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Dynamics of an impurity ion transport in oil-paper insulation under various electric fields

High Voltage 2024年第1期9卷 66-80页

作者： Yuanyang Ren Yang Wang Qiankai Zhang Jiayu Xiong Wen Cao zepeng lv Kai Wu State Key Laboratory of Electrical Insulation and Power Equipment Xi'an Jiaotong UniversityXi'anChina School of Electronics and Information Xi'an Polytechnic UniversityXi'anChina State Grid Sichuan Electric Power Research Institute ChengduChina

The ionic transport process is an important counterpart to charge transport in oil-paper insulation,and it significantly impacts oil flow electrification at the oil-paper *** this,the dynamics of this phenomenon and the underlying mechanisms remain unclear,particularly at the molecular *** understand this fundamental aspect,we conduct Molecular Dynamics study on the transport behaviour of an impurity ion in different oil-paper insulation models under various external electric *** influence factors,such as external electric fields,temperatures,and local structural characteristics,are investigated in relation to the corresponding ionic mobility in different polymer *** to the simulations,ionic mobility and its response to electric fields are higher in weaker electrostatic *** a result,mineral oil exhibits the highest ionic mobility and the most substantial enhancement of ionic mobility by external electric fields,followed by vegetable oil,oil-paper blends,and insulating *** significant deviation in ionic mobility between oil and paper leads to the formation of an electric double layer near the oil-paper *** underlying physical mechanisms of different ionic mobility and its response to the electric field in different polymer models could be explained by the different polymer structural influences in terms of interaction energy and coordination numbers in a static manner,as well as by the interactions between the impurity ion and its surrounding atoms in terms of lifetime correlation functions and velocity autocorrelation functions in a dynamic *** addition,the influence of temperature on ionic mobility in mineral and vegetable oil is examined,and their activation energies are *** in the fundamental understanding of the dynamics of the ion transport process in oil-paper insulation is vital to improving their insulating properties for oil-impregnated power transformers.

关键词： insulation transport fields

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Synergism and anion-cation dual chemical substitution in heterostructure sprouted on MXene enable high-efficiency and stable overall water splitting

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Journal of Materials Science & Technology 2023年第16期147卷 207-216页

作者： zepeng lv Jinshuai Fei Yang You Xuewei lv Qian Li Jie Dang College of Materials Science and Engineering Chongqing UniversityChongqing 400044China National Engineering Research Center for Magnesium Alloys Chongqing UniversityChongqing 400044China State Key Laboratory of Advanced Special Steels&Shanghai Key Laboratory of Advanced Ferrometallurgy School of Materials Science and EngineeringShanghai UniversityShanghai 200444China

The exploration of novel,super-potent and low-cost electrocatalysts for water splitting has always been the kernel in the field of renewable ***,exfoliated Ti_(3)C_(2)T_(x) MXenes work as a substrate to vertically grow polypore N,Ni-Co2P nanoarrays(N,Ni-Co2P@TC)through an in situ interface-growth strategy and subsequent phosphorization and *** well-defined heterointerfaces with positive and negative ions co-modulation as coupled hydrogen evolution reaction(HER)and oxygen evolution reaction(OER)catalysts for efficient overall water splitting are investigated,which possesses excellent durability even at a large current density(±500 mA cm^(-2)).For HER,suitable H_(2)O∗and H∗absorption energies and accelerated electronic transmission make N,Ni-Co2P@TC display a low overpotential of 27 mV at-10 mA cm^(-2) and Tafel slope of 38 mV dec^(–1) in 1 mol/L *** OER,the synergy of N,Ni-Co2P@TC with selfreconfiguration can give enhanced activity with a low overpotential of 232 mV at 10 mA cm^(-2) and a Tafel slope of 57 mV dec^(–1).Additionally,the excellent bifunctional activity allows easily combining for efficient overall water splitting with a low driving voltage(1.51 V)at 10 mA cm^(-2),and the electrolyzer can be driven by a 1.5 V AAA battery.

关键词： Synergism Chemical substitution Heterostructure Overall water splitting MXene

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Constructing heterostructures of ZIF-67 derived C,N doped Co_(2)P and Ti_(2)VC_(2)T_(x)MXene for enhanced OER

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Journal of Materials Science & Technology 2023年第14期145卷 74-82页

作者： Jinzhou Li Chao Chen zepeng lv Wansen Ma Meng Wang Qian Li Jie Dang College of Materials Science and Engineering Chongqing UniversityChongqing 400044China College of Materials Science and Engineering Taiyuan University of TechnologyTaiyuan 030024China State Key Laboratory of Advanced Special Steels&Shanghai Key Laboratory of Advanced Ferrometallurgy School of Materials Science and EngineeringShanghai UniversityShanghai 200444China

Oxygen evolution reaction(OER)is central to technologies such as electrochemical water splitting,and developing efficient and low-cost non-precious metal electrocatalysts for OER is of great significance to reducing cell voltage and developing hydrogen production by electrochemical water ***,we prepared a carbon,nitrogen co-doped porous Co_(2)P derived from the metal-organic framework(ZIF-67),which is anchored on bimetallic MXene nanosheets(named MX@MOF-Co_(2)P).It was used as the OER catalyst and exhibited great electrocatalytic performance with very small overpotentials(246 mV at 10 mA^(-2)and 407 mV at 200 mA cm^(-2))as well as ultralow Tafel slope(28.18 mV dec^(-1)).Combining charac-terizations and theoretical calculations,it was found that the remarkable performance was from follows:the obtained MX@MOF-Co_(2)P inherited the porous structure of the pristine MOF with a large number of open active sites;carbon and nitrogen doping also modulated the electronic structure of the active center;the synergistic effect between cobalt phosphide and MXenes booted the electronic *** work represents a promising strategy for the development of non-precious metal catalysts derived from metal-organic frameworks to achieve efficient energy conversion.

关键词： Mxene mof doping cobalt phosphide electrocatalysts

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MoS_(2)/Co_(9)S_(8)/MoC heterostructure connected by carbon nanotubes as electrocatalyst for efficient hydrogen evolution reaction

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Journal of Materials Science & Technology 2021年第20期79卷 29-34页

作者： Meng Wang Kailiang Jian zepeng lv Dong Li Gangqiang Fan Run Zhang Jie Dang College of Materials Science and Engineering Chongqing UniversityChongqing400044China Chongqing Key Laboratory of Vanadium-Titanium Metallurgy and New Materials Chongqing UniversityChongqing400044China

High-performance multifunctional materials for water splitting driven by low voltage are crucial for hydrogen evolution reaction(HER),but developing such materials is ***,a simple strategy was designed to build a MoS_(2)/Co_(9)S_(8)/MoC@CNT-N(MCM@CNT-N)heterostructure with a large number of *** the HER,the synthesized MCM@CNT-N heterostructure catalyst showed high efficiency and stable electrocatalytic performance,with a low overpotential of 174.2 mV and a small Tafel slope of 84.7 mV dec^(-1) at a current density of 10 mA cm^(-2) in 0.5 M H_(2)SO_(4).In addition to the function of heterojunctions,the excellent activity is also attributed to the introduction of Co and N atoms and the formation of carbon *** work provides a new approach to build efficient and low-cost electrocatalysts for electrochemical reactions.

关键词： MoS_(2) Heterostructure Hydrogen Electrocatalysis CNT

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Fullerene-derived boron-doped defective nanocarbon for highly selective H_(2)O_(2) electrosynthesis

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Nano Research 2024年第3期17卷 1217-1224页

作者： Wangqiang Shen Chang Zhang Muneerah Alomar Zhiling Du zepeng Yang Junjie Wang Guangqing Xu Jian Zhang Jun lv Xing Lu School of Materials Science and Engineering Hefei University of TechnologyHefei 230009China School of Energy and Environmental Hebei University of EngineeringHandan 056038China School of Materials Science and Engineering Huazhong University of Science and TechnologyWuhan 430074China Department of Physics College of SciencesPrincess Nourah bint Abdulrahman UniversityP.O.Box 84428Riyadh 11671Saudi Arabia

Electrochemical production of hydrogen peroxide(H_(2)O_(2))via the two-electron(2e-)pathway of oxygen reduction reaction(ORR)supplies an auspicious alternative to the current industrial anthraquinone ***,it still lacks efficient electrocatalysts to achieve high ORR activity together with 2e-selectivity ***,a boron-doped defective nanocarbon(B-DC)electrocatalyst is synthesized by using fullerene frameworks as the precursor and boric oxide as the boron *** obtained B-DC materials have a hierarchical porous structure,befitting boron dopants,and abundant topological pentagon defects,exhibiting a high ORR onset potential of 0.78 V and a dominated 2e-selectivity(over 95%).Remarkably,when B-DC electrocatalyst is employed in a real device,it achieves a high H_(2)O_(2) yield rate(247 mg·L^(-1)·h^(-1)),quantitative Faraday efficiency(~100%),and ultrafast organic pollutant degradation *** theoretical calculation reveals that the synergistic effect of topological pentagon defects and the incorporation of boron dopants promote the activation of the O_(2) molecule and facilitates the desorption of oxygen *** finding will be very helpful for the comprehension of the synergistic effect of topological defects and heteroatom dopants for boosting the electrocatalytic performance of nanocarbon toward H_(2)O_(2) production.

关键词： fullerene electrochemical hydrogen peroxide production oxygen reduction reaction carbon nanomaterials

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浅析运维人员在变电站改扩建工程中的现场安全管控

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现代工业经济和信息化 2014年第16期4卷 25-27页

作者：吕泽鹏顿凯国网山西省电力公司检修公司山西太原030032

文章通过总结此次工程在施工过程中出现的问题提出了运维人员在变电站改扩建工程中如何保证施工安全的几点体会和建议,为后续的变电站改扩建工程施工安全提供技术参考。

关键词：变电站安全管控现场监护

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福瑞500kV智能变电站数字化技术的应用

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现代工业经济和信息化 2014年第14期4卷 93-94,97页

作者：顿凯吕泽鹏山西省电力公司省检修分公司山西太原030006

智能变电站是智能电网的重要组成部分,通过对福瑞500kV智能变电站结构、网络及告警报文的分析研究,对智能变电站进行了直观的阐述。

关键词：智能变电站三层两网 GOOS断链

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高压直流XLPE电缆研究现状

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绝缘材料 2014年第1期47卷 22-25页

作者：王亚吕泽鹏吴锴王霞刘通李锐海西安交通大学电力设备电气绝缘国家重点实验室西安710049 南方电网科学研究院有限责任公司广州510080

介绍了国际高压直流输电电缆绝缘的应用情况,概述了高压直流电缆的空间电荷与直流电缆测试方法的研究情况,展望了高压直流电缆材料及测试技术的发展方向。

关键词：高压直流 XLPE电缆纳米技术空间电荷老化直流电缆测试技术

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高灰难选细粒煤泥煤质分析及其浮选工艺探讨

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中国煤炭 2010年第11期36卷 78-80页

作者：王市委陶秀祥吕则鹏程敢胡忠波中国矿业大学化工学院江苏省徐州市221008

以开滦地区钱家营选煤厂的难选细粒煤泥为研究对象,分析了该煤泥的煤质特性,并提出了新的浮选降灰工艺。

关键词：煤泥煤质特性浮选工艺

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Cross section measurement for the^(232)Th(n,f)reaction in the 4.50−5.40 MeV region using a time projection chamber

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Chinese Physics C 2024年第10期48卷 157-167页

作者： Haofan Bai Han Yi Yankun Sun Yiwei Hu Jie Liu zepeng Wu Cong Xia Wenkai Ren Wentian Cao Tieshuan Fan Guohui Zhang Ruirui Fan Yang Li Wei Jiang Yonghao Chen You lv Changjun Ning Weihua Jia Zhiyong Zhang Haolei Chen Zhen Chen Maoyuan Zhao Changqing Feng Shubin Liu State Key Laboratory of Nuclear Physics and Technology Institute of Heavy Ion PhysicsPeking UniversityBeijing 100871China Institute of High Energy Physics Chinese Academy of SciencesBeijing 100049China Spallation Neutron Source Science Center Dongguan 523803China National Key Laboratory of Intense Pulsed Radiation Simulation and Effect Northwest Institute of Nuclear TechnologyXi'an 710024China Department of Nuclear Science and Technology School of Energy and Power EngineeringXi’an Jiaotong UniversityXi’an 710049China State Key Laboratory of Particle Detection and Electronics University of Science and Technology of ChinaHefei 230026China Department of Modern Physics University of Science and Technology of ChinaHefei 230026China

Accurate cross sections of neutron induced fission reactions are required in the design of advanced nuclear systems and the development of fission *** projection chambers(TPCs),with their track reconstruction and particle identification capabilities,are considered the best detectors for high-precision fission cross section *** TPC developed by the back-streaming white neutron source(Back-n)team of the China Spallation Neutron Source(CSNS)was used as the fission fragment detector in *** this study,the cross sections of the ^(232)Th(n,f)reaction at five neutron energies in the 4.50−5.40 MeV region were *** fission fragments and α particles were well identified using our TPC,which led to a higher detection efficiency of the fission fragments and smaller uncertainty of the measured cross *** is the first measurement of the ^(232)Th(n,f)reaction using a TPC for the detection of fission *** uncertainties less than 5%,our cross sections are consistent with the data in different evaluation libraries,including JENDL-4.0,ROSFOND-2010,CENDL-3.2,ENDF/B-VⅢ.0,and BROND-3.1,whose uncertainties can be reduced after future improvement of the measurement.

关键词： ^(232)Th(n,f)fission cross section time projection chamber(TPC) ^(232)Th

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