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Fabrication of MXene-Bi_(2)WO_(6)heterojunction by Bi_(2)Ti_(2)O_(7)hinge for extraordinary LED-light-driven photocatalytic performance

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Nano Research 2024年第6期17卷 4729-4736页

作者： Zhiwen Li Liangliang Xu Zaheer Ud Din Babar Ali Raza Yifei Zhang Xinrui Gu Yu-Xin Miao zhen zhao Gao Li Institute of Catalysis for Energy and Environment College of Chemistry and Chemical EngineeringShenyang Normal UniversityShenyang 110034China State Key Laboratory of Catalysis Dalian Institute of Chemical PhysicsChinese Academy of SciencesDalian 116023China Scuola Superiore Meridionale(SSM) University of Naples Federico IILargo S.Marcellino1080138Italy Department of Chemical and Biomolecular Engineering Korea Advanced Institute of Science and Technology(KAIST)Daejeon 34141Republic of Korea University of Chinese Academy of Sciences Beijing 100049China

Heterojunction composites with intimate interfaces can shorten the diffusion distance,which leads to a shorter path for photogenerated carriers,thereby increasing photocatalytic ***,we report the fabrication of Ti_(3)C_(2)-Bi_(2)WO_(6)(TC-BW)heterojunctions hinged by Bi_(2)Ti_(2)O_(7)joints via an in situ hydrothermal reaction of Ti_(3)C_(2)in the presence of Na_(2)WO_(4)and Bi(NO_(3))_(3).The TC-BW was characterized using X-ray diffraction(XRD),scanning transmission electron microscopy(STEM),and Raman ***-BW showed superior photocatalytic activity(productivity over 15TC-WB reaches up to 5.0 mmolreacted BA·gcat.^(−1)·h^(−1))in the oxidation of benzyl alcohol using light-emitting diode(LED)light,arising from the surface defects and intimate heterojunction interface between the Ti_(3)C_(2)MXene and Bi_(2)WO_(6)***-BW heterojunctions provide an enhanced separation efficiency of photogenerated charges,which in turn yields superior photocatalytic ***,it is well substantiated by density functional theory(DFT)*** summary,this study elucidates the preparation of heterojunction composites with intimate interfaces for highly efficient photooxidation.

关键词： MXene-Bi_(2)WO_(6) heterojunction LED-light-driven photocatalysis Bi_(2)Ti_(2)O_(7) photooxidation

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Recent development of three-dimension printed graphene oxide and MXene-based energy storage devices

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Tungsten 2024年第1期6卷 196-211页

作者： Liang-Hao Yu Xin Tao Shang-Ru Feng Jin-Tao Liu Lin-Lin Zhang Guang-zhen zhao Guang Zhu Key Laboratory of Spin Electron and Nanomaterials of Anhui Higher Education Institutes Suzhou UniversitySuzhou 234000China Key Laboratory of Leather of Zhejiang Province College of Chemistry and Materials EngineeringWenzhou UniversityWenzhou 325035China

The research for three-dimension(3D)printing carbon and carbide energy storage devices has attracted widespread exploration *** designable in structure and materials,graphene oxide(GO)and MXene accompanied with a direct ink writing exhibit a promising prospect for constructing high areal and volume energy density *** review not only summarizes the recent advances in 3D printing energy storage devices including printing methods,ink rheological properties,and different energy storage systems,but also discusses the printing methods related to energy *** addition,the binder or additive free of two-dimensional carbide materials is quite important for the present electrochemical energy storage devices,which also are presented.

关键词： 3D printing Two-dimensional materials Energy storage device Ink theological MXene

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A high-speed true random number generator based on Ag/SiNx/n-Si memristor

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Frontiers of physics 2024年第1期19卷 241-250页

作者： Xiaobing Yan Zixuan Zhang Zhiyuan Guan Ziliang Fang Yinxing Zhang Jianhui zhao Jiameng Sun Xu Han Jiangzhen Niu Lulu Wang Xiaotong Jia Yiduo Shao zhen zhao zhenqiang Guo Bing Bai Institute of Life Science and Green Development Key Laboratory of Brain-Like Neuromorphic Devices and Systems of Hebei ProvinceCollege of Electron and Information EngineeringHebei UniversityBaoding 071002China

The intrinsic variability of memristor switching behavior can be used as a natural source of randomness,this variability is valuable for safe applications in hardware,such as the true random number generator(TRNG).However,the speed of TRNG is still be further ***,we propose a reliable Ag/SiNx/n-Si volatile memristor,which exhibits a typical threshold switching device with stable repeat ability and fast switching *** volatile-memristor-based TRNG is combined with nonlinear feedback shift register(NFSR)to form a new type of high-speed dual output ***,the bit generation rate reaches a high speed of 112 kb/*** addition,this new TRNG passed all 15 National Institute of Standards and Technology(NIST)randomness tests without post-processing steps,proving its performance as a hardware security *** work shows that the SiNx-based volatile memristor can realize TRNG and has great potential in hardware network security.

关键词： volatile memristor true random number generator(TRNG) delay time threshold switching device

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Engineered wettability-gradient porous structure enabling efficient water manipulation in regenerative fuel cells

Energy and AI

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Energy and AI 2024年第3期17卷 357-367页

作者： Zhefei Pan Lizhen Wu Fengjia Xie Zhewei Zhang zhen zhao Oladapo Christopher Esan Xuming Zhang Rong Chen Liang An Key Laboratory of Low-grade Energy Utilization Technologies and Systems(Chongqing University) Ministry of EducationChongqing 400030China Institute of Engineering Thermophysics Chongqing UniversityChongqing 400030China Department of Mechanical Engineering The Hong Kong Polytechnic UniversityHung HomKowloonHong Kong Special Administrative Regions of China Department of Applied Physics The Hong Kong Polytechnic UniversityHung HomKowloonHong Kong Special Administrative Regions of China Department of Mechanical Aerospaceand Biomedical EngineeringUniversity of TennesseeKnoxvilleTN 37996USA Research Institute for Sports Science and Technology The Hong Kong Polytechnic UniversityHung HomKowloonHong Kong Special Administrative Regions of China

Regenerative fuel cells can operate alternately as an electrolyzer and as a fuel cell,frequently involving water as a reactant or *** the electrode surface to manipulate water can prevent electrode flooding and enhance the electrode's mass transfer efficiency by facilitating better contact with gaseous ***,conventional electrodes face difficulties in allowing water droplets to penetrate in a single direction leaving *** this work to address this issue,a wettability gradient electrode is designed and fabricated for efficient water manipulation in regenerative fuel *** findings demonstrate that the water removal strategy in the electrolyzer mode yields the highest ammonia yield and Faradaic efficiency of 3.39×10-10 mol s-1 cm-2 and 0.49%,***,in the fuel cell mode,the discharging process sustains for approximately 20.5 h,which is six times longer than the conventional *** ability to sustain the discharging process for extended periods is particularly advantageous in regenerative fuel cells,as it enables the cells to operate for longer periods without the need for regeneration.

关键词： Regenerative fuel cells Electrode flooding Water manipulation Wettability gradient Water fluxes

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TiO_(2) nanofiber-supported copper nanoparticle catalysts for highly efficient methane conversion to C1 oxygenates under mild conditions

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Nano Research 2024年第5期17卷 3844-3852页

作者： Wencui Li Yu Ren Zean Xie Yipeng Wang Hang Zhang Dianxiang Peng Hengfang Shen Hongfei Shi Jiaxin Cai Peng Wang Tongxin Zhang zhen zhao State Key Laboratory of Heavy Oil Processing China University of Petroleum(Beijing)Beijing 102249China Institute of Catalysis for Energy and Environment College of Chemistry&Chemical EngineeringShenyang Normal UniversityShenyang 110034China Institute of Petrochemical Technology Jilin Institute of Chemical TechnologyJilin 132022China

The selective oxidation of methane under mild conditions remains the“Holy Grail of Catalysis”.The key to activating methane and inhibiting over-oxidation of target oxygenates lies in designing active *** nanoparticles were loaded onto TiO_(2) nanofibers using the photo-deposition *** resulting catalysts were found to effectively convert methane into C1 oxygenated products under mild *** with previously reported catalysts,it delivers a superior performance of up to 2510.7 mmol·g_(Cu)^(-1)·h^(-1) productivity with a selectivity of around 100%at 80℃for 5 *** characterizations and density functional theory(DFT)calculations indicate that TiO_(2) in the mixed phase of anatase and rutile significantly increases the Cu^(+)/CuO ratio of the supported Cu species,and this ratio is linearly related to the formation rate of oxygen-containing *** CuI site promotes the generation of active O species from H_(2)O_(2) dissociation on Cu_(2)O(111).These active O species reduce the energy barrier for breaking the C-H bond of CH_(4),thus boosting the catalytic *** methane conversion mechanism was proposed as a methyl radical pathway to form CH_(3)OH and CH_(3)OOH,and then the generated CH_(3)OH is further oxidized to HOCH_(2)OOH.

关键词： TiO_(2)nanofiber copper nanoparticles photo-deposition method methane oxidation C1 oxygenates

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Global dust density in two-dimensional complex plasma

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Chinese Physics B 2024年第6期33卷 445-450页

作者：赵逸真刘松芬孔伟杨芳 School of Physics Nankai UniversityTianjin 300071China College of Science Civil Aviation University of ChinaTianjin 300300China

The driven-dissipative Langevin dynamics simulation is used to produce a two-dimensional(2D) dense cloud, which is composed of charged dust particles trapped in a quadratic potential. A 2D mesh grid is built to analyze the center-to-wall dust density. It is found that the local dust density in the outer region relative to that of the inner region is more nonuniform,being consistent with the feature of quadratic potential. The dependences of the global dust density on equilibrium temperature, particle size, confinement strength, and confinement shape are investigated. It is found that the particle size, the confinement strength, and the confinement shape strongly affect the global dust density, while the equilibrium temperature plays a minor effect on it. In the direction where there is a stronger confinement, the dust density gradient is bigger.

关键词： dust particles quadratic potential two-dimensional mesh grid

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Microstructure and properties of LZQT600-3 HCCDIBs for plunger pump cylinder

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China Foundry 2024年第2期21卷 197-204页

作者： Chun-jie Xu Yuan-ying Jin Dong Ma zhen zhao Jia-wei Qi Shang Sui Xiang-quan Wu Can Guo Zhong-ming Zhang Yong-hui Liu Dan Shechtman School of Materials Science and Engineering Xi'an University of TechnologyXi'an 710048China Xi'an Shechtman Nobel Prize New Materials Institute Xi'an 710048China Tongchuan Huazhu Precision Technology Co. Ltd.Tongchuan 727100ShaanxiChina Faculty of Materials Science and Engineering Technion-Israel Insititue of TechnologyHaifa 3200003Israel

It is important to improve the comprehensive performance of the ductile iron bars(DIBs)for the cylinder block of the extra high pressure hydraulic plunger pump and accelerate the industrial *** this work,the LZQT600-3 DIBs with the diameter of 145 mm were prepared by the horizontal continuous casting(HCC)process,that is,LZQT600-3 *** microstructure and room temperature tensile properties of different sections[left-edge(surface layer),left-1/2R(left half of the radius),and the center of the HCCDIBs]were *** results show that the spheroidization of LZQT600-3 HCCDIBs matrix from the left-edge,left-1/2R to the center is at nodulizing grade II and *** the cooling rate gradually decreases from surface to the center of the HCCIBs,the number of spheroidized graphite is gradually reduced,the size is gradually increased,the shape factor is decreased,and the pearlite content and lamellate spacing are *** the horizontal direction of the section,the hardness of the material is distributed symmetrically around the center of the *** the vertical direction,the hardness distribution in the center of the HCCDIBs is asymmetrical due to the gravity during the solidification ***,the microstructure in the lower part of the section solidifies relatively *** left-edge has the best tensile mechanical properties,and the ultimate tensile strength,yield tensile strength and elongation are 597.3 MPa,418.5 MPa and 9.6%,*** tensile fracture belongs to the ductile-brittle hybrid *** comprehensive performances of LZQT600-3 HCCDIBs meet the actual application requirements of ultra-high pressure hydraulic plunger pump cylinder.

关键词： horizontal continuous casting(HCC) nodular cast iron ductile iron bars microstructure mechanical properties

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论网络攻击溯源困境下的战争伦理规制

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太平洋学报 2024年第3期32卷 49-61页

作者：赵阵国防科技大学湖南长沙410072

网络攻击溯源旨在确定虚拟网络空间中发起攻击的行为主体,使得攻击者受到应有制裁,这对于实现网络空间的安全具有重大意义。然而,现实中网络攻击溯源遭遇困境,通过技术手段难以最终锁定发动攻击者,通过法律途径也难以将某攻击责任归因... 详细信息

网络攻击溯源旨在确定虚拟网络空间中发起攻击的行为主体,使得攻击者受到应有制裁,这对于实现网络空间的安全具有重大意义。然而,现实中网络攻击溯源遭遇困境,通过技术手段难以最终锁定发动攻击者,通过法律途径也难以将某攻击责任归因于一国政府。解决溯源问题需要转换研究视域,从问题追溯的理路转向直面攻击行为本身,从各种网络攻击中区分出国家网络攻击并进行伦理规制。国家网络攻击本质上是一种新型战争方式,是体现国家意志有组织的暴力行为,已有战争伦理规范难以适用于这种新型战争,国际网络空间实质上处于一种伦理缺失状态,只有重塑战争伦理才能规制国家网络攻击,也才能从根本上破解溯源困境。要抛弃“武力至上”的现实主义伦理观念,在网络空间中树立正义战争观。通过宣告原则主动标识国家网络行为,要遵循恰当性原则接受正义性审视。要遵循网络平等均衡原则促进构建和平正义的国际环境。

关键词：网络攻击溯源归因伦理规制

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基于增量式Q学习的固定翼无人机跟踪控制性能优化

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控制与决策 2024年第2期39卷 391-400页

作者：赵振根程磊南京航空航天大学自动化学院南京211106

针对固定翼无人机纵向控制的高性能需求,提出一种控制系统性能优化结构.该结构包括一个使系统稳定的标称控制器和一个参与性能优化的增量式控制器.控制系统增量式的实现不会改变原有的控制系统,而是仅对标称控制系统做控制输入的补偿与... 详细信息

针对固定翼无人机纵向控制的高性能需求,提出一种控制系统性能优化结构.该结构包括一个使系统稳定的标称控制器和一个参与性能优化的增量式控制器.控制系统增量式的实现不会改变原有的控制系统,而是仅对标称控制系统做控制输入的补偿与控制性能的优化.基于Q学习理论进行增量式控制器设计,针对状态信息完全可获得的系统,设计一种基于状态反馈的增量式Q学习算法.当状态信息不能完全获得时,利用系统输入、输出和参考信号数据,设计一种基于输出反馈的增量式Q学习算法.两种增量式控制器均是在数据驱动环境下自适应学习增量式控制律,无需提前知道系统动力学模型以及标称控制器的控制增益.此外,证明了增量式Q学习方法在满足持续激励条件的激励噪声下,对Q函数贝尔曼方程的求解没有偏差.最后,通过对F-16飞行器纵向模型实例的仿真验证该方法的有效性.

关键词：强化学习 Q学习增量式控制性能优化跟踪控制无人机

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Insufficient Physical Activity among Students Aged 6-17 Years in China,2016-2017

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Biomedical and Environmental Sciences 2024年第5期37卷 531-536页

作者： XUE Tao Tao GAO Xing Xing WANG Li Min ZHANG Xiao zhao zhen Ping LI Chun NYASHA Grace Mudoti LIU Chen Yi ZHANG Mei Division of Chronic Disease and Risk Factor Surveillance National Center for Chronic and Non-communicable Disease Control and PreventionChinese Center for Disease Control and PreventionBeijing 100050China International Education School China Medical UniversityShenyang 110122LiaoningChina

Regular physical activity of sufficient duration and intensity can provide health benefits such as improved physical fitness,which promotes bone health,prevents hypertension,improves mental health,and reduces adiposit... 详细信息

关键词： hypertension Regular benefits

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