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Cr-containing wastewater treatment based on Cr self-catalysis: a critical review

Frontiers of Environmental Science & Engineering 2024年第1期18卷 1-22页

作者： Manshu zhao Xinhua wang Shuguang wang Mingming Gao School of Environmental Science and Engineering Shandong UniversityQingdao 266237China Shandong Key Laboratory of Environmental Processes and Health Shandong UniversityQingdao 266237China Shandong Key Laboratory of Water Pollution Control and Resource Reuse Shandong UniversityQingdao 266237China Weihai Research Institute of Industrial Technology of Shandong University Weihai 264209China

Chromium (Cr), as a transition metal material with multiple redox states, has exhibited the catalysis toward Fenton-like reactions over a wide pH range. Although it is not sensible to add Cr reagents as catalysts due to its toxicity, it is highly promising to remediate Cr-containing wastewater through Cr-initiated advanced oxidation processes (Cr-initiated AOPs), which are clean and low-cost. Moreover, the widely concerned Cr-complexes, considered as obstacles in the remediation process, can be effectively destroyed by AOPs. Cr self-catalysis is defined as Cr species is both substrate and catalyst. However, the full understanding of Cr self-catalysis, including the generation of intermediates Cr(IV)/Cr(V), the synergetic effects with co-existing ions, and the accumulation of toxic Cr(VI), remains a challenge for the practical application of Cr-initiated AOPs. In this review, relevant researches on Cr self-catalysis during Cr-initiated AOPs are summarized. Specifically, the Cr-Fenton-like reaction, Cr substituted materials, and Cr-sulfite reactions are explored as key mechanisms contributing to Cr self-catalysis. Moreover, Cr transformation processes, including synchronously Cr removal, Cr redox reactions, and Cr(VI) accumulation, in AOPs-based synergistic systems are systematically analyzed. Detailed approaches for the detection of active species in AOPs-based systems are also presented. The primary objective of this review is to explore the application of AOPs for Cr-containing wastewater remediation based on Cr self-catalysis, and provide fundamental insights and valuable information for future research on Cr-initiated AOPs.

关键词： Self-catalysis Cr-initiated AOPs Cr transformation Cr intermediates Cr-containing wastewater

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Underwater Directional Acoustic Source Based on Pentamode Material

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Acta Mechanica Solida Sinica 2024年第1期37卷 1-9页

作者： Binghao zhao Peng wang Dongwei wang Gengkai Hu School of Aerospace Engineering Beijing Institute of TechnologyBeijing 100081China Wuhan Second Ship Design and Research Institute Wuhan 430205China

An underwater directional acoustic emitter is conceived with a highly anisotropic lattice material,whose acoustic characteristics manifest strong dependence on the orientation of the lattice material’s principal *** these features,a cylindrical structure made of such anisotropic lattice material is engineered to possess distinct impedance values in different directions,thereby facilitating wave emission along the principal axis while inducing reflection in other ***,through numerical simulations,it is demonstrated that the emission direction can be effectively manipulated by adjusting the principal axis orientation,concurrently enhancing the emitted *** contrast to previous directional acoustic structures,the compact emitter presented in this study can get rid of the size-wavelength constraint,enabling effective control of low-frequency waves.

关键词： Underwater Directional emission Pentamode material Broadband frequency

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Quaternion-Based Adaptive Trajectory Tracking Control of a Rotor-Missile with Unknown Parameters Identification

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Defence Technology（防务技术） 2024年第1期31卷 375-386页

作者： Jie zhao Zhongjiao Shi Yuchen wang Wei wang Beijing Institute of Technology Beijing 100081China

This paper investigates the adaptive trajectory tracking control problem and the unknown parameter identification problem of a class of rotor-missiles with parametric system ***,considering the uncertainty of structural and aerodynamic parameters,the six-degree-of-freedom(6Do F) nonlinear equations describing the position and attitude dynamics of the rotor-missile are established,respectively,in the inertial and body-fixed reference ***,a hierarchical adaptive trajectory tracking controller that can guarantee closed-loop stability is proposed according to the cascade characteristics of the 6Do F ***,a memory-augmented update rule of unknown parameters is proposed by integrating all historical data of the regression *** long as the finitely excited condition is satisfied,the precise identification of unknown parameters can be ***,the validity of the proposed trajectory tracking controller and the parameter identification method is proved through Lyapunov stability theory and numerical simulations.

关键词： Rotor-missile Adaptive control Parameter identification Quaternion control

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The storage and utilization of carbohydrates in response to elevation mediated by tree organs in subtropical evergreen broad-leaved forests

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Forest Ecosystems 2024年第1期11卷 52-61页

作者： Bin xu xueli Jiang Yingying Zong G.Geoff wang Fusheng Chen Zhenyu zhao Xiangmin Fang Key Laboratory of National Forestry and Grassland Administration on Forest Ecosystem Protection and Restoration of Poyang Lake Watershed College of ForestryJiangxi Agricultural UniversityNanchang330045China Jiulianshan National Observation and Research Station of Chinese Forest Ecosystem College of ForestryJiangxi Agricultural UniversityNanchang330045China Department of Forestry and Environmental Conservation Clemson UniversityClemsonSC29634USA

Global climate change can affect tree growth and carbon sink function by influencing plant carbohydrate synthesis and utilization,while elevation can be used as an ideal setting under natural conditions to simulate climate change *** effect of elevation on tree growth may depend on organ ***,the allocation patterns of nonstructural and structural carbohydrates(NSCs and SCs,respectively)in different tree organs and their response to elevation remain *** selected four dominant tree species,Schima superba,Castanopsis eyrei,Castanopsis fargesii and Michelia maudiae,along an elevation gradient from 609 to 1,207 m in subtropical evergreen broad-leaved forests and analyzed leaf,trunk,and fine root NSCs,carbon(C),nitrogen(N)and phosphorus(P)concentrations and the relative abundance of *** NSCs increased initially and then decreased,and trunk NSCs increased with increasing ***,root NSCs decreased with increasing *** relative abundance of SCs in leaves and trunks decreased,while the relative abundance of root SCs increased with increasing *** significant correlations between SCs and NSCs in leaves were detected,while there were negative correlations between SCs and NSCs in trunks,roots,and all *** partitioning analysis indicated that plant C/N and C/P were the main predictors of changes in SCs and *** results suggest that tree organs have divergent responses to elevation and that increasing elevation will inhibit the aboveground part growth and enhance the root growth of trees.A tradeoff between the C distribution used for growth and storage was confirmed along the elevation gradient,which is mainly manifested in the"sink"organs of *** results provide insight into tree growth in the context of global climate change scenarios in subtropical forest ecosystems.

关键词： Nonstructural carbohydrates Structural carbohydrates Elevation Subtropical evergreen broad-leaved forests Tree organs

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On the Infinite-Dimensional Modular Lie Superalgebras of O-Type

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Algebra Colloquium 2024年第2期31卷 347-360页

作者： Xiaoning xu Jing zhao Yucai Su School of Mathematics and Statistics Liaoning UniversityShenyang 110036China 不详

The natural filtrations of infinite-dimensional Lie superalgebras of O-type over a field of positive characteristic are proved to be invariant under automorphisms by studying ad-nilpotent *** observe that two Lie superalgebras of O-type are isomorphic if and only if the integers in the definition of these Lie superalgebras are ***,all the Lie superalgebras of O-type are classified in the sense of isomorphism.

关键词： filtration isomorphism classification

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Ultraviolet‑Irradiated All‑Organic Nanocomposites with Polymer Dots for High‑Temperature Capacitive Energy Storage

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Nano-Micro Letters 2024年第3期16卷 398-406页

作者： Jiale Ding Yao Zhou Wenhan xu Fan Yang Danying zhao Yunhe Zhang Zhenhua Jiang Qing wang College of Chemistry Jilin UniversityChangchun 130012People’s Republic of China Department of Materials Science and Engineering The Pennsylvania State UniversityUniversity ParkPA 16802USAs Deutsches Elektronen-Synchrotron DESY Notkestr.8522607 HamburgGermany

Polymer dielectrics capable of operating efficiently at high electric fields and elevated temperatures are urgently demanded by next-generation electronics and electrical power *** inorganic fillers have been extensively utilized to improved high-temperature capacitive performance of dielectric polymers,the presence of thermodynamically incompatible organic and inorganic components may lead to concern about the long-term stability and also complicate film ***,zero-dimensional polymer dots with high electron affinity are introduced into photoactive allyl-containing poly(aryl ether sulfone)to form the all-organic polymer composites for hightemperature capacitive energy *** ultraviolet irradiation,the crosslinked polymer composites with polymer dots are efficient in suppressing electrical conduction at high electric fields and elevated temperatures,which significantly reduces the high-field energy loss of the composites at 200℃.Accordingly,the ultraviolet-irradiated composite film exhibits a discharged energy density of 4.2 J cm^(−3)at 200℃.Along with outstanding cyclic stability of capacitive performance at 200℃,this work provides a promising class of dielectric materials for robust high-performance all-organic dielectric nanocomposites.

关键词： High-temperature energy storage Polymer dots Ultraviolet irradiation All-organic composite dielectrics

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Experimental investigation on the permeability of gap-graded soil due to horizontal suffusion considering boundary effect

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Journal of Rock Mechanics and Geotechnical Engineering 2024年第3期16卷 1072-1084页

作者： xuwei wang Yeshuang xu State Key Laboratory of Ocean Engineering School of Naval ArchitectureOceanand Civil EngineeringShanghai Jiao Tong UniversityShanghai200240China Shanghai Key Laboratory for Digital Maintenance of Buildings and Infrastructure Department of Civil EngineeringShanghai Jiao Tong UniversityShanghai200240China

The boundary condition is a crucial factor affecting the permeability variation due to *** experimental investigation on the permeability of gap-graded soil due to horizontal suffusion considering the boundary effect is conducted,where the hydraulic head difference(DH)varies,and the boundary includes non-loss and soil-loss *** samples are filled into seven soil storerooms connected in *** evaluation,the variation in content of fine sand(ΔR_(f))and the hydraulic conductivity of soils in each storeroom(C_(i))are *** the non-loss test,the soil sample filling area is divided into runoff,transited,and accumulated areas according to the negative or positive ΔR_(f) values.ΔR_(f) increases from negative to positive along the seepage path,and Ci decreases from runoff area to transited area and then rebounds in accumulated *** the soil-loss test,all soil sample filling areas belong to the runoff area,where the gentle-loss,strengthened-loss,and alleviated-loss parts are further divided.ΔR_(f) decreases from the gentle-loss part to the strengthened-loss part and then rebounds in the alleviated-loss part,and C_(i) increases and then decreases along the seepage *** relationship between ΔR_(f) and Ci is different with the boundary *** exponentially decreases with ΔR_(f) in the non-loss test and increases with ΔR_(f) generally in the soil-loss test.

关键词： Suffusion Permeability Experimental investigation Boundary effect Horizontal seepage

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IQABC-Based Hybrid Deployment Algorithm for Mobile Robotic Agents Providing Network Coverage

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Tsinghua Science and Technology 2024年第2期29卷 589-604页

作者： Shuang xu Xiaojie Liu Dengao Li Jumin zhao College of Computer Science and Technology(College of Data Science) Taiyuan University of TechnologyTaiyuan 030024China Pengcheng Laboratory Shenzhen 518055China College of Information and Computer Taiyuan University of TechnologyTaiyuan 030024China

Working as aerial base stations,mobile robotic agents can be formed as a wireless robotic network to provide network services for on-ground mobile devices in a target ***,a challenging issue is how to deploy these mobile robotic agents to provide network services with good quality for more users,while considering the mobility of on-ground *** this paper,to solve this issue,we decouple the coverage problem into the vertical dimension and the horizontal dimension without any loss of optimization and introduce the network coverage model with maximum coverage ***,we propose a hybrid deployment algorithm based on the improved quick artificial bee *** algorithm is composed of a centralized deployment algorithm and a distributed *** proposed deployment algorithm deploy a given number of mobile robotic agents to provide network services for the on-ground devices that are independent and identically *** results have demonstrated that the proposed algorithm deploys agents appropriately to cover more ground area and provide better coverage uniformity.

关键词： wireless robotic networks network coverage deployment algorithm improved quick artificial bee colony

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One-pot Synthesis of MoO_(3)/PI Composite with Enhanced Photocatalytic Performance for Oxidative Coupling of Amines to Imines

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China Petroleum Processing & Petrochemical Technology 2024年第2期26卷 57-71页

作者： zhao Wenjie Du Chengxin Song Yu Zhou Yafen wang Qing Zhou Limei xu Bin Chemical Synthesis and Pollution Control Key Laboratory of Sichuan Province College of Chemistry and Chemical EngineeringChina West Normal UniversityNanchongChina Key Laboratory of Green Chemistry of Sichuan Institutes of Higher Education Sichuan University of Science&EngineeringZigongChina

Organic-inorganic MoO_(3)/PI(MoPI)composites were prepared using a simple one-pot thermal copolymerization *** resulting composites exhibited enhanced photocatalytic activity for the selective oxidation of benzylamine to N-benzylidene benzylamine(N-BDBA)in ambient air under simulated solar light irradiation compared to pristine MoO_(3) or polyimide(PI).In particular,the MoPI composite with a 0.3:1 molar ratio of Mo to melamine,referred to as MoPI-0.3,demonstrated the best performance in the photo-oxidation of benzylamine,achieving a benzylamine conversion of 95%with a N-BDBA selectivity exceeding 99%after 3 h *** enhanced photocatalytic activity of the MoPI-0.3 catalyst was attributed to the formation of a direct Z-scheme heterojunction between MoO_(3) and PI,facilitating more efficient separation of the photoinduced electrons and ***,the MoPI-0.3 composite maintained considerably high activity over four consecutive cycles,highlighting its good stability and ***,the MoPI-0.3 composite could photo-oxidize benzylamine derivatives and heterocyclic amines to their corresponding imines,demonstrating the universal applicability of this composite catalyst.

关键词： MoO3/PI composite photocatalysis amine oxidation imine

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Understanding Human and Machine Interaction from Decision Perspective: An Empirical Study Based on the Game of Go

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Journal of Systems Science & Complexity 2024年第2期37卷 647-667页

作者： zhao Ping LI xuerong wang Shouyang Academy of Mathematics and Systems Science Chinese Academy of SciencesBeijing 100190China School of Mathematical Sciences University of Chinese Academy of SciencesBeijing 100190China

The authors aim to interpret human and AI interactions from the decision *** authors decompose the interaction analysis into the following main components in the context of interactions:Individual behavior patterns,interaction relationships,and comprehensive *** authors interpret intertemporal decisions from a physical perspective and employ cross-discipline concepts and methodologies to extract the behavior characteristics of players in the empirical case *** the individual behavior patterns,the authors find that human players prefer short-term periods to AI in *** interaction relationship analysis reveals a dynamic relationship between possible short-term co-movement and nearly counter-movement in the long *** authors apply principal component analysis to descriptive indicators and discover a regular decision *** main behavior pattern of players in the game of Go is switching between careful and daring *** differences in the decision hierarchies imply a discrepancy of patience between humans and AI.

关键词： Coherence analysis decision hierarchy machine behaviour multitaper spectral analysis

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