeng Han Yifang Liang Sanqiao Yao Weidong Wu Jia Cao Linqiang Tian Yichun Bai Wenjie Ren Health School of Public Health Xinxiang Medical UniversityXinxiang 453003HenanChina Toxicology Research Institute PLA Army Medical UniversityChongqing 400038China Institute of Trauma and Orthopaedics Xinxiang Medical UniversityXinxiang 453003HenanChina Institutes of Health Central Plains Xinxiang Medical UniversityXinxiang 453003HenanChina

Gas explosions,a major occupational hazard in China’s coal industry,endanger the lives and health of *** explosions cause a specific type of traumatic brain injury with complex mechanisms,leading to disability and death.A study by Zhao et *** magnetic resonance imaging on 49 gas explosion survivors revealed significant damage to brain regions like the hippocampus and cerebral cortex.

关键词： damage Nrf2 cerebral

Broadband light-active optoelectronic FeFET memory for in-sensor non-volatile logic

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Science China(Information Sciences) 2024年第9期67卷 346-347页

作者： Yong ZHANG Dongxin TAN Cizhe FANG zheng-Dong luo Qiyu YANG Qiao ZHANG Yu ZHANG Xuetao GAN Yan LIU Yue HAO Genquan HAN State Key Discipline Laboratory of Wide Band Gap Semiconductor Technology School of MicroelectronicsXidian University Hangzhou Institute of Technology Xidian University Key Laboratory of Light Field Manipulation and Information Acquisition Ministry of Industry and Information Technologyand Shaanxi Key Laboratory of Optical Information Technology School of Physical Science and TechnologyNorthwestern Polytechnical University

Machine vision has become crucial in the modern intelligence era, especially in rapidly developing applications such as autonomous vehicles and robotic visual sensors [1].With the ever-increasing requirements of visual recognition,tremendous amounts of data are captured by sensors and must be processed and stored [2].

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冲击荷载下节段拼装梁的响应与破坏特征研究

中国公路学报 2024年第5期37卷 188-200页

作者：王银辉石宝斌陈闯罗征浙江大学建筑工程学院浙江杭州310000 浙大宁波理工学院土木建筑工程学院浙江宁波315100

由于节段拼装梁在接缝处混凝土和钢筋均不连续,导致其剪切破坏机制更加突出,冲击荷载作用会进一步加剧其破坏向更具局部特征的剪切破坏演变。为了解冲击荷载下节段拼装梁的响应与破坏特征,开展了试验梁落锤冲击试验,并结合LS-DYNA数值... 详细信息

由于节段拼装梁在接缝处混凝土和钢筋均不连续,导致其剪切破坏机制更加突出,冲击荷载作用会进一步加剧其破坏向更具局部特征的剪切破坏演变。为了解冲击荷载下节段拼装梁的响应与破坏特征,开展了试验梁落锤冲击试验,并结合LS-DYNA数值模拟分析,得到冲击荷载作用下梁的裂缝发展、破坏过程、形态等破坏特征,获得梁体变形、支座反力、内力分布等动力响应,揭示了节段长度、冲击能量、冲击作用位置等因素对节段拼装梁的动力响应与破坏特征的影响规律。结果表明:冲击荷载作用下节段拼装梁的局部剪切破坏特征突出,损伤和破坏位置集中于冲击作用点所在节段及接缝,典型破坏形式有斜截面破坏和接缝截面直剪破坏2种,冲击作用点与接缝的相对位置对破坏形式影响显著;混凝土和预应力筋的变形是冲击能量耗散的主要原因,普通钢筋耗能贡献可以忽略;梁体变形在接缝位置呈折线状,位移响应时间比整体梁更长,残余变形小;冲击作用点附近截面剪力峰值达到冲击力峰值的40%左右,较大剪力是导致节段拼装梁在局部形成斜截面破坏和直剪破坏的主要原因。

关键词：桥梁工程冲击破坏特征落锤冲击试验节段预制拼装梁数值模拟

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基于机器学习的珠三角秋季臭氧浓度预测

环境科学 2024年第1期45卷 1-7页

作者：陈镇刘润罗征薛鑫汪瑶赵志军暨南大学环境与气候研究院广州511443 粤港澳环境质量协同创新联合实验室广州511443 复旦大学信息与工程学院上海200438

基于2015~2022年珠三角地区的臭氧(O_(3))日最大8 h浓度平均值[MDA8-O_(3),ρ(O_(3)-8h)]的观测数据和气象再分析数据,运用支持向量回归(SVR)、随机森林(RF)、多层感知机(MLP)和轻量级梯度提升机(LG)这4种机器学习方法,建立MDA8-O_(3)... 详细信息

基于2015~2022年珠三角地区的臭氧(O_(3))日最大8 h浓度平均值[MDA8-O_(3),ρ(O_(3)-8h)]的观测数据和气象再分析数据,运用支持向量回归(SVR)、随机森林(RF)、多层感知机(MLP)和轻量级梯度提升机(LG)这4种机器学习方法,建立MDA8-O_(3)预测模型.结果表明,对于全年MDA8-O_(3)预测而言,SVR模型的效果最好,决定系数(R^(2))达0.86,均方根误差(RMSE)和平均绝对误差(MAE)分别为16.3μg·m^(-3)和12.3μg·m^(-3);对于秋季MDA8-O_(3)预测而言,SVR模型的效果依然略优于LG和MLP,其R2、RMSE和MAE分别为0.88、19.8μg·m^(-3)和16.1μg·m^(-3),RF模型在秋季的预测效果最差.采用全年数据构建的模型对秋季MDA8-O_(3)的预测效果比仅采用秋季数据构建的模型效果好,R2相差0.08~0.14.

关键词：珠三角(PRD) 臭氧(O_(3)) 日最大8 h浓度平均值(MDA8-O_(3)) 机器学习预测

地方高校商务英语专业校企合作困局与出路——基于组织间关系视角

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鄂州大学学报 2024年第1期31卷 52-54页

作者：骆铮平顶山学院外国语学院河南平顶山467000

校企合作是地方高校商务英语专业提高人才培养质量的重要手段,组织间关系视角能够解释校企双方合作的基本逻辑。当前地方高校商务英语专业的校企合作面临不稳定性联结、不信任性联结与不确定性联结的困局。因此,双方合作的出路应以政策... 详细信息

校企合作是地方高校商务英语专业提高人才培养质量的重要手段,组织间关系视角能够解释校企双方合作的基本逻辑。当前地方高校商务英语专业的校企合作面临不稳定性联结、不信任性联结与不确定性联结的困局。因此,双方合作的出路应以政策支持为依托,关注交换资源,实现均衡发展。

关键词：地方高校商务英语专业校企合作组织间关系