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Encoding innumerable charge density waves of FeGe into polymorphs of LiFe_(6)Ge_(6)

Science China(Physics,Mechanics & Astronomy) 2024年第9期67卷 126-132页

作者： Yilin wang School of Emerging Technology University of Science and Technology of ChinaHefei 230026China Hefei National Laboratory University of Science and Technology of ChinaHefei 230088China New Cornerstone Science Laboratory University of Science and Technology of ChinaHefei 230026China

Kagome metals exhibit rich quantum states by the intertwining of lattice,charge,orbital and spin degrees of ***,a novel charge density wave(CDW)ground state was discovered in kagome magnet FeGe and was revealed to be driven by lowering magnetic energy via large ***,based on DFTcalculations,we show that such mechanism will yield infinitely many metastable CDWs in FeGe due to different ways to arrange the Ge1-dimerization in enlarged ***,utilizing these metastable CDWs,innumerable polymorphs of kagome magnet LiFe_(6)Ge_(6) can be stabilized by filling Li atoms in the voids right above/below the dimerized Ge1-sites in the CDW *** polymorphs are very stable due to the presence of magnetic-energy-saving mechanism,in sharp contrast to the non-magnetic“166”kagome *** this way,a one-to-one mapping of the metastable CDWs of FeGe to stable polymorphs of LiFe_(6)Ge_(6) is *** one hand,the fingerprints of these metastable CDWs,i.e.,the induced in-plane atomic distortions and band gaps,are encoded into the corresponding stable polymorphs of LiFe_(6)Ge_(6),such that further study of their properties becomes *** the other hand,such innumerable polymorphs of LiFe_(6)Ge_(6) offer great degrees of freedom to explore the rich physics of magnetic kagome *** thus reveal a novel connection between the unusually abundant CDWs and structural polymorphism in magnetic kagome materials,and establish a new route to obtain structural polymorphism on top of CDW states.

关键词： kagome magnet unconventional charge density wave structural polymorphism magnetic energy saving

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Time-sensitive prediction of NO_(2) concentration in China using an ensemble machine learning model from multi-source data

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Journal of Environmental Sciences 2024年第3期137卷 30-40页

作者： Chenliang Tao Man Jia Guoqiang wang Yuqiang Zhang Qingzhu Zhang Xianfeng wang Qiao wang Wenxing wang Big Data Research Center for Ecology and Environment Environment Research InstituteShandong UniversityQingdao 266237China Shandong Provincial Eco-environment Monitoring Center Jinan 250101China

Nitrogen dioxide(NO_(2))poses a critical potential risk to environmental quality and public health.A reliable machine learning(ML)forecasting framework will be useful to provide valuable information to support government *** on the data from1609 air quality monitors across China from 2014-2020,this study designed an ensemble ML model by integrating multiple types of spatial-temporal variables and three sub-models for time-sensitive prediction over a wide *** ensemble ML model incorporates a residual connection to the gated recurrent unit(GRU)network and adopts the advantage of Transformer,extreme gradient boosting(XGBoost)and GRU with residual connection network,resulting in a 4.1%±1.0%lower root mean square error over XGBoost for the test *** ensemble model shows great prediction performance,with coefficient of determination of 0.91,0.86,and 0.77 for 1-hr,3-hr,and 24-hr averages for the test results,*** particular,this model has achieved excellent performance with low spatial uncertainty in Central,East,and North China,the major site-dense *** the interpretability analysis based on the Shapley value for different temporal resolutions,we found that the contribution of atmospheric chemical processes is more important for hourly predictions compared with the daily scale predictions,while the impact of meteorological conditions would be ever-prominent for the *** with existing models for different spatiotemporal scales,the present model can be implemented at any air quality monitoring station across China to facilitate achieving rapid and dependable forecast of NO_(2),which will help developing effective control policies.

关键词： Air quality prediction Deep learning Ensemble method Nitrogen dioxide Spatiotemporal covariates

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高尚堡深层低电阻率油层的识别方法

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测井技术 2010年第3期34卷 242-245页

作者：王友净宋新民刘明新俞宏伟中国石油勘探开发研究院北京100083

高尚堡深层油藏复杂的地质条件导致在淡地层水环境下低电阻率油层与中、高电阻率油层间互发育,油水层识别难度大。受沉积特征和成岩作用的控制,主要发育薄互层型、复杂孔隙结构成因型、黏土矿物附加导电型和因压实作用导致物性变差形成... 详细信息

高尚堡深层油藏复杂的地质条件导致在淡地层水环境下低电阻率油层与中、高电阻率油层间互发育,油水层识别难度大。受沉积特征和成岩作用的控制,主要发育薄互层型、复杂孔隙结构成因型、黏土矿物附加导电型和因压实作用导致物性变差形成的低电阻率油层。在地质成因控制因素定性识别和预测低电阻率油层的基础上,提出应用多元统计分析的主因素分析法确定常规测井信息中油水层识别的敏感性参数,建立交会图版以提高识别准确率的方法。主因素分析表明,自然伽马、自然电位是高尚堡深层油藏油水层识别常规测井信息中的敏感性参数,建立ΔGR与视地层水电阻率Rwa的交会图版,低电阻率油气层主要分布在Rwa0.3区域。

关键词：测井解释低电阻率油层识别高尚堡深层

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Effect of Operation Parameters on the Thermal Characteristics in a Planar Solid Oxide Fuel Cell

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Journal of Thermal Science 2024年第5期33卷 1974-1989页

作者： wang Mingyuan wang Ke wang Yongqing CHEN Jiangshuai AN Bo TU Shantung School of Mechanics and Safety Engineering Zhengzhou UniversityZhengzhou 450001China Key Laboratory of Process Heat Transfer and Energy Saving of Henan Province Zhengzhou UniversityZhengzhou 450002China School of Mechanical and Power Engineering Zhengzhou UniversityZhengzhou 450001China Key Laboratory of Pressure Systems and Safety(MOE) East China University of Science&TechnologyShanghai 200237China

Effective operation strategies in the solid oxide fuel cell(SOFC)can adjust the spatial distribution of temperature gradient favoring the long-term *** investigate the effects of different operating conditions on the thermal behavior inside SOFC,a three-dimensional model is developed in this *** model is verified by comparing it with the experimental *** heat generation rate and its variation under different operating conditions are *** combined effects of operating voltage and gas temperature are considered to be the key factor influencing the temperature *** to the original case,the temperature of SOFC decreases by 21.4 K when the fuel velocity reaches 5 m/*** the maximum temperature gradient increases by21.2%.Meanwhile,higher fuel velocities can eliminate about 32%of the area with higher temperature *** when the oxidant velocity reaches 7.5 m/s,the peak temperature gradient effectively decreases by 16.59%.Simultaneous adjustment of the oxidant and fuel velocities can effectively reduce the peak temperature gradient and increase the safety *** effects of operation conditions on the temperature gradient of the cell are clarified in this study,which can be a reference for further research on the reliability of SOFCs.

关键词： SOFC heat generation temperature gradient distribution heat source thermal behavior

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Extending the detection limit:innovations in infrared quantum dot photodetectors reaching up to 18μm

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Light(Science & Applications) 2024年第8期13卷 1445-1447页

作者： Chong Wu wang Qi Jie wang Centre for OptoElectronics and Biophotonics School of Electrical and Electronic EngineeringNanyang Technological UniversitySingapore 639798Singapore Centre for Disruptive Photonic Technologies School of Physical and Mathematical SciencesNanyang Technological UniversitySingaporeSingapore

A regrowth method was used to synthesize large-sized colloidal quantum dots(CQDs).With the assistance of doping engineering,the synthesized CQD detectors demonstrate exceptional long-wavelength infrared detection performance,reaching up to 18μm,significantly extending the spectral response limit for CQD-based infrared *** detectors also achieve a reasonably high detectivity of 6.6×10^(8)Jones.

关键词： limit quantum sized

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Recent advances in solving Li_(2)CO_(3) problems in garnet-based solid-state battery: A systematic review(2020-2023)

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Journal of Energy Chemistry 2024年第3期90卷 58-76,I0004页

作者： Shaoxiong Han Ziqi wang Yue Ma Yanlan Zhang Yongzhen wang Xiaomin wang College of Materials Science and Engineering Taiyuan University of TechnologyTaiyuan 030024ShanxiChina Shanxi Joint Laboratory of Coal based Solid Waste Resource Utilization and Green Ecological Development Taiyuan 030024ShanxiChina

Garnet solid electrolytes are one of the most promising electrolytes for solid-state ***,Li_(2)CO_(3) is a critical issue that hinders the practical application of garnet-based solid-state lithium-ion *** are two sources of Li_(2)CO_(3) *** main one is the aging of garnet electrolytes in the *** electrolytes can react with H_(2)O and CO_(2) in the air to form Li_(2)CO_(3),which reduces ion conductivity,increases electrode/garnet electrolyte interface resistance,and deteriorates the electrochemical performance of the *** strategies,such as elemental doping,grain boundary manipulation,and interface engineering,have been suggested to address these *** other is the passivation layer(Li_(2)CO_(3),Li_3N,LiOH,Li_(2)O) formed on the surface of the lithium foil after long-term storage,which is ignored by most *** better understand the current strategies and future trends to address the Li_(2)CO_(3) problem,this perspective provides a systematic review of journals published in this field from 2020-2023.

关键词： Solid-state batteries Garnet electrolytes Air stability Interface engineering Lithium foil contamination

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中—高含水期低渗透储层优势渗流通道研究——以温米油田温西一区块三间房组储层为例

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油气地质与采收率 2015年第6期22卷 74-79页

作者：惠钢王友净李佳鸿康波葛启兵戴立波中国石油勘探开发研究院北京100083 中国石油吐哈油田分公司勘探开发研究院新疆哈密839009

中—高含水期低渗透储层经过长期注水开发容易形成优势渗流通道,造成注入水无效循环加剧,严重影响油藏注水开发的效果。以温米油田温西一区块三间房组低孔、中—低渗透储层为例,基于岩性、沉积及微观特征分析优势渗流通道形成的控制因素... 详细信息

中—高含水期低渗透储层经过长期注水开发容易形成优势渗流通道,造成注入水无效循环加剧,严重影响油藏注水开发的效果。以温米油田温西一区块三间房组低孔、中—低渗透储层为例,基于岩性、沉积及微观特征分析优势渗流通道形成的控制因素,综合动、静态资料确定识别优势渗流通道的方法及评价标准,并优选动、静态参数建立综合评价指数模型。研究结果表明,温西一区块三间房组优势渗流通道的形成受岩性、沉积相及微观特征控制;其静态特征表现为岩性粗、物性好,沉积于水下分流河道的主流线上;动态特征表现为吸水剖面存在差异,油井含水率突然升高,示踪剂水线推进快,突破厚度小。研究区优势渗流通道的识别标准为:层内渗透率大于或等于40×10-3μm2,层内渗透率级差大于或等于20,孔喉半径大于或等于3.6μm,月含水率上升率大于或等于30%,单层吸水率大于或等于50%。

关键词：低渗透优势渗流通道识别方法综合评价指数温西-区块

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Molecular design of recyclable thermosetting polyimide and its composite with excellent mechanical and tribological properties

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Friction 2024年第3期12卷 452-461页

作者： Xiaoyue wang Zenghui YANG Tingmei wang Qihua wang Xinrui ZHANG Song LI Key Laboratory of Science and Technology on Wear and Protection of Materials Lanzhou Institute of Chemical PhysicsChinese Academy of SciencesLanzhou 730000China Center of Materials Science and Optoelectronics Engineering University of Chinese Academy of SciencesBeijing 100049China State Key Laboratory of Solid Lubrication Lanzhou Institute of Chemical PhysicsChinese Academy of SciencesLanzhou 730000China

Recyclability of thermosetting polymers and their composites is a challenge for alleviating environmental pollution and resource *** this study,solvent-recyclable thermosetting polyimide(PI)and its composite were successfully *** tensile strength,elongation at break,and Young’s modulus of PI are 108.70±7.29 MPa,19.35%±3.89%,and 2336.42±128.00 MPa,*** addition of reduced graphene oxide(RGO)not only enhances the mechanical properties of PI but also endows it with excellent tribological *** PI illustrates a high recycling efficiency of 94.15%,but the recycled composite exhibits inferior mechanical *** recycling and utilization of PI and its composite are realized through imine bonds(-C=N),which provides new guidance for solving the problem of environmental pollution and resource waste and is potential application in the field of sustainable tribology.

关键词： thermosetting polyimide(PI) recyclability dynamic covalent bonds friction and wear polymer composites

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Enrichment of anammox biomass during mainstream wastewater treatment driven by achievement of partial denitrification through the addition of bio-carriers

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Journal of Environmental Sciences 2024年第3期137卷 181-194页

作者： Yuqing Ma Bo wang Xiaodi Li Shuo wang Wen wang Yongzhen Peng National Engineering Laboratory for Advanced Municipal Wastewater Treatment and Reuse Technology Engineering Research Center of BeijingBeijing University of TechnologyBeijing 100124China

Anammox is widely considered as the most cost-effective and sustainable process for nitrogen ***,how to achieve the enrichment of anammox biomass remains a challenge for its large-scale application,especially in mainstream wastewater *** this study,the feasibility of enrichment of anammox biomass was explored through the realization of partial denitrification and the addition of *** using ordinary activated sludge,a sequencing batch reactor(SBR)followed by an up-fow anaerobic sludge bed(UASB)was operated at 25±2℃ for 214 *** long-term operation was divided into five phases,in which SBR and UASB were started-up in Phases I and II,*** eliminating oxygen and adjusting the infow ratios in Phases III-V,advanced nitrogen removal was achieved with the effuent total nitrogen being 4.7 mg/L and the nitrogen removal efficiency being 90.5%in Phase *** in-situ and ex-situ activity tests demonstrated the occurrence of partial denitrification and ***,16S rRNA high-throughput sequencing analysis revealed that Candidatus Brocadia was enriched from below the detection limit to in biofilms(0.4%in SBR,2.2%in UASB)and the foc sludge(0.2%in SBR,1.3%in UASB),while Thauera was mainly detected in the foc sludge(8.1%in SBR,8.8%in UASB),which might play a key role in partial ***,this study provides a novel strategy to enrich anammox biomass driven by rapid achievement of partial denitrification through the addition of bio-carriers,which will improve large-scale application of anammox processes in mainstream wastewater treatment.

关键词： Enrichment Anammox biomass Bio-carriers Partial denitrification Mainstream wastewater

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A Novel Method for Forecasting Freak Wave Occurrence in A Short Crested Coastal Sea

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China Ocean Engineering 2024年第1期38卷 104-116页

作者： wang Ying-guang State Key Laboratory of Ocean Engineering Shanghai Jiao Tong UniversityShanghai 200240China School of Ocean and Civil Engineering Shanghai Jiao Tong UniversityShanghai 200240China

In order to forecast the distribution of crest amplitudes and the occurrence of freak waves in a short crested coastal sea,a novel transformed linear simulation method is initially proposed in this paper.A Hermite transformation model expressed as a monotonic cubic polynomial serves as the foundation for the novel simulation *** wave crest amplitude exceedance probabilities of two sea states-one with a directional wave spectrum based on the measured wave elevation data at the Yura coast and the other with a typical directional JONSWAP wave spectrum-have been predicted using the novel simulation method that has been *** likelihood that a particular critical wave crest amplitude will be exceeded is directly correlated with the probability that freak waves will *** is shown that the novel simulation approach suggested can provide predictions that are more precise than those obtained from the Rayleigh crest amplitude distribution model,the Jahns and Wheeler crest amplitude distribution model,or the conventional linear simulation *** study also demonstrated that the nonlinear simulation method is less effective than the novel simulation method in terms of efficiency.

关键词： wave crest amplitude freak waves short crested sea transformed linear simulation

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