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Impact of warming and nitrogen addition on soil greenhouse gas fluxes:A global perspective

Journal of Environmental Sciences 2025年第5期151卷 88-99页

作者： Hongze Ma Xiaoyu Jia Weiguang Chen jingyi yang jin Liu Xiaoshan Zhang Ke Cui Zhouping Shangguan Weiming Yan State Key Laboratory of Soil Erosion and Dryland Farming on the Loess Plateau College of Soil and Water Conservation Science and EngineeringNorthwest A&F UniversityYanglingShaanxi 712100China Institute of Soil and Water Conservation Chinese Academy of SciencesYanglingShaanxi 712100China University of Chinese Academy of Sciences Beijing 100049China Shaanxi Institute of Geo-Environment Monitoring Xi’an 710000China

Global warming and nitrogen(N)deposition have a profound impact on greenhouse gas(GHG)fluxes and consequently,they also affect climate ***,the global combined effects of warming and N addition on GHG fluxes remain to be fully *** address this knowledge gap,a globalmeta-analysis of 197 datasets was performed to assess the response of GHG fluxes to warming and N addition and their interactions under various climate and experimental *** results indicate that warming significantly increased CO_(2)emissions,while N addition and the combined warming and N addition treatments had no impact on CO_(2)***,both warming and N addition and their interactions exhibited positive effects on N_(2)O *** the combined warming and N addition treatments,warming was observed to exert a positive main effect on CO_(2)emissions,while N addition had a positive main effect on N_(2)O *** interactive effects of warming and N addition exhibited antagonistic effects on CO_(2),N_(2)O,and CH_(4)emissions,with CH_(4)uptake dominated by additive ***,we identified biome and climate factors as the two *** findings indicate that both warming and N addition substantially impact soil GHG fluxes and highlight the urgent need to investigate the influence of the combination of warming and N addition on terrestrial carbon and N cycling under ongoing global change.

关键词： Warming Nitrogen(N)addition Greenhouse gas(GHG)fluxes Interactive effects Biome

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Plastic flow and interfacial bonding behaviors of embedded linear friction welding process:Numerical simulation combined with thermophysical experiment

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Chinese Journal of Aeronautics 2025年第1期38卷 87-98页

作者： Tiejun MA Zhenguo GUO Xiawei yang Junlong jin Xi CHEN Jun TAO Wenya LI Achilles VAIRIS Liukuan YU State Key Laboratory of Solidification Processing Shaanxi Key Laboratory of Friction Welding TechnologiesNorthwestern Polytechnical UniversityXi'an 710072China Aeronautical Key Laboratory for Welding and Joining Technologies AVIC Manufacturing Technology InstituteBeijing 100024China Mechanical Engineering Department University of West AtticaAthens 12241Greece Mathematic and Physic Department Xianjiaotong-liverpool UniversitySuzhou 215123China

In this study,a new linear friction welding(LFW)process,embedded LFW process,was put forward,which was mainly applied to combination manufacturing of long or overlong loadcarrying titanium alloy structural components in *** interfacial plastic flow behavior and bonding mechanism of this process were investigated by a developed coupling EulerianLagrangian numerical model using software ABAQUS and a novel thermo-physical simulation method with designed embedded hot compression *** addition,the formation mechanism and control method of welding defects caused by uneven plastic flow were *** results reveal that the plastic flow along oscillating direction of this process is even and *** the direction perpendicular to oscillation,thermo-plastic metals mainly flow downward along welding interface under coupling of shear stress and interfacial pressure,resulting in the interfacial plastic zone shown as an inverted“V”*** upward plastic flow in this direction is relatively weak,and only a small amount of flash is extruded from top of ***,the wedge block and welding components at top of joint are always in un-steady friction stage,leading to nonuniform temperature field distribution and un-welded *** to the results of numerical simulation,high oscillating frequency combined with low pressure and small amplitude is considered as appropriate parameter selection scheme to improve the upward interfacial plastic flow at top of joint and suppress the un-welded *** results of thermo-physical simulation illustrate that continuous dynamic recrystallization(CDRX)induces the bonding of interface,accompanying by intense dislocation movement and creation of many low-angle grain *** the interfacial bonding area,grain orientation is random with relatively low texture density(5.0 mud)owing to CDRX.

关键词： Embedded linear friction welding Plastic flow Interfacial bonding behavior Numerical simulation Thermo-physical simulation Temperature field Dynamic recrystallization

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H_6P_2W_(18)O_(62)/TiO_2-SiO_2光催化降解有机染料

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精细化工 2015年第5期32卷 571-577页

作者：杨志远刘晓霞徐玉林杨水金湖北师范学院化学化工学院稀有金属化学湖北省协同创新中心湖北黄石435002

采用浸渍法制备了H6P2W18O62/Ti O2-Si O2光催化剂,并采用傅里叶变换红外光谱（FTIR）、X射线粉末衍射（XRD）、扫描电子显微镜（SEM）对其进行了表征。通过光催化剂H6P2W18O62/Ti O2-Si O2对含甲基橙模拟废水进行处理,结果表明,H6P2W18... 详细信息

采用浸渍法制备了H6P2W18O62/Ti O2-Si O2光催化剂,并采用傅里叶变换红外光谱（FTIR）、X射线粉末衍射（XRD）、扫描电子显微镜（SEM）对其进行了表征。通过光催化剂H6P2W18O62/Ti O2-Si O2对含甲基橙模拟废水进行处理,结果表明,H6P2W18O62/Ti O2-Si O2光催化剂表现出较高的光催化性能,在催化剂用量为1.39 g/L,甲基橙溶液质量浓度为5 mg/L,初始p H=3.5,反应时间2.5 h的条件下,甲基橙的降解率可达99.2%,且产生了协同效应。H6P2W18O62/Ti O2-Si O2光催化剂对罗丹明B、亚甲基蓝和甲基红均具有较高的光催化性能,降解率达84.0%~100.0%。光催化剂还表现出较好的重复使用性能,第5次降解率仍为94.4%。

关键词： H6P2W18O62/Ti O2-Si O2 光催化降解甲基橙水处理技术与环境保护

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H_2O_2处理H_3PW_6Mo_6O_(40)/ZrO_2-SiO_2光催化降解甲基橙

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化学研究与应用 2017年第4期29卷 459-464页

作者：杨水金段国滨徐玉林湖北师范大学化学化工学院污染物分析与资源化技术湖北省重点实验室湖北黄石435002

采用浸渍法制备了H_3PW_6Mo_6O_(40)/ZrO_2-SiO_2催化剂,用H_2O_2进行敏化处理,并通过FT-IR、XRD对其进行了表征。探讨了该催化剂对甲基橙溶液的催化降解活性,较系统地研究了溶液的初始浓度、溶液的pH、催化剂用量对光催化降解甲基橙的... 详细信息

采用浸渍法制备了H_3PW_6Mo_6O_(40)/ZrO_2-SiO_2催化剂,用H_2O_2进行敏化处理,并通过FT-IR、XRD对其进行了表征。探讨了该催化剂对甲基橙溶液的催化降解活性,较系统地研究了溶液的初始浓度、溶液的pH、催化剂用量对光催化降解甲基橙的影响。研究发现:H_3PW_6Mo_6O_(40)/ZrO_2-SiO_2对甲基橙有良好的降解效果。在甲基橙溶液初始浓度为10mg·L^(-1),溶液pH为2.5,催化剂用量为溶液总质量0.5%的条件下光照2.5h,甲基橙的降解率达到91.1%。H_3PW_6Mo_6O_(40)/ZrO_2-SiO_2催化剂光催化降解甲基橙溶液为一级动力学反应。

关键词： H3PW6Mo6O4i/ZrO2-SiO2 光催化降解甲基橙

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Broadband low-frequency sound absorption of multifunctional composite metastructure

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Science China(Technological Sciences) 2025年第2期68卷 114-124页

作者： Yilong yang Shanshan LIU Yan LI Tong GAO Yongdong PAN Yong LI Yabin jin School of Aerospace Engineering and Applied Mechanics Tongji UniversityShanghai 200092China State International Joint Research Center of Aerospace Design and Additive Manufacturing Northwestern Polytechnical UniversityXi’an 710072China Institute of Acoustics School of Physics Science and EngineeringTongji UniversityShanghai 200092China Shanghai Key Laboratory of Intelligent Sensing and Detection Technology School of Mechanical and Power EngineeringEast China University of Science and TechnologyShanghai 200237China Shanghai Institute of Aircraft Mechanics and Control Shanghai 200092China

In this study,we fabricated multifunctional metastructures from carbon fiber-reinforced plastic composites using additive manufacturing *** metastructures are characterized by their lightweight,load-bearing capacity,and broadband low-frequency sound absorption *** metastructure consists of 36 unit cells,and non-local coupling mechanism was considered for designing the sound absorption *** developed an acoustic impedance theory tailored for the metastructure,facilitating an analysis of thermal and viscous dissipation *** is proven theoretically and experimentally that the proposed composite metastructure can achieve a noise reduction with an average sound absorption coefficient greater than 0.9 across frequencies in the rage of 330-1500 *** also studied the metastructure’s quasi-static and cyclic compression performance,confirming its efficient absorption capabilities after cyclic *** proposed design and additive manufacturing method for composite metastructures provides a novel pathway for creating lightweight,multifunctional structures with diverse applications,such as aerospace engineering.

关键词： composite metastructure broadband sound absorption additive manufacturing

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H3PW6Mo6O40／SiO2催化合成7-羟基4-甲基香豆素

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化学研究与应用 2012年第9期24卷 1354-1358页

作者：杨水金黄永葵李萍徐明波湖北师范学院化学与环境工程学院污染物分析与资源化技术湖北省重点实验室湖北黄石435002

采用溶胶-凝胶法制备了二氧化硅负载磷钨钼杂多酸催化剂H3PW6Mo6O40/SiO2,该催化剂制备的适宜条件是:m(H3PW6Mo6O40)∶m(SiO2)=40%,煅烧温度150℃,活化时间3 h。以二氧化硅负载磷钨钼酸为催化剂,在无溶剂条件下由间苯二酚和乙酰乙酸乙... 详细信息

采用溶胶-凝胶法制备了二氧化硅负载磷钨钼杂多酸催化剂H3PW6Mo6O40/SiO2,该催化剂制备的适宜条件是:m(H3PW6Mo6O40)∶m(SiO2)=40%,煅烧温度150℃,活化时间3 h。以二氧化硅负载磷钨钼酸为催化剂,在无溶剂条件下由间苯二酚和乙酰乙酸乙酯为原料进行Pechmann反应合成7-羟基-4-甲基香豆素。考察了反应物间苯二酚与乙酰乙酸乙酯摩尔比,催化剂用量,反应温度,反应时间等因素对收率的影响,并对反应条件进行优化。结果表明,在间苯二酚与乙酰乙酸乙酯的摩尔比为1∶1.5(其中间苯二酚为0.1mol),反应时间为16 h,H3PW6Mo6O40/SiO2的用量为1.3 g,在油浴加热120℃左右的优化条件下,7-羟基-4-甲基香豆素的收率可达86.1%。

关键词： H3PW6Mo6O40/SiO2 Pechmann反应 7-羟基4-甲基香豆素

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Distinct MLT asymmetry of auroral kilometric radiation observed by the FAST satellite

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Earth and Planetary Physics 2025年第1期9卷 188-193页

作者： JiaWen Tang Sai Zhang FuLiang Xiao HongMing yang Si Liu YiHua He Chang yang YuYue jin ZhouKun Deng Ping Li Archie James Johnston School of Physics and Electronic Sciences Changsha University of Science and TechnologyChangsha 410114China Hunan Province Higher Education Key Laboratory of Modeling and Monitoring on the Near-Earth Electromagnetic Environments Changsha University of Science and TechnologyChangsha 410114China School of Electrical and Information Engineering Changsha University of Science and TechnologyChangsha 410114China

Auroral Kilometric Radiation (AKR) is a common radio emission,which can contribute to the magnetosphere-ionosphereatmosphere co u *** emissions have been observed in all magnetic planet magnetospheres of the solar *** this study,using observations from the FAST satellite from 30 August 1996 to 9 September 2001,the distribution of AKR in altitude=500-4500 km and invariant latitude (|ILAT|)=60°-80°has been analyzed.63045 AKR samples have been identified with~48%(52%) samples on the dayside (nightside).Of considerable interest,there is a distinct MLT asymmetry with the high occurrence rate in MLT=05-08 and 18-22(02-05 and 12-17) in the northern (southern) *** distinct MLT asymmetry is associated with the direction of Bxof the interplaneta ry magnetic *** addition,the occurrence rate on the nightside clearly increases as the AE^(*) index *** study further enriches the information and understanding of AKR in the magnetosphere as well as other similar radio emissions.

关键词： asymmetry auroral kilometric radiation interplanetary magnetic field

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磷钨酸借自然光催化甲基橙溶液降解脱色的研究

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化学试剂 2006年第9期28卷 515-517页

作者：王敏朱佐毅白爱民杨水金华中师范大学化学学院湖北武汉430079 湖北师范学院生化分析技术湖北省重点实验室湖北黄石435002

研究了以磷钨酸为光催化剂,在自然光照条件下模拟染料废水甲基橙溶液的光催化脱色性能。实验结果表明,催化剂类型,光照条件,催化剂的投入量,甲基橙的初始浓度,光照时间以及光照强度是影响甲基橙溶液脱色率的重要因素。当磷钨酸的浓度为2... 详细信息

研究了以磷钨酸为光催化剂,在自然光照条件下模拟染料废水甲基橙溶液的光催化脱色性能。实验结果表明,催化剂类型,光照条件,催化剂的投入量,甲基橙的初始浓度,光照时间以及光照强度是影响甲基橙溶液脱色率的重要因素。当磷钨酸的浓度为2.0 g/L,甲基橙的初始浓度为10 mg/L,自然光照时间为2.5 h时,甲基橙溶液的脱色率可达95.9%。

关键词：磷钨酸光催化降解甲基橙

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Synthesis of 4-Methyl-2-Isopropyl-1,3-Dioxolane by TiSiW_(12)O_(40)/TiO_2 as Catalyst

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合成化学 2004年第Z1期12卷 66-66页

作者： yang shui-jin YU Xie-qing Department of Chemistry and Environmental Engineering Hubei Normal University Huangshi 435002 China Department of Chemistry and Environmental Engineering Hubei Normal University Huangshi 435002 China

Acetals and ketals are a kind of the important compounds and used to protect carbonyl,middle material of the organic synthesis. What's more, they are a sort of the widely use flavor substance. 4-Methyl-2-isopropyl-1,3-dioxolane has fresh fruit odor and apple note. It is used to producing many sorts of essence. And the conventional method to synthesize 4-methyl-2-isopropyl-1,3-dioxolane makes use of sulfuric acid as catalyst in factories. But it causes many problems, such as the erosion of production equipment, difficulty after-treatment, low quality of the products, etc. HPA and its salts shows excellent catalytic activity to the esterification and have recently attracted much attention as catalysts for various industrial processes, because their acidic and redox properties can be controlled at atomic/molecular levels. Misono, Pope [1], and Wang [2]have reviewed the homogeneous catalysis and fine organic synthesis catalyzed by heteropoly compounds. However, there is no report on the synthesis of 4-methyl-2-isopropyl-1,3-dioxolane catalyzed by TiSiW12O40/TiO2. TiSiW12O40/TiO2 was prepared according to reference [3] and identified by means of IR and XRD. The reaction was carried out in a three-neck flask equipped with a stirrer, a reflux condenser, and a thermometer. A certain amounts of isobutyraldehyde,1,2-propanediol and the catalyst was heated to boiling and refluxed until no water flowed off. The purified product was analyzed by IR spectra and *** this paper, we report 4-methyl-2-isopropyl-1,3-dioxolane was synthesized from isobutyraldehyde and 1,2-propanediol in the presence of TiSiW12O40/TiO2. The factors influencing the yield of product and the optimum reaction conditions were discussed. The optimum conditions are molar ratio of isobutyraldehyde to 1,2-propanediol was 1:1.5, the quantity of catalyst was equal to 0.5% feed stock, and the reaction time was 1.0 h. TiSiW12O40/TiO2 was an excellent catalyst to synthesize 4-methyl-2-isopropyl-1,3-dioxolane and

关键词： 4-Methyl-2-isopropyl-1,3-dioxolane, TiSiW12O40/TiO2, catalysis, acetalation.

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微藻去除重金属镉的抗性机理研究进展

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微生物学通报 2017年第8期44卷 1980-1987页

作者：孔祥雪李宝珍杨金水农业生物技术国家重点实验室中国农业大学生物学院北京100193

与水体中重金属去除的传统方法相比,生物吸附法是一种更具经济效益和环境效益的技术。微藻由于自身的廉价性和高吸附性已成为高效生物吸附剂的材料来源。要评价微藻在镉(Cd)去除方面的应用潜力,解析微藻抗重金属的机理是必要条件。因此... 详细信息

与水体中重金属去除的传统方法相比,生物吸附法是一种更具经济效益和环境效益的技术。微藻由于自身的廉价性和高吸附性已成为高效生物吸附剂的材料来源。要评价微藻在镉(Cd)去除方面的应用潜力,解析微藻抗重金属的机理是必要条件。因此,本文从抗Cd微藻种类,Cd对微藻光合作用、生长及结构的影响,胞外吸附的机理,胞内积累的机理,以及基因调控水平,阐述了目前微藻抗Cd的研究进展,以期为后续的研究提供理论帮助。

关键词：微藻镉抗性机理胞外吸附胞内积累

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