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Journal of Energy Chemistry 2024年第8期95卷 511-518,I0011页

作者： Hongfei Bao Diancheng Chen Jiaqi Cao Pengfeng Jiang Kaili Li Runtao Liu Yuling Zhao Yichun Zheng Beiqi Liao Yaming Zhang Xia Lu yang Sun School of Materials Shenzhen Campus of Sun Yat-sen UniversityShenzhen 518107GuangdongChina

Solid-state electrolytes(SSEs)play a pivotal role in advancing next-generation lithium metal battery ***,they commonly encounter substantial interfacial resistance and poor stability when interfacing with lithium metal,hindering practical ***,we introduce a flexible metal-organic framework(MOF:NUS-6)-incorporated polymeric layer,denoted as NP,designed to protect the sodium superionic conductor(NASICON)-type Li_(1.3)Al_(0.3)Ti_(1.7)(PO_(4))_(3)(LATP)electrolyte from Li metal *** NP matrix establishes a soft interface with the LATP surface,effectively reducing voids and gaps that may arise between the LATP electrolyte and Li ***,the MOF component in NP enhances ionic conductivity,offers abundant Li^(+)transport sites,and provides hierarchical ion channels,ensuring a homogeneous Li^(+)flow and thus effectively inhibiting Li dendrite *** NP,we fabricate Li symmetrical cells cycled for over 1600 h at 0.2 mA cm^(-2)and all-solid-state LiINP-LATPI LiFePO_(4)batteries,achieving a remarkable 99.3%capacity retention after 200 cycles at 0.2 *** work outlines a general strategy for designing long-lasting and stable solid-state Li metal batteries.

关键词： All-solid-state Li metal battery MOF-based polymeric layer Li dendrite Interfacial contact LATP electrolyte stability

探矿找油六十载：黄汲清与中国石油、天然气的普查勘探

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地质学报 2024年第3期98卷 647-652页

作者：杨丽娟浙江大学历史学院

黄汲清(1904～1995),著名地质学家，中国科学院院士，我国近现代地质事业开拓者和奠基人之一。他在开创中国区域地质调查和地质制图事业、建立中国大地构造理论基础、勘察中国石油天然气资源等方面均作出了卓越贡献。早在20世纪30年代... 详细信息

黄汲清(1904～1995),著名地质学家，中国科学院院士，我国近现代地质事业开拓者和奠基人之一。他在开创中国区域地质调查和地质制图事业、建立中国大地构造理论基础、勘察中国石油天然气资源等方面均作出了卓越贡献。早在20世纪30年代，黄汲清即着手石油地质的考察研究工作；20世纪50年代，黄汲清参与规划、部署并实地指导全国范围的石油、天然气的普查，为大庆等油田的发现作出了突出贡献。本文利用黄汲清回忆录、年谱和自然资源部档案等原始材料，系统整理黄汲清数十年来在中国石油、天然气的方面研究工作，分析中国石油勘探工作在理论和实践上的突破。

关键词：黄汲清石油天然气松辽盆地

Al-enabled properties distribution prediction for high-pressure die casting Al-Si alloy

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Advances in Manufacturing 2024年第3期12卷 591-602页

作者： Yu-Tong yang Zhong-Yuan Qiu Zhen Zheng Liang-Xi Pu Ding-Ding Chen Jiang Zheng Rui-Jie Zhang Bo Zhang Shi-Yao Huang Key Laboratory for Light-Weight Materials Nanjing Tech UniversityNanjing211816People’s Republic of China Xi’an Jiaotong-Liverpool University Suzhou215000JiangsuPeople’s Republic of China Materials Academy JITRI Suzhou215100JiangsuPeople’s Republic of China Key Laboratory for Light-weight Materials Nanjing University of Science and TechnologyNanjing210009People’s Republic of China College of Materials Science and Engineering Chongqing UniversityChongqing400044People’s Republic of China Collaborate Innovation Center of Steel Technology University of Science and Technology BeijingBeijing100083People’s Republic of China Chongqing Millison Technologies Inc. Chongqing401321People’s Republic of China

High-pressure die casting(HPDC)is one of the most popular mass production processes in the automotive industry owing to its capability for part ***,the nonuniform distribution of mechanical properties in large-sized HPDC products adds complexity to part property ***,a methodology for property prediction must be *** characterization,simulation technologies,and artificial intelligence(AI)algorithms were ***,an image recognition technique was employed to construct a temperature-microstructure characteristic model for a typical HPDC Al7Si0.2Mg ***,a porosity/microstructure-mechanical property model was established using a machine learning method based on the finite element method and representative volume element model ***,the computational results of the casting simulation software were mapped with the porosity/microstructure-mechanical property model,allowing accurate prediction of the property distribution of the HPDC Al-Si *** AI-enabled property distribution model developed in this study is expected to serve as a foundation for intelligent HPDC part design platforms in the automotive industry.

关键词： Artificial intelligence(AI) Properties prediction High-pressure die-casting(HPDC) Image recognition Machine learning

Bismuth clusters pinned on TiO_(2) porous nanowires boosting charge transfer for CO_(2) photoreduction to CH_(4)

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Nano Research 2024年第3期17卷 1190-1198页

作者： Jiazhi Meng Kaiwen Wang yang Wang Jiangping Ma Chaogang Ban Yajie Feng Bin Zhang Kai Zhou Liyong Gan Guang Han Danmei Yu Xiaoyuan Zhou College of Physics and Institute of Advanced Interdisciplinary Studies Chongqing UniversityChongqing 401331China School of Chemistry and Chemical Engineering Chongqing UniversityChongqing 401331China College of Materials Science and Engineering Chongqing UniversityChongqing 400044China Beijing Key Lab of Microstructure and Properties of Advanced Materials Beijing University of TechnologyBeijing 100124China Analytical and Testing Center Chongqing UniversityChongqing 401331China

Artificial photosynthesis in carbon dioxide(CO_(2))conversion into value-added chemicals attracts considerable attention but suffers from the low activity induced by sluggish separation of photogenerated carriers and the kinetic bottleneck-induced unsatisfied ***,we prepare a new-style Bi/TiO_(2) catalyst formed by pinning bismuth clusters on TiO_(2) nanowires through being confined by pores,which exhibits high activity and selectivity towards photocatalytic production of CH_(4) from CO_(2).Boosted charge transfer from TiO_(2) through Bi to the reactants is revealed via in situ X-ray photon spectroscopy and time-resolved photoluminescence(PL).Further,in situ Fourier transform infrared results confirm that Bi/TiO_(2) not only overcomes the multi-electron kinetics challenge of CO_(2) to CH_(4) via boosting charge transfer,but also facilitates proton production and transfer as well as the intermediates*CHO and*CH_(3)O generation,ultimately achieving the tandem catalysis towards *** calculation also underlies that the more favorable reaction step from*CO to*CHO on Bi/TiO_(2) results in CH_(4) production with higher *** work brings new insights into rational design of photocatalysts with high performance and the formation mechanism of CO_(2) to CH_(4) for solar energy storage in future.

关键词： carbon dioxide(CO_(2))photoreduction charge transfer tandem catalysis methanation

Seasonal compensation implied no weakening of the land carbon sink in the Northern Hemisphere under the 2015/2016 El Niño

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Science China Earth Sciences 2024年第1期67卷 281-294页

作者： Fangzhong SHI Xiuchen WU Xiaoyan LI Philippe CIAIS Hongyan LIU Chao YUE Yuting yang Shulei ZHANG Shushi PENG Yi YIN Benjamin POULTER Deliang CHEN State Key Laboratory of Earth Surface Processes and Resource Ecology Beijing Normal UniversityBeijing 100875China Faculty of Geographical Science Beijing Normal UniversityBeijing 100875China Key Laboratory of Tibetan Plateau Land Surface Processes and Ecological Conservation Qinghai Normal UniversityXining 810016China Research and Development Center for Watershed Environmental Eco-Engineering Beijing Normal University(Zhuhai)Zhuhai 519085China Laboratoire des Sciences du Climat et de l’Environnement(LSCE) CEA-CNRS-UVSQUMR821291191Gif-sur-YvetteFrance College of Urban and Environmental Science MOE Laboratory for Earth Surface ProcessesPeking UniversityBeijing 100871China State Key Laboratory of Hydroscience and Engineering Department of Hydraulic EngineeringTsinghua UniversityBeijing 100084China Southern Marine Science and Engineering Guangdong Laboratory(Zhuhai) School of Atmospheric SciencesSun Yat-sen UniversityGuangzhou 510275China California Institute of Technology PasadenaCA 91125USA Biospheric Sciences Laboratory NASA Goddard Space Flight CenterGreenbeltMaryland 20771USA Regional Climate Group Department of Earth SciencesUniversity of GothenburgGothenburg SE-40530Sweden

The recurrent extreme El Niño events are commonly linked to reduced vegetation growth and the land carbon sink over many but discrete regions of the Northern Hemisphere(NH).However,we reported here a pervasive and continuous vegetation greening and no weakened land carbon sink in the maturation phase of the 2015/2016 El Niño event over the NH(mainly in the extra-tropics),based on multiple evidences from remote sensing observations,global ecosystem model simulations and atmospheric CO_(2)*** discovered a significant compensation effect of the enhanced vegetation growth in spring on subsequent summer/autumn vegetation growth that sustained vegetation greening and led to a slight increase in the land carbon sink over the spring and summer of 2015(average increases of 23.34%and 0.63%in net ecosystem exchange from two independent datasets relative to a 5-years average before the El Niño event,respectively)and spring of 2016(6.82%),especially in the extra-tropics of the NH,where the water supply during the pre-growing-season(November of the previous year to March of the current year)had a positive *** seasonal compensation effect was much stronger than that in 1997 and 1998 and significantly alleviated the adverse impacts of the 2015/2016 El Niño event on vegetation growth during its maturation *** legacy effect of water supply during the pre-growing-season on subsequent vegetation growth lasted up to approximately six *** findings highlight the role of seasonal compensation effects on mediating the land carbon sink in response to episodic extreme El Niño events.

关键词： El Niño Seasonal compensation effect Vegetation greening Land carbon sink Net ecosystem exchange Legacy effect

Achieving a superior Na storage performance of Fe-based Prussian blue cathode by coating perylene tetracarboxylic dianhydride amine

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Carbon Energy 2024年第5期6卷 53-64页

作者： Xin-Yuan Fu Lu-Lu Zhang Zhao-Yao Chen Yunkai Xu Junxiu Wu Cheng-Cheng Wang Xiao-Kai Ding Xue-Lin yang Jun Lu Hubei Provincial Collaborative Innovation Center for New Energy Microgrid College of Electrical Engineering&New EnergyChina Three Gorges UniversityYichangHubeiChina College of Materials and Chemical Engineering China Three Gorges UniversityYichangHubeiChina College of Chemical and Biological Engineering Zhejiang UniversityHangzhouChina

Fe-based Prussian blue(Fe-PB)cathode material shows great application potential in sodium(Na)-ion batteries due to its high theoretical capacity,long cycle life,low cost,and simple preparation ***,the crystalline water and vacancies of Fe-PB lattice,the low electrical conductivity,and the dissolution of metal ions lead to limited capacity and poor cycling *** this work,a perylene tetracarboxylic dianhydride amine(PTCDA)coating layer is successfully fabricated on the surface of Fe-PB by a liquid-phase *** aminated PTCDA(PTCA)coating not only increases the specific surface area and electronic conductivity but also effectively reduces the crystalline water and vacancies,which avoids the erosion of Fe-PB by ***,the PTCA layer reduces the charge transfer resistance,enhances the Na-ion diffusion coefficient,and improves the structure *** PTCA-coated Fe-PB exhibits superior Na storage performance with a first discharge capacity of 145.2 mAh g^(−1) at 100 mA g^(−1).Long cycling tests exhibit minimal capacity decay of 0.027%per cycle over 1000 cycles at 1 A g^(−1).Therefore,this PTCA coating strategy has shown promising competence in enhancing the electrochemical performance of Fe-PB,which can potentially serve as a universal electrode coating strategy for Na-ion batteries.

关键词： cathode material coating Fe-based Prussian blue Na-ion batteries perylene tetracarboxylic dianhydride amine

Single crystal growth and characterization of 166-type magnetic kagome metals

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Chinese Physics B 2024年第9期33卷 145-150页

作者： Huangyu Wu Jinjin Liu Yongkai Li Peng Zhu Liu yang Fuhong Chen Deng Hu Zhiwei Wang Centre for Quantum Physics Key Laboratory of Advanced Optoelectronic Quantum Architecture and Measurement(MOE)School of PhysicsBeijing Institute of TechnologyBeijing 100081China Beijing Key Laboratory of Nanophotonics and Ultrafine Optoelectronic Systems Beijing Institute of TechnologyBeijing 100081China Beijing Institute of Technology Zhuhai 519000China Material Science Center Yangtze Delta Region Academy of Beijing Institute of TechnologyJiaxing 314011China

Kagome magnets were predicted to be a good platform to investigate correlated topology band structure,Chern quantum phase,and geometrical frustration due to their unique lattice *** we reported single crystal growth of 166-type kagome magnetic materials,including HfMn_(6)Sn_(6),ZrMn_(6)Sn_(6),GdMn_(6)Sn_(6)and GdV_(6)Sn_(6),by using the flux method with Sn as the *** them,HfMn_(6)Sn_(6)and ZrMn_(6)Sn_(6)single crystals were grown for the first time.X-ray diffraction measurements reveal that all four samples crystallize in HfFe6Ge6-type hexagonal structure with space group P6/*** samples show metallic behavior from temperature dependence of resistivity measurements,and the dominant carrier is hole,except for GdV6Sn6 which is electron *** samples have magnetic order with different transition temperatures,HfMn_(6)Sn_(6),ZrMn_(6)Sn_(6)and GdV_(6)Sn_(6)are antiferromagnetic with TN of 541 K,466 K and 4 K respectively,while GdMn_(6)Sn_(6)is ferrimagnetic with the critical temperature of about 470 *** study will enrich the research platform of magnetic kagome materials and help explore the novel quantum phenomena in these interesting *** dataset of specific crystal structure parameters for HfMn_(6)Sn_(6)are available in Science Data Bank,with the link.

关键词： kagome metal single crystal growth crystal structure physical property

Asperochones A and B,two antimicrobial aromatic polyketides from the endophytic fungus Aspergillus ***-2

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Chinese Chemical Letters 2024年第9期35卷 206-209页

作者： Hong Zhang Cui-Ping Li Li-Li Wang Zhuo-Da Zhou Wen-Sen Li Ling-Yi Kong Ming-Hua yang Jiangsu Key Laboratory of Bioactive Natural Product Research and State Key Laboratory of Natural Medicines China Pharmaceutical UniversityNanjing 210009China

Two novel fungal metabolites,asperochones A and B,were obtained from an Aspergillus *** structures were determined by 1D/2D nuclear magnetic resonance(NMR)spectroscopy,high resolution electrospray ionization mass spectroscopy(HRESIMS),and single-crystal X-ray diffraction *** A possesses an intriguing skeleton bearing 5/6/6/6/7/5/5/5 octacyclic ring system,and asperochone B also exhibits an unusual carbon skeleton with five stereochiral *** structures were proposed as heterotrimeric and heterodimeric products of aromatic *** addition,asperochone A exhibited a potential anti-tuberculosis effect since it showed a moderate potency against Mycobacterium smegmatis.

关键词： Aspergillus sp. Asperochones A and B Aromatic polyketides Heterotrimeric compound Anti-tuberculosis effect Antifibrotic activity

Self-synchronized multi-color Q-switched fiber laser using a parallel-integrated fiber Bragg grating

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Chinese Optics Letters 2024年第6期22卷 148-153页

作者： Chao Zeng Guangwei yang Dong Li Pengtao Luo Ruohui Wang Yueqing Du Dong Mao Jianlin Zhao Key Laboratory of Light Field Manipulation and Information Acquisition Ministry of Industry and Information TechnologySchool of Physical Science and TechnologyNorthwestern Polytechnical UniversityXi’an 710072China Research&Development Institute of Northwestern Polytechnical University in Shenzhen Shenzhen 518063China School of Physics Northwest UniversityXi’an 720127China

We demonstrate an intracavity self-synchronized multi-color Q-switched fiber laser using a parallel-integrated fiber Bragg grating(PI-FBG), fabricated by a femtosecond laser with a point-by-point parallel inscription method. The multi-color Q-switched pulses can be always self-synchronized when the group delay differences between neighboring spectra range from-3.4 to 3.4 *** starting and evolution dynamics indicate that the saturable absorption effect of the carbon nanotube plays a dual role: synchronously triggering the startup of the pulse at successive colors by active Q-switching and spontaneously compensating to some extent the temporal walk-off of the multi-color pulses through the cross saturable absorption modulation. This work unveils the intracavity self-synchronization mechanism of the multi-color Q-switched pulses and also demonstrates the potential of PI-FBGs for the customizable generation of the synchronized multi-color pulse in a single cavity.

关键词： synchronized pulse sources Q-switched fiber lasers saturable absorption effect fiber Bragg grating

CMKLR1 senses chemerin/resolvin E1 to control adipose thermogenesis and modulate metabolic homeostasis

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Fundamental Research 2024年第3期4卷 575-588页

作者： Zewei Zhao Siqi Liu Bingxiu Qian Lin Zhou Jianglin Shi Junxi Liu Lin Xu Zhonghan yang Department of Biochemistry Molecular Cancer Research CenterSchool of MedicineSun Yat-sen UniversityShenzhenGuangdong 518107China Department of Biochemistry Zhongshan School of MedicineSun Yat-sen UniversityGuangzhouGuangdong 510080China School of Public Health Sun Yat-sen UniversityGuangzhouGuangdong 510080China

Induction of beige fat for thermogenesis is a potential therapy to improve homeostasis against obesity.β3-adrenoceptor(β3-AR),a type of G protein-coupled receptor(GPCR),is believed to mediate the thermogenesis of brown fat in ***,β3-AR has low expression in human adipose tissue,precluding its activation as a standalone clinical *** study aimed at identifying a potential GPCR target to induce beige *** found that chemerin chemokine-like receptor 1(CMKLR1),one of the novel GPCRs,mediated the development of beige fat via its two ligands,chemerin and resolvin E1(RvE1).The RvE1 levels were decreased in the obese mice,and RvE1 treatment led to a substantial improvement in obese features and augmented beige fat ***,despite sharing the same receptor as RvE1,the chemerin levels were increased in obesogenic conditions,and chemerin treatment led to an augmented obese phenotype and a decline of beige fat ***,RvE1 and chemerin induced or restrained the development of beige fat,respectively,via the mechanistic target of rapamycin complex 1(mTORC1)signaling *** further showed that RvE1 and chemerin regulated mTORC1 signaling differentially by forming hydrogen bonds with different binding sites of *** conclusion,our study showed that RvE1 and chemerin affected metabolic homeostasis differentially,suggesting that selectively modulating CMKLR1 may be a potential therapeutic target for restoring metabolic homeostasis.

关键词： Obesity Insulin resistance Thermogenesis CMKLR1 Resolvin E1 Chemerin