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Journal of Modern Power Systems and Clean Energy 2024年第3期12卷 958-970页

作者： Jialiang Wu zh.n wang Ruixu Liu Yu shan Chenxuan wang the College of Electrical Engineering Zhejiang UniversityHangzhou 310027China the Economic Research Institute of State Grid zhejiang Electric Power Co. Ltd.Hangzhou 310016China

Hybrid multi-terminal direct current(MTDC)transmission technology has been a research focus,and primary frequency regulation(FR)improvement in the receiving-end system is one of the problems to be *** paper presents a decentralized primary FR scheme for hybrid MTDC power systems considering multi-source enhancement to help suppress frequency disturbance in the receiving-end *** the converters only need local frequency or DC voltage signal input to respond to system disturbance without communication or a control center,i.e.,a decentralized control *** proposed scheme can activate appropriate power sources to assist in FR in various system disturbance severities with fine-designed thresholds,ensuring sufficient utilization of each power *** better balance FR performance and FR resource participation,an evaluation index is proposed and the parameter optimization problem is further ***,the validity of the proposed scheme is verified by simulations in MATLAB/Simulink.

关键词： Decentralized control scheme primary frequency regulation(FR) rate of change of frequency(ROCOF) system frequency disturbance

Promoted nH_(3)-SCR activity and hydrothermal stability of Cu-SSZ-50 catalyst synthesized by one-pot method

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Chinese Chemical Letters 2024年第3期35卷 135-139页

作者： Jinpeng Du Jingyi wang Yulong shan Shichao Han Wenpo shan Hong He Center for Excellence in Regional Atmospheric Environment Institute of Urban EnvironmentChinese Academy of SciencesXiamen 361021China zhejiang Key Laboratory of Urban Environmental Processes and Pollution Control Ningbo Urban Environment Observation and Research StationInstitute of Urban EnvironmentChinese Academy of SciencesNingbo 315800China University of Chinese Academy of Sciences Beijing 100049China State Key Joint Laboratory of Environment Simulation and Pollution Control Research Center for Eco-Environmental SciencesChinese Academy of SciencesBeijing 100085China

nitrogen oxide(nO_(x))is one of the most critical contaminants in the air,and the control of nO_(x)emission from diesel vehicles is very ***-based small-pore zeolites have already been applied for nO_(x)abatement on diesel *** the small-pore zeolites,Cu-SSZ-50 catalysts with good nH_(3)-SCR catalytic activity were believed to have potential for *** this study,a one-pot synthesis method for Cu-SSZ-50 catalysts was developed for the first time,using the co-templates of Cu-TEPA and 2,6-dimethyl-n-methylpyridinium *** this synthesis method,Cu-SSZ-50 with various Cu contents can be obtained by adjusting the amount of Cu-TEPA without the need for a further after-treatment *** addition of Cu-TEPA affected the framework atoms and Cu species,and a lower Si/Al ratio and more SCR active Cu species were *** synthesized catalyst with a Cu/Al ratio of 0.40 exhibited over 90%nO_(x)conversion between 200℃and 450℃for the selective catalytic reduction of nO_(x)with nH_(3)(nH_(3)-SCR).Meanwhile,over 80%nO_(x)conversion could be obtained from 250℃to 450℃after hydrothermal aging at 750℃for 16 *** addition,both L-H and E-R mechanisms were proven to exist for the one-pot-synthesized Cu-SSZ-50 by in situ DRIFTS *** simple synthesis procedure,excellent catalytic activity and hydrothermal stability brighten the prospects for the application of Cu-SSZ-50.

关键词： nH_(3)-SCR Cu-SSZ-50 One-pot synthesis Si/Al ratio Cu species distribution Reaction mechanism

Research on the Effect of Dance Therapy on Improving Social Communication Ability of Children with Autism

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International Journal of Mental Health Promotion 2024年第5期26卷 407-416页

作者： Xiaorui Cui shan wang Institute of Education Xinyang UniversityXinyang464000China Hengshui College Conservatory of Music Hengshui053000China

Research motivation:Through the 12 weeks dance therapy intervention for children with autism,the purpose is to explore the intervention model of dance therapy for children with autism and the changes in motor ability,social ability,and communication ability of children with autism after dance therapy *** results of the research are expected to expand the intervention mode of dance therapy in my country and provide practical reference for rehabilitation intervention of children with *** methods:24 autistic boys aged 6 to 12 with mild to moderate symptoms were recruited and screened through the Internet as the subjects of this *** randomly divided them into experimental group(n=12)and control group(n=12).All children with autism have an autism diagnosis certificate issued by Children’s Hospital or a tertiary hospital,excluding other mental diseases(such as epilepsy,major physical disability,mental illness,no history of drugs and other interventions,etc.).We used the paired sample t-test to compare the score difference between the dance treatment group and the control group before and after the two groups,and used the observation method to record the basic communication behavior and the number of active communication behaviors in the experimental group during the intervention *** data analysis is used in SPSS *** results:After 12 weeks of dance therapy intervention,there were statistically significant differences in the gross movement,balance,and coordination abilities of the children in the experimental group compared with those before the intervention(pno significant difference between the children in the control group(p>0.05).After 12 weeks of dance therapy intervention,there were statistically significant differences in the scores of the social response scale for children with autism in the experimental group(pno significant change in the scores of each item of the SRS scale before an

关键词： Dance therapy movement ability children with autism social interaction communication

n-octyl acrylate is a candidate sex pheromone component involved in courtship in parasitoid wasp Microplitis mediator

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Insect Science 2024年第4期31卷 1200-1210页

作者： Yu-Xiao Tao Shuang shan Youssef Dewer shan-ning wang Adel Khashaveh Rui-Jun Li Yong-Jun zh.ng State Key Laboratory for Biology of Plant Diseases and Insect Pests Institute of Plant ProtectionChinese Academy of Agricultural SciencesBeijingChina College of Plant Protection Agricultural University of HebeiBaodingHebei ProvinceChina Bioassay Research Department Central Agricultural Pesticide LaboratorySabahia Plant Protection Research StationAgricultural Research CenterAlexandriaEgypt Beijing Key Laboratory of Environment Friendly Management on Fruit Diseases and Pests in north China Institute of Plant ProtectionBeijing Academy of Agriculture and Forestry SciencesBeijingChina

Sex pheromones are considered to play critical roles in partner communication of most parasitic ***,the identification of sex pheromone components remains limited to a few families of parasitoid *** this study,we functionally characterized a candidate sex pheromone component in Microplitis mediator(Hymenoptera:Braconidae),a solitary parasitoid of noctuidae *** found that the body surface extract from female wasps could significantly stimulate courtship behavior of *** chromatography-electroantennographic detection(GC-EAD)analysis revealed that a candidate semiochemical from extract triggered significant electrophysiological response of antennae of *** performing gas chromatography-mass spectrometer(GC-MS)measurement,GC-EAD active compound was identified as n-octyl acrylate,a candidate sex pheromone component in female *** electroantennogram(EAG)tests,antennae of male wasps showed significantly higher electrophysiological responses to n-octyl acrylate than those of females.Y-tube olfactometer assays indicated that male wasps significantly chose n-octyl acrylate compared with the ***,male wasps showed a remarkable preference for n-octyl acrylate in a simulated field condition behavioral trial;simultaneously,n-octyl acrylate standard could also trigger significant courtship behavior in *** propose that n-octyl acrylate,as a candidate vital sex pheromone component,could be utilized to design behavioral regulators of *** to implement the protection and utilization of natural enemies.

关键词： behavioral assay courtship behavior GC-EAD analysis Microplitis mediator sex pheromone

Isotopic dependence of the yield ratios of light fragments from different projectiles and their unified neutron skin thicknesses

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nuclear Science and Techniques 2024年第3期35卷 228-236页

作者： Ting-zhi Yan shan Li School of Energy and Power Engineering Northeast Electric Power UniversityJilin 132012China

The yield ratios of neutron-proton(R(n/p))and^(3)H-^(3)He(R(^(3)H∕^(3)He))with reduced rapidity from 0 to 0.5 were simulated at 50 MeV/u even-even ^(36−56)Ca+^(40)Ca,even-even ^(48−78)ni+^(58)ni,and ^(100−139)Sn(every third isotopes)+112 Sn for full reduced impact parameters using the isospin-dependent quantum molecular dynamics(IQMD)*** neutron and proton density distributions and root-mean-square radii of the reaction systems were obtained using the Skyrme-Hartree-Fock model,which was used for the phase space initialization of the projectile and target in *** defined the unified neutron skin thickness asΔRnp=^(1∕2) n−^(1∕2)p,which was negative for neutron-deficient *** unifiedΔRnp values for nuclei with the same relative neutron excess from different isotopic chains were nearly equal,except for extreme neutron-rich isotopes,which is a type of scaling *** yield ratios of the three isotopic chain-induced reactions,which depended on the reduced impact parameter and unified neutron skin thickness,were *** results showed that both R(n/p)and R(^(3)H∕^(3)He)decreased with a reduced impact parameter for extreme neutron-deficient isotopes;however,they increased with reduced impact parameters for extreme neutron-rich isotopes,and increased with theΔRnp of the projectiles for all reduced impact *** addition,a scaling phenomenon was observed betweenΔR np and the yield ratios in peripheral colli-sions from different isotopic chain projectiles(except for extreme neutron-rich isotopes).Thus,R(n/p)and R(^(3)H∕^(3)He)from peripheral collisions were suggested as experimental probes for extracting the neutron or proton skin thicknesses of non-extreme neutron-rich nuclei from different isotopic chains.

关键词： Exotic nuclei Unified neutron skin thickness Yield ratios IQMD

Tuning interface mechanism of FeCo alloy embedded n,S-codoped carbon substrate for rechargeable Zn-air battery

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Journal of Energy Chemistry 2024年第6期93卷 400-410,I0010页

作者： Hui Chang Lulu zhao shan zhao Zong-Lin Liu Peng-Fei wang Ying Xie Ting-Feng Yi School of Materials Science and Engineering Northeastern UniversityShenyang 110819LiaoningChina Key Laboratory of Functional Inorganic Material Chemistry Ministry of EducationSchool of Chemistry and Materials ScienceHeilongjiang UniversityHarbin 150080HeilongjiangChina Key Laboratory of Dielectric and Electrolyte Functional Material Hebei Province School of Resources and MaterialsNortheastern University at QinhuangdaoQinhuangdao 066004HebeiChina

The interface mechanism between catalyst and carbon substrate has been the focus of *** this paper,the FeCo alloy embedded n,S co-doped carbon substrate bifunctional catalyst(FeCo/S-nC)is obtained by a simple one-step pyrolysis *** experimental results and density functional theory(DFT)calculation show that the formation of FeCo alloy is conducive to promoting electron transfer,and the introduction of S atom can enhance the interaction between FeCo alloy and carbon substrate,thus inhibiting the migration and agglomeration of particles on the surface of carbon *** FeCo/SnC catalysts show outstanding performance for oxygen reduction reaction(ORR)and oxygen evolution reaction(OER).FeCo/S-nC shows a high half-wave potential(E_(1/2)=0.8823 V)for ORR and a low overpotential at 10 mA cm^(-2)(E_(j=10)=299 mV)for *** addition,compared with Pt/C+RuO_(2) assembled Zn-air battery(ZAB),the FeCo/S-nC assembled ZAB exhibits a larger power density(198.8 mW cm^(-2)),a higher specific capacity(786.1 mA h g_(zn)~(-1)),and ultra-stable cycle *** results confirm that the optimized composition and the interfacial interaction between catalyst and carbon substrate synergistically enhance the electrochemical performance.

关键词： FeCo alloy n S co-doped carbon DFT calculation Zn-air batteries Interfacial interaction

nanoindentation behavior and creep-induced cracking of long-term crept austenitic steel at 650℃

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Journal of Iron and Steel Research International 2024年第2期31卷 464-474页

作者： zh.n zh.ng Yu-hang Duan Shuai wang Jin-shan Chen An-zhe wang Xiang-yang Mao Yuan-ji Shi Jie zh.ng Ming Liu zh.ng-fei Hu School of Materials Science and Engineering Nanjing Institute of TechnologyNanjing211167JiangsuChina Jiangsu Key Laboratory of Advanced Structural Materials and Application Technology Nanjing211167JiangsuChina Jiangsu Wind Power Engineering Technology Center Nanjing210023JiangsuChina nanjing Vocational University of Industry Technology Nanjing210023JiangsuChina Baoshan Iron&Steel Co. Ltd.Shanghai201900China Fujian Provincial Key Laboratory of Terahertz Functional Devices and Intelligent Sensing School of Mechanical Engineering and AutomationFuzhou UniversityFuzhou350116FujianChina School of Materials Science and Engineering Tongji UniversityShanghai201804China

The grain boundary(GB)damage of long-term crept HR3C(25Cr–20ni–nb–n)austenitic steel with solid solution state was investigated by nanoindentation test accompanied with in-situ electron back-scattered *** corresponding microstructure was characterized by scanning electron microscopy and transmission electron *** show that the increase in nanoindentation hardness at the GBs and triple grain junctions may be related to the dislocation accumulation and carbide growth during the *** M23C6 and dislocations piling-up at the GB accelerate the nucleation and coalescence of creep cavity along the *** nanoindentation hardness in grains varies with orientation of the stress *** orientation difference of neighbor grains may induce local high geometrically necessary dislocation densities and strain gradients near the GB,consequently causing stress concentration and subsequent crack growth at specific GBs.

关键词： Austenitic steel Creep nanoindentation Grain orientation Creep-induced cracking

Tuning SMSI to stabilize metallic Pd species:A case study on Pd/TiO_(2) for HCHO oxidation

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Chinese Chemical Letters 2024年第3期35卷 162-166页

作者： Chunying wang Xiaofeng Liu Jingyi wang Yaobin Li Shaohua Xie Fudong Liu Changbin zh.ng Yuming zh.ng Wenpo shan Hong He Center for Excellence in Regional Atmospheric Environment Key Laboratory of Urban Pollutant ConversionInstitute of Urban EnvironmentChinese Academy of SciencesXiamen 361021China zhejiang Key Laboratory of Urban Environmental Processes and Pollution Control Ningbo Urban Environment Observation and Research StationChinese Academy of SciencesNingbo 315800China Department of Civil Environmentaland Construction Engineering(CECE)Catalysis Cluster for Renewable Energy and Chemical Transformations(REACT)Nano Science Technology Center(NSTC)University of Central FloridaOrlandoFL 32816USA State Key Joint Laboratory of Environment Simulation and Pollution Control Research Center for Eco-environmental SciencesChinese Academy of SciencesBeijing 100085China

Pretreatment of the carrier for supported catalysts can effectively improve the strong metal-support interaction(SMSI)and increase the dispersion of precious metals,which are critical to many important catalytic *** this work,we tuned SMSI on Pd/TiO_(2)catalysts through inducing surface defects of TiO_(2)by pretreated with different atmospheres(H_(2)/n_(2),n_(2),O_(2)/n_(2))at the high temperature(800℃).Multiple characterization results illustrated that surface defects anchored Pd species and thus enhanced their *** reduction,Ti^(3+)species formed and transferred onto the metallic Pd species and then induced SMSI,which effectively stabilize Pd species in the metallic *** stronger MSI,the more stability of Pd *** a case,Pd/TiO_(2)–800H_(2),with strongest MSI,displayed the best HCHO oxidation performance at low temperature(10℃).

关键词： Pd/TiO_(2) Surface defects SMSI Formaldehyde Stability of Pd species

High-Efficiency Photo-Induced Charge Transfer for SERS Sensing in n-Doped 3D-Graphene on Si Heterojunction

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Energy & Environmental Materials 2024年第2期7卷 272-280页

作者： Guanglin zh.ng Jie Sun Genwang Wei shan zh.ng zh.ngyi He Huijuan Wu Bingkun wang Siwei Yang Guqiao Ding zhiduo Liu zhiwen Jin Caichao Ye Gang wang Department of Microelectronic Science and Engineering School of Physical Science and Technology Ningbo University Department of Biochemistry and Molecular Biology School of Basic Medical Sciences Shenzhen University Academy for Advanced Interdisciplinary Studies & Department of Materials Science and Engineering Guangdong Provincial Key Laboratory of Computational Science and Material Design Southern University of Science and Technology State Key Laboratory of Functional Materials for Informatics Shanghai Institute of Microsystem and Information Technology Chinese Academy of Sciences Centre for Quantum Physics Key Laboratory of Advanced Optoelectronic Quantum Architecture and Measurement (MOE) School of Physics Beijing Institute of Technology School of Physical Science and Technology & Key Laboratory for Magnetism and Magnetic Materials of the Ministry of Education Lanzhou University

nitrogen-doped three-dimensional graphene（n-doped 3D-graphene） is a graphene derivative with excellent adsorption capacity, large specific surface area, high porosity, and optoelectronic properties. Herein, n-doped 3Dgraphene/Si heterojunctions were grown in situ directly on silicon（Si）substrates via plasma-assisted chemical vapor deposition（PACVD）, which is promising for surface-enhanced Raman scattering（SERS） substrates candidates. Combined analyses of theoretical simulation, incorporating n atoms in 3D-graphene are beneficial to increase the electronic state density of the system and enhance the charge transfer between the substrate and the target molecules. The enhancement of the optical and electric fields benefits from the stronger light-matter interaction improved by the natural nano-resonator structure of n-doped 3D-graphene. The as-prepared SERS substrates based on n-doped 3D-graphene/Si heterojunctions achieve ultralow detection for various molecules: 10-8M for methylene blue（MB） and10-9M for crystal violet（CRV） with rhodamine（R6G） of 10-10M. In practical detected, 10-8M thiram was precisely detected in apple peel extract. The results indicate that n-doped 3D-graphene/Si heterojunctions based-SERS substrates have promising applications in low-concentration molecular detection and food safety.

关键词： charge transfer DFT simulation n-doped 3D-graphene SERS Thiram detection

Geochemistry and origins of hydrogen-containing natural gases in deep Songliao Basin,China:Insights from continental scientific drilling

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Petroleum Science 2024年第2期21卷 741-751页

作者： Shuang-Biao Han Chao-Han Xiang Xin Du Lin-Feng Xie Jie Huang Cheng-shan wang College of Geoscience and Surveying Engineering China University of Mining and TechnologyBeijing100083China State Key Laboratory of Biogeology and Environmental Geology China University of GeosciencesBeijing100083China

The different reservoirs in deep Songliao Basin have non-homogeneous lithologies and include multiple layers with a high content of hydrogen *** gas composition and stable isotope characteristics vary significantly,but the origin analysis of different gas types has previously been *** on the geochemical parameters of gas samples from different depths and the analysis of geological settings,this research covers the diverse origins of natural gas in different *** gas components are mainly methane with a small amount of C_(2+),and non-hydrocarbon gases,including nitrogen(n_(2)),hydrogen(H_(2)),carbon dioxide(CO_(2)),and helium(He).At greater depth,the carbon isotope of methane becomes heavier,and the hydrogen isotope points to a lacustrine sedimentary *** increasing depth,the origins of n_(2)and CO_(2)change gradually from a mixture of organic and inorganic to *** origins of hydrogen gas are complex and include organic sources,water radiolysis,water-rock(Fe^(2+)-containing minerals)reactions,and *** shales of Denglouku and Shahezi Formations,as source rocks,provide the premise for generation and occurrence of organic ***,the deep faults and fluid activities in Basement Formation control the generation and migration of mantle-derived *** discovery of a high content of H_(2)in study area not only reveals the organic and inorganic association of natural-gas generation,but also provides a scientific basis for the exploration of deep hydrogen-rich gas.

关键词： Gas compositions Stable isotopes Gas origins Hydrogen gas Songliao Basin