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Chinese Chemical Letters 2024年第2期35卷 484-488页

作者： hao Zhang Qian Liu Zhurui Shen School of Materials Science and Engineering Nankai UniversityTianjin 300350China

Photoreduction of CO_(2) to solar fuels has caused great interest,but suffers from low catalytic efficiency and poor ***,we designed a S-scheme heterojunction(Cu-TiO_(2)/WO_(3))with Cu single atom to significantly boost the photoreduction of CO_(2).Notably,the developed Cu-TiO_(2)/WO_(3) achieved the solardriven conversion of CO_(2) to CH_(4) with an evolution rate of 98.69μmol g^(−1) h^(−1),and the electron selectivity of CH_(4) reached 88.5%.The yield was much higher than those of pristine WO_(3),TiO_(2)/WO_(3) and Cu-TiO_(2) *** and theoretical analysis suggested that the S-scheme heterojunction accelerated charge migration and inhibited the recombination of electron-hole ***,the charge separation effect of the heterojunction meliorated the position of the *** uplifted d-band centers of Cu and Ti on Cu-TiO_(2)/WO_(3) not only improved the electron interaction between Cu single atoms and substrate-TiO_(2),accelerated the adsorption and activation of CO_(2) on the active sites of Cu single atom,but also optimized the Gibbs free energies of CH 4 formation pathway,leading to excellent selectivity toward CH_(4).This work provides new insights into the design of photocatalyst systems with high photocatalytic performance.

关键词： Cu single atom Heterojunction CO_(2)photoreduction d-band center DFT

MODIFIED SPLIT-STEP THETA METHOD FOR STOCHASTIC DIFFERENTIAL EQUATIONS DRIVEN BY FRACTIONAL BROWNIAN MOTION

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Journal of Computational Mathematics 2024年第5期42卷 1226-1245页

作者： Jingjun Zhao hao Zhou Yang Xu School of Mathematics Harbin Institute of TechnologyHarbin 150001China

For solving the stochastic differential equations driven by fractional Brownian motion,we present the modified split-step theta method by combining truncated Euler-Maruyama method with split-step theta *** the problem under a locally Lipschitz condition and a linear growth condition,we analyze the strong convergence and the exponential stability of the proposed ***,for the stochastic delay differential equations with locally Lipschitz drift condition and globally Lipschitz diffusion condition,we give the order of ***,numerical experiments are done to confirm the theoretical conclusions.

关键词： Stochastic differential equation Fractional Brownian motion Split-step theta method Strong convergence Exponential stability

Restricted Arc-Connectivity of Harary Digraphs

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Journal of the Operations Research Society of China 2024年第2期12卷 540-547页

作者： Jun-hao Zhang Ji-Xiang Meng College of Mathematics and System Science Xinjiang UniversityUrumqi 830046XinJiangChina

The h-restricted arc-connectivity of a digraph is an important parameter to measure fault-tolerance of interconnection *** paper determines that the h-restricted arc-connectivity of the Harary digraph D=G(n;1,2,.:,k)i... 详细信息

关键词： Restricted arc-connectivity λ_(h)(D) Super-λ_(h) λ_(h)-Atom λ_(h)-Superatom

IR-YOLO: Real-Time Infrared Vehicle and Pedestrian Detection

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Computers, Materials & Continua 2024年第2期78卷 2667-2687页

作者： Xiao Luo hao Zhu Zhenli Zhang Department of Electrical Engineering and Automation Jiangxi University of Science and TechnologyGanzhou341000China Jiangxi Provincial Key Laboratory of Maglev Technology Ganzhou341000China Graduate School of Information Production and SystemsWaseda UniversityKitakyushu-shiFukuoka808-0135Japan

Road traffic safety can decrease when drivers drive in a low-visibility *** application of visual perception technology to detect vehicles and pedestrians in infrared images proves to be an effective means of reducing the risk of *** tackle the challenges posed by the low recognition accuracy and the substan-tial computational burden associated with current infrared pedestrian-vehicle detection methods,an infrared pedestrian-vehicle detection method A proposal is presented,based on an enhanced version of You Only Look Once version 5(YOLOv5).First,A head specifically designed for detecting small targets has been integrated into the model to make full use of shallow feature information to enhance the accuracy in detecting small ***,the Focal Generalized Intersection over Union(GIoU)is employed as an alternative to the original loss function to address issues related to target overlap and category ***,the distribution shift convolution optimization feature extraction operator is used to alleviate the computational burden of the model without significantly compromising detection *** test results of the improved algorithm show that its average accuracy(mAP)reaches 90.1%.Specifically,the Giga Floating Point Operations Per second(GFLOPs)of the improved algorithm is only *** contrast,the improved algorithms outperformed the other algorithms on similar GFLOPs,such as YOLOv6n(11.9),YOLOv8n(8.7),YOLOv7t(13.2)and YOLOv5s(16.0).The mAPs that are 4.4%,3%,3.5%,and 1.7%greater than those of these algorithms show that the improved algorithm achieves higher accuracy in target detection tasks under similar computational resource *** the other hand,compared with other algorithms such as YOLOv8l(91.1%),YOLOv6l(89.5%),YOLOv7(90.8%),and YOLOv3(90.1%),the improved algorithm needs only 5.5%,2.3%,8.6%,and 2.3%,respectively,of the *** improved algorithm has shown significant advancements in balancing accuracy and computati

关键词： Traffic safety infrared image pedestrians and vehicles focal GIoU distributed shift convolution

How to achieve energy efficiency in buildings without compromising indoor air quality:A case study on enthalpy exchangers

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Science China(Technological Sciences) 2024年第9期67卷 2648-2658页

作者： LI hao ZHANG Tao LIU XiaoHua Department of Building Science Tsinghua UniversityBeijing 100084China

As a representative heat recovery device,the fixed-plate enthalpy exchanger possesses the advantages of high recovery effectiveness,low pressure drop,and small space ***,indoor contaminants may transfer to fresh air through the enthalpy exchanger simultaneously,causing cross-contamination ***,the cross-contamination risk of the fixed-plate enthalpy exchanger has been under-researched in previous *** a result,this study experimentally investigates the energy performance,formaldehyde and ammonia transfer rates of paper-based and membrane-based enthalpy *** results illustrate that the enthalpy recovery effectiveness of the plate exchangers ranges from 60%–85%.The formaldehyde transfer rate through the exchangers varies from 5%–23%,and the ammonia transfer rate is 0–15%.The high effectiveness and low contaminant transfer rates are conducive to the promising application of the fixed-plate enthalpy *** addition,the energy reclaimed increases with the increase of the absolute indoor-outdoor enthalpy *** formaldehyde and ammonia transfer rates and cross-contamination risk slightly decrease with increasing temperature but significantly increase with increasing ***,the experimental results demonstrate that the contaminant transfer rates through the membranebased exchanger are lower than those of the paper-based *** study provides a reference for the fixed-plate enthalpy exchanger design in practical applications.

关键词： building energy efficiency enthalpy recovery heat recovery effectiveness cross-contamination

Deciphering the cellular heterogeneity of the insect brainwith single-cell RNA sequencing

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Insect Science 2024年第2期31卷 314-327页

作者： Xiaofei Wang Yifan Zhai hao Zheng Institute of Plant Protection Shandong Academy of Agricultural SciencesJinanChina College of Food Science and Nutritional En-gineering China Agricultural UniversityBeijingChina Key Laboratory of Natural Enemies Insects Ministry of Agriculture and RuralAffairsJinanChina Shandong Provincial Engineering Technology Research Center on Biocontrol of Crops Diseases and In-sectPests JinanChina

Insects show highly complicated adaptive and sophisticated behaviors, includ-ing spatial orientation skills, learning ability, and social interaction. These behaviors arecontrolled by the insect brain, the central part of the nervous system. The tiny insect brainconsists of millions of highly differentiated and interconnected cells forming a complexnetwork. Decades of research has gone into an understanding of which parts of the insectbrain possess particular behaviors, but exactly how they modulate these functional conse-quences needs to be clarified. Detailed description of the brain and behavior is required todecipher the complexity of cell types, as well as their connectivity and function. Single-cell RNA-sequencing (scRNA-seq) has emerged recently as a breakthrough technologyto understand the transcriptome at cellular resolution. With scRNA-seq, it is possible touncover the cellular heterogeneity of brain cells and elucidate their specific functions andstate. In this review, we first review the basic structure of insect brains and the links toinsect behaviors mainly focusing on learning and memory. Then the scRNA applicationson insect brains are introduced by representative studies. Single-cell RNA-seq has allowedresearchers to classify cell subpopulations within different insect brain regions, pinpointsingle-cell developmental trajectories, and identify gene regulatory networks. These devel-opments empower the advances in neuroscience and shed light on the intricate problemsin understanding insect brain functions and behaviors.

关键词： behavior brain cell type insect single-cell RNA sequencing

Reverse metabolomics as a novel strategy to annotate the human metabolome

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Chinese Journal of Natural Medicines 2024年第4期22卷 289-290页

作者： YAN Tingting NIE Liangliang hao Haiping State Key Laboratory of Natural Medicines China Pharmaceutical UniversityNanjing 211198China Laboratory of Metabolic Regulation and Drug Target Discovery School of PharmacyChina Pharmaceutical UniversityNanjing 210009China

Identifying chemical structures inhuman-derived samples presents significant challenges due to limited structural data obtained from untargeted metabolomics *** the chemical structures of molecules are closely related to the phenotypic status of human ecosystems,it becomes invaluable to devise a method for efficiently and systematically determining structures that correlate with the pathophysiological status of humans in a high-throughput approach.

关键词： Reverse metabolomics Human metabolome Combinational synthesis Bile amidates

Guest-adaptive chiral coassembly of a conformationally locked host into supramolecular boxes and ladders through arene-perfluoroarene force

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Science China Chemistry 2024年第10期67卷 3482-3492页

作者： Weilong Ma Xinyi Li Aiyou hao Pengyao Xing School of Chemistry and Chemical Engineering Shandong UniversityJinan 250100China

Unveiling the role of weak non-covalent forces in chiral self-assembly is pivotal in the design and fabrication of functional chiroptical *** nature of arene-perfluoroarene(AP)force is the electrostatic attraction betweenπ-hole andπplanes of perfluoroarenes and polyaromatic hydrocarbons(PAHs),which is emerging in constructing supramolecular motifs and coassembled optical *** this work,we reveal the potential of AP forces in building diversified levels of chiral coassemblies adaptive to the geometries of *** naphthalene-F8was covalently conjugated with a chiral amine,which folded into a semi-rectangular geometry via two intramolecular F···H *** of naphthalene,anthracene,pyrene,carbazole,perylene and benzoperylene were introduced to afford coassemblies in the crystalline state.X-ray structures suggest the formation of supramolecular boxes that encapsulate the PAHs with a 2:1 stoichiometric ratio,as well as the formation of consecutive layered ladders with a 1:1 stoichiometric *** preference is adaptive to the geometries of PAHs,and experimental and computational results evidenced the ladder structures possess strong binding *** this top,the selective chiral recognition in the mixtures of PAHs was realized,which shows promising applications in the separation of PAHs and rational design of crystalline chiroptical materials.

关键词： arene-perfluoroarene force coassembly supramolecular chirality selectivity

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Variational data encoding and correlations in quantum-enhanced machine learning

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Chinese Physics B 2024年第9期33卷 298-306页

作者： Ming-hao Wang Hua L¨u School of Physics Hubei UniversityWuhan 430062China School of Science Hubei University of TechnologyWuhan 430068China

Leveraging the extraordinary phenomena of quantum superposition and quantum correlation,quantum computing offers unprecedented potential for addressing challenges beyond the reach of classical *** paper tackles two pivotal challenges in the realm of quantum computing:firstly,the development of an effective encoding protocol for translating classical data into quantum states,a critical step for any quantum *** encoding strategies can significantly influence quantum computer ***,we address the need to counteract the inevitable noise that can hinder quantum *** primary contribution is the introduction of a novel variational data encoding method,grounded in quantum regression algorithm *** adapting the learning concept from machine learning,we render data encoding a learnable *** allowed us to study the role of quantum correlation in data *** numerical simulations of various regression tasks,we demonstrate the efficacy of our variational data encoding,particularly post-learning from instructional ***,we delve into the role of quantum correlation in enhancing task performance,especially in noisy *** findings underscore the critical role of quantum correlation in not only bolstering performance but also in mitigating noise interference,thus advancing the frontier of quantum computing.

关键词： quantum machine learning variational data encoding quantum correlation

Tanaka Formula and Local Time for a Class of Interacting Branching Measure-valued Diffusions

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Acta Mathematica Sinica,English Series 2024年第4期40卷 1059-1098页

作者： Donald A.DAWSON Jean VAILLANCOURT hao WANG School of Mathematics and Statistics Carleton UniversityOttawaCanada Department of Decision Sciences HECMontrealCanada Department of Mathematics University of OregonEugeneUSA

We construct superprocesses with dependent spatial motion(SDSMs)in Euclidean spaces R^(d)with d≥1 and show that,even when they start at some unbounded initial positive Radon measure such as Lebesgue measure on R^(d),... 详细信息

关键词： Measure-valued diffusions stochastic partial differential equations superprocesses branching processes local time Tanaka formula