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Atomic Ni directional-substitution on ZnIn_(2)S_(4) nanosheet to achieve the equilibrium of elevated redox capacity and efficient carrier-kinetics performance in photocatalysis

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Journal of Energy Chemistry 2024年第1期88卷 272-281,I0007页

作者： Haibin Huang Guiyang yu Xingze zhao Boce Cui Jinshi yu Chenyang zhao Heyuan Liu Xiyou Li School of Materials Science and Engineering China University of Petroleum(East China)Qingdao 266580ShandongChina Key Laboratory of Optic-electric Sensing and Analytical Chemistry for Life Science(MOE) College of Chemistry and Molecular EngineeringQingdao University of Science and TechnologyQingdao 266042ShandongChina College of New Energy China University of Petroleum(East China)Qingdao 266580ShandongChina

It is a challenge to coordinate carrier-kinetics performance and the redox capacity of photogenerated charges synchronously at the atomic level for boosting photocatalytic ***,the atomic Ni was introduced into the lattice of hexagonal ZnIn_(2)S_(4) nanosheets(Ni/ZnIn_(2)S_(4))via directionalsubstituting Zn atom with the facile hydrothermal *** electronic structure calculations indicate that the introduction of Ni atom effectively extracts more electrons and acts as active site for subsequent reduction *** the optimized light absorption range,the elevation of Efand ECBendows Ni/ZnIn_(2)S_(4) photocatalyst with the increased electron concentration and the enhanced reduction ability for surface ***,ultrafast transient absorption spectroscopy,as well as a series of electrochemical tests,demonstrates that Ni/ZnIn_(2)S_(4) possesses 2.15 times longer lifetime of the excited charge carriers and an order of magnitude increase for carrier mobility and separation efficiency compared with pristine ZnIn_(2)S_(4).These efficient kinetics performances of charge carriers and enhanced redox capacity synergistically boost photocatalytic activity,in which a 3-times higher conversion efficiency of nitrobenzene reduction was achieved upon Ni/ZnIn_(2)S_(4).Our study not only provides in-depth insights into the effect of atomic directional-substitution on the kinetic behavior of photogenerated charges,but also opens an avenue to the synchronous optimization of redox capacity and carrier-kinetics performance for efficient solar energy conversion.

关键词： ZnIn_(2)S_(4) Substitution Carrier kinetics Redox capacity Photocatalysis

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Endoscopic band ligation or endoscopic tissue adhesive injection in the treatment of gastric varices:Which is better?

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World Journal of Gastroenterology 2024年第21期30卷 2827-2828页

作者： Li-Zhi Yi sheng-Bing zhao Department of Gastroenterology The People’s Hospital of LeshanLeshan 614000Sichuan ProvinceChina Department of Gastroenterology Changhai HospitalThe Second Military Medical University/Naval Medical UniversityShanghai 200433China

The combination of endoscopic ultrasound with endoscopic treatment of type 1 gastric variceal hemorrhage may improve the robustness and generalizability of the findings in future ***,the esophageal varices should also... 详细信息

关键词： Gastric varices Esophageal varices Endoscopic band ligation Endoscopic tissue adhesive injection Endoscopic ultrasound

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Probing the Kinematic Signatures of Planet Formation in the Gas Disk of MWC 480

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Research in Astronomy and Astrophysics 2024年第6期24卷 110-118页

作者： Min zhao Haochuan yu Zhengxiang Li Department of Astronomy Beijing Normal UniversityBeijing 100875China Sub-department of Astrophysics Department of PhysicsUniversity of OxfordOxfordOX13RHUK

The disk around MWC 480 has shown multiple substructures in both dust and gas observations,possibly suggesting ongoing planet formation in *** this paper,we explore the gas kinematics of the MWC 480 disk by analyzing the archival Atacama Large Millimeter/submillimeter Array observations of^(12)CO(J=2-1),^(13)CO(J=2-1),and C^(18)O(J=2-1).By modeling the line-of-sight velocities,inferred from the Doppler shifts of the emission lines,we are able to decompose the three-dimensional(3D)velocity field of the disk into rotational,radial,and vertical *** analysis reveals the presence of large-scale gas flows in the(r,z)***,we identify potential meridional flows across various heights as traced by all three CO isotopologues in the 80–120 au region,possibly associated with ongoing planet formation activities in this ***,we find upward flows near 200 au for all three CO isotopologues,which may point to the presence of disk winds.

关键词： protoplanetary disks planet-disk interactions planet-star interactions

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A review on covalent organic frameworks for rechargeable zinc-ion batteries

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Chinese Chemical Letters 2024年第7期35卷 107-120页

作者： yunyu zhao Chuntao Yang Yingjian yu College of Physics Science and Technology Kunming UniversityKunming 650214China

In recent years,rechargeable zinc-ion batteries(ZIBs)are considered to be a promising alternative to lithium-ion batteries owing to their high safety and theoretical capacity with low ***,the in-depth development of rechargeable zinc-ion batteries is restricted by a sequence of issues,such as the dissolution and structure collapse of cathode materials,the formation of by-products,severe anode corrosion,passivation,and the growth of zinc *** covalent organic frameworks(COFs)can solve the above problems to a certain extent owing to their ideal characteristics,such as rigid structure,insolubility,high porosity,and abundant active ***,as advanced materials for ZIBs,have attracted researchers'*** this review,we systematically summarized the synthesis methods of COFs and discussed the application of several advanced characterization technologies in COFs,which would provide a reference for the in-depth research of *** addition,we elucidated the use of COFs as cathode materials and anode protective layers in rechargeable ***,we discussed the challenges and solutions in the development of COF materials,which would provide constructive insights into the future direction of COFs.

关键词： Covalent organic framework Zn-ion battery Zinc dendrite Anode Cathode

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A New Equalization Method for Lithium-Ion Battery Packs Based on CUK

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Energy Engineering 2024年第6期121卷 1459-1472页

作者： yu Zhang sheng Tian Yongkang Zhang School of Electrical and Electronic Engineering Hubei University of TechnologyWuhan430000China

Aiming at the traditional CUK equalizer can only perform energy equalization between adjacent batteries,if the two single batteries that need to be equalized are far away from each other,there will be the problem of longer energy transmission path and lower equalization efficiency,this paper optimizes the CUK equalizer and optimizes its peripheral selection circuit,which can support the equalization of single batteries at any two *** control strategy adopts the open-circuit voltage(OVC)of the battery and the state of charge(SOC)of the battery as the equalization variables,and selects the corresponding equalization variables according to the energy conditions of the two batteries that need to be equalized,and generates the adaptive equalization current with an adaptive PID controller in order to improve the equalization *** modeling is performed in Matlab/Simulink 2021b,and the experimental results show that the optimized CUK equalizer in this paper improves the equalization time by 25.58%compared with the traditional CUK *** addition,compared with the mean value difference(MVD)method,the adaptive PID method reduces the equalization time by about 30%in the static and charging and discharging experimental environments,which verifies the superiority of this equalization scheme.

关键词： battery balancing CUK equalizer adaptive PID SOC

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Beamspace maximum likelihood algorithm based on sum and difference beams for elevation estimation

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Journal of Systems Engineering and Electronics 2024年第3期35卷 589-598页

作者： CHEN sheng zhao Yongbo HU Yili PANG Xiaojiao National Laboratory of Radar Signal Processing Xidian UniversityXi’an 710071China

Beamspace super-resolution methods for elevation estimation in multipath environment has attracted significant attention, especially the beamspace maximum likelihood(BML)algorithm. However, the difference beam is rarely used in superresolution methods, especially in low elevation estimation. The target airspace information in the difference beam is different from the target airspace information in the sum beam. And the use of difference beams does not significantly increase the complexity of the system and algorithms. Thus, this paper applies the difference beam to the beamformer to improve the elevation estimation performance of BML algorithm. And the direction and number of beams can be adjusted according to the actual needs. The theoretical target elevation angle root means square error(RMSE) and the computational complexity of the proposed algorithms are analyzed. Finally, computer simulations and real data processing results demonstrate the effectiveness of the proposed algorithms.

关键词： elevation estimation beamspace multipath environment maximum likelihood

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CP violation of baryon decays with Nπrescatterings

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Chinese Physics C 2024年第10期48卷 1-10页

作者： Jian-Peng Wang Fu-sheng yu MOE Frontiers Science Center for Rare Isotopes and School of Nuclear Science and TechnologyLanzhou UniversityLanzhou 730000China

There is a long-standing puzzle that the CP violation(CPV)in the baryon systems has never been wellestablished in experiments,while the CPV of mesons have been observed by *** this paper,we propose thatthe CpV of baryon decays can be generated with the rescatterings of a nucleon and a pion into some final states,i.e Nπ→Nπor Nππ.Benelited by the fruitful data of Nπscatterings,we can model-independently analyse the strongphases of b-baryon decays using the partial wave amplitudes of Nπ*** the most difficult problemof non-perturbative dynamics,it makes a great advantage to predict the CpV of baryon decays with a relatively *** understanding of the decay *** study the processes of∧_(b)^(0)→(pπ^(+)π^(-))h^(-)and(pπ^(0))h^(-)with h=πor *** is found that the global CPV of the above processes in the invariant mass regions of Nπscatterings are at theorder of several *** importantly,the local CPV in some regions of the Dalitz plots can reach the order of 10%,or be even *** the predicted results and the experimental data samples,we strong suggest tomeasure the CPV of∧_(b)^(0)→(pπ^(+)π^(-))K^(-),which has a large possibility to achieve the first observation of CPV in thebaryon system.

关键词： CP violation baryon decays Nπscatterings

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2D DOA Estimation of Coherent Signals with a Separated Linear Acoustic Vector-Sensor Array

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China Communications 2024年第2期21卷 155-165页

作者： sheng Liu Jing zhao Decheng Wu Yiwang Huang Kaiwu Luo School of Data Science Tongren UniversityTongren 554300China School of Automation Chongqing University of Posts and TelecommunicationsChongqing 400065China

In this paper, a two-dimensional(2D) DOA estimation algorithm of coherent signals with a separated linear acoustic vector-sensor(AVS) array consisting of two sparse AVS arrays is proposed. Firstly,the partitioned spatial smoothing(PSS) technique is used to construct a block covariance matrix, so as to decorrelate the coherency of signals. Then a signal subspace can be obtained by singular value decomposition(SVD) of the covariance matrix. Using the signal subspace, two extended signal subspaces are constructed to compensate aperture loss caused by *** elevation angles can be estimated by estimation of signal parameter via rotational invariance techniques(ESPRIT) algorithm. At last, the estimated elevation angles can be used to estimate automatically paired azimuth angles. Compared with some other ESPRIT algorithms, the proposed algorithm shows higher estimation accuracy, which can be proved through the simulation results.

关键词： acoustic vector-sensor coherent signals extended signal subspace sparse array

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Three-Component Transformation of CO_(2),Propargyl Alcohols and Secondary Amines intoβ-Oxopropylcarbamates Promoted by a Noble Metal-Free Metal–Organic Framework Catalyst

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CCS Chemistry 2024年第9期6卷 2333-2345页

作者： Xiao-Lei Jiang Fang-yu Ren Ying Shi Yao Xie sheng-Li Hou Bin zhao Department of Chemistry Key Laboratory of Advanced Energy Material Chemistry(Ministry of Education)MOERenewable Energy Conversion and Storage Center(RECAST)Nankai UniversityTianjin 300071 College of Chemistry and Chemical Engineering Yantai UniversityYantai 264010

The three-component reaction of CO_(2),propargyl alcohols,and secondary amines frequently applies noble metal or homogeneous catalysts,therefore it is necessary and important to seek a recyclable catalyst without noble metals for this reaction,despite the multitude of ***,a unique framework{[Ce3(Cu4I4)2(CNA)8(DMF)8](NO3)}n(CuCe-CNA)with two kinds of metal cluster nodes[Ce3]and[Cu4I4]was synthesized,displaying high thermal and chemical ***-CNA-300 was obtained by removing the coordinated DMF molecules with[Ce3]cluster at 300°C,in which more metal sites are exposed and the pores are enlarged,but the three-dimensional framework still remains ***-CNA-300 can effectively catalyze the three-component reaction of 2-methyl-3-butyn-2-alcohol,CO_(2),and pyrrolidine toβ-oxopropylcarbamates with a yield of 98%under mild conditions,and the catalytic activity is higher than those of noble metal ***,CuCe-CNA-300 exhibits high catalytic efficiency for various kinds of propargyl alcohols and secondary amines,and also shows good *** studies suggest that theα-alkylidene cyclic carbonates derived from the cycloaddition of propargyl alcohols and CO_(2) are the intermediates,which further react with secondary amines through ammonolysis reaction to generateβ-***,this work may open a new avenue for the one-pot transformation of CO_(2) with two or more components into value-added chemicals activated by noble metal-free metal–organic frameworks catalysts.

关键词： three-component reaction CO_(2)conversion metal-organic frameworks noble metal-free catalyst synergistic catalysis

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Simulation of nanofluid natural convection based on single-particle hydrodynamics in energy-conserving dissipative particle dynamics(eDPD)

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Applied Mathematics and Mechanics(English Edition) 2024年第8期45卷 1429-1446页

作者： Wei LU Shuo CHEN Zhiyuan yu Jiayi zhao School of Aerospace Engineering and Applied Mechanics Tongji UniversityShanghai 200092China Shanghai Key Laboratory of Vehicle Aerodynamics and Vehicle Thermal Management Systems Tongji UniversityShanghai 201804China School of Energy and Power Engineering University of Shanghai for Science and TechnologyShanghai 200093China

In the present study,the nanofliud natural convection is investigated by the energy-conserving dissipative particle dynamics(eDPD)method,where the nanoparticles are considered at the single-particle *** thermal expansion coefficientβand the viscosityμof the simulated system containing nanoparticles are calculated and found to be in close alignment with the previous simulation *** single-particle hydrodynamics in e DPD enables simulations of nanofluid natural convection with higher Rayleigh numbers and greater nanoparticle volume ***,this approach is utilized to simulate the nanoparticle distribution during the enhanced heat transfer process in the nanofluid natural *** localized aggregation of nanoparticles enhances the heat transfer performance of the nanofluid under specific Rayleigh numbers and nanoparticles volume fractions.

关键词： single-particle hydrodynamics energy-conserving dissipative particle dynamics(eDPD) nanoparticle nanofluid heat transfer

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