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Drought decreases the positive impact of warming on an alpine grassland community

Science china Earth Sciences 2024年第10期67卷 3226-3238页

作者： Wang A Wangwang LV yang ZHOU Bowen LI Jianping SUN Jingya LV Lanying CHEN Dorji TSECHEO Shiping WANG Key Laboratory of Tibetan Plateau Earth Resources and EnvironmentInstitute of Tibetan Plateau ResearchChinese Academy of SciencesBeijing 100101China School of Ecology and Environment Tibet UniversityLhasa 850000China University of the chinese Academy of Sciences Beijing 100049China

Temperature and precipitation are the main factors determining plant community succession and aboveground net primary productivity(ANPP)in natural ***,most climate manipulative experiments have mainly focused on their impacts in isolation,especially in alpine *** we explored the relative effects and interaction of warming and precipitation alteration on succession and ANPP using a 7-year experiment involving warming with precipitation alteration(increase(IP)or decrease(DP))in precipitation relative to ambient precipitation(AP)on the Tibetan *** results showed that warming and warm-wet conditions increased species richness,diversity index,height and cover of overall ***,decreasing precipitation reduced them,but increased *** and the rate of change in community ***,warming mitigated the impacts of decreased precipitation on plant community composition,and the interactive effects of warming and altered precipitation on cover,height and plant ANPP varied with year and plant ***,warming increased community ANPP through increases in forb ANPP or non-dominant species ANPP and biodiversity regardless of change in ***,decreased precipitation reduced community ANPP via decreases in the ANPP of sedges and forbs and *** alteration affected the relationship between biodiversity and community ANPP regardless of warming(IP

关键词： Alpine grassland Climate warming Precipitation alteration Community composition Biodiversity Above-ground net primary productivity

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Engineering S-scheme W_(18)O_(49)/ZnIn_(2)S_(4)heterojunction by Co_(x)P nanoclusters for enhanced charge transfer capability and solar hydrogen evolution

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Nano Research 2024年第9期17卷 8095-8103页

作者： Xiaojie Liu Erkang Liu Zixian Wang Wen Zhang Mingyu Dou Hua yang Changhua An Dacheng Li Jianmin Dou Shandong Provincial Key Laboratory of Chemical Energy Storage and Novel Cell Technology School of Chemistry and Chemical EngineeringLiaocheng UniversityLiaocheng 252059China Tianjin Key Laboratory of Organic Solar Cell and Photochemical Conversion School of Chemistry and Chemical EngineeringTianjin Key Laboratory of Advanced Functional Porous MaterialsInstitute for New Energy Materials and Low-Carbon TechnologiesTianjin University of TechnologyTianjin 300384China Institute of Powder Metallurgy and Advanced Ceramics School of Materials Science and EngineeringUniversity of Science and Technology BeijingBeijing 100083China

Enhancement of the light-absorption response and utilization of the photogenerated carriers represent a robust strategy for the design of high-performance *** this work,grafting Co_(x)P nanoclusters onto S-scheme heterojunction of W18O49/ZnIn2S4(WO/ZIS-CoxP)with strong response to the ultraviolet-visible-near infrared ray(UV-vis-NIR)region has been achieved,which possesses efficient electron-transfer-channel,and boosts charge-separation and transport *** as-prepared WO/ZIS-Co_(x)P yields an impressive solar-driven hydrogen production rate of 45 mmol·g^(-1)·h^(-1).The increased photocatalytic performance is attributed to the synergistic effect of the composite catalyst:(1)The local surface plasmon resonance-induced“hot electron”injection of W_(18)O_(49)significantly increases the electron density;(2)the engineered S-scheme directional electron transfer promotes charge separation and enhances the reducing capability of photoexcited electrons;and(3)Co_(x)P as electron-trap site for accelerating surface proton reduction *** work provides a platform to impart nonprecious co-catalyst for engineering S-scheme heterojunction,serving a class of efficient solar-driven photocatalyst towards hydrogen production.

关键词： hydrogen cocatalyst photocatalysis S-scheme hot electron

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甲烷化学链干重整制合成气的氧载体La_(1-x)Sr_(x)Fe_(0.8)Al_(0.2)O_(3)性能研究

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工程热物理学报 2024年第9期45卷 2551-2557页

作者：杨天龙张晋睿饶琼盖忠睿李扬潘莹金红光西安交通大学可再生能源国际研究中心暨动力工程多相流国家重点实验室西安710049 中国科学院工程热物理研究所北京100190 中国科学院大学北京100049

通过化学链方法使用氧载体中的晶格氧进行甲烷的部分氧化反应制合成气,可以实现高的产物选择性。本文采用溶胶凝胶法制备了氧载体La_(1-x)Sr_(x)Fe_(0.8)Al_(0.2)O_(3)用于甲烷化学链干重整反应,使用热重和固定床反应器对不同比例Sr掺... 详细信息

通过化学链方法使用氧载体中的晶格氧进行甲烷的部分氧化反应制合成气,可以实现高的产物选择性。本文采用溶胶凝胶法制备了氧载体La_(1-x)Sr_(x)Fe_(0.8)Al_(0.2)O_(3)用于甲烷化学链干重整反应,使用热重和固定床反应器对不同比例Sr掺杂氧载体的反应性能进行测试。实验结果表明La_(1-x)Sr_(x)Fe_(0.8)Al_(0.2)O_(3)中x=0.4的氧载体氧容量高达1.88 mmol·g^(-1),反应性能优异,同时积碳量较少。进一步对氧载体La_(0.6)Sr_(0.4)Fe_(0.8)Al_(0.2)O_(3)进行了20次循环稳定性测试,发现氧载体保持优异的氧化还原性能,实现了61.2%的甲烷转化率,97.1%的CO选择性,1.81的H_(2)/CO。氧载体的表征结果显示,反应前后氧载体的微观形貌以及晶相结构均未发生改变。本文的结果表明La_(0.6)Sr_(0.4)Fe_(0.8)Al_(0.2)O_(3)是适用于甲烷化学链干重整反应的高性能氧载体。

关键词：化学链甲烷干重整钙钛矿合成气

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Exosomes:the next-generation therapeutic platform for ischemic stroke

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Neural Regeneration Research 2025年第5期20卷 1221-1235页

作者： Wenjing Yin Hongyin Ma yang Qu Jiaxin Ren yingying Sun Zhen-Ni Guo Yi yang Stroke Center Department of NeurologyFirst Hospital of Jilin UniversityChangchunJilin ProvinceChina Neuroscience Research Center Department of NeurologyFirst Hospital of Jilin UniversityChangchunJilin ProvinceChina

Current therapeutic strategies for ischemic stroke fall short of the desired objective of neurological functional ***,there is an urgent need to develop new methods for the treatment of this *** are natural cell-derived vesicles that mediate signal transduction between cells under physiological and pathological *** have low immunogenicity,good stability,high delivery efficiency,and the ability to cross the blood–brain *** physiological properties of exosomes have the potential to lead to new breakthroughs in the treatment of ischemic *** rapid development of nanotechnology has advanced the application of engineered exosomes,which can effectively improve targeting ability,enhance therapeutic efficacy,and minimize the dosages *** in technology have also driven clinical translational research on *** this review,we describe the therapeutic effects of exosomes and their positive roles in current treatment strategies for ischemic stroke,including their antiinflammation,anti-apoptosis,autophagy-regulation,angiogenesis,neurogenesis,and glial scar formation reduction ***,it is worth noting that,despite their significant therapeutic potential,there remains a dearth of standardized characterization methods and efficient isolation techniques capable of producing highly purified *** optimization strategies should prioritize the exploration of suitable isolation techniques and the establishment of unified workflows to effectively harness exosomes for diagnostic or therapeutic applications in ischemic ***,our review aims to summarize our understanding of exosome-based treatment prospects in ischemic stroke and foster innovative ideas for the development of exosome-based therapies.

关键词： blood–brain barrier electroacupuncture engineering exercise exosomes ischemic stroke mesenchymal stem cells microglia neuroprotection stents

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3D interlocked all-textile structured triboelectric pressure sensor for accurately measuring epidermal pulse waves in amphibious environments

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Nano Research 2024年第3期17卷 1923-1932页

作者： Shaobo Si Chenchen Sun Yufen Wu Jingjing Li Han Wang yinggang Lin Jin yang Zhong Lin Wang Department of Optoelectronic Engineering Key Laboratory of Optoelectronic Technology and Systems Ministry of EducationChongqing UniversityChongqing 400044China College of Physics and Electronic Engineering Chongqing Normal UniversityChongqing 401331China Beijing Institute of Nanoenergy and Nanosystems Chinese Academy of SciencesBeijing 100083China School of Materials Science and Engineering Georgia Institute of TechnologyAtlantaGA 30332USA

The performance degradation and even damage of the e-textiles caused by sweat,water,or submersion during all-weather health monitoring are the main reasons that e-textiles have not been commercialized and routinized so ***,we developed an amphibious,high-performance,air-permeable,and comfortable all-textile triboelectric sensor for continuous and precise measurement of epidermal pulse waves during full-day *** on the principle of preparing gas by acid-base neutralization reaction,a one-piece preparation process of amphibious conductive yarn(ACY)with densely porous structures is *** innovative three-dimensional(3D)interlocking fabric knitted from ACYs(0.6 mm in diameter)and polytetrafluoroethylene yarns exhibit high sensitivity(0.433 V·kPa^(-1)),wide bandwidth(up to 10 Hz),and stability(>30,000 cycles).With these benefits,98.8%agreement was achieved between wrist pulse waves acquired by the sensor and a high-precision laser ***,the polytetrafluoroethylene yarn with good compression resilience provides sufficient mechanical support for the contact separation of the ***,the unique skeletonized design of the 3D interlocking structure can effectively relieve the water pressure on the sensor surface to obtain stable and accurate pulse waves(underwater depth of 5 cm).This achievement represents an important step in improving the practicality of e-textiles and early diagnosis of cardiovascular diseases.

关键词： triboelectric pressure sensor amphibious fabric interlocking fabric pulse wave measurement one-piece preparation method

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Origin of the near-room temperature resistance transition in lutetium with H2/N2 gas mixture under high pressure

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National Science Review 2024年第7期11卷 26-32页

作者： Di Peng Qiaoshi Zeng Fujun Lan Zhenfang Xing Zhidan Zeng Xiaoxing Ke yang Ding Ho-kwang Mao Key Laboratory of Materials Physics Institute of Solid State Physics Hefei Institutes of Physical Science(HFIPS)Chinese Academy of Sciences Science Island Branch Graduate School of University of Science and Technology of China Center for High Pressure Science and Technology Advanced Research Shanghai Key Laboratory of Material Frontiers Research in Extreme Environments(MFree) Shanghai Advanced Research in Physical Sciences(SHARPS) State Key Laboratory of Superhard Materials Institute of PhysicsJilin University College of Materials Science&Engineering Beijing University of Technology

The recent report of room-temperature superconductivity at near-ambient pressure in nitrogen-doped lutetium hydride（Lu-H-N） by Dasenbrock-Gammon et al. [Nature 615, 244–250（2023）] has attracted tremendous attention due to its anticipated great impact on technology. However, the results could not be independently reproduced by other groups worldwide in follow-up studies, which elicited intense controversy. Here, we develop a reliable experimental protocol to minimize the extensively concerned extrinsic influences on the sample by starting the reaction from pure lutetium loaded with an H2/N2gas mixture in a diamond anvil cell under different pressures and temperatures and simultaneously monitoring the entire chemical reaction process using in situ four-probe resistance measurements. Therefore, we could repeatedly reproduce the near-room temperature upsurge of electrical resistance at a relatively early stage of the chemical reaction. However, the mechanism is suggested to be a metal-to-semiconductor/insulator transition associated with the structural modulation in the non-stoichiometric Lu-H-N, rather than superconductivity.

关键词： superconductivity high pressure lutetium hydride resistance transition metal-to-semiconductor/insulator transition

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Analysis of the Effect of Problem-Oriented Nursing Intervention on Patients with Lower Extremity Arteriosclerosis Obliterans in Vascular Surgery

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Journal of Clinical and Nursing Research 2024年第4期8卷 1-6页

作者： yang An Shanxi Provincial People’s Hospital Taiyuan 030012China

Objective: To analyze the effect of problem-oriented nursing intervention on patients with lower extremity arteriosclerosis obliterans (ASO) in vascular surgery. Methods: The clinical data of 128 patients with lower extremity ASO in vascular surgery were selected and randomly divided into groups A and B, with 64 cases each. Group A is the control group, and Group B is the observation group. Group A received the routine nursing intervention, and Group B received the problem-oriented nursing intervention. The compliance, self-care ability, psychological state, quality of life, and nursing satisfaction of the two groups of patients were evaluated based on various indicators. Results: After the intervention, the evaluation of self-care ability (ESCA) score of the patients in Group B was higher than that of Group A, and the symptom checklist-90 (SCL-90) score was lower than that of Group A. The differences were significant (t = 10.019, t = 3.118, P < 0.01). After the intervention, the World Health Organization Quality of Life Brief (WHOQOL-BREF) index scores of the two groups increased and the increase in Group B was significantly higher than Group A (P < 0.001). The compliance rate of Group B (62/ 96.88%) was higher than that of Group A (52/ 81.25%), and the difference was extremely significant (χ2 = 8.020, P < 0.01). Conclusion: Problem-oriented nursing intervention for patients with lower extremity ASO in vascular surgery improved the patient’s self-care ability, and quality of life, reduced the patient’s negative emotions, and enhanced their overall satisfaction.

关键词： Problem orientation Nursing intervention Vascular surgery Lower extremity arteriosclerosis obliterans

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Adsorption behavior of CO2/H2S mixtures in calcite slit nanopores for CO2 storage:An insight from molecular perspective

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Petroleum Science 2024年第4期21卷 2444-2456页

作者： Cheng Qian Zhen-Hua Rui Yue-Liang Liu Kai Du Chen Liu yang Zhao Xiao-Min Ma State Key Laboratory of Petroleum Resources and Engineering China University of Petroleum College of Petroleum Engineering China University of Petroleum College of Carbon Neutrality Future Technology China University of Petroleum College of Petroleum China University of Petroleum-Beijing at Karamay College of Mining Engineering Taiyuan University of Technology

It is acknowledged that injecting CO2into oil reservoirs and saline aquifers for storage is a practical and affordable method for *** CO2produced from industrial exhaust contains impurity gases such as H2S that might impact CO2sequestration due to competitive *** study makes a commendable effort to explore the adsorption behavior of CO2/H2S mixtures in calcite slit *** Canonical Monte Carlo（GCMC） simulation is employed to reveal the adsorption of CO2,H2S as well as their binary mixtures in calcite *** show that the increase in pressure and temperature can promote and inhibit the adsorption capacity of CO2and H2S in calcite nanopores,***2exhibits stronger adsorption on calcite surface than *** energy plays the dominating role in the adsorption *** energy accounts for 97.11% of the CO2-calcite interaction energy and 56.33% of the H2S-calcite interaction energy at 10 MPa and 323.15 *** presence of H2S inhibits the CO2adsorption in calcite nanopores due to competitive adsorption,and a higher mole fraction of H2S leads to less *** quantity of CO2adsorbed is lessened by approximately 33% when the mole fraction of H2S reaches ***2molecules preferentially occupy the regions near the po re wall and H2S molecules tend to reside at the center of nanopore even when the molar ratio of CO2is low,indicating that CO2has an adsorption priority on the calcite surface over *** addition,moisture can weaken the adsorption of both CO2and H2S,while CO2is more *** interestingly,we find that pure CO2is more suitable to be sequestrated in the shallower formations,i.e.,500-1500 m,whereas CO2with H2S impurity should be settled in the deeper reservoirs.

关键词： Adsorption behavior CO2/H2S binary mixtures Molecular perspective Calcite slit nanopores CO2 sequestration

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富硒纳豆芽孢杆菌发酵鹰嘴豆风味物质和活性成分研究

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中国粮油学报 2024年第5期39卷 62-68页

作者：徐颖王洋徐瑶魏丽娜蒋国振陕西科技大学食品科学与工程学院西安710021 陕西省产品质量监督检验研究院西安710048 陕西省粮食质量安全中心西安710016

为了评价富硒纳豆芽孢杆菌发酵鹰嘴豆风味和活性成分,研究了富硒纳豆芽孢杆菌固态和液态发酵鹰嘴豆所产生的挥发性物质、游离氨基酸及其他活性物质组成和含量。结果表明,纳豆芽孢杆菌液态发酵鹰嘴豆(L-SD1)的主要挥发性成分是2-甲基丁酸... 详细信息

为了评价富硒纳豆芽孢杆菌发酵鹰嘴豆风味和活性成分,研究了富硒纳豆芽孢杆菌固态和液态发酵鹰嘴豆所产生的挥发性物质、游离氨基酸及其他活性物质组成和含量。结果表明,纳豆芽孢杆菌液态发酵鹰嘴豆(L-SD1)的主要挥发性成分是2-甲基丁酸和3-甲基丁酸,纳豆芽孢杆菌固态发酵鹰嘴豆(G-SD1)、富硒纳豆芽孢杆菌液态发酵(L-Se-SD1)及固态发酵鹰嘴豆(G-Se-SD1)的最主要挥发性成分均为2,5-二甲基吡嗪。液态发酵比固态发酵所产生的挥发性物质种类较多,富硒对主要挥发性物质的种类和相对含量影响较大(P<0.05)。采用氨基酸自动分析仪法检测出L-SD1、L-Se-SD1、G-SD1和G-Se-SD1中均含有16种氨基酸,包括7种人体必需氨基酸和9种其他氨基酸,且苦味氨基酸含量均最高。不同发酵方式对氨基酸种类影响无差异;液态发酵比固态发酵产生的总游离氨基酸含量高。富硒纳豆芽孢杆菌液态发酵鹰嘴豆总黄酮含量为(1.91±0.02)mg/mL,维生素K 2含量为(755.70±0.11)μg/100 g,卵磷脂质量分数为(2.41±0.03)%,相比于未富硒组,分别提高了80.2%、81.6%、10.6%。

关键词：纳豆芽孢杆菌富硒鹰嘴豆风味物质活性物质

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可调高式无砟轨道结构研究

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中国铁路 2024年第9期 77-84页

作者：李莹李晨颖杨荣山中国铁路上海局集团有限公司上海上铁建筑工程(集团)有限公司上海 200040 利丰工程技术(天津)有限公司天津 300000 西南交通大学土木工程学院四川成都 610031

针对无砟轨道基础变形适应能力小的难题,提出一种可调高式无砟轨道结构,由"扣件+垫板"组成,能够灵活调节轨道结构高度,主动适应轨下基础变形.建立可调高式无砟轨道结构整体受力分析有限元模型,分析轨道结构合理尺寸;建立轨道局部受力计... 详细信息

针对无砟轨道基础变形适应能力小的难题,提出一种可调高式无砟轨道结构,由"扣件+垫板"组成,能够灵活调节轨道结构高度,主动适应轨下基础变形.建立可调高式无砟轨道结构整体受力分析有限元模型,分析轨道结构合理尺寸;建立轨道局部受力计算模型,分析垫板厚度变化的影响及锚固螺栓受力状态.结果表明:轨枕块高度为200 mm,埋深为140 mm时,各部件受力较小;通过更换不同厚度的垫板能够实现轨道结构0～60 mm的垂向调整量;锚固螺栓能够正常工作,满足强度设计要求.

关键词：无砟轨道竖向调高基础沉降活动承轨台垫板锚固螺栓扣件轨枕块

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