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Durable K-ion batteries with 100% capacity retention up to 40,000 cycles

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Carbon Energy 2024年第5期6卷 201-212页

作者： Xianlu Lu Zhao Liang Zhi Fang Dongdong Zhang yapeng Zheng Qiao liu Dingfa Fu Jie Teng Weiyou Yang Institute of Micro/Nano Materials and Devices Ningbo University of TechnologyNingboZhejiangChina College of Materials Science and Engineering Hunan UniversityChangshaChina College of Mechanical and Vehicle Engineering Hunan UniversityChangshaChina

Currently,the major challenge in terms of research on K-ion batteries is to ensure that they possess satisfactory cycle stability and specific capacity,especially in terms of the intrinsically sluggish kinetics induced by the large radius of K+***,we explore high-performance K-ion half/full batteries with high rate capability,high specific capacity,and extremely durable cycle stability based on carbon nanosheets with tailored N dopants,which can alleviate the change of volume,increase electronic conductivity,and enhance the K+ion *** as-assembled K-ion half-batteries show an excellent rate capability of 468 mA h g^(−1) at 100 mA g^(−1),which is superior to those of most carbon materials reported to ***,the as-assembled half-cells have an outstanding life span,running 40,000 cycles over 8 months with a specific capacity retention of 100%at a high current density of 2000 mA g^(−1),and the target full cells deliver a high reversible specific capacity of 146 mA h g^(−1) after 2000 cycles over 2 months,with a specific capacity retention of 113%at a high current density of 500 mA g^(−1),both of which are state of the art in the field of K-ion *** study might provide some insights into and potential avenues for exploration of advanced K-ion batteries with durable stability for practical applications.

关键词： carbon nanosheet cycle stability K-ion batteries rate performance specific capacity

A model with multiple intracranial aneurysms: possible hemodynamic mechanisms of aneurysmal initiation, rupture and recurrence

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中华神经外科杂志(英文) 2024年第02期10卷 107-114页

作者： Li Wenqiang Wang Chao Wang Yanmin Zhao yapeng Yang Xinjian liu Xianzhi liu Jian Department of Interventional Neuroradiology and Neurosurgery Beijing Neurosurgical Institute and Beijing Tiantan Hospital Beijing China Department of Neurosurgery The First Affiliated Hospital of Zhengzhou University Zhengzhou China

Background Hemodynamic factors play an important role in aneurysm initiation, growth, rupture, and recurrence, while the mechanism of the hemodynamic characteristics is still controversial. A unique model of multiple aneurysms (initiation, growth, rupture, and recurrence) is helpful to avoids the confounders and further explore the possible hemodynamic mechanisms of aneurysm in different *** We present a model with multiple aneurysms, and including the states of initiation, growth, rupture, and recurrence, discuss the proposed mechanisms, and describe computational fluid dynamic model that was used to evaluate the likely hemodynamic effect of different states of the *** The hemodynamic analysis suggests that high flow impingement and high WSS distribution at normal parent artery was found before aneurysmal initiation. The WSS distribution and flow velocity were decreased in the new sac after aneurysmal growth. Low WSS was the risk hemodynamic factor for aneurysmal rupture. High flow concentration region on the neck plane after coil embolization still marked in recanalized *** Associations have been identified between high flow impingement and aneurysm recanalization, while low WSS is linked to the rupture of aneurysms. High flow concentration and high WSS distribution at normal artery associated with aneurysm initiation and growth, while after growth, the high-risk hemodynamics of aneurysm rupture was occurred, which is low WSS at aneurysm dome.

关键词： Multiple intracranial aneurysms Hemodynamic Aneurysm initiation and growth Rupture Recurrence

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高阶煤孔隙特征的低场核磁共振实验研究

中国安全生产科学技术 2016年第11期12卷 63-69页

作者：杨明刘亚鹏煤炭安全生产河南省协同创新中心河南焦作454003 河南省瓦斯地质与瓦斯治理重点实验室-省部共建国家重点实验室培育基地河南焦作454003 河南理工大学安全科学与工程学院河南焦作454003

研究孔裂隙特征对煤层中甲烷的产出及运移具有重要的意义。为了得到高阶煤的孔裂隙特征信息,采用低场核磁共振仪对高阶煤样做低场核磁共振实验,测得煤样的T2图谱,进一步分析得到了煤样的核磁渗透率、核磁孔隙度、可动流体饱和度、束缚... 详细信息

研究孔裂隙特征对煤层中甲烷的产出及运移具有重要的意义。为了得到高阶煤的孔裂隙特征信息,采用低场核磁共振仪对高阶煤样做低场核磁共振实验,测得煤样的T2图谱,进一步分析得到了煤样的核磁渗透率、核磁孔隙度、可动流体饱和度、束缚流体饱和度以及孔径分布等参数的实验结果,并测出煤样的工业分析参数。分析结果得出:原煤中孔隙体积与煤的挥发分含量呈正比的关系;高阶煤孔隙发育而裂隙不发育,并且在孔隙中微孔和小孔占有较大的比例而中孔和大孔占有较少的比例;煤样渗透率与煤样内小孔和大孔所占的比例成正比,与煤样内微孔所占的比例成反比等结论。

关键词：孔隙低场核磁共振渗透率孔径分布

Integrated causal inference modeling uncovers novel causal factors and potential therapeutic targets of Qingjin Yiqi granules for chronic fatigue syndrome

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Acupuncture and Herbal Medicine 2024年第1期4卷 122-133页

作者： Junrong Li Xiaobing Zhai Jixing liu Chi Kin Lam Weiyu Meng Yuefei Wang Shu Li yapeng Wang Kefeng Li Faculty of Applied Sciences Macao Polytechnic UniversityMacao SARChina Center for Artificial Intelligence Driven Drug Discovery Faculty of Applied SciencesMacao Polytechnic UniversityMacao SARChina National Key Laboratory of Chinese Medicine Modernization Tianjin Key Laboratory of TCM Chemistry and AnalysisTianjin University of Traditional Chinese MedicineTianjinChina Haihe Laboratory of Modern Chinese Medicine TianjinChina

Objective:Chronic fatigue syndrome(CFS)is a prevalent symptom of post-coronavirus disease 2019(COVID-19)and is associated with unclear disease *** herbal medicine Qingjin Yiqi granules(QJYQ)constitute a clinically approved formula for treating post-COVID-19;however,its potential as a drug target for treating CFS remains largely *** study aimed to identify novel causal factors for CFS and elucidate the potential targets and pharmacological mechanisms of action of QJYQ in treating ***:This prospective cohort analysis included 4,212 adults aged≥65 years who were followed up for 7 years with 435 incident CFS *** modeling and multivariate logistic regression analysis were performed to identify the potential causal determinants of CFS.A proteome-wide,two-sample Mendelian randomization(MR)analysis was employed to explore the proteins associated with the identified causal factors of CFS,which may serve as potential drug ***,we performed a virtual screening analysis to assess the binding affinity between the bioactive compounds in QJYQ and CFS-associated ***:Among 4,212 participants(47.5%men)with a median age of 69 years(interquartile range:69–70 years)enrolled in 2004,435 developed CFS by *** graph analysis with multivariate logistic regression identified frequent cough(odds ratio:1.74,95%confidence interval[CI]:1.15–2.63)and insomnia(odds ratio:2.59,95%CI:1.77–3.79)as novel causal factors of ***-wide MR analysis revealed that the upregulation of endothelial cell-selective adhesion molecule(ESAM)was causally linked to both chronic cough(odds ratio:1.019,95%CI:1.012–1.026,P=2.75 e^(−05))and insomnia(odds ratio:1.015,95%CI:1.008–1.022,P=4.40 e^(−08))in *** major bioactive compounds of QJYQ,ginsenoside Rb2(docking score:−6.03)and RG4(docking score:−6.15),bound to ESAM with high affinity based on virtual ***:Our integrated analytical framework combining epidemiological,genet

关键词： Causal factors Causal graph analysis Chronic fatigue syndrome Drug targets Mendelian randomization Qingjin Yiqi

基于混淆布鲁姆过滤器的云外包隐私集合比较协议

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计算机应用 2016年第10期36卷 2723-2727,2732页

作者：张恩刘亚鹏河南师范大学计算机与信息工程学院河南新乡453007 智慧商务与物联网技术河南省工程实验室河南新乡453007

针对基于混淆布鲁姆过滤器的隐私集合比较(PSI)协议中存在参与方信息获取不对等及协议不能有效应用于云环境等问题,将混淆布鲁姆过滤器算法与代理不经意传输协议相结合,提出了一种基于混淆布鲁姆过滤器和代理不经意传输的云外包隐私集... 详细信息

针对基于混淆布鲁姆过滤器的隐私集合比较(PSI)协议中存在参与方信息获取不对等及协议不能有效应用于云环境等问题,将混淆布鲁姆过滤器算法与代理不经意传输协议相结合,提出了一种基于混淆布鲁姆过滤器和代理不经意传输的云外包隐私集合比较协议。首先,该算法通过引入混淆布鲁姆过滤器的概念,解决了传统标准布鲁姆过滤器产生误判的问题,进而达到高效存储和传输大数据的目的;其次,采用代理不经意传输协议,能够将复杂耗时的计算外包给云代理服务器,使得云租户不需实时在线、仅需进行少量计算;最后,在云外包隐私集合比较过程中,云租户间无需交互,能够公平地得到集合比较结果。理论分析和性能对比表明,该算法的通信复杂度和计算复杂度是线性的,并且协议是安全和有效的。

关键词：隐私集合比较云外包布鲁姆过滤器代理不经意传输

Negative enthalpy alloys and local chemical ordering:a concept and route leading to synergy of strength and ductility

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National Science Review 2024年第4期11卷 172-184页

作者： Zibing An Tao Yang Caijuan Shi Shengcheng Mao Lihua Wang Ang Li Wei Li Xianmeng Xue Ming Sun Yifan Bai yapeng He Fuzeng Ren Zhouguang Lu Ming Yan Yang Ren Chain-Tsuan liu Ze Zhang Xiaodong Han Beijing Key Lab of Microstructure and Property of Advanced Materials College of Materials Science &Engineering Beijing University of Technology Department of Materials Science and Engineering City University of Hong Kong Key Laboratory of Partial Acceleration Physics& Technology Institute of High Energy PhysicsChinese Academy of Sciences Department of Materials Science &Engineering Southern University of Science and Technology Department of Physics City University of Hong Kong State Key Laboratory of Silicon Materials Department of Materials Science and Engineering Zhejiang University

Solid solutions are ubiquitous in metals and alloys. Local chemical ordering(LCO) is a fundamental sub-nano/nanoscale process that occurs in many solid solutions and can be used as a microstructure to optimize strength and ductility. However, the formation of LCO has not been fully elucidated, let alone how to provide efficient routes for designing LCO to achieve synergistic effects on both superb strength and ductility. Herein, we propose the formation and control of LCO in negative enthalpy alloys. With engineering negative enthalpy in solid solutions, genetic LCO components are formed in negative enthalpy refractory high-entropy alloys(RHEAs). In contrast to conventional ‘trial-and-error' approaches, the control of LCO by using engineering negative enthalpy in RHEAs is instructive and results in superior strength(1160 MPa) and uniform ductility(24.5%) under tension at ambient temperature, which are among the best reported so far. LCO can promote dislocation cross-slip, enhancing the interaction between dislocations and their accumulation at large tensile strains; sustainable strain hardening can thereby be attained to ensure high ductility of the alloy. This work paves the way for new research fields on negative enthalpy solid solutions and alloys for the synergy of strength and ductility as well as new functions.

关键词： negative enthalpy alloys local chemical ordering strength ductility dislocation

激光冲击与喷丸复合强化对TC4钛合金细节疲劳额定强度截止值DFRcutoff的影响

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中国激光 2020年第5期47卷 362-369页

作者：刘亚鹏史志俊赵一昭朱亮刘马宝西安交通大学航天航空学院陕西西安710049 西安交通大学机械结构强度与振动国家重点实验室陕西西安710049 中国航空工业集团公司西安飞机设计研究所陕西西安710089 陕西省先进飞行器服役环境与控制重点实验室陕西西安710049

为研究激光冲击与喷丸复合强化对TC4钛合金疲劳性能的影响,在测试不同强化工艺状态(未强化状态、喷丸强化状态、激光冲击强化状态、激光冲击与喷丸复合强化状态)TC4钛合金表面残余应力的基础上,进行了细节疲劳额定强度截止值(DFRcutoff... 详细信息

为研究激光冲击与喷丸复合强化对TC4钛合金疲劳性能的影响,在测试不同强化工艺状态(未强化状态、喷丸强化状态、激光冲击强化状态、激光冲击与喷丸复合强化状态)TC4钛合金表面残余应力的基础上,进行了细节疲劳额定强度截止值(DFRcutoff)试验,并利用ABAQUS有限元仿真分析其表层残余应力分布。试验结果表明:复合强化TC4钛合金的表面残余压应力和DFRcutoff最大,相比于未强化状态分别提高了189.1%和62.3%。仿真结果表明:表面处理会在试样表面形成残余压应力,激光冲击与喷丸复合强化状态试样的表面残余压应力最大,喷丸强化试样的次之,激光冲击强化试样的最小;激光冲击与喷丸复合强化试样中的残余压应力层最深,激光冲击强化试样的次之,喷丸强化试样的最浅。结合试验结果与有限元分析可知,TC4钛合金的DFRcutoff与表面残余压应力和残余压应力层深度呈正相关。

关键词：激光技术 TC4钛合金喷丸强化激光冲击强化复合强化 DFRcutoff 残余应力

合作机器人微操作力提升系统的控制策略及实验研究

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高技术通讯 2007年第5期17卷 493-497页

作者：董玉红张立勋刘亚鹏哈尔滨理工大学机械动力学院哈尔滨150080 哈尔滨工程大学机电学院哈尔滨150001

根据合作机器人提升系统的组成和工作原理,提出了顺应操作者特性的阻抗控制策略,建立了微操作力提升系统的数学模型和Simulink仿真模型,对阻抗控制策略进行了仿真分析。基于dSPACE半物理仿真平台对提升系统的控制策略进行了实验研究。... 详细信息

根据合作机器人提升系统的组成和工作原理,提出了顺应操作者特性的阻抗控制策略,建立了微操作力提升系统的数学模型和Simulink仿真模型,对阻抗控制策略进行了仿真分析。基于dSPACE半物理仿真平台对提升系统的控制策略进行了实验研究。研究结果表明,该控制策略是可行的,操作者施加较小的操作力,提升系统就能顺应人的操作升降重物,且能满足操作者提升操作的柔顺性要求。

关键词：合作机器人微操作力阻抗控制策略

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超高效液相色谱法测定大黄与铜离子络合能力

色谱 2023年第4期41卷 323-329页

作者：刘亚鹏张旺刘心洁吴欢周安安徽中医药大学科研技术中心安徽合肥230038 中药复方安徽省重点实验室中药研究与开发安徽省重点实验室安徽合肥230012

中药肝豆汤治疗铜代谢障碍疾病具有疗效显著、副作用小的优势,但由于缺乏评价铜离子(Cu^(2+))络合能力的技术手段,限制了肝豆汤配位活性成分的筛查和发现。为评价复方肝豆汤中主药大黄对铜离子的络合能力,该文通过优化大黄活性成分与铜... 详细信息

中药肝豆汤治疗铜代谢障碍疾病具有疗效显著、副作用小的优势,但由于缺乏评价铜离子(Cu^(2+))络合能力的技术手段,限制了肝豆汤配位活性成分的筛查和发现。为评价复方肝豆汤中主药大黄对铜离子的络合能力,该文通过优化大黄活性成分与铜离子配位反应条件,建立了超高效液相色谱法(UHPLC)测定中药大黄与铜离子络合能力的方法。样品经Agilent Eclipse Plus C18色谱柱(50 mm×2.1 mm,1.8μm)分离,以甲醇-0.1%(v/v)磷酸水溶液为流动相进行梯度洗脱,柱温30℃,流速为0.3 mL/min,检测波长为254 nm,进样体积为5μL。研究通过UHPLC分析比较大黄与铜离子配位反应前后色谱峰变化,超高效液相色谱四极杆-飞行时间质谱(UPLC-Q-TOF-MS)鉴定大黄提取物中配位活性成分,计算大黄提取物与铜离子配位反应前后其色谱峰面积变化率来评价大黄中活性成分与Cu^(2+)的络合能力。结果显示,大黄提取物与Cu^(2+)在pH为9的体系中配位反应12 h达到平衡;鉴定出大黄提取物中20种主要成分,根据Cu^(2+)配位率筛选出8种具有较强配位能力的化合物,其中没食子酸-3-O-β-D-(6′-O-没食子酰基)-吡喃葡萄糖苷、芦荟大黄素-8-O-β-D-葡萄糖苷、番泻苷B、l-O-没食子酰基-2-O-肉桂酰基-葡萄糖苷、大黄酚-8-O-β-D-(6″-O-乙酰)-葡萄糖苷、芦荟大黄素、大黄酸和大黄素的Cu^(2+)配位率依次为62.50%、29.94%、70.58%、32.77%、34.61%、26.07%、28.73%和31.78%。该方法的建立可用于筛选与Cu^(2+)具有络合能力的中药活性成分,同时可为其他中药与金属离子络合能力的评估和筛选提供借鉴。

关键词：超高效液相色谱配位反应铜离子大黄肝豆状核变性