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Single-atom catalysts supported on graphene/electride heterostructures for the enhanced sulfur reduction reaction in lithium-sulfur batteries

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Journal of Energy Chemistry 2024年第10期97卷 738-746,I0015页

作者： Siyun qi Chuanchuan li Gang Chen Mingwen Zhao School of Physics and Electronics Shandong Normal UniversityJinan 250358ShandongChina qingdao Industrial Energy Storage Research Institute Qingdao Institute of Bioenergy and Bioprocess TechnologyChinese Academy of SciencesQingdao 26611ShandongChina School of Physics&State Key Laboratory of Crystal Materials Shandong UniversityJinan 250100ShandongChina

Single-atom catalysts(SACs)hold great promise in addressing the sluggish kinetics of the sulfur reduction reaction(SRR)in lithium-sulfur(li-S)batteries for their unique catalytic activity and maximum atom *** these SACs must be dispersed on solid substrates,the underlying support is usually limited to carbon materials that have a poor ability to modulate the coordination environment and electronic structures of single atoms,and consequently their catalytic activity toward the SRR is *** we propose two-dimensional(2D)graphene/electride heterostructu res as substrates to enhance the catalytic activities of SACs for li-S batteries.2D electrides featuring the anionic electron gas on their surface enable efficient electron transfer to SACs,which alters their electronic structures,resulting in the shifts of the d orbital and Fermi *** unique electronic structure decreases the filling of antibonding states such that the bonding with adsorbates at active sites is *** demonstrate the enhanced catalytic performance of SACs in terms of the Gibbs free energy of SRR and li_(2)S *** addition,a universal descriptor for the rapid screening of SACs is established by a linear regression fitting *** work provides a new design strategy to modulate SAC activity through electrides for li-S batteries.

关键词： Electrides DFT calculations Kinetics Universal descriptors Charge transfers

Real-time Energy Management Method for Electric-hydrogen Hybrid Energy Storage Microgrids Based on DP-MPC

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CSEE Journal of Power and Energy Systems 2024年第1期10卷 324-336页

作者： qi li Xueli Zou Yuchen Pu Weirong Chen School of Electrical Engineering Southwest Jiaotong UniversityChengdu 611756China

With the increasing presence of intermittent energy resources in microgrids,it is difficult to precisely predict the output of renewable resources and their load *** order to realize the economical operations of the system,an energy management method based on a model predictive control(MPC)and dynamic programming(DP)algorithm is *** method can reasonably distribute the energy of the battery,fuel cell,electrolyzer and external grid,and maximize the output of the distributed power supply while ensuring the power balance and cost optimization of the *** on an ultra-shortterm forecast,the output power of the photovoltaic array and the demand power of the system load are *** offline global optimization of traditional dynamic programming is replaced by the repeated rolling optimization in a limited period of time to obtain power values of each unit in the energy storage *** with the traditional DP,MILP-MPC and the logic based real-time management method,the proposed energy management method is proved to be feasible and effective.

关键词： Electric-hydrogen hybrid energy economic energy management improved dynamic programming microgrid model predictive control

High dimensional proteomic mapping of bone marrow immune characteristics in immune thrombocytopenia

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Science China(life Sciences) 2024年第8期67卷 1635-1647页

作者： Feng-qi liu qing-yuan Qu Ying Lei qi Chen Yu-Xiu Chen Meng-lin li Xue-Yan Sun Ye-Jun Wu qiu-Sha Huang Hai-Xia Fu yuan Kong Yue-Ying li qian-Fei Wang Xiao-Jun Huang Xiao-Hui Zhang Peking University People’s Hospital Peking University Institute of HematologyBeijing 100044China Beijing Key Laboratory of Hematopoietic Stem Cell Transplantation Beijing 100044China National Clinical Research Center for Hematologic Disease Beijing 100044China Collaborative Innovation Centre of Hematology Peking UniversityBeijing 100044China CAS Key Laboratory of Genomic and Precision Medicine Beijing Institute of GenomicsChinese Academy of Sciences and China National Center for BioinformationBeijing 100101China University of Chinese Academy of Sciences Beijing 100049China Peking-Tsinghua Center for life Sciences Academy for Advanced Interdisciplinary StudiesPeking UniversityBeijing 100074China State Key Laboratory of Natural and Biomimetic Drugs Peking UniversityBeijing 100191China

To investigate the role of co-stimulatory and co-inhibitory molecules on immune tolerance in immune thrombocytopenia(ITP),this study mapped the immune cell heterogeneity in the bone marrow of ITP at the single-cell level using Cytometry by Time of Flight(CyTOF).Thirtysix patients with ITP and nine healthy volunteers were enrolled in the *** soluble immunomodulatory molecules,more sCD25 and sGalectin-9 were detected in ITP *** the cell surface,co-stimulatory molecules like ICOS and HVEM were observed to be upregulated in mainly central memory and effector T *** contrast,co-inhibitory molecules such as CTLA-4 were significantly reduced in Th1 and Th17 cell *** a platelet count of 30×10^(9)L^(−1)as the cutoff value,ITP patients with high and low platelet counts showed different T cell immune ***-presenting cells such as monocytes and B cells may regulate the activation of T cells through CTLA-4/CD86 and HVEM/BTLA interactions,respectively,and participate in the pathogenesis of *** conclusion,the proteomic and soluble molecular profiles brought insight into the interaction and modulation of immune cells in the bone marrow of *** may offer novel targets to develop personalized immunotherapies.

关键词： immune thrombocytopenia autoimmune diseases co-stimulatory co-inhibitory immune checkpoint CTLA4 Cytometry by Time of Flight bone marrow

Design and calibration of spoke piezoelectric six-dimensional force/torque sensor for space manipulator

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Chinese Journal of Aeronautics 2024年第1期37卷 218-235页

作者： Yingjun li Guicong WANG Shuai ZHANG yuanqin ZHOU Hongyu li Zhenguang qi School of Mechanical Engineering University of JinanJinan 250022China

The large manipulator outside the space cabin is a multi-degree of freedom actuator for space *** order to realize the automatic control and flexible operation of the space manipulator,a novel spoke structure piezoelectric six-dimensional force/torque sensor with redundancy ability,high stiffness and good decoupling performance is innovatively *** on the deformation coordination relationship,the redundancy measurement mechanism is *** mathematical models of the sensor with and without branch fault are established *** finite element model is established to verify the feasibility of structure and redundancy measuring principle of the *** on the theoretical analysis and simulation analysis,the prototype of the sensor is *** and dynamic calibration experiments are carried *** actual output voltage signal of the six-dimensional force/torque sensor is collected to establish the equation between the standard input applied load and the actual output voltage *** on ant colony optimized BP algorithm,performance indexes of the sensor with and without branch fault are analyzed *** experimental results show that the spoke piezoelectric sixdimensional force/torque sensor with the eight-point support structure has good accuracy and ***,it has strong decoupling characteristic that can effectively shield the coupling between *** nonlinear errors and maximum interference errors of decoupled data with and without branch faults are less than 1% and 2%,*** natural frequency of the sixdimensional force sensor can reach 2856.45 Hz and has good dynamic *** research content lays a theoretical and experimental foundation for the design,development and application of the new six-dimensional force/torque sensors with ***,it will significantly improve the research level in this field,and provide a strong guarantee for the smoot

关键词： Decoupling algorithm Piezoelectric Redundancy Six-dimensional force/torque sensor Space manipulator

Multiscale causes of the 2022 Yangtze mega-flash drought under climate change

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Science China Earth Sciences 2024年第8期67卷 2649-2660页

作者： Xing yuan Yumiao WANG Shiyu ZHOU Hua li Chenyuan li School of Hydrology and Water Resources Nanjing University of Information Science and TechnologyNanjing 210044China Institute of Atmospheric Physics Chinese Academy of SciencesBeijing 100029China Key Laboratory of Hydrometeorological Disaster Mechanism and Warning of Ministry of Water Resources Nanjing University of Information Science and TechnologyNanjing 210044China

The 2022 Yangtze mega-flash drought is characterized by strong intensity and rapid development both in time and space,accompanied by a persistent anticyclonic circulation ***,the causes of the extreme event remain elusive given the multiscale nature of *** we presented a brief overview for the oceanic and terrestrial causes of the megaflash drought during the summer of 2022,and estimated the risk in a changing *** the soil moisture percentile as the drought index,it was found that the drought expanded to the entire Yangtze River basin within two months,with 80%of basin under severe drought conditions at the end of *** the intensity and onset speed of the 2022 mega-flash drought were ranked as the first during the past 62 years,with return periods of 86 and 259 years,*** results of composite analysis showed that the spring La Ni?a can facilitate the abrupt change from a wet/normal condition in May–June to drought in July–August over the Yangtze River basin,which was beneficial for the increase of flash drought intensity and onset speed *** analysis through the linear regression also indicated that the unprecedented intensity was associated with the negative phase of the Pacific Decadal *** by a coupling strength index for soil moisture and vapor pressure deficit,it was found that there was a strong land-atmosphere coupling over the Yangtze River basin during July–August *** attribution by using CMIP6 climate models suggested that land-atmosphere coupling increased the risks of flash drought intensity and onset speed like 2022 by 61%±6%and 64%±7%under natural climate forcings,and the synergy of coupling and anthropogenic climate change would increase the risks by 75%±22%and 85%±12%.Our findings emphasized the role of landatmosphere coupling combined with anthropogenic climate change in intensifying flash droughts.

关键词： Flash drought Yangtze River basin Land-atmosphere coupling Climate change Attribution

Effect of geometry simplification and boundary condition specification on flow field and aerodynamic noise in the train head and bogie region of high-speed trains

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Journal of Zhejiang University-Science A(Applied Physics & Engineering) 2024年第9期25卷 716-731页

作者： Jiawei SHI yuan HE Jiye ZHANG Tian li State Key Laboratory of Rail Transit Vehicle System Southwest Jiaotong UniversityChengdu 610031China Institute of Sound and Vibration Research Faculty of Engineering and Physical SciencesUniversity of SouthamptonSouthampton SO171BJUK

The purpose of this study is to determine a suitable modeling method to make computational fluid dynamics(CFD)simulation more efficient for aeroacoustics optimization of the bogie region of high-speed *** this end,four modeling methods are considered,which involve different geometry simplifications and boundary condition *** corresponding models are named the three-car marshalling model,computational domain shortening model,carbody shortening model,and sub-domain *** the detached eddy simulation(DES)model and Ffowcs Williams-Hawkings(FW-H)equation,the unsteady flow field and far-field noise of the four models are *** evaluate the effect of the different modeling methods,the time-averaged flow field,fluctuating flow field,and far-field noise results of the four models are compared and analyzed in detail with the results of the three-car marshalling model used as basis for *** results show that the flow field results of the bogie region predicted by the four models have relatively high ***,the usage of the non-time varying outlet boundary conditions in the computational domain shortening model and sub-domain model could affect the pressure fluctuation on the upstream carbody *** only the bogie region is used as the source surface,the differences between the far-field noise results of the three simplified models and the three-car marshalling model are all within 1 dB;when the train head is used as the source surface,the results of the carbody shortening model and the three-car marshalling model are more consistent.

关键词： Bogie region Train head Flow field Aerodynamic noise Geometry simplification Boundary conditions

Decoupled deep hough voting for point cloud registration

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Frontiers of Computer Science 2024年第2期18卷 147-155页

作者： Mingzhi yuan Kexue FU Zhihao li Manning WANG Digital Medical Research Center School of Basic Medical SciencesFudan UniversityShanghai 200032China Shanghai Key Laboratory of Medical Image Computing and Computer Assisted Intervention Shanghai 200032China

Estimating rigid transformation using noisy correspondences is critical to feature-based point cloud ***,a series of studies have attempted to combine traditional robust model fitting with deep *** them,DHVR proposed a hough voting-based method,achieving new state-of-the-art ***,we find voting on rotation and translation simultaneously hinders achieving better ***,we proposed a new hough voting-based method,which decouples rotation and translation ***,we first utilize hough voting and a neural network to estimate *** based on good initialization on rotation,we can easily obtain accurate rigid *** experiments on 3DMatch and 3DLoMatch datasets show that our method achieves comparable performances over the state-of-the-art *** further demonstrate the generalization of our method by experimenting on KITTI dataset.

关键词： point cloud registration robust model fitting deep learning hough voting

Finite-Time Stabilization for Constrained Discrete-time Systems by Using Model Predictive Control

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IEEE/CAA Journal of Automatica Sinica 2024年第7期11卷 1656-1666页

作者： Bing Zhu Xiaozhuoer yuan li Dai Zhiwen qiang IEEE the Seventh Research Division Beihang UniversityBeijing 100191China the School of Automation Beijing Institute of TechnologyBeijing 100081China

In this paper, a model predictive control(MPC)framework is proposed for finite-time stabilization of linear and nonlinear discrete-time systems subject to state and control constraints. The proposed MPC framework guarantees the finite-time convergence property by assigning the control horizon equal to the dimension of the overall system, and only penalizing the terminal cost in the optimization, where the stage costs are not penalized explicitly. A terminal inequality constraint is added to guarantee the feasibility and stability of the closed-loop *** feasibility can be improved via augmentation. The finite-time convergence of the proposed MPC is proved theoretically,and is supported by simulation examples.

关键词： Constraints deadbeat control finite-time stabilization model predictive control(MPC)

Wind-sand flow simulation and radius optimization of highway embankment under different vertical curve radius

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Journal of Mountain Science 2024年第8期21卷 2533-2546页

作者： li liangying li qi WANG Xu XIN Guowei WANG Zhenqiang School of Civil Engineering Lanzhou Jiaotong UniversityLanzhou 730070China

It is of great practical value to explore the correlation between the vertical curve radius of desert highway and the increase of sand accumulation in local lines,and to select the appropriate vertical curve radius for reducing the risk of sand *** this study,three-dimensional models of desert highway embankments with different vertical curve radii were constructed,and Fluent software was used to simulate the wind-sand flow field and sand accumulation distribution of vertical curve *** results show that:(1)Along the direction of the road,the concave and the convex vertical curve embankments have the effect of collecting and diverging the wind-sand flow,*** the radius of the concave vertical curve is 3000 m,5000 m,8000 m,10000 m and 20000 m,the wind velocity in the middle of the vertical curve is 31.76%,22.58%,10.78%,10.53%and 10.44%,higher than that at both *** the radius of the convex vertical curve is 6500 m,8000 m,10000 m,20000 m and 30000 m,the wind velocity at both ends of the vertical curve is 14.06%,9.99%,6.14%,3.22%and 2.41%,higher than that in the *** diversion effect also decreases with the increase of the radius.(2)The conductivity of the concave and convex vertical curve embankments with different radii is greater than 1,which is the sediment transport *** conductivity increases with the increase of radius and gradually tends to be *** the radius of the concave and convex vertical curves reaches 8000 m and 20000 m respectively,the phenomenon of sand accumulation is no longer *** the same radius condition,the concave vertical curve embankment is more prone to sand accumulation than the convex one.(3)Considering the strength of the collection and diversion of the vertical curve embankment with different radii,and the sand accumulation of the vertical curve embankment in the desert section of Wuma Expressway,the radius of the concave vertical curve is not less than 8000 m,and the r

关键词： Highway engineering Vertical curve Numerical simulation Embankment wind-sand flow Radius optimization