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A novel strategy of tannery sludge disposal–converting into biochar and reusing for Cr(Ⅵ)removal from tannery wastewater

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Journal of Environmental Sciences 2024年第4期138卷 637-649页

作者： Zhiwei Li Di Yu Xingdong wang Xuejiao Liu zhen Xu Yin wang CAS Key Laboratory of Urban Pollutant Conversion Institute of Urban EnvironmentChinese Academy of SciencesXiamen 361021China University of Chinese Academy of Sciences Beijing 100049China Zhejiang Key Laboratory of Urban Environmental Processes and Pollution Control CAS Haixi Industrial Technology Innovation Center in BeilunNingbo 315830China Key Laboratory of Urban Environment and Health Ningbo Observatio

Tannery sludge with high chromium content has been identified as hazardous solid waste due to its potential toxic *** safety disposal and valorization of the tannery sludge remains a *** this study,the chromium stabilization mechanism was systematically investigated during chromium-rich tannery sludge was converted to biochar and the removal performance of the sludge biochar(SBC)for Cr(Ⅵ)from tannery wastewater was also *** results showed that increase in pyrolysis temperature was conductive to the stabilization of Cr and significant reduction of the proportion of Cr(Ⅵ)in *** was confirmed that the stabilization of chromium mainly was attributed to the embedding of chromium in the C matrix and the transformation of the chromium-containing substances from the amorphous Cr(OH)_(3)to the crystalline state,such as(FeMg)Cr_(2)O_(5).The biochar presented high adsorption capacity of Cr(Ⅵ)at low pH and the maximal theoretical adsorption capacity of SBC produced at 800°C can reach 352 mg Cr(Ⅵ)/g,the process of which can be well expressed by Langmuir adsorption isotherm and pseudo second order *** electrostatic effect and reduction reaction were dominantly responsible for the Cr(Ⅵ)adsorption by ***,this study provided a novel strategy for the harmless disposal and resource utilization for the solid waste containing chromium in leather industry.

关键词： Chromium-rich tannery sludge Pyrolysis Biochar Stabilizationmechanisms Cr(Ⅵ)adsorption

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Track-Pattern-Based Characteristics of Extratropical Transitioning Tropical Cyclones in the Western North Pacific

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Advances in Atmospheric Sciences 2024年第6期41卷 1251-1263页

作者： Hong huaNG Dan WU Yuan wang zhen wang Yu LIU College of Meteorology and Oceanography National University of Defense TechnologyChangsha 410000China No.31631 Army of PLA Huizhou 516000China School of Atmospheric Sciences and Key Laboratory of Mesoscale Severe Weather/Ministry of Education Nanjing 210023China No.93721 Army of PLA Shuozhou 038300China

Based on the Regional Specialized Meteorological Center(RSMC)Tokyo-Typhoon Center best-track data and the NCEP-NCAR reanalysis dataset,extratropical transitioning(ET)tropical cyclones(ETCs)over the western North Pacific(WNP)during 1951–2021 are classified into six clusters using the fuzzy c-means clustering method(FCM)according to their track *** characteristics of the six hard-clustered ETCs with the highest membership coefficient are *** tropical cyclones(TCs)that were assigned to clusters C2,C5,and C6 made landfall over eastern Asian countries,which severely threatened these *** landfalling TCs,93.2%completed their ET after landfall,whereas 39.8%of ETCs completed their transition within one *** frequency of ETCs over the WNP has decreased in the past four decades,wherein cluster C5 demonstrated a significant decrease on both interannual and interdecadal timescales with the expansion and intensification of the western Pacific subtropical high(WPSH).This large-scale circulation pattern is favorable for C2 and causes it to become the dominant track pattern,owning to it containing the largest number of intensifying ETCs among the six clusters,a number that has increased insignificantly over the past four *** surface roughness variation and three-dimensional background circulation led to C5 containing the maximum number of landfalling TCs and a minimum number of intensifying *** results will facilitate a better understanding of the spatiotemporal distributions of ET events and associated environment background fields,which will benefit the effective monitoring of these events over the WNP.

关键词： Western North Pacific tropical cyclone extratropical transition fuzzy c-means clustering method

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Tongxinluo Activates PI3K/AKT Signaling Pathway to Inhibit Endothelial Mesenchymal Transition and Attenuate Myocardial Fibrosis after Ischemia-Reperfusion in Mice

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Chinese Journal of Integrative Medicine 2024年第7期30卷 608-615页

作者： WEI Ya-ru HOU Yun-long YIN Yu-jie LI zhen LIU Yi HAN Ning-xin wang Zi-xuan LIU Lu wang Xiao-qi HAO Yuan-jie MA Kun GU Jiao-jiao JIA zhen-hua Graduate School Hebei University of Chinese MedicineShijiazhuang050090China Shijiazhuang Yiling Pharmaceutical New Drug Evaluation Center Shijiazhuang050035China Hebei Institute of Integrated Traditional and Western Medicine Shijiazhuang050035China National Key Laboratory for Innovation and Transformation of Luobing Theory Shijiazhuang050035China Department of Cardiology Hebei Yiling HospitalShijiazhuang050091China Graduate School Hebei Medical UniversityShijiazhuang050017China

Objective To investigate the potential role of Tongxinluo(TXL)in attenuating myocardial fibrosis after myocardial ischemia-reperfusion injury(MIRI)in *** A MIRI mouse model was established by left anterior descending coronary artery ligation for 45 *** to a random number table,66 mice were randomly divided into 6 groups(n=11 per group):the sham group,the model group,the LY-294002 group,the TXL group,the TXL+LY-294002 group and the benazepril(BNPL)*** day after modeling,TXL and BNPL were administered by *** injection of LY-294002 was performed twice a week for 4 consecutive *** was used to measure cardiac function in *** staining was used to evaluate the degree of myocardial fibrosis in *** and quantitative analysis of endothelial mesenchymal transition(EndMT)after MIRI was performed by immunohistochemistry,immunofluorescence staining and flow cytometry,*** protein expressions of platelet endothelial cell adhesion molecule-1(CD31),α-smoth muscle actin(α-SMA),phosphatidylinositol-3-kinase(PI3K)and phospho protein kinase B(p-AKT)were assessed using Western *** TXL improved cardiac function in MIRI mice,reduced the degree of myocardial fibrosis,increased the expression of CD31 and inhibited the expression ofα-SMA,thus inhibited the occurrence of EndMT(P0.05).In addition,the use of the PI3K/AKT pathway-specific inhibitor LY-294002 to block this pathway and combination with TXL intervention,eliminated the protective effect of TXL,further supporting the protective effect of *** TXL activated the PI3K/AKT signaling pathway to inhibit EndMT and attenuated myocardial fibrosis after MIRI in mice.

关键词： myocardial fibrosis endothelial mesenchymal transition myocardial ischemia-reperfusion injury phosphatidylinositol-3-kinase/protein kinase B(PI3K/AKT)pathway

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Effect of Cyclic Annealing on Microstructure and Mechanical Properties of Medium Carbon Steel

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Journal of Iron and Steel Research(International) 2016年第2期23卷 145-150页

作者： Zhi-qing LÜ Hui-fang ZHANG Qing MENG zhen-hua wang Wan-tang FU College of Mechanical Engineering Yanshan UniversityQinhuangdao 066004HebeiChina State Key Laboratory of Metastable Material Science and Technology Yanshan UniversityQinhuangdao 066004HebeiChina

The microstructure and mechanical properties of medium carbon steel after cyclic heat treatment were in- vestigated. The effects of cyclic numbers and long time annealing on the microstructure and mechanical properties of the experimental steel were compared. A short duration （5 min） holding at 1023 K （above A1 temperature） and a short-duration （3 min） holding at 893 K are adopted in each cyclic heat treatment. The spheroidization is accelerated during cyclic heat treatment, and the spheroidizing ratio grows with cyclic numbers. After 12-cycle heat treatments, there are few incompletely spheroidized regions in the specimens, and cementite lamellae mostly change into cement- ite particles. The morphological character of cementite for 12 cycles is similar to that undergoing annealing for 10 h at 973 K. The strength of the experimental steel after 5-cycle heat treatment is the lowest in the following cyclic heat treatment, but it is still higher than that of specimens with subcritical annealing over a long period （10 h）. After 12- cycle heat treatment, the strength of the experimental steel is close to that of the normalized steel, and the plasticity is the best in all heat treated specimens.

关键词： rapid spheroidizing mechanical property cyclic annealing cementite medium carbon steel

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Phase and CCT Diagram of an N-Containing 8%Cr Roller Steel

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Journal of Harbin Institute of Technology(New Series) 2013年第6期20卷 112-117页

作者： Shu-hua Sun Bo wang zhen-hua wang Yang Gao Ming-Wei Guo Wan-Tang Fu State Key Laboratory of Metastable Materials Science and Technology Yanshan University College of Sciences Yanshan University Key Laboratory of Advanced Forging & Stamping Technology and Science (Yanshan University) Ministry of Education of China China First Heavy Industries

The pseudo-equilibrium phase diagram and continuous cooling transformation diagram of an N-containing 8% Cr roller steel were investigated by using thermodynamic calculation,differential scanning calorimetry, X-ray diffraction, expansion method, and so on. Under equilibrium conditions, the main carbonitrides are MX,M7C3,and M23C6types. The measured Ac1,Ac3,start temperature of martensitic transformation,and M7C3transformation temperatures are 811,855,324,and 1100 ℃,respectively. Bainite appears at cooling rates ranging from 0. 5 to 5 ℃ / s and ferrite forms at grain boundaries at a cooling rate lower than 0. 5 ℃ / s. Finally,the effects of adding N and lowering the C content on workability and mechanical properties of common 8%Cr steel were discussed.

关键词： high Cr roller steel phase diagram continuous cooling transformation N alloying

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Impact of sourdough fermentation on nutrient transformations in cereal-based foods:Mechanisms,practical applications,and health implications

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Grain & Oil Science and Technology 2024年第2期7卷 124-132页

作者： zhen wang Luyang wang State Key Laboratory of Crop Stress Adaptation and Improvement College of AgricultureHenan UniversityKaifeng 475004China

Sourdough is often considered a healthy choice and quality improver for use in cereal production due to its unique microbial composition and fermentation *** sourdough fermentation of cereals,biotransformation of nutrients occurs,resulting in notable changes to proteins,carbohydrates,fats,vitamins,and *** nutrient undergoes specific transformations,providing various advantages for human *** undergo hydrolysis to produce small molecular weight peptides and amino acids that are more easily digested and absorbed by the human *** break down to improve the digestibility and absorption of cereals and lower the glycemic *** acids experience oxidation to produce new substances with health ***,the application of sourdough fermentation can enhance the texture,flavor,and nutritional value of cereal foods while also extending their shelf life and improving food *** conclusion,sourdough fermentation has a broad range of applications in cereal food *** research is encouraged to investigate the mechanisms and processes of sourdough fermentation to develop even more nutritious,healthy,and flavorful cereal-based foods.

关键词： Sourdough fermentation Lactic acid bacteria Proteolysis Starch hydrolysis Low-GI Nutrients

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Progress and challenges of electrolyte modulation in aqueous zinc-ion batteries

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Rare Metals 2024年第7期43卷 2940-2967页

作者： Qi-Hang Yang Lu-Fei wang Xiao-Yu wang Meng-Meng zhen Tianjin Key Laboratory of Clean Energy and Pollution Control School of Energy and Environmental EngineeringHebei University of Technology

As a new type of green battery system,aqueous zinc-ion batteries（AZIBs） have gradually become a research hotspot due to their low cost,high safety,excellent stability,high theoretical capacity(820 mAh·g-1) of zinc anode,and low redox potential(-0.76 V *** hydrogen electrode（SHE）).AZIBs have been expected to be an alternative to lithium-ion batteries for large-scale commercial energy storage ***,they are facing thorny issues such as degradation of cycling performance,zinc dendrites,and side *** the same time,these problems cause short cycling life of batteries,thus severely limiting their commercial *** recent years,many more researches have been conducted on the modification of anode and cathode materials of AZIBs,but there is a lack of in-depth discussion on the characteristics and mechanism of electrolyte *** this review,we will make a systematic summary of the current problems with two electrodes in AZIBs,as well as the types and functions of electrolyte ***,we further systematically describe the modulation mechanism of electrolyte additives in the performance of the cathode and *** prospects and development directions of additive modulation strategies for AZIBs electrolytes are prospected.

关键词： Electrolyte additives Aqueous zinc-ion batteries Zinc anode protection Cathode chemistry

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Performance improvements in complementary metal oxide semiconductor devices and circuits based on fin field-effect transistors using 3-nm ferroelectric Hf0.5Zr0.5O2

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Rare Metals 2024年第7期43卷 3242-3249页

作者： Zhao-Hao Zhang Yan-Na Luo Gao-Bo Xu Jia-Xin Yao zhen-hua Wu Hong-Bin Zhao Qing-Zhu Zhang hua-Xiang Yin Jun Luo Wen-Wu wang Hai-Ling Tu Integrated Circuit Advanced R&D Center Institute of Microelectronics of Chinese Academy of Sciences School of Integrated Circuits University of Chinese Academy of Sciences State Key Laboratory of Advanced Materials for Smart Sensing General Research Institute for Nonferrous Metals

In this work,a conventional HfO2gate dielectric layer is replaced with a 3-nm ferroelectric（Fe） HZO layer in the gate stacks of advanced fin field-effect transistors（FinFETs）.Fe-induced characteristics,e.g.,negative drain induced barrier lowering（N-DIBL） and negative differential resistance（NDR）,are clearly observed for both p-and n-type HZO-based *** characteristics are attributed to the enhanced ferroelectricity of the 3-nm hafnium zirconium oxide（HZO） film,caused by Al doping from the TiAlC capping *** mechanism is verified for capacitors with structures similar to the *** to the enhanced ferroelectricity and N-DIBL phenomenon,the drain current(IDS)of the HZO-FinFETs is greater than that of HfO2-FinFETs and obtained at a lower operating ***,circuits based on HZO-FinFET achieve higher performance than those based on HfO2-FinFET at a low voltage drain(VDD),which indicates the application feasibility of the HZO-FinFETs in the ultralow power integrated circuits.

关键词： FinFET Ferroelectric Hafnium zirconium oxide Subthreshold swing Low power

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Sputtered MoN nanolayer as a multifunctional polysulfide catalyst for high-performance lithium–sulfur batteries

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eScience 2022年第3期2卷 329-338页

作者： Xin-Yang Yue Jing Zhang Jian Bao Yi-Fan Bai Xun-Lu Li Si-Yu Yang zheng-Wen Fu zhen-hua wang Yong-Ning Zhou Department of Materials Science Fudan UniversityShanghai200433China Beijing Key Laboratory for Chemical Power Source and Green Catalysis School of Chemistry and Chemical EngineeringBeijing Institute of TechnologyBeijing100081China Beijing Key Laboratory of Green Chemical Reaction Engineering and Technology Department of Chemical EngineeringTsinghua UniversityBeijing100084China Department of Chemistry Fudan UniversityShanghai200433China

Two major obstacles for the practical application of lithium–sulfur batteries are sluggish redox kinetics and the shuttle effect of lithium polysulfides(LiPSs).Herein,MoN nanolayer-decorated multilayer graphene is fabricated via magnetron sputtering then serves as a multifunctional interlayer in Li–S batteries to suppress the shuttle effect and enhance redox *** is revealed that after the initial discharge process,the MoN layers break up into independent microreaction units consisting of MoN bodies and MoS_(2) edges,forming a heterogeneous composite catalyst in *** MoN bodies not only have high sulfur affinity to trap LiPSs but also enhance their redox *** the same time,the MoS_(2) edge weakens the mobility of LiPSs via the anchoring *** a result,Li–S cells using the interlayer present superior cycling stability under a high sulfur loading of 4.8 mg cm^(-2).This work may open a new avenue for developing high-performance Li–S batteries.

关键词： Li–S batteries Polysulfide Barrier interlayer MoN Magnetron sputtering

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Optimal Model Average Prediction in Orthogonal Kriging Models

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Journal of Systems Science & Complexity 2024年第3期37卷 1080-1099页

作者： wang Jun HE Jiabei LIANG hua LI Xinmin School of Mathematics and Statistics Qingdao UniversityQingdao 266071China Department of Statistics George Washington UniversityWashington DC 20052USA

The main objective of this paper is to consider model averaging methods for kriging *** paper proposes a Mallows model averaging procedure for the orthogonal kriging model and demonstrate the asymptotic optimality of the model averaging estimators in terms of mean square *** studies are conducted to evaluate the performance of the proposed method and compare it with the competitors to demonstrate its *** authors also analyse a real dataset for an illustration.

关键词： Asymptotic optimality Mallows criterion optimal model averaging orthogonal kriging model

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