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Enhanced energy storage properties and good stability of novel(1-x)Na_(0.5)Bi_(0.5)TiO_(3)-xCa(Mg_(1/3)Nb_(2/3))O_(3) relaxor ferroelectric ceramics prepared by chemical modification

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Journal of Materiomics 2024年第4期10卷 770-782页

作者： Ying zhang Meng-Han Yan Zhi-Fei zhang Hai-Rui Bai Peng Li Wei-Fang Han Ji-Gong Hao Wei Li Yu-Chao Li chun-Ming Wang Peng fu School of Materials Science and Engineering Liaocheng UniversityLiaocheng252059China Shandong Laboratory of Yantai Advanced Materials and Green Manufacturing 300 Changjiang RoadYantai264006China School of Physics Shandong UniversityJinan250100China

The increase in energy consumption and its collateral damage on the environment has encouraged the development of environment-friendly ceramic materials with good energy storage *** this work,(1-x)Na_(0.5)Bi_(0.5)TiO_(3)-xCa(Mg_(1/3)Nb_(2/3))O_(3) ceramics were synthesized by the solid-state reaction *** 0.88Na_(0.5)Bi_(0.5)TiO_(3)-0.12Ca(Mg_(1/3)Nb_(2/3))O_(3) ceramic exhibited a high recoverable energy storage density of 8.1 J/cm3 and energy storage efficiency of 82.4% at 550 kV/*** introduction of Ca(Mg_(1/3)Nb_(2/3))O_(3) reduced the grain size and increased the band gap,thereby enhancing the breakdown field strength of the ceramic *** method also resulted in good temperature stability(20–140℃),frequency stability(1–200 Hz),and fatigue stability over 106 *** addition,an ultrahigh power density of 187 MW/cm^(3) and a fast charge-discharge rate(t0.9=57.2 ns)can be obtained *** element method analysis revealed that the decrease of grain size was beneficial to the increase of breakdown field ***,the 0.88Na_(0.5)Bi_(0.5)TiO_(3)-0.12Ca(Mg_(1/3)Nb_(2/3))O_(3) ceramics resulted in high energy storage properties with good stability and were promising environment-friendly materials for advanced pulsed power systems applications.

关键词： (1-x)Na_(0.5)Bi_(0.5)TiO_(3)-xCa(Mg_(1/3)Nb_(2/3))O_(3)ceramics Relaxor ferroelectrics Breakdown field strength Energy storage properties Stability

Off-farm employment,agriculture production activities,and household dietary diversity in environmentally and economically vulnerable areas of Asia

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Journal of Integrative Agriculture 2024年第2期23卷 359-373页

作者： Yunli Bai Xuanye Zeng Chao fu Linxiu zhang Key Laboratory of Ecosystem Network Observation and Modeling Institute of Geographic Sciences and Natural Resources ResearchChinese Academy of SciencesBeijing 100101China United Nations Environment Programme-International Ecosystem Management Partnership(UNEP-IEMP) Beijing 100101China University of Chinese Academy of Sciences Beijing 100101China

Access to off-farm employment has been expected to be a critical approach to ending hunger and all forms of malnutrition,two important targets of achieving Zero *** study aims to investigate the role of off-farm employment in improving dietary diversity through substitution effect and complementary effect with agricultural production activities and income *** study adopts Poisson/Tobit/Probit/OLS regressions and the instrument variable method based on the primary survey data collected among 1,282 households at 12 sites in environmentally and economically vulnerable areas of China,Nepal,Cambodia,Thailand,and Myanmar in *** results show that off-farm employment is positively associated with household dietary diversity and the consumption of flesh meat,fish and other aquatic animals,fruits,and milk and dairy products,which are rich in protein and *** results of mechanism analysis show that off-farm employment contributes to household dietary diversity by improving crop diversity,especially for poor households,boosting the probability of livestock raising for households with the middle one-third disposal income,and increasing household *** positive association between off-farm employment and household dietary diversity is much higher for households with the bottom one-third disposal income,low illiteracy,and from upper-middle income *** findings imply that off-farm employment does play a vital role in achieving multiple benefits of poverty alleviation,malnutrition reduction,and agrobiodiversity conservation in environmentally and economically vulnerable ***,it may enlarge the gaps in dietary diversity between households with low human capital and from low and lower-middle income countries and those with high human capital and from middle-high countries.

关键词： off-farm employment dietary diversity income effect substitution effect complementary effect

3D printed grafts with gradient structures for organized vascular regeneration

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International Journal of Extreme Manufacturing 2024年第3期6卷 505-520页

作者： Yuewei Chen Zhongfei Zou Tao fu Zhuang Li Zhaojie zhang Meng Zhu Qing Gao Shaofei Wu Guosheng fu Yong He Jiayin fu State Key Laboratory of Fluid Power and Mechatronic Systems School of Mechanical EngineeringZhejiang UniversityHangzhou 310027People’s Republic of China School of Mechanical Engineering Guizhou UniversityGuiyang 550025People’s Republic of China Key Laboratory of Cardiovascular Intervention and Regenerative Medicine of Zhejiang Province Department of CardiologySir Run Run Shaw HospitalZhejiang UniversityHangzhou 310016People’s Republic of China School of Mechanical Engineering Guizhou Institute of TechnologyGuiyang 550003People’s Republic of China Department of Oral and Maxillofacial Surgery The Second Affiliated Hospital of Zhejiang University School of MedicineSchool of Stomatologyand Key Laboratory of Oral Biomedical Research of Zhejiang ProvinceHangzhouZhejiang 310006People’s Republic of China

Synthetic vascular grafts suitable for small-diameter arteries(<6 mm) are in great ***,there are still no commercially available small-diameter vascular grafts(SDVGs) in clinical practice due to thrombosis and stenosis after in vivo *** designing SDVGs,many studies emphasized reendothelization but ignored the importance of reconstruction of the smooth muscle layer(SML).To facilitate rapid SML regeneration,a high-resolution 3D printing method was used to create a novel bilayer SDVG with structures and mechanical properties mimicking natural *** by the collagen alignment of SML,the inner layer of the grafts had larger pore sizes and high porosity to accelerate the infiltration of cells and their circumferential alignment,which could facilitate SML reconstruction for compliance restoration and spontaneous *** outer layer was designed to induce fibroblast recruitment by low porosity and minor pore size and provide SDVG with sufficient mechanical *** month after implantation,the arteries regenerated by 3D-printed grafts exhibited better pulsatility than electrospun grafts,with a compliance(8.9%) approaching that of natural arteries(11.36%) and significantly higher than that of electrospun ones(1.9%).The 3D-printed vascular demonstrated a three-layer structure more closely resembling natural arteries while electrospun grafts showed incomplete endothelium and immature *** study shows the importance of SML reconstruction during vascular graft regeneration and provides an effective strategy to reconstruct blood vessels through 3D-printed structures rapidly.

关键词： small-diameter vascular graft smooth muscle layer 3D printing endothelialization

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Co掺杂闪锌矿ZnO的磁性和光学性质

发光学报 2015年第5期36卷 508-514页

作者：张富春崔红卫延安大学物理与电子信息学院陕西延安716000

采用自旋极化密度泛函理论方法对Co掺杂闪锌矿Zn O的能带结构、态密度、磁学和光学属性进行了研究。计算结果显示:Co掺杂闪锌矿Zn O的基态是反铁磁态,具有金属性特征;而铁磁态具有半金属性特征。铁磁耦合在费米能级附近出现了明显的自... 详细信息

采用自旋极化密度泛函理论方法对Co掺杂闪锌矿Zn O的能带结构、态密度、磁学和光学属性进行了研究。计算结果显示:Co掺杂闪锌矿Zn O的基态是反铁磁态,具有金属性特征;而铁磁态具有半金属性特征。铁磁耦合在费米能级附近出现了明显的自旋劈裂现象,表现出明显的不对称性和强烈的Co 3d和O 2p杂化效应。磁矩主要来源于Co 3d轨道电子以及部分近邻耦合的O 2p轨道电子,大小与Co原子的掺杂位置有关。光学性质计算结果显示,Co掺杂闪锌矿Zn O在可见光范围内都有较强的光吸收能力,吸收峰在高能区发生了红移现象。理论计算结果表明,Co掺杂闪锌矿Zn O或许是一种优异的磁光材料。

关键词： Co掺杂闪锌矿ZnO 第一性原理铁磁和反铁磁光学性质

Proteomics Study of Benzene Metabolite Hydroquinone Induced Hematotoxicity in K562 Cells

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Biomedical and Environmental Sciences 2024年第4期37卷 341-353页

作者： JIN Yi Shan YI Zong chun zhang Yu Jing RONG Long YU chun Hong School of Biological Science and Medical Engineering Beihang UniversityBeijing 100191China School of Engineering Medicine Beihang UniversityBeijing 100191China

Objective Hydroquinone(HQ),one of the phenolic metabolites of benzene,is widely recognized as an important participant in benzene-induced ***,there are few relevant proteomics in HQ-induced hematotoxicity and the mechanism hasn’t been fully understood *** In this study,we treated K562 cells with 40μmol/L HQ for 72 h,examined and validated protein expression changes by Label-free proteomic analysis and Parallel reaction monitoring(PRM),and performed bioinformatics analysis to identify interaction *** One hundred and eighty-seven upregulated differentially expressed proteins(DEPs)and 279 downregulated DEPs were identified in HQ-exposed K562 cells,which were involved in neutrophilmediated immunity,blood microparticle,and other GO terms,as well as the lysosome,metabolic,cell cycle,and cellular senescence-related *** on the 23 DEGs and 5 DEPs in erythroid differentiation-related pathways,we constructed the network of protein interactions and determined 6 DEPs(STAT1,STAT3,CASP3,KIT,STAT5B,and VEGFA)as main hub proteins with the most interactions,among which STATs made a central impact and may be potential biomarkers of HQ-induced *** Our work reinforced the use of proteomics and bioinformatic approaches to advance knowledge on molecular mechanisms of HQ-induced hematotoxicity at the protein level and provide a valuable basis for further clarification.

关键词： Hydroquinone Proteomics Hematotoxicity K562 cells

Ni-catalyzed highly regio- and stereo-selective diborylative cyclization of 1,6-enynes with diboron reagent

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Science China Chemistry 2024年第3期67卷 981-989页

作者： Qitao Guan Zhen Shen Yiqiang Tian Genping Huang chun zhang Institute of Molecular Plus Tianjin Key Laboratory of Molecular Optoelectronic ScienceDepartment of ChemistrySchool of SciencesTianjin UniversityTianjin 300072China State Key Laboratory of Elemento-Organic Chemistry Nankai UniversityTianjin 300071China

The Ni-catalyzed highly selective diborylative cyclization of 1,6-enynes with diboron reagent has been developed. When pinB-Bdan was used, multiple types of boron-containing functional groups could be installed into organic molecule with great chemoselectivity and regioselectivity though this reaction. Meanwhile, if B_2pai_2 was employed, the asymmetric diborylative cyclization could be well induced by using strategy of dynamic kinetic resolution. Importantly, the above reactions could afford desired product with 100% atomic economy, and could be compatible with different series of substituents. The studies of further transformation well illustrated that different type products could serve diverse synthetic strategy. Notably, the reaction mechanism was intensively studied by density functional theory(DFT) calculations, which could reveal the mechanism of regio- and enantio-selective control.

关键词： nickel-catalyzed organoboron cyclization regioselectivity enantioselectivity

Special issue on electrochemical conversion and utilization of hydrogen energy

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Frontiers in Energy 2024年第3期18卷 263-264页

作者： Yun ZHENG Bo YU Xiaogang fu Jiujun zhang Institute of New Energy Materials and Engineering School of Materials Science and EngineeringFuzhou UniversityFuzhou 350108China State Key Laboratory of Solidification Processing Atomic Control&Catalysis Engineering LaboratorySchool of Materials Science and EngineeringNorthwestern Polytechnical UniversityXi’an 710072China Institute of Nuclear and New Energy Technology Tsinghua UniversityBeijing 100084China

The concerns over energy crisis and climate change caused by the excessive consumption of fossil fuels and the associated emission of greenhouse gases, have driven many countries to develop policies for an energy transition into zero-carbon energy sources, essentially aiming at decarbonizing their energy systems. Among various renewable sources, hydrogen has been hailed as an ideal alternative to provide secure, cost-effective, and non-polluting energy. In recent years, there has been noteworthy progress in hydrogen electrochemical conversion and utilization techniques and devices, including water electrolyzers, proton-exchange membrane fuel cells (PEMFCs), solid oxide fuel cells (SOFCs), etc. Each of these technologies has yielded a series of encouraging advances. To showcase these recent advances, Frontiers in Energy is launching a special issue titled “electrochemical conversion and utilization of hydrogen energy”.

关键词： hydrogen energy. electrochemical

Deep learning CNN-APSO-LSSVM hybrid fusion model for feature optimization and gas-bearing prediction

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Petroleum Science 2024年第4期21卷 2329-2344页

作者： Jiu-Qiang Yang Nian-Tian Lin Kai zhang Yan Cui Chao fu Dong zhang College of Earth Sciences and Engineering Shandong University of Science and Technology Laboratory for Marine Mineral Resources Qingdao National Laboratory for Marine Science and Technology Transportation Institute of Inner Mongolia University Key Laboratory of Gas Hydrate Qingdao Institute of Marine Geology Ministry of Natural Resources

Conventional machine learning(CML) methods have been successfully applied for gas reservoir prediction. Their prediction accuracy largely depends on the quality of the sample data; therefore, feature optimization of the input samples is particularly important. Commonly used feature optimization methods increase the interpretability of gas reservoirs; however, their steps are cumbersome, and the selected features cannot sufficiently guide CML models to mine the intrinsic features of sample data efficiently. In contrast to CML methods, deep learning(DL) methods can directly extract the important features of targets from raw data. Therefore, this study proposes a feature optimization and gas-bearing prediction method based on a hybrid fusion model that combines a convolutional neural network(CNN)and an adaptive particle swarm optimization-least squares support vector machine(APSO-LSSVM). This model adopts an end-to-end algorithm structure to directly extract features from sensitive multicomponent seismic attributes, considerably simplifying the feature optimization. A CNN was used for feature optimization to highlight sensitive gas reservoir information. APSO-LSSVM was used to fully learn the relationship between the features extracted by the CNN to obtain the prediction results. The constructed hybrid fusion model improves gas-bearing prediction accuracy through two processes of feature optimization and intelligent prediction, giving full play to the advantages of DL and CML methods. The prediction results obtained are better than those of a single CNN model or APSO-LSSVM model. In the feature optimization process of multicomponent seismic attribute data, CNN has demonstrated better gas reservoir feature extraction capabilities than commonly used attribute optimization methods. In the prediction process, the APSO-LSSVM model can learn the gas reservoir characteristics better than the LSSVM model and has a higher prediction accuracy. The constructed CNN-APSO-LSSVM mode

关键词： Multicomponent seismic data Deep learning Adaptive particle swarm optimization Convolutional neural network Least squares support vector machine Feature optimization Gas-bearing distribution prediction

A Radiative-Cooling Hierarchical Aligned Porous Poly(vinylidene fluoride)Film by Freeze-Thaw-Promoted Nonsolvent-Induced Phase Separation

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Chinese Journal of Polymer Science 2024年第7期42卷 976-983,I0009页

作者： Yiting zhang Jiahui Sun Yufeng Wang Yunchen Wu chun Huang Chao zhang Tianxi Liu Key Laboratory of Synthetic and Biological Colloids Ministry of Education School of Chemical and Material EngineeringJiangnan UniversityWuxi214122China State Key Laboratory for Modification of Chemical Fibers and Polymer Materials College of Materials Science and EngineeringDonghua UniversityShanghai201620China

Passive daytime radiative cooling(PDRC)is an innovative and sustainable cooling technology that holds immense potential for addressing the energy *** the numerous reports on radiative coolers,the design of a straightforward,efficient,and readily producible system remains a ***,we present the development of a hierarchical aligned porous poly(vinylidene fluoride)(HAP-PVDF)film through a freeze-thaw-promoted nonsolvent-induced phase separation *** film features oriented microporous arrays in conjunction with random nanopores,enabling efficient radiative cooling performance under direct sunlight *** incorporation of both micro-and nano-pores in the HAP-PVDF film results in a remarkable solar reflectance of 97%and a sufficiently high infrared thermal emissivity of 96%,facilitating sub-environmental cooling at 18.3℃ on sunny days and 13.1℃ on cloudy ***,the HAP-PVDF film also exhibits exceptional flexibility and *** calculations further confirm a radiative cooling power of 94.8 W·m^(-2)under a solar intensity of 1000W·m^(-2),demonstrating a performance comparable to the majority of reported radiative coolers.

关键词： Daytime radiative cooling Hierarchical porosity PVDF porous film Thermal insulation Nonsolvent-induced phase separation