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Rechargeable Na-MnO_(2) battery with modified cell chemistry

Journal of Energy Chemistry 2023年第9期84卷 414-423页

作者： Sirugaloor Thangavel Senthilkumar Rebeca Marcilla youngsik kim Jesus Palma Mani Ulaganathan Jeong-Sun Park School of Energy&Chemical Engineering Ulsan National Institute of Science and Technology(UNIST)Ulsan 689-798Republic of Korea Electrochemical Processes Unit IMDEA Energy InstituteAvda.Ramón de La Sagra 328935MóstolesSpain Center for Advanced Materials Research Research Institute of Science and TechnologyUniversity of SharjahP.O.Box 27272SharjahUnited Arab Emirates Energy Materials and Devices Lab 4TOONE CorporationUNIST-gil 50Ulsan 689-798Republic of Korea Department of Sciences Amrita School of Physical SciencesAmrita Vishwa VidyapeethamCoimbatore 641112India

High voltage,high energy density,nominal cycle life,and low cost are the most critical requirements of rechargeable batteries for their widespread energy storage applications in electric vehicles and renewable energy ***-MnO_(2) battery could be a low-cost contender,but it suffers extensively from its low cell voltage and poor *** this study,we modified the conventional cell structure of Na-MnO_(2) battery and established altered cell chemistry through a hybrid electrochemical process consisting of Na striping/plating at the anode and Zn^(2+) insertion/de-insertion along with MnO_(2) dissolution/deposition at the *** the modification,Na-MnO_(2) battery exhibits a discharge capacity of 267.10 mA h/g and a cell voltage of 3.30 V(***/Na^(+)),resulting in a high specific energy density of 881.43 Wh/*** 300 cycles,the battery retains 98% of its first-cycle discharge capacity with100% coulombic ***,Na metal-free battery assembled using sodium biphenyl as a safer anode also delivers an excellent energy density of 810.0 Wh/*** work could provide a feasible method to develop an advanced Na-MnO_(2) battery for real-time energy storage applications.

关键词： Hybrid battery Sodium metal Sodium biphenyl High cell voltage Manganese dioxide battery Modified cell chemistry

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Nanocomposite quasi-solid-state electrolyte for high-safety lithium batteries

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Nano Research 2017年第9期10卷 3092-3102页

作者： Hyunji Choi Hyun Woo kim Jae-Kwang kim Young Jun Lim youngsik kim Jou-Hyeon Ahn School of Energy & Chemical Engineering Ulsan National Institute of Science and Technology (UNIST) Ulsan 689-798 Republic of Korea Department of Solar & Energy Engineering Cheongju University Cheongju Chungbuk 28503 Republic of Korea School of Energy & Chemical Engineering and Research Institute for Green Energy Convergence Technology Gyeongsang National University 900 Gajwa-dong Jinju 660-70 I Republic of Korea

Rechargeable lithium batteries are attractive power sources for electronic devices and are being aggressively developed for vehicular use. Nevertheless, problems with their safety and reliability must be solved for the large-scale use of lithium batteries in transportation and grid-storage applications. In this study, a unique hybrid solid-state electrolyte composed of an ionic liquid electrolyte (LiTFSI/Pyr14TFSI) and BaTiO3 nanosize ceramic particles was prepared without a polymer. The electrolyte exhibited high thermal stability, a wide electrochemical window, good ionic conductivity of 1.3 × 10−3 S·cm−1 at 30 °C, and a remarkably high lithium-ion transference number of 0.35. The solid-state LiFePO4 cell exhibited the best electrochemical properties among the reported solid-state batteries, along with a reasonable rate capability. Li/LiCoO2 cells prepared using this nanocomposite solid electrolyte exhibited high performance at both room temperature and a high temperature, confirming their potential as lithium batteries with enhanced safety and a wide range of operating temperatures.

关键词： nanocomposition solidified ionic liquid shell charge space safety lithium battery

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