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Safer solid-state lithium metal batteries:Mechanisms and strategies

InfoMat 2024年第2期6卷 1-27页

作者： Shi-Jie Yang jiang-Kui Hu Feng-Ni jiang Hong Yuan Ho Seok Park Jia-Qi huang School of Materials Science&Engineering Beijing Institute of TechnologyBeijingthe People's Republic of China Advanced Research Institute of Multidisciplinary Science Beijing Institute of TechnologyBeijingthe People's Republic of China College of Chemical Engineering and Technology Taiyuan University of TechnologyTaiyuanShanxithe People's Republic of China Beijing Key Laboratory of Green Chemical Reaction Engineering and Technology Department of Chemical EngineeringTsinghua UniversityBeijingthe People's Republic of China Center for Next-Generation Energy Materials and School of Chemical Engineering Sungkyunkwan UniversitySuwonRepublic of Korea

Solid-state batteries that employ solid-state electrolytes(SSEs)to replace routine liquid electrolytes are considered to be one of the most promising solutions for achieving high-safety lithium metal *** with high mechanical modulus,thermal stability,and non-flammability can not only inhibit the growth of lithium dendrites but also enhance the safety of lithium metal ***,several internal materials/electrodes-related thermal hazards demonstrated by recent works show that solid-state lithium metal batteries(SSLMBs)are not ***,understanding the potential thermal hazards of SSLMBs is critical for their more secure and widespread *** this contribution,we provide a comprehensive overview of the thermal failure mechanism of SSLMBs from materials to ***,strategies to improve the thermal safety performance of SSLMBs are included from the view of material enhancement,battery design,and external ***,the future directions are further *** hope that this work can shed bright insights into the path of constructing energy storage devices with high energy density and safety.

关键词： lithium metal batteries safety improvements solid-state batteries thermal failures thermal runaway

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TransTM:A device-free method based on time-streaming multiscale transformer for human activity recognition

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Defence Technology（防务技术） 2024年第2期32卷 619-628页

作者： Yi Liu Weiqing huang Shang jiang Bobai Zhao Shuai Wang Siye Wang Yanfang Zhang Institute of Information Engineering Chinese Academy of Sciences School of Cyber SecurityUniversity of Chinese Academy of SciencesBeijingChina School of Information Management Beijing Information Science and Technology UniversityBeijingChina

RFID-based human activity recognition(HAR)attracts attention due to its convenience,noninvasiveness,and privacy *** RFID-based HAR methods use modeling,CNN,or LSTM to extract features ***,they have shortcomings:1)requiring complex hand-crafted data cleaning processes and 2)only addressing single-person activity recognition based on specific RF *** solve these problems,this paper proposes a novel device-free method based on Time-streaming Multiscale Transformer called *** model leverages the Transformer's powerful data fitting capabilities to take raw RFID RSSI data as input without ***,we propose a multiscale convolutional hybrid Transformer to capture behavioral features that recognizes singlehuman activities and human-to-human *** with existing CNN-and LSTM-based methods,the Transformer-based method has more data fitting power,generalization,and ***,using RF signals,our method achieves an excellent classification effect on human behaviorbased classification *** results on the actual RFID datasets show that this model achieves a high average recognition accuracy(99.1%).The dataset we collected for detecting RFID-based indoor human activities will be published.

关键词： Human activity recognition RFID Transformer

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AHLNet:Adaptive Multihead Structure and Lightweight Feature Pyramid Network for Detection of Live Working in Substations

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Machine Intelligence Research 2024年第5期21卷 983-992页

作者： Mengle Peng Xiaoyong jiang Langyue huang Zhongyi Li Haiteng Wu Xiaotang Geng Zhejiang University of Science and Technology Hangzhou310023China Zhejiang Key Laboratory of Intelligent Operation and Maintenance Robot Hangzhou311100China

With the increasing demand for power in society,there is much live equipment in substations,and the safety and standardization of live working of workers are facing *** at these problems of scene complexity and object diversity in the real-time detection of the live working safety of substation workers,an adaptive multihead structure and lightweight feature pyramid-based network(AHLNet)is proposed in this study,which is based on ***,we take AH-Darknet53 as the backbone network of YOLOV3,which can introduce an adaptive multihead(AMH)structure,reduce the number of network parameters,and improve the feature extraction ability of the backbone ***,to reduce the number of convolution layers of the deeper feature map,a lightweight feature pyramid network(LFPN)is proposed,which can perform feature fusion in advance to alleviate the problem of feature imbalance and gradient ***,the proposed AHLNet is evaluated on the datasets of 16 categories of substation safety operation scenarios,and the average prediction accuracy MAP_(50)reaches 82.10%.Compared with YOLOV3,MAP_(50)is increased by 2.43%,and the number of parameters is 90 M,which is only 38%of the number of parameters of *** addition,the detection speed is basically the same as that of YOLOV3,which can meet the real-time and accurate detection requirements for the safe operation of substation staff.

关键词： Adaptive multihead structure lightweight feature pyramid substation feature imbalance multiobject detection

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Selective leaching of calcium from mechanically activated mixed rare earth concentrate

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Journal of Rare Earths 2024年第6期42卷 1149-1156,I0006页

作者： jiang Liu Bingxue Chen Yuanqi Feng Yijun Cao Yukun huang Yuan Shi Meng Li Zhongyuan Critical Metals Laboratory School of Chemical EngineeringZhengzhou UniversityZhengzhou450001China State Key Laboratory of Advanced Processing and Recycling of Nonferrous Metals Lanzhou University of TechnologyLanzhou730050China

The loss of rare earths(REs)takes place during the pre-decalcification process of mixed rare earth *** an effort to reduce such RE loss,a novel idea to improve the leaching selectivity of Ca to REs by applying selective mechanical activation was ***,regarding the key minerals affecting the leaching selectivity of Ca to REs,the differences in the mechanical activation behaviors of CaF_(2) and REFCO_(3) were studied,and we find that the lattice strain of CaF_(2) increases from 0.21%to 0.42%,whereas that of REFCO_(3) increases from 0.31%to 0.40%.Notably,CaF_(2) demonstrates a larger lattice strain than REFCO_(3),indicating greater mechanical activation energy storage and higher leaching ***,the HCl leaching process was studied.A significant leaching selectivity of Ca to REs,from 21.6 to 35.1,is achieved through mechanical *** Ca leaching rate reaches 80.7%when the RE loss is 2.3%in the activated *** study provides an novel approach for achieving selective extraction of specific components via mechanical activation pretreatment.

关键词： Mixed rare earth concentrate Pre-decalcification Selective mechanical activation Selective leaching

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Single‑cell sequencing reveals the reproductive variations between primiparous and multiparous Hu ewes

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Journal of Animal Science and Biotechnology 2024年第2期15卷 614-631页

作者： Ting Ge Yifan Wen Bo Li Xiaoyu huang Shaohua jiang Enping Zhang Key Laboratory of Animal Genetics Breeding and Reproduction of Shaanxi ProvinceCollege of Animal Science and TechnologyNorthwest A&F UniversityYangling 712100China

Background In the modern sheep production systems,the reproductive performance of ewes determines the economic profitability of *** the genetic mechanisms underlying differences in the litter size is important for the selection and breeding of highly prolific *** sheep,a high-quality Chinese sheep breed,is known for its high fecundity and is often used as a model to study prolificacy *** the current study,animals were divided into two groups according to their delivery rates in three consecutive lambing seasons(namely,the high and low reproductive groups with≥3 lambs and one lamb per season,n=3,respectively).The ewes were slaughtered within 12 h of estrus,and unilateral ovarian tissues were collected and analyzed by 10×Genomics single-cell RNA *** A total of 5 types of somatic cells were identified and corresponding expression profiles were mapped in the ovaries of each ***,the differences in the ovary somatic cell expression profiles between the high and low reproductive groups were mainly clustered in the granulosa ***,four granulosa cell subtypes were *** analysis revealed that the abundance of JPH1 expression and the reduction of LOC101112291 expression could lead to different evolutionary directions of the granulosa ***,the expression levels of FTH1 and FTL in mural granulosa cells of the highly reproductive group were significantly *** genes inhibit necroptosis and ferroptosis of mural granulosa cells,which helps prevent follicular *** This study provides insights into the molecular mechanisms underlying the high fecundity of Hu *** differences in gene expression profiles,particularly in the granulosa cells,suggest that these cells play a critical role in female *** findings also highlight the importance of genes such as JPH1,LOC101112291,FTH1,and FTL in regulating granulosa cell function and follicular development.

关键词： Granulosa cells Hu sheep Lambing number Ovarian somatic cells Single-cell RNA sequencing

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Problem identification and revitalization strategies for the recovery and reconstruction of traditional villages in the Ms 6.8 Luding Earthquake

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Journal of Mountain Science 2024年第2期21卷 361-379页

作者： huang Chao QIU Jian LIU Chun jiang Rui ZHAO Chuanrong ZHANG Yi School of Architecture and Research Center of Space Planning and Engineering Design Southwest Jiaotong UniversityChengdu 611756China Sichuan Provincial Rural Construction and Development Center Chengdu 610041China Sichuan Institute of Urban and Rural Construction Chengdu 610043China China Association for Promoting Democracy(CAPD)Sichuan Provincial Committee Chengdu 610016China Sichuan Provincial Architectural Design and Research Institute(SADI) Chengdu 610095China

Post-disaster reconstruction is a topic of global concern,and traditional villages have special heritage attributes and need to face more requirements and obstacles in post-disaster *** paper summarizes four concepts based on the research on post-disaster reconstruction both domestically and internationally,as well as the recovery and reconstruction of cultural *** a field survey of traditional villages in the Ms 6.8 Luding earthquake-stricken area,it is found that there are problems such as insufficient awareness of heritage value,misalignment of scientific reconstruction technology,and insufficient protection of reconstruction elements during the reconstruction *** villages face the risk of declining or even loss of heritage *** order to effectively protect traditional villages and inherit the carrier of regional culture,four targeted reconstruction response strategies are proposed,i.e.,to"establish special planning for traditional village preservation","emphasize recovery of the authenticity of village heritage","ensure elements for village heritage recovery"and"promote the activation and utilization of village heritage",based on the problems discovered during the survey and the four concepts summarized in the research on post-disaster reconstruction of traditional *** research results hope to provide useful reference for ancient cultural areas affected by earthquakes on how to protect cultural heritage during the post-disaster reconstruction process.

关键词： Seismic hazard Decision making Traditional village Cultural heritage protection Post-earthquake recovery and reconstruction Revitalization strategy

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Optical two-dimensional coherent spectroscopy of excitons in transition-metal dichalcogenides

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Frontiers of physics 2024年第2期19卷 141-148页

作者： YanZuo Chen ShaoGang Yu Tao jiang XiaoJun Liu XinBin Cheng Di huang State Key Laboratory of Magnetic Resonance and Atomic and Molecular Physics Wuhan Institute of Physics and MathematicsInnovation Academy for Precision Measurement Science and TechnologyChinese Academy of SciencesWuhan 430071China MOE Key Laboratory of Advanced Micro-Structured Materials Shanghai Frontiers Science Center of Digital OpticsInstitute of Precision Optical Engineeringand School of Physics Science and EngineeringTongji UniversityShanghai 200092China Shanghai Institute of Intelligent Science and Technology Tongji UniversityShanghai 200092China

Exciton physics in atomically thin transition-metal dichalcogenides(TMDCs)holds paramount importance for fundamental physics research and prospective ***,the experimental exploration of exciton physics,including excitonic coherence dynamics,exciton many-body interactions,and their optical properties,faces challenges stemming from factors such as spatial heterogeneity and intricate many-body *** this perspective,we elaborate upon how optical two-dimensional coherent spectroscopy(2DCS)emerges as an effective tool to tackle the challenges,and outline potential directions for gaining deeper insights into exciton physics in forthcoming experiments with the advancements in 2DCS techniques and new materials.

关键词： monolayer transition-metal dichalcogenides two-dimensional coherent spectroscopy

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The dynamics beamline at SSRF

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NUCLEAR SCIENCE AND TECHNIQUES 2024年第9期35卷 1-12页

作者： Liu, Zhen Wang, Li-Hua jiang, yong Tong, Ya-Jun Zhu, Hua-Chun Ji, Te Chen, Min jiang, Zheng Wei, Xiang-Jun Chinese Acad Sci Shanghai Adv Res Inst Shanghai 201204 Peoples R China ShanghaiTech Univ Shanghai 201210 Peoples R China

The dynamics beamline (D-Line), which combines synchrotron radiation infrared spectroscopy (SR-IR) and energy-dispersive X-ray absorption spectroscopy (ED-XAS), is the first beamline in the world to realize concurrent ED-XAS and SR-IR measurements at the same sample position on a millisecond time-resolved scale. This combined technique is effective for investigating rapid structural changes in atoms, electrons, and molecules in complicated disorder systems, such as those used in physics, chemistry, materials science, and extreme conditions. Moreover, ED-XAS and SR-IR can be used independently in the two branches of the D-Line. The ED-XAS branch is the first ED-XAS beamline in China, which uses a tapered undulator light source and can achieve approximately 2.5 x 1012 photons/s300 eV BW@7.2 keV at the sample position. An exchangeable polychromator operating in the Bragg-reflection or Laue-transmission configuration is used in different energy ranges to satisfy the requirements for beam size and energy resolution. The focused beam size is approximately 3.5 mu m (H) x 21.5 mu m (V), and the X-ray energy range is 5-25 keV. Using one- and two-dimensional position-sensitive detectors with frame rates of up to 400 kHz enables time resolutions of tens of microseconds to be realized. Several distinctive techniques, such as the concurrent measurement of in situ ED-XAS and infrared spectroscopy, time-resolved ED-XAS, high-pressure ED-XAS, XMCD, and pump-probe ED-XAS, can be applied to achieve different scientific goals.

关键词： ED-XAS SR-IR Time-resolved D-line SSRF SYNCHROTRON-RADIATION DISPERSIVE MODE SPECTROSCOPY PRESSURE EXAFS SPECTROMETER DICHROISM DETECTOR XAFS IR

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Aero-Hydro-Elastic-Servo Modeling and Dynamic Response Analysis of A Monopile Offshore Wind Turbine Under Different Operating Scenarios

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China Ocean Engineering 2024年第3期38卷 379-393页

作者： XIE Shuang-yi GAO Jian LI yong-ran jiang Shu-xin ZHANG Cheng-lin HE Jiao College of Mechanical Engineering Chongqing University of TechnologyChongqing 400044China Beijing Institute of Precision Mechatronics and Controls Beijing 100076China College of Mechanical and Vehicle Engineering Chongqing UniversityChongqing 400044China Fishery Machinery and Instrument Research Institute Chinese Academy of Fishery SciencesShanghai 200092China School of Mechanical and Power Engineering Chongqing University of Science&TechnologyChongqing 401331China

This paper constructs a coupled aero-hydro-elastic-servo simulation framework for a monopile offshore wind turbine(OWT).In this framework,a detailed multi-body dynamics model of the monopile OWT including the gearbox,blades,tower and other components(nacelle,hub,bedplate,etc.)has been explicitly *** effects of pile−soil interaction,controller and operational conditions on the turbine dynamic responses are studied systematically in time domain and frequency *** results show that(1)a comprehensive drivetrain model has the capability to provide a more precise representation of the complex dynamic characteristics exhibited by drivetrain components,which can be used as the basis for further study on the dynamic characteristics of the drivetrain.(2)The pile−soil interaction can influence the wind turbine dynamic responses,particularly under the parked condition.(3)The effect of the pile−soil interaction on tower responses is more significant than that on blade responses.(4)The use of the controller can substantially affect the rotor characteristics,which in turn influences the turbine dynamic responses.(5)The tower and blade displacements under the operational condition are much larger than those under the parked *** model and methodology presented in this study demonstrate potential for examining complex dynamic behaviors of the monopile *** ensure accuracy and precision,it is imperative to construct a detailed model of the wind turbine system,while also taking into account simulation efficiency.

关键词： offshore wind turbine(OWT) pile−soil interaction dynamic response parked condition operating condition

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Recovery and in-situ reduction of precious metals by graphdiyne and graphdiyne oxide for antibacterial use

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Rare Metals 2024年第4期43卷 1747-1757页

作者： Ming-Ji jiang Ya-Na Zhang Ling-Shen Meng Jing Kang yong-Jun Li Alideertu Dong College of Chemistry and Chemical Engineering Inner Mongolia UniversityHohhot010021China Engineering Research Center of Dairy Quality and Safety Control Technology Ministry of EducationInner Mongolia UniversityHohhot010021China Department of Chemistry University of ZurichCH-8057ZurichSwitzerland Laboratory of Organic Solids and Beijing National Laboratory for Molecular Sciences Institute of ChemistryChinese Academy of SciencesBeijing100190China

Based on the in-situ self-reduction and chemical stability,graphdiyne(GDY)and graphdiyne oxide(GDYO)are used as trapping agents to investigate the ability for recovering Au^(3+),Ag^+,and Pd^(2+)under different pH values and interfering *** strong acidity at pH=1,these two agents demonstrate high select recovery towards the three precious metal ions,which could be insitu reduced to nanoparticles(NPs).In addition,superparamagnetic Fe_(3)O_(4)NPs are deposited on the surfaces of GDY and *** magnetic responses enable GDYFe_(3)O_(4)to recover precious metals conveniently and efficiently by the aid of an external magnetic *** study also confirms the antibacterial activity of the as-recovered NPs deposited on GDY and GDYO against Escherichia coli and Staphylococcus aureus(1×10^(5)colony-forming unit(CFU)·mL^(-1)),and the antibacterial rates are 100%.This strategy of recovering precious metals and subsequently reusing to combat pathogens will be of great significance for environmental remediation and biomedical applications.

关键词： Graphdiyne In-situ reduction Recovery Precious metals Antibacterial

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