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Rare Metals 2024年第9期43卷 4356-4366页

作者： Qin-Ke Tang Jiang-Chuan Liu Rui Shi yun-feng zhu Ji-Guang Zhang Ya-Na Liu Jun Wang Yao Zhang Xiao-Hui Hu Zhi-Bin Liu Li-Quan Li College of Materials Science and Engineering Jiangsu Collaborative Innovation Centre for Advanced Inorganic Function CompositesNanjing Tech UniversityNanjing 211816China School of Materials Science and Engineering Southeast UniversityNanjing 211189China

Magnesium-based hydrides have been widely recognized as an appropriate choice for solid-state hydrogen ***,its undesirable thermodynamics and sluggish hydrogenation/dehydrogenation kinetics are major bottlenecks for its ***,a highly stable and highly dispersed Ni-based catalyst(Ni/Al_(2)O_(3)/GN)was fabricated to promote the hydrogen storage performance of MgH_(2)via the electrostatic effect of NiAl-LDH/GN precursor with a co-calcination reduction ***_(2)-5wt%Ni/Al_(2)O_(3)/GN exhibits excellent hydrogen storage performance,releasing about 5.7 wt%hydrogen in 3500 s at 250℃,and can reach a saturation hydrogen absorption of about 6.15 wt%in 3000 s at 100℃.Furthermore,it also shows low dehydrogenation apparent activation energy of 89.1 and 118.2 kJ·mol^(-1).Impressively,the catalyst ensures the stability of both the physical phase and structure during ball milling and cycling *** role of each phase in Ni/Al_(2)O_(3)/GN on the hydrogen storage performance of MgH_(2)was also discussed through experiments and theoretical calculation,and the synergistic catalytic mechanism of Ni/Al_(2)O_(3)/GN was clearly *** work provides a unique perspective for the preparation of highly stable and highly dispersible catalysts.

关键词： Magnesium hydride Ni/Al_(2)O_(3)/GN Hydrogen storage performance Catalytic mechanism

Phase transformation and thermal analysis during combustion synthesis of Mg_(17)Al_(12) alloy

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Rare Metals 2014年第1期33卷 37-40页

作者： Yu-Li Zhou yun Lu yun-feng zhu Li-Quan Li College of Materials Science and Engineering Nanjing University of Technology

The Mg-A1 hydrogen storage alloy was suc- cessfully prepared by combustion synthesis （CS） method. The formation of alloy phases during the CS process was studied using X-ray diffraction （XRD）, scanning electron microscope （SEM）, and differential scanning calorimetry （DSC）. When the time increases from 0, 0.5, 1.0 to 2.0 h at 733 K, the products are Mg and A1; Mg2A13, Mg and A1; Mgl7All2, Mg2A13; and Mg; and eventually only MgI7A112, respectively. Combined with three peaks in the DSC traces, it is concluded that the formation of MglyAll2 during the CS includes three processes, namely, the formation of MgzA13 first; then the unsaturated solid solution, MglvAla2; and finally the complete MglvA112 alloy. The formation of MgzA13 prior to MglvA112 in this work is different from those prepared by mechanical alloying. This is thought to be related to the instant high temperature during the ther- mal explosion of CS.

关键词： Mg-A1 alloy Combustion synthesis Phasetransformation Thermal analysis

Enhancing the Interaction of Carbon Nanotubes by Metal-Organic Decomposition with Improved Mechanical Strength and Ultra-Broadband EMI Shielding Performance

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Nano-Micro Letters 2024年第7期16卷 281-294页

作者： Yu-Ying Shi Si-Yuan Liao Qiao-feng Wang Xin-yun Xu Xiao-yun Wang Xin-Yin Gu You-Gen Hu Peng-Li zhu Rong Sun Yan-Jun Wan Shenzhen Institute of Advanced Electronic Materials Shenzhen Institutes of Advanced TechnologyChinese Academy of SciencesShenzhen 518055People’s Republic of China Southern University of Science and Technology Shenzhen 518055People’s Republic of China National Key Laboratory of Materials for Integrated Circuits Shanghai Institute of Microsystem and Information TechnologyChinese Academy of SciencesShanghai 200050People’s Republic of China

The remarkable properties of carbon nanotubes(CNTs)have led to promising applications in the field of electromagnetic inter-ference(EMI)***,for macroscopic CNT assemblies,such as CNT film,achieving high electrical and mechanical properties remains challenging,which heavily depends on the tube-tube interac-tions of ***,we develop a novel strategy based on metal-organic decomposition(MOD)to fabricate a flexible silver-carbon nanotube(Ag-CNT)*** Ag particles are introduced in situ into the CNT film through annealing of MOD,leading to enhanced tube-tube *** a result,the electrical conductivity of Ag-CNT film is up to 6.82×10^(5) S m^(-1),and the EMI shielding effectiveness of Ag-CNT film with a thickness of~7.8μm exceeds 66 dB in the ultra-broad frequency range(3-40 GHz).The tensile strength and Young’s modulus of Ag-CNT film increase from 30.09±3.14 to 76.06±6.20 MPa(~253%)and from 1.12±0.33 to 8.90±0.97 GPa(~795%),***,the Ag-CNT film exhibits excellent near-field shield-ing performance,which can effectively block wireless *** innovative approach provides an effective route to further apply macroscopic CNT assemblies to future portable and wearable electronic devices.

关键词： EMI shielding Mechanical strength Carbon nanotubes Metal-organic decomposition Flexibility

Evaluation of transmission risk of respiratory particles under different ventilation strategies in an elevator

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Building Simulation 2024年第5期17卷 771-784页

作者： Liangyu zhu Xian Li Bujin feng Fan Liu School of Civil Engineering and Architecture Linyi UniversityLinyi276000China College of Agriculture Shandong Agricultural UniversityTaian271018China School of Environment and Architecture University of Shanghai for Science and TechnologyShanghai200093China

People in elevators are at risk of respiratory infection because the elevator cabin is crowded and has poor *** exhaled particles may be inhaled by the susceptible person,deposited on the surface and suspended in the elevator,which can result in direct and indirect ***,whether the air vent designs adopted in the elevator can effectively reduce the transmission risk of respiratory particles remains *** this study,the dispersion of particles under four common ventilation strategies used in the commercial elevator was investigated by proven computational fluid dynamics(CFD)*** flow field was simulated with the RNG κ-ξ turbulence model and the Lagrangian method was adopted to track particle *** effects of air vent layout and airflow rate on particle transmission were *** found that more than 50% of exhaled particles(average value)were suspended in the cabin and difficult to discharge under the investigated ventilation *** deposited fraction of particles on the susceptible person reached up to 39.14% for infiltration ventilation,which led to a high risk of contact *** the ventilation rate could not significantly reduce the inhalation proportion of particles due to the poor airflow distribution inside the elevator.A more proper ventilation strategy should be explored for the elevator to control transmission risk.

关键词： particle dispersion transmission risk elevator ventilation strategy computational fluid dynamics(CFD)

High-efficiency crystalline white organic lightemitting diodes

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Light(Science & Applications) 2024年第4期13卷 747-759页

作者： Yijun Liu feng zhu Yue Wang Donghang Yan State Key Laboratory of Polymer Physics and Chemistry Changchun Institute of Applied ChemistryChinese Academy of SciencesChangchun 130022China. School of Applied Chemistry and Engineering University of Science and Technology of ChinaHefei 230026China. State Key Laboratory of Supramolecular Structure and Materials Jilin UniversityChangchun 130012China

Crystalline white organic light-emitting diodes(C-WOLEDs)are promising candidates for lighting and display *** is urgently necessary,however,to develop energy-saving and high-efficiency C-WOLEDs that have stable and powerful emission to meet commercial ***,we report a crystalline host matrix(CHM)with embedded nanoaggregates(NA)structure for developing high-performance C-WOLEDs by employing a thermally activated delayed fluorescence(TADF)material and orange phosphorescent dopants(Phos.-D).The CHM-TADFNA-D WOLED exhibit a remarkable EQE of 12.8%,which is the highest performance WOLEDs based on crystalline *** device has a quick formation of excitons and a well-designed energy transfer process,and possesses a fast ramping of luminance and current *** to recently reported high-performance WOLEDs based on amorphous material route,the C-WOLED achieves a low series-resistance Joule-heat loss ratio and an enhanced photon output,demonstrating its significant potential in developing the next-generation WOLEDs.

关键词： diodes dopant crystalline

Photodegradation of xylene isomers:Kinetics,mechanism,secondary pollutant formation potential and health risk evaluation

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Journal of Environmental Sciences 2024年第2期136卷 658-669页

作者： Xiaoyan Chen Weikun zhu Sufen feng Jiangyao Chen Guangdong Key Laboratory of Environmental Catalysis and Health Risk Control Guangdong Technology Research Center for Photocatalytic Technology Integration and Equipment EngineeringInstitute of Environmental Health and Pollution ControlGuangdong University of TechnologyGuangzhou 510006China Guangzhou Key Laboratory of Environmental Catalysis and Pollution Control Guangdong-Hong Kong-Macao Joint Laboratory for Contaminants Exposure and HealthSchool of Environmental Science and EngineeringGuangdong University of TechnologyGuangzhou 510006China

Photodegradation technology has been widely applied in the purification of industrial aromatic ***,whether this technology efficiently removes the pollutants to prevent secondary pollution and health risk is still ***,the photodegradation processes of three xylenes were compared under designed reaction atmospheres and light *** lamp showed poor photodegradation ability toward xylenes,no matter in N_(2) or N_(2)+O_(2)system,while much higher photodegradation performance of xylenes were obtained under ultraviolet(UV)and vacuum ultraviolet(VUV)irradiation,especially in N_(2)+O_(2)+VUV system,where 97.9%of m-xylene,99.0%of o-xylene or 87.5%of p-xylene with the initial concentration of 860 mg/m^(3) was removed within 240 *** xylenes underwent three processes of photo-isomerization,photodecomposition and photo-oxidation to produce intermediates of aromatics,alkanes and *** them,the photo-isomerization products showed the highest concentration percentage(e.g.,≥50%in o-xylene system),confirming that photo-isomerization reaction was the dominated photodegradation process of ***,these isomerized products not only contributed about 97%and91%to the formation potential of O3(OFP)and secondary organic aerosols(SOAFP),but also displayed obvious non-carcinogenic risk,although one of photodecomposition product—benzene showed the highest occupational exposure ***,the secondary pollution and health risks of photodegradation products of xylenes were non-ignorable,although the OFP,SOAFP and health risks of the generated products reduced at least 4.5 times in comparison with that of the degraded *** findings are helpful for the appropriate application of this technology in the purification of industrial organic waste gas.

关键词： Isomer aromatics Photodegradation Ozone formation Secondary organic aerosols Health risk

Precise determination of the pole position of the exotic Z_(c)(3900)

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Science China(Physics,Mechanics & Astronomy) 2024年第9期67卷 84-90页

作者： yun-Hua Chen Meng-Lin Du feng-Kun Guo School of Mathematics and Physics University of Science and Technology BeijingBeijing 100083China School of Physics University of Electronic Science and Technology of ChinaChengdu 611731China CAS Key Laboratory of Theoretical Physics Institute of Theoretical PhysicsChinese Academy of SciencesBeijing 100190China School of Physical Sciences University of Chinese Academy of SciencesBeijing 100049China Peng Huanwu Collaborative Center for Research and Education Beihang UniversityBeijing 100191China

We perform a unified description of the experimental data of the π^(+)π^(-)and J/ψπ^(±)invariant mass spectra for e^(+)e^(-)→J/ψπ^(+)π^(-)and the D^(0)D^(*-)mass spectrum for e^(+)e^(-)→D^(0)D^(*-)π^(+)at e^(+)e^(-)center-of-mass energies 4.23 and 4.26 *** analysis takes into account open-charm meson loops that contain triangle singularities,the J/ψπ-DD^(*)coupled-channel interaction respecting unitarity,and the strong ππ-KK final state interaction using dispersion *** analysis leads to a precise determination of the Z_(c)(3900)pole with the pole mass and width(3880.7±1.7_(stat)±22.4_(syst))MeV and(35.9±1.4_(stat)±15.3_(syst))MeV,respectively,and hints at that the DD^(*)molecular and non-molecular components are of similar importance in the Z_(c)(3900)formation.

关键词： exotic hadrons dispersion relations final state interaction triangle singularity

Global classical solutions for 3D compressible magneto-micropolar fluids without resistivity and spin viscosity in a strip domain

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Science China Mathematics 2024年第11期67卷 2485-2514页

作者： Zefu feng Guangyi Hong Changjiang zhu School of Mathematical Sciences Chongqing Normal University School of Mathematics South China University of Technology

In this paper,we consider 3D compressible magneto-micropolar fluids without resistivity and spin viscosity in a strip *** prominent character of the governing model is the presence of the microstructure,a linear coupling structure involving derivatives of the velocity fields,which along with the lack of spin viscosity brings several challenges to the *** exploiting the two-tier energy method developed in Guo and Tice(Arch Ration Mech Anal,2013),we prove the global existence of classical solutions to the governing model around a uniform magnetic field that is non-parallel to the horizontal ***,we show that the solution converges to the steady state at an almost exponential rate as time goes to *** of the main ingredients in our analysis,compared with previous works on micropolar fluids,is that we deal with the microstructure by establishing some delicate estimates based on the analysis of the div-curl decomposition,and the coupling between the fluid velocity and the vorticity of angular velocity.

关键词： magneto-micropolar fluids compressible global existence large-time behavior

SMSTracker:A Self-Calibration Multi-Head Self-Attention Transformer for Visual Object Tracking

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Computers, Materials & Continua 2024年第7期80卷 605-623页

作者： Zhongyang Wang Hu zhu feng Liu School of Communications and Information Engineering Nanjing University of Posts and TelecommunicationsNanjing210003China

Visual object tracking plays a crucial role in computer *** recent years,researchers have proposed various methods to achieve high-performance object *** these,methods based on Transformers have become a research hotspot due to their ability to globally model and contextualize ***,current Transformer-based object tracking methods still face challenges such as low tracking accuracy and the presence of redundant feature *** this paper,we introduce self-calibration multi-head self-attention Transformer(SMSTracker)as a solution to these *** employs a hybrid tensor decomposition self-organizing multihead self-attention transformermechanism,which not only compresses and accelerates Transformer operations but also significantly reduces redundant data,thereby enhancing the accuracy and efficiency of ***,we introduce a self-calibration attention fusion block to resolve common issues of attention ambiguities and inconsistencies found in traditional trackingmethods,ensuring the stability and reliability of tracking performance across various *** integrating a hybrid tensor decomposition approach with a self-organizingmulti-head self-attentive transformer mechanism,SMSTracker enhances the efficiency and accuracy of the tracking *** results show that SMSTracker achieves competitive performance in visual object tracking,promising more robust and efficient tracking systems,demonstrating its potential to providemore robust and efficient tracking solutions in real-world applications.

关键词： Visual object tracking tensor decomposition transformer self-attention

Stability of Gas Diffusion Flame in Laterally Confined Space

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Journal of Thermal Science 2024年第6期33卷 2437-2449页

作者： WANG Xiuzhen zhu feng WANG Shuangfeng Key Laboratory of Microgravity Institute of MechanicsChinese Academy of Sciences School of Engineering Science University of Chinese Academy of Sciences

Lateral-confined coaxial jet diffusion flame is common in micro thrusters,and the specific impulse is mainly obtained through thermodynamic calculations with an assumption of fuel combustion with an equivalence ratio,regardless of the stability of the combustion ***,the flame behavior plays an important impact on the performance of a micro thruster through the varied combustion *** stability of confined coaxial jet diffusion flames with air coflow was studied by experiments and numerical ***,hydrogen,and propane were used as *** attachment,liftoff,blowout(extinction limits of lifted flame),and blowoff(extinction limits of attached flame) behaviors with the effect of confinement ratios and fuel properties were focused *** the range of the jet flow velocity in this research,the hydrogen flame is always attached to the jet exit,the flame tip goes from closed to open as the jet velocity increases,while the flame transitions from attachment to liftoff in the case of CH4 and ***,in a narrow confined space,the attached flame for both CH4 and C3H8 undergoes liftoff followed by ***,in a space with a high confinement ratio,the CH4 flame transitions directly from attachment to *** critical modified Craya-Curtet number,which is used to predict the onset of the recirculation,is determined through simulation and experiment,and the number is about *** work provides valuable data on flame stability inside a confined space and gives insights into the design of a thruster.

关键词： confined space Craya-Curtet number flame stability jet diffusion flame