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Changes of nutrients and microbial communities in recovery process of abandoned rare earth tailings

Pedosphere 2024年第4期34卷 826-836页

作者： bing zhang Junli WU Mengyuan HUANG Yan zhang Jin ZHAO Chuntao HE Zhongyi YANG School of Environmental Science and Engineering Sun Yat-sen UniversityGuangzhou 510006China School of Life Sciences Sun Yat-sen UniversityGuangzhou 510275China School of Agriculture State Key Laboratory for BiocontrolShenzhen Campus of Sun Yat-sen UniversitySun Yat-sen UniversityShenzhen 518107China

Rare earth element(REE)mining has wrought severe ecosystem destruction,particularly in the loss of carbon(C),nitrogen(N),and phosphorus(P).Furthermore,its effects on nutrient recovery characteristics and associated microbial abundance are still poorly *** this study,an investigation was conducted to determine C,N,and P recovery patterns and microbial communities in abandoned REE mining tailings with different abandoned durations of 1.5(1.5-Y),7(7-Y),10(10-Y),and 14(14-Y)years and at an unmined site(the control group)in Jiangxi Province,*** tailing delamination at each site was investigated in 0–15(layer 1)and 15–30(layer 2)cm tailing *** the abandoned duration of REE tailings,C and P in layer 1 continued to recover from 1.62 to 8.51 g kg^(-1) and from 0.71 to 1.94 g kg^(-1),respectively;N losses of 0.60 and 0.22 g kg^(-1) occurred at the 1.5-Y and 10-Y sites,while N in layer 1 slightly increased at the 14-Y ***,Methylosinus,Bradyrhizobium,Pseudomonas,and Azospirillum were dominant bacteria at the 14-Y site and in the *** relative abundances of N-fixing bacteria Mesorhizobium(32.94%),Sinorhizobium(0.24%),Frankia(0.71%),and Burkholderia(2.38%)at the 14-Y site were 1.33–3.97 times those in the control(24.19%,0.18%,0.32%and 0.60%,respectively),which was helpful for tailing N *** the 14-Y site,Tylospora(50.24%),Luellia(11.02%),Tomentella(6.94%),and Chaetomium(4.34%)were the dominant fungal genera,while Tylospora(56.93%),Suillus(11.45%),and Penicillium(6.78%)predominated in the *** relative abundance of the P-dissolving fungus Aspergillus at the 14-Y site(0.42%)was 4.2 times that in the control(0.1%),which may lead to the improved tailing P *** the 14-Y site,woody plants such as Pinus massoniana and native pioneering herbs and ferns such as Dicranopteris dichotoma and Nephrolepis auriculata probably invaded from adjacent *** study unraveled the natural restoration of plant and micro

关键词： abandoned duration mining tailing N-fixing bacteria nutrient recovery P-solubilizing fungi rare earth element

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Online preparation of high-quality BN coatings with atomic diffusion based on carbon-free water-soluble precursor

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Journal of Advanced Ceramics 2024年第3期13卷 272-281页

作者： Yiang Du bing Wang Yunbo zhang Quzhi Song Fuwen Wang Cheng Han Xiaoshan zhang yingde Wang Science and Technology on Advanced Ceramic Fibers and Composites Laboratory College of Aerospace Science and EngineeringNational University of Defense TechnologyChangsha 410073China

Efficient and environmentally friendly production of high-quality continuous fiber coatings using current preparation methods is highly challenging due to issues such as scale and batch processing restrictions,low deposition rate,high energy consumption,and utilization of multiple environmentally hazardous *** address these challenges,we propose a stable and efficient wet chemical deposition coating method for high-throughput online continuous preparation of boron nitride(BN)coatings on ceramic fibers under an ambient *** process involves surface modification,in-situ wet chemical deposition,and heat treatment,and all seamlessly connecting with the ceramic fiber preparation process through continuous *** groups were introduced via surface modification enhancing wettability of the fiber surface with impregnating *** in-situ reaction and atom migration improve uniformity and binding of the *** a result,outstanding impregnation and adhesion properties are achieved.A comprehensive analysis to evaluate the impact of the BN coatings was conducted,which demonstrates that the BN-coated fibers exhibit a remarkable 36%increase in tensile strength,a 133%increase in fracture toughness,and enhanced temperature resistance of up to 1600℃.It provides a secure and efficient platform for cost-effective production of functional and high-quality coatings through targeted surface modification and rapid stretching impregnation.

关键词： polymer-derived ceramics SiC fibers wet chemical deposition atomic diffusion boron nitride(BN)coatings

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Experimental study on the CO_(2) concentration and age of air distribution inside tiny sleeping spaces

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Building Simulation 2024年第4期17卷 591-605页

作者： Jingying zhang Yanyan Li Haiguo yin Linfeng Liang Songmei Zu Le Gao ying zhang Angui Li School of Building Services Science and Engineering Xi’an University of Architecture and TechnologyXi’anShaanxi710055China

In recent years,rapid urban development has led to capsule hotels,sleep pods,and other tiny sleeping spaces that adapt to people’s fast-paced lives,achieving maximum functionality with a very small ***,due to the small space,human metabolic pollutant(such as CO_(2))is more likely to accumulate,and the air is not easily *** this paper,a full-size experimental platform is set up with three types of ventilation modes to explore the exclusion efficiency of metabolic pollutants and the overall distribution of age of air under these ventilation *** conclusions showed that the mean values of metabolic pollutant exclusion rates for the different ventilation modalities varied very little across the spatial dimensions of the confined space but varied considerably in the area around the *** double-side attached ventilation method was the most effective in removing human metabolic pollutants,especially in the head region(CN≥0.92),while the single-wall attached ventilation method had the best air exchange efficiency(η≥0.85).This suggests an inconsistent distribution of CO_(2) and age of air,which is contrary to general common *** conclusions of this paper can guide the design of ventilation for tiny sleeping spaces.

关键词： attached ventilation mode human metabolic pollutant indoor air quality air exchange efficiency tiny sleeping spaces

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Dynamic-based model for calculating the boulder impact force in debris flow

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Journal of Mountain Science 2024年第6期21卷 1930-1940页

作者： YANG Chaoping zhang Shaojie yin Yueping YANG Hongjuan WEI Fangqiang State Key Laboratory of Mountain Hazards and Engineering Resilience Institute of Mountain Hazards and EnvironmentChinese Academy of SciencesChengdu 610299China University of Chinese Academy of Sciences Beijing 100049China China Institute of Geological Environment Monitoring Beijing 100081China Chongqing Institute of Green and Intelligent Technology Chinese Academy of SciencesChongqing 400714China Chongqing School University of Chinese Academy of SciencesChongqing 400714China

The boulder impact force in debris flow is generally calculated by static methods such as the cantilever beam ***,these methods cannot describe the dynamic scenario of boulder collision on structures,so the inertia and damping effects of the structures are not involved causing an overestimation on the boulder impact *** order to address this issue,a dynamic-based model for calculating the boulder impact force of a debris flow was proposed in this study,and the dynamic characteristics of a cantilever beam with multiple degrees of freedom under boulder collision were *** using the drop-weight method to simulate boulders within debris flow,seven experiments of drop-weight impacting the cantilever beam were used to calibrate the error of the dynamicbased *** indicate that the dynamic-based model is able to reconstruct the impact force history on the cantilever beam during impact time and the error of dynamic-based model is 15.3%in calculating boulder impact force,significantly outperforming the cantilever beam model’s error of 285%.Therefore,the dynamic-based model can overcome the drawbacks of the static-based models and provide a more reliable theoretical foundation for the engineering design of debris flow control structures.

关键词： Debris flow Impact force Boulder collision Dynamic-based model Engineering design

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Efficient adsorption separation of methane from C_(2)-C_(3) hydrocarbons in a Co(Ⅱ)-nodes metal-organic framework

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Chinese Journal of Chemical Engineering 2024年第5期69卷 192-198页

作者： Jie zhang Xingzhe Guo bing Lin Guangzu Xiong Hanshuang Wang Min zhang Liwen Fan bingwen Li Shuisheng Chen Department of Chemistry and Chemical Engineering Taiyuan Institute of TechnologyTaiyuan 030008China Engineering Research Center of Oligosaccharides Fuyang Normal UniversityFuyang 236041China Shandong Key Laboratory of Biophysics Institute of BiophysicsDezhou UniversityDezhou 253023China

Methane(CH_(4))as a substitute for other mineral fuels plays a crucial role in reducing energy consumption and preventing environmental *** present study employs a solvothermal method to fabricate a porous framework Co-metal-organic framework(Co-MOF)containing two distinct secondary building units(SBUs):an anionic[Co_(2)(μ_(2)-OH)(COO)_(4)(H_(2)O)]and a neutral[CoN_(2)(COO)_(2)].Notably,within the anionic SBUs,the coordinated water molecules induce the generation of divergent unsaturated Co(Ⅱ)centers in the unidirectional porous channels,thereby creating open metal *** adsorption performance of Co-MOF towards pure component gases was systematically *** results demonstrated that Co-MOF exhibits superior adsorption capacity for C_(2)-C_(3) hydrocarbons compared to CH_(4),which offers the potential for efficient adsorption and separation of CH_(4) from C_(2)-C_(3) *** gas selectivity separation ratios of Co-MOF for C_(2)H_(6)/CH_(4) and C_(3)H_8/CH_(4) were calculated using the ideal adsorbed solution theory method at 273/298 K and 0.1 *** results revealed that Co-MOF achieved remarkable equilibrium separation selectivity for CH_(4) and C_(2)-C_(3) hydrocarbon gases among non-modified MOFs,signifying the potential of the synthesized Co-MOF for efficient recovery and purification of CH_(4) from C_(2)-C_(3) *** experiments further demonstrate the ability of Co-MOF to purify methane from C_(2)-C_(3) hydrocarbons in practical gas separation ***,molecular simulation calculations further substantiate the propensity of anionic SBUs to interact with C_(2)-C_(3) hydrocarbon *** study provides a novel paradigm for the development of porous MOF materials in the application of gas mixture separation.

关键词： Co-MOF Separation hydrocarbons Dynamic breakthrough curves Molecular simulations adsorbent Monte Carlo simulation

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Manipulating Crystal Growth and Secondary Phase PbI_(2)to Enable Efficient and Stable Perovskite Solar Cells with Natural Additives

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Nano-Micro Letters 2024年第9期16卷 432-448页

作者： Yirong Wang Yaohui Cheng Chunchun yin Jinming zhang Jingxuan You Jizheng Wang Jinfeng Wang Jun zhang Institute of Chemistry Chinese Academy of Sciences(CAS)Beijing 100190People’s Republic of China University of Chinese Academy of Sciences Beijing 100049People’s Republic of China Nanjing University Nanjing 210023People’s Republic of China Wuhan Textile University Wuhan 430200People’s Republic of China

In perovskite solar cells(PSCs),the inherent defects of perovskite film and the random distribution of excess lead iodide(PbI_(2))prevent the improvement of efficiency and ***,natural cellulose is used as the raw material to design a series of cellulose derivatives for perovskite crystallization *** cationic cellulose derivative C-Im-CN with cyano-imidazolium(Im-CN)cation and chloride anion prominently promotes the crystallization process,grain growth,and directional orientation of ***,excess PbI_(2)is transferred to the surface of perovskite grains or formed plate-like crystallites in local *** effects result in suppressing defect formation,decreasing grain boundaries,enhancing carrier extraction,inhibiting non-radiative recombination,and dramatically prolonging carrier ***,the PSCs exhibit a high power conversion efficiency of 24.71%.Moreover,C-Im-CN has multiple interaction sites and polymer skeleton,so the unencapsulated PSCs maintain above 91.3%of their initial efficiencies after 3000 h of continuous operation in a conventional air atmosphere and have good stability under high humidity *** utilization of biopolymers with excellent structure-designability to manage the perovskite opens a state-of-the-art avenue for manufacturing and improving PSCs.

关键词： Perovskite Solar cells Defect passivation Biomass additives Crystal orientation

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Developmental toxicity assessment of neonicotinoids and organophosphate esters with a human embryonic stem cell-and metabolism-based fast-screening model

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Journal of Environmental Sciences 2024年第3期137卷 370-381页

作者： Shuxian zhang Miaomiao Zhao Shichang Li Renjun Yang Nuoya yin Francesco Faiola State Key Laboratory of Environmental Chemistry and Ecotoxicology Research Center for Eco-Environmental SciencesChinese Academy of SciencesBeijing 100085China College of Resources and Environment University of Chinese Academy of SciencesBeijing 100049China

In recent years,neonicotinoids(NEOs)and organophosphate esters(OPEs)have been widely used as substitutes for traditional pesticides and brominated fame-retardants,*** studies have shown that those compounds can be frequently detected in environmental and human samples,are able to penetrate the placental barrier,and are toxic to ***,it is reasonable to speculate that NEOs and OPEs may have potential adverse effects in humans,especially during *** employed a human embryonic stem cell differentiation-and liver S9 fraction metabolism-based fast screening model to assess the potential embryonic toxicity of those two types of *** show that four NEO and five OPE prototypes targeted mostly ectoderm specification,as neural ectoderm and neural crest genes were down-regulated,and surface ectoderm and placode markers *** liver S9 fraction's treatment could generally reduce the effects of the chemicals,except in a few specific instances,indicating the liver may detoxify NEOs and *** findings suggest that NEOs and OPEs interfere with human early embryonic development.

关键词： Neonicotinoids Organophosphate esters Human embryonic stem cells Fast screening model Developmental toxicity

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Insight into the Role and Evidence of Oxygen Vacancies in Porous Single-Crystalline Oxide to Enhance Catalytic Activity and Durability

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Research 2024年第2期2023卷 675-683页

作者： Lingting Ye Jiaming Ma Jie zhang Wen yin Yuanguang Xia Kui Xie Key Laboratory of Optoelectronic Materials Chemistry and Physics Fujan Institute of Research on the Structure of MatterChinese Academy of SciencesFuzhouFujian 350002China Fujian Science&Technology Innovation Laboratory for Optoelectronic Information of China FuzhouFujian 350108China Advanced Energy Science and Technology Guangdong Laboratory 29 Sanxin North RoadHuizhouGuangdong 116023China Spallation Neutron Source Science Center DongguanGuangdong 523803China

Introducing and stabilizing oxygen vacancies in oxide catalysts is considered to be a promising strategy for improving catalytic activity and ***,we quantitatively create oxygen vacancies in the lattice of porous single-crystallineβ-Ga_(2)O_(3)monoliths by reduction treatments and stabilize them through the long-range ordering of crystal lattice to enhance catalytic activity and *** combination analysis of time-of-flight neutron powder diffraction and extended x-ray absorption fine structure discloses that the preferential generation of oxygen vacancy tends to occur at the site of tetrahedral coordination oxygen ions(O_(Ⅲ)sites),which contributes to the formation of unsaturated Ga-O coordination in the monoclinic *** oxygen vacancies are randomly distributed in lattice even though some of them are present in the form of domain defect in the PSC Ga_(2)O_(3)monoliths after the reduction *** number of oxygen vacancies in the reduced monoliths gives 2.32×10^(13),2.87×10^(13),and 3.45×10^(13)mg^(-1)for the Ga_(2)O_(2.952),Ga_(2)O_(2.895),and Ga_(2)O_(2.880),*** therefore demonstrate the exceptionally high C_(2)H_(4)selectivity of~100%at the C_(2)H_(6)conversion of~37%for nonoxidative dehydrogenation of C_(2)H_(6)to C_(2)H_(4).We further demonstrate the excellent durability even at 620℃for 240 h of continuous operation.

关键词： durability coordination Oxygen

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Bionic lightweight design of limb leg units for hydraulic quadruped robots by additive manufacturing and topology optimization

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Bio-Design and Manufacturing 2024年第1期7卷 1-13页

作者： Huaizhi Zong Junhui zhang Lei Jiang Kun zhang Jun Shen Zhenyu Lu Ke Wang Yanli Wang bing Xu The State Key Laboratory of Fluid Power and Mechatronic Systems Zhejiang UniversityHangzhou 310058China Unmanned Vehicle Research and Development Center China North Vehicle Research InstituteBeijing 100072China School of Mechatronic Engineering Nanchang UniversityNanchang 330031China Auclean High-Tech Ltd. Wuxi 214108China

Galloping cheetahs,climbing mountain goats,and load hauling horses all show desirable locomotion capability,which motivates the development of quadruped *** various quadruped robots,hydraulically driven quadruped robots show great potential in unstructured environments due to their discrete landing positions and large *** the most critical movement unit of a quadruped robot,the limb leg unit(LLU)directly affects movement speed and reliability,and requires a compact and lightweight *** by the dexterous skeleton–muscle systems of cheetahs and humans,this paper proposes a highly integrated bionic actuator system for a better dynamic performance of an *** propose that a cylinder barrel with multiple element interfaces and internal smooth channels is realized using metal additive manufacturing,and hybrid lattice structures are introduced into the lightweight design of the piston *** addition,additive manufacturing and topology optimization are incorporated to reduce the redundant material of the structural parts of the *** mechanical properties of the actuator system are verified by numerical simulation and experiments,and the power density of the actuators is far greater than that of cheetah *** mass of the optimized LLU is reduced by 24.5%,and the optimized LLU shows better response time performance when given a step signal,and presents a good trajectory tracking ability with the increase in motion frequency.

关键词： Additive manufacturing Bionic lightweight design Limb leg unit Quadruped robot Trajectory tracking

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Current collectors' effects on the electrochemical performance of LiNi0.6Co0.2Mn0.2O2 suspension electrodes for lithium slurry battery

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Green Energy & Environment 2024年第8期9卷 1306-1313页

作者： Linshan Peng Yufei Ren Zhaoqiang yin Zhitong Wang Xiangkun Wu Lan zhang CAS Key Laboratory of Green Process and Engineering Beijing Key Laboratory of Ionic Liquids Clean ProcessState Key Laboratory of Multiphase Complex SystemsInstitute of Process EngineeringChinese Academy of Sciences School of Chemical Engineering University of Chinese Academy of Sciences Hefei University Institute of Mechanics Chinese Academy of Sciences Langfang Green Industrial Technology Center

Take after the advantages of lithium-ion battery（LIB） and redox flow battery（RFB）, semi-solid flow battery（SSFB） is a promising electrochemical energy storage device in renewable energy utilization. The flowable slurry electrode realizes decouple of energy and power density,while it also brings about new challenge to SSFBs, electron transport between active material and the out circuit. In this consideration, three types of current collectors（CCs） are applied to study the resistance and electrochemical performances of slurry cathodes within pouch cells for the first time. It proves that the electronic resistance（Re） between slurry electrode and the CC plays a decisive role in SSFB operation, and it is so large when Al foil is adopted that the cell cannot even work. Contact angle between Ketjen black（KB） slurry without active material（AM） and the CC is a preliminarily sign for the Re, the smaller the angle, the lower the resistance, and the better electrochemical performance of the cell.

关键词： Semi-solid flow battery Slurry electrode Current collector Electronic resistance Carbon coated Al

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