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Regulation of the pore structure of carbon nanosheets based electrocatalyst for efficient polysulfides phase conversions

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Journal of Materials Science & Technology 2024年第4期171卷 37-46页

作者： Xiaoyang Liu Jingbo zhang Kangli Liu Shijie zhang Rouhan Hou Xiaoyi Hu peng zhang Guosheng Shao State Center for International Cooperation on Designer Low-Carbon&Environmental Materials(CDLCEM) School of Materials Science and EngineeringZhengzhou UniversityZhengzhou 450001China Zhengzhou Materials Genome Institute(ZMGI) Xingyang 450100China

The practical applications of lithium-sulfur(Li-S)batteries are hampered by the sluggish redox kinetics and polysulfides shuttle in the cyclic process,which leads to a series of problems including the loss of active materials and poor cycling *** this paper,the pore structures of carbon nanosheets based electrocatalysts were precisely controlled by regulating the content of water-soluble KCl *** relationship between pore structures and Li-S electrochemical behavior was studied,which demonstrates a key influence of pore structure in polysulfides phase *** the liquid-sloid redox reaction of polysulfides,the micropores and small mesopores(d20 nm)and macropores played a decisive *** a typical exhibition,the nickel-embedded carbon nanosheets(Ni-CNS)with a high content of large mesopores and macropores can aid Li-S batteries in exhibiting stable cycling performance(760.1 mAh g^(-1)at 1 C after 300 cycles)and superior rate capac-ity(847.8 mAh g^(-1)at 2 C).Furthermore,even with high sulfur loading(8 mg cm^(−2))and low electrolyte(E/S is around 6μL mg^(-1)),the high area capacity of 7.7 mAh cm^(−2)at 0.05 C could be *** work can provide a guideline for the design of the pore structure of carbon-based electrocatalysts toward high-efficiency sulfur species redox reactions,and afford a general,controllable,and simple approach to constructing high performance Li-S batteries.

关键词： Hierarchical porous carbon network Electrocatalyst Molten salt templating method Modified separators Li-S batteries

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Properties, hazards and valuable metal recovery technologies of red mud: A review

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Particuology 2024年第10期93卷 328-348页

作者： Peixin Du peng Wang Xueqian zhang Guangwu Wen Yishan Wang School of Materials Science and Engineering Shandong University of TechnologyZibo255000China

This review presents a summary of the research conducted thus far on the recovery of various types of valuable metals from red mud. The composition, properties, environmental hazards, and current status of comprehensive utilization of red mud were studied. A number of studies have been conducted on the use of red mud as a modifying additive for cement, the development of various catalysts based on red mud, and the recovery of various valuable metals from red mud. Furthermore, we examine several techniques for extracting various types of valuable metals from red mud, including pyrometallurgical recovery, wet leaching recovery, and emerging biobased technology recovery. We investigate the underlying principles, processes, research progress, and the potential for industrial application of these methods, and assess the advantages and disadvantages of each from the perspectives of economic and environmental benefits. Although these methods have certain disadvantages, in general, the recovery of various types of valuable metals from red mud is an effective way to solve the problem of red mud and the supply of metal raw materials. In conclusion, this paper presents an overview of the current state of red mud development and utilization, as well as the various methods employed for the recovery of valuable metals from red mud.

关键词： Red mud Utilization Environment hazard Valuable metal Recovery

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Bimetal MOF-derived NiFe-P nanocomposites coupled with Cu_(3)P nanoparticles to construct tandem electron transfer channels for photocatalytic hydrogen evolution

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Journal of Environmental Sciences 2024年第3期137卷 333-346页

作者： Haiyan zhang Shitao Yang peng Zhu Senpei Tang Ming Li College of Chemistry and Chemical Engineering Jishou UniversityJishou 416000China School of Account Hunan University of Technology and BusinessChangsha 410205China

Finely modulated light-induced charge separation and transfer is a central challenge to achieve efficient *** progress has been made in this field,most of the previous research works focused on the separation or migration of photogenerated carriers but did not build a bridge between the *** to realize the strong driving and precise migration of carriers has become the focus of our *** report an ingeniously designed ternary *** NiFe-MOF as the“parent material”,the FeP_(4)/Ni_(x)P_(y)heterojunction is derived in situ while maintaining the frame structure through gas-solid reaction,and finally the Z-type electron transfer is *** Cu_(3)P anchoring spindle matrix,an electron transport tunnel is opened up in Cu_(3)P/FeP_(4)/Ni_(x)P_(y)ternary heterojunction under the action of p-n heterojunction built-in electric field driving and accurate energy band *** strong driving force of the built-in electric field provides an inexhaustible power for the transmission of electrons,and the fine series of electron transmission channels realizes the precise transmission of *** above fine design makes the perfect fit between the built-in electric field and the electron transfer channel,which not only effectively improves the embarrassing situation of insufficient electron driving force of hydrogen evolution reaction in the previous research,but also makes up for the weakening of semi-conductor reduction ability caused by the construction of traditional p-n *** research work provides a new idea for the construction of multiple heterostructures and the design of fine interface engineering in the future.

关键词： Cu_(3)P/FeP_(4)/Ni_(x)P Built-in electric field Electron transfer channels Photocatalysis

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Assessment of piloting behavior impact on landing risk of transport aircraft

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Chinese Journal of Aeronautics 2024年第9期37卷 178-192页

作者： Zhiyue XIONG Shuguang zhang Mingkai WANG peng TANG Mengmeng WANG School of Transportation Science and Engineering Beihang UniversityBeijing 102206China

The human factors and their interaction with other factors play an important role in the flight safety of transport *** this paper,a paradigm of risk assessment for transport aircraft interacting with piloting behaviors is proposed,with focus on landing which is the most accident-prone flight stage in aviation safety ***-based flight simulation serves as our data source for landing risk analysis under uncertainties.A digital pilot in the loop that reflects the human piloting behaviors is employed to facilitate simulation *** types of unsafe events in landing are identified from *** this basis,the landing safety boundary is extracted via stochastic simulation to divide safety and hazardous flight status domains,which con-tributes to flight status management and risk *** simulation results indicate that appro-priate piloting behavior,which is active response and fast target acquisition with minimum overshoot and fluctuation,shows benefit to landing *** subset simulation technique is employed to further refine the boundary with less computational ***,the effect of airspeed,windspeed,and other factors on landing risk is also *** proposed risk assess-ment method would help optimize operation procedure and develop targeted pilot training program.

关键词： Landing risk assessment Risk parameterization Human factors Piloting behavior model Landing safety boundary Subset simulation

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Glucose-sensitive Membrane with PBA-based Contraction-type Linear Polymer as Chemical Valves Prepared by Surface Grafting

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Chinese Journal of Polymer Science 2024年第8期42卷 1067-1076页

作者： Chun-peng zhang Si-Jia Gao Ying Luo Lei Zou Yong-Jun zhang State Key Laboratory of Separation Membranes and Membrane Processes School of Material Science and EngineeringTiangong UniversityTianjin 300387China State Key Laboratory of Separation Membranes and Membrane Processes School of Pharmaceutical SciencesTiangong UniversityTianjin 300387China Tianjin Key Laboratory of Extracorporeal Life Support for Critical Diseases Institute of Hepatobiliary DiseaseNankai University Affiliated Third Center HospitalTianjin 300170China Cangzhou Institute of Tiangong University Cangzhou 061000China

Glucose-sensitive membrane has potential application in self-regulating insulin *** acid(PBA)is a well-known glucose ***,most PBA-based glucose-sensitive materials are expansion-type,which are not suitable as chemical valves in membrane pores for self-regulating insulin *** to a new glucose-sensitive mechanism,we synthesized PBA-based contraction-type glucose-sensitive liner polymer and ***,a glucose-sensitive membrane was prepared by grafting PBA-based contraction-type glucose-sensitive linear polymer on the membrane *** adjusting the chain length and chain density,the glucose-sensitivity of the membrane was *** membrane can reversibly regulate insulin release at physiologically relevant glucose concentrations in simulates body fluids and fetal bovine *** membrane also has good stability,anti-fouling and biocom *** has potential application in selfregulating insulin release.

关键词： Phenylboronic acid Glucose-sensitive Membrane Surface grafting Insulin

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Explainable Neural Network for Sensitivity Analysis of Lithium-ion Battery Smart Production

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IEEE/CAA Journal of Automatica Sinica 2024年第9期11卷 1944-1953页

作者： Kailong Liu Qiao peng Yuhang Liu Naxin Cui Chenghui zhang School of Control Science and Engineering Shandong UniversityJinan 250061China Information Technology Analytics&Operations groupQueen’s University BelfastBelfast BT71NNUK

Battery production is crucial for determining the quality of electrode,which in turn affects the manufactured battery *** battery production is complicated with strongly coupled intermediate and control parameters,an efficient solution that can perform a reliable sensitivity analysis of the production terms of interest and forecast key battery properties in the early production phase is urgently *** paper performs detailed sensitivity analysis of key production terms on determining the properties of manufactured battery electrode via advanced data-driven *** be specific,an explainable neural network named generalized additive model with structured interaction(GAM-SI)is designed to predict two key battery properties,including electrode mass loading and porosity,while the effects of four early production terms on manufactured batteries are explained and *** experimental results reveal that the proposed method is able to accurately predict battery electrode properties in the mixing and coating *** addition,the importance ratio ranking,global interpretation and local interpretation of both the main effects and pairwise interactions can be effectively visualized by the designed neural *** to the merits of interpretability,the proposed GAM-SI can help engineers gain important insights for understanding complicated production behavior,further benefitting smart battery production.

关键词： Battery management battery manufacturing data science explainable artificial intelligence sensitivity analysis

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Contact engineering for temperature stability improvement of Bi-contacted MoS2 field effect transistors

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Science China(Information Sciences) 2024年第06期67卷 172-179页

作者： Zizheng LIU Qing zhang Xiaohe HUANG Chunsen LIU peng ZHOU State Key Laboratory of Integrated Chip and Systems School of MicroelectronicsZhangjiang Fudan International Innovation CenterFudan University Frontier Institute of Chip and System Shanghai Key Lab for Future Computing Hardware and SystemFudan University Shaoxin Laboratory

Semimetallic bismuth（Bi） is one of the most effective strategies for reducing the contact resistance of two-dimensional transition metal dichalcogenide field effect transistors（FETs）. However, the low melting point of Bi contact（271.5℃） limits its reliable applications. In this study, we demonstrated that the temperature stability of Bi-contacted electrodes could be improved by inserting a high-melting point semimetallic antimony（Sb） between the Bi contacting layer and the gold（Au） capping layer. The proposed Bi/Sb/Au contact electrodes tended to form a metal mixture with a continuous surface during the heating process（Voids appeared on the surface of the Bi/Au contact electrodes after heating at 120℃）. Because of the improved contacting layer formed by the semimetal Bi/Sb alloy, the fabricated Bi/Sb/Au-contacted molybdenum sulfide（MoS2） FETs with different gate lengths demonstrated higher on-state current stability after heating treatment than the Bi/Au contact. Because of the Bi/Sb/Au contact and poly（methyl methacrylate） package, the MoS2FETs demonstrated time stability of at least two months from the almost unchanged transfer characteristics. The electrical stability indicates that the insertion of semimetallic Sb is a promising technology for reliable Bi-based contact.

关键词： temperature stability semimetallic bismuth contact semimetallic antimony contact MoS2 FETs time stability

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Application of magnetotactic bacteria as engineering microrobots:Higher delivery efficiency of antitumor medicine

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Chinese Chemical Letters 2024年第10期35卷 139-146页

作者： Jing zhang Charles Wang Yaoyao zhang Haining Xia Yujuan Wang kun Ma junfeng Wang High Magnetic Field Laboratory CAS Key Laboratory of High Magnetic Field and lon Beam Physical BiologyHefei Institutes of Physical ScienceChinese Academy of SciencesHefei 230031China University of Science and Technology of China Hefei 230026China University of California San DiegoLa JollaCA 92093United States International Magnetobiology Frontier Research Center Hefei 230031China

For a significant duration,enhancing the efficacy of cancer therapy has remained a critical *** bacteria(MTB),often likened to micro-robots,hold substantial promise as a drug delivery ***,classified as anaerobic,aquatic,and gram-negative microorganisms,exhibit remarkable motility and precise control over their internal biomineralization *** unique ability results in the formation of magnetic nanoparticles arranged along filamentous structures in a catenary fashion,enclosed within a *** bacteria possess distinctive biochemical properties that facilitate their precise positioning within complex *** harnessing these biochemical attributes,MTB could potentially offer substantial advantages in the realm of cancer *** article reviews the drug delivery capabilities of MTB in tumor treatment and explores various applications based on their inherent *** objective is to provide a comprehensive understanding of MTB-driven drug delivery and stimulate innovative insights in this field.

关键词： Magnetotactic bacteria Engineering microrobot Tumor treatment Drug delivery Bioconjugation

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Machining dynamics and chatters in micro-milling:A critical review on the state-of-the-art and future perspectives

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Chinese Journal of Aeronautics 2024年第7期37卷 59-80页

作者： Qingshun BAI peng WANG Kai CHENG Liang ZHAO Yabo zhang School of Mechanical and Electrical Engineering Harbin Institute of TechnologyHarbin 150001China Department of Mechanical and Aerospace Engineering Brunel University LondonUxbridge UB83PHUK

Micro-milling technology is widely applied in micro manufacturing,particularly for the fabrication of miniature and micro ***,the chatters and machining dynamics related issues in micro-milling are often the main challenges restricting its machining quality and *** research works have rendered that the machining dynamics and chatters in micro-milling are more complex compared with the conventional macro-milling process,likely because of the size effect and rigidity of the micro-milling system including the tooling,workpiece,process variables,materials involved,and the high-speed milling machines,and further their collective dynamic ***,in this paper,the state of the art focusing on micro-milling chatters and dynamics related issues over the past years are comprehensively and critically reviewed to provide some insights for potential researchers and ***,typical applications and the problems caused by the machining dynamics and chatters in micro-milling have been put forward in this ***,the research on the underlying micro-cutting mechanics and dynamics,stability analysis,chatters detection,and chatter suppression are summarized ***,the underlying scientific and technological challenges are discussed particularly against typical precision engineering ***,the possible future directions and trends in research and development of micro-milling have been discussed.

关键词： Micro-milling Machining dynamics Micro-cutting mechanics Stability lobe diagram(SLD) Chatters suppression Digital twin

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Structure characterization of the oxide film on FGH96 superalloy powders with various oxidation degrees

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International Journal of Minerals,Metallurgy and Materials 2024年第9期31卷 2037-2047页

作者： Yang Liu Yufeng Liu Sha zhang Lin zhang peng zhang Shaorong zhang Na Liu Zhou Li Xuanhui Qu Beijing Advanced Innovation Center for Materials Genome Engineering Institute for Advanced Materials and TechnologyUniversity of Science and Technology BeijingBeijing 100083China Institute of Materials Intelligent Technology Liaoning Academy of MaterialsShenyang 110004China Science and Technology on Advanced High Temperature Structural Materials Laboratory AECC Beijing Institute of Aeronautical MaterialsBeijing 100095China

The structure of the oxide film on FGH96 alloy powders significantly influences the mechanical properties of *** this study,FGH96 alloy powders with various oxygen contents were investigated using high-resolution transmission electron microscopy and atomic probe technology to elucidate the structure evolution of the oxide *** dispersive spectrometer analysis revealed the presence of two distinct components in the oxide film of the alloy powders:amorphous oxide layer covering the γ matrix and amorphous oxide particles above the *** alloying elements within the oxide layer showed a laminated distribution,with Ni,Co,Cr,and Al/Ti,which was attributed to the decreasing oxygen equilibrium pressure as oxygen diffused from the surface into the γ *** the other hand,Ti enrichment was observed in the oxide particles caused by the oxidation and decomposition of the carbide *** analysis of the oxide film with oxygen contents of 140,280,and 340 ppm showed similar element distributions,while the thickness of the oxide film varies approximately at 9,14,and 30 nm,*** findings provide valuable insights into the structural analysis of the oxide film on FGH96 alloy powders.

关键词： Ni-based superalloys surface structure oxide layer thickness oxidation behavior element distribution

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