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Enhanced post-combustion CO_(2) capture and direct air capture by plasma surface functionalization of graphene adsorbent

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Journal of Energy Chemistry 2025年第1期100卷 653-664页

作者： Rahul Navik Eryu Wang Xiao ding Huang yunyi yiyu Liu Jia Li Guangdong-Hong Kong Joint Laboratory for Carbon Neutrality Jiangmen Laboratory of Carbon and Science and TechnologyJiangmen 529100GuangdongChina Guangzhou HKUST Fok ying Tung Research Institute Guangzhou 511458GuangdongChina The Hong Kong University of Science and Technology(Guangzhou) Guangzhou 511453GuangdongChina Stoddart Institute of Molecular Science Department of ChemistryZhejiang UniversityHangzhou 310058ZhejiangChina Carbon Neutrality and Climate Change Thrust Society HubThe Hong Kong University of Science and Technology(Guangzhou)Guangzhou 511453GuangdongChina

Graphene has enormous potential to capture CO_(2)due to its unique properties and ***,graphene-based adsorbents have drawbacks of lower CO_(2)adsorption capacity and poor *** work demonstrates a one-step rapid and sustainable N_(2)/H_(2)plasma treatment process to prepare graphene-based sorbent material with enhanced CO_(2)adsorption *** treatment directly enriches amine species,increases surface area,and improves textural *** CO_(2)adsorption capacity increases from 1.6 to 3.3 mmol/g for capturing flue gas,and from 0.14 to 1.3 mmol/g for direct air capture (DAC).Importantly,the electrothermal property of the plasma-modified aerogels has been significantly improved,resulting in faster heating rates and significantly reducing energy consumption compared to conventional external heating for regeneration of *** aerogels display improved selectivity of 42 and 87 after plasma modification for 5 and 10 min,*** plasma-treated aerogels display minimal loss between 17%and 19% in capacity after 40 adsorption/desorption cycles,rendering excellent *** N_(2)/H_(2)plasma treatment of adsorbent materials would lower energy expenses and prevent negative effects on the global economy caused by climate change.

关键词： Carbon neutrality CO_(2)capture Climate change Plasma treatment Graphene aerogel

Study on the off situ reconstruction of the core neutron field based on dual-task hybrid network architecture

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Nuclear Science and Techniques 2025年第1期36卷 175-191页

作者： Pei Cao Hui ding Cheng-Long Cao Zi-Hui yang Guo-Min Sun School of Artificial Intelligence and Big Data Hefei UniversityHefei 230001China College of Electronic Engineering National University of Defense TechnologyHefei 230001China Institute of Nuclear Energy Safety Technology HFIPSChinese Academy of SciencesHefei 230027China

The off situ accurate reconstruction of the core neutron field is an important step in realizing real-time reactor *** existing off situ reconstruction method of the neutron field is only applicable to cases wherein a single region changes at a specified location of the ***,when the neutron field changes are complex,the accurate identification of the individual changed regions becomes challenging,which seriously affects the accuracy and stability of the neutron field ***,this study proposed a dual-task hybrid network architecture(DTHNet)for off situ reconstruction of the core neutron field,which trained the outermost assembly reconstruction task and the core reconstruction task jointly such that the former could assist the latter in the reconstruction of the core neutron field under core complex ***,to exploit the characteristics of the ex-core detection signals,this study designed a global-local feature upsampling module that efficiently distributed the ex-core detection signals to each reconstruction unit to improve the accuracy and stability of *** experiments were performed on the simulation datasets of the CLEAR-I reactor to verify the accuracy and stability of the proposed *** results showed that when the location uncertainty of a single region did not exceed nine and the number of multiple changed regions did not exceed ***,the reconstructed ARD was within 2%,RD_(max)was maintained within 17.5%,and the number of RD≥10%was maintained within ***,when the noise interference of the ex-core detection signals was within±2%,although the average number of RD≥10%increased to 16,the average ARD was still within in 2%,and the average RD_(max)was within 22%.Collectively,these results show that,theoretically,the DTHNet can accurately and stably reconstruct most of the neutron field under certain complex core changes.

关键词： Real-time reactor monitoring Core neutron field reconstruction Dual-task hybrid network architecture Global-local feature upsampling module

Aqueous indium metal batteries

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Chinese Chemical Letters 2025年第2期36卷 34-35页

作者： Jingjing Zhang Lan ding Vadim Popkov Kezhen Qi College of Pharmacy Dali University Hydrogen Energy Laboratory Ioffe Institute

Energy storage devices have been extensively owing to their critical role in addressing the energy and environment *** trivalent metal batteries are promising due to their unique three-electron redox reactions for high reversible capacity and high safety [1]. Especially, aqueous aluminum-based batteries have attracted significant attention [2]. However, severe water decomposition occurs due to their low redox potential (Al3+/Al,-1.66 V vs. SHE)[3]. In contrast, the metallic indium (In)/or In3+has a more suitable redox potential (-0.34 V vs. SHE), which is within the water stability window, minimizingwater decomposition [4]. Recently, a study on trivalent indium metal batteries was firstly reported by Wu’s group in Journal of the American Chemical Society [5].

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World Journal of Gastroenterology 2025年第8期31卷 115-129页

作者： Han ding Zhi-Guo ding Song Liu Xu-Nan Mao Xing-Sheng Lu Department of Endoscopy Center and Endoscopy Research Institute Zhongshan HospitalThe Affiliated to Fudan UniversityShanghai 200032China Department of General Surgery Xinhua Hospital Affiliated to Shanghai Jiao Tong University School of MedicineShanghai 200092China Department of General Surgery The Third People’s Hospital of YangzhouYangzhou 225126Jiangsu ProvinceChina Department of General Surgery The Fourth Affiliated Hospital of Soochow UniversitySuzhou 215000Jiangsu ProvinceChina Medical College Yangzhou UniversityYangzhou 225009Jiangsu ProvinceChina

BACKGROUND Ras-related protein Rab24,which belongs to the small GTPase family,plays a crucial role in regulating intracellular protein *** of Rab24 has been recently identified in hepatocellular carcinoma(HCC).However,its clinical significance and tumor related effects remain to be further *** To explore the expression pattern of Rab24 and its role in HCC *** The expression profile of Rab24 was tested in HCC tissues together with adjacent tissues from transcriptional,mRNA,and protein *** prognostic role of Rab24 in HCC was assessed by univariate and multivariate *** outcomes were evaluated by the Kaplan-Meier analysis and log-rank *** effect of Rab24 on cell proliferation was tested through cellular experiments and xenograft *** Rab24 expression was elevated in HCC tissues compared to adjacent liver *** expression of Rab24 was significantly associated with larger tumor size and advanced tumor ***,HCC patients with high Rab24 expression showed poorer overall survival,and Rab24 was identified as an independent prognosis factor according to multivariate *** using overexpression and shRNA knockdown strategies in HCC cell lines,we found that Rab24 can promote HCC ***,we validated that silencing Rab24 significantly attenuated xenograft growth in *** Our study demonstrated that high expression of Rab24 was significantly correlated with poorer prognosis of HCC patients,indicating the potential of Rab24 as a novel clinical biomarker and therapeutic target.

关键词： Hepatocellular carcinoma Ras-related protein Rab24 Prognosis Proliferation

Mossbauer,optical and structural properties of Fe^(3+) ion in borate glass

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Journal of Rare Earths 2025年第1期43卷 162-170,I0006页

作者： Essam A.Elkelany Hesham y.Amin A.Samir M.M.EL-Hady H.H.El-Bahnasawy Moukhtar A.Hassan Basic Science Department Faculty of EngineeringSinai UniversityAl-Arish45511Egypt School of Information and Electrical Engineering Hangzhou City UniversityHangzhou30015China State Key Laboratory of Modern Optical Instrumentation College of Optical Science and EngineeringZhejiang UniversityHangzhou310027China Basic Science Department Faculty of Engineering at ShoubraBenha University11629Egypt Physics Department Faculty of ScienceAl-Azhar University11884CairoEgypt

Lanthanum-bearing iron lithium borate glass is a quaternary system for oxide glasses and was prepared via the melt-quenching *** present article correlates the structure,optical,ligand field and M?ssbauer data on iron lithium borate glass co ntaining La^(3+).The density was measured,while the molar volume was *** physical parameters are *** increasing the La_(2)O_(3) content within the glass network,infrared spectra analysis reveals structural modifications such as the increase in BO_(4) units and the decline in both BO_(3) units and NBO bonds ***,optical absorption spectra were *** absorption spectra disclose a plethora of electronic transitions that are related to Fe^(3+)in tetrahedral and octahedral sites,however,Fe^(2+)phase is not observed in optical spectra,but it has a clear signature in M?ssbauer ***,the glass absorption edges undergo a clear blue shift,reflecting an increased band gap energy(1.96-2.28 eV).The decline in NBO bonds justifies this ***,the values of crystal field splitting are increased,while the values of Racah parameters are *** trend is justified by the decline in NBO bonds and increases electron localization around Fe cations.M?ssbauer spectra confirm the existence of Fe^(3+)in tetrahedral and octahedral sites,while Fe^(2+)exists in only a tetrahedral *** increasing La_(2)O_(3) content,the isomer shift of Fe^(3+)in tetrahedral sites changes to be 0.312-0.329 mm/s,while the isomer shift of octahedral Fe^(3+)is 0.424-0.456 mm/*** findings coincide with optical *** the isomer shift of tetrahedral Fe^(2+)is 0.902-0.911 mm/*** results of structural,optical and ligand field associated with M?ssbauer spectra open more vistas toward the utility of these samples in the optics realm.

关键词： Fe3+ions Rare-earth oxide Mossbauer spectra Ligand field parameters Optical properties

Improvement of charge-transfer kinetics via MXene and cobalt containing polyoxometalate loading on CdS for photocatalytic hydrogen production

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Science China Chemistry 2025年第2期68卷 772-780页

作者： yu Feng Xiao Fang Jinnuo Zang Bin Song Chunlian Hu Xiaoyu Dong yong ding State Key Laboratory of Applied Organic Chemistry Key Laboratory of Advanced Catalysis of Gansu ProvinceCollege of Chemistry and Chemical EngineeringLanzhou UniversityLanzhou 730000China State Key Laboratory of Low Carbon Catalysis and Carbon Dioxide Utilization State Key Laboratory for Oxo Synthesis and Selective OxidationLanzhou Institute of Chemical PhysicsChinese Academy of SciencesLanzhou 730000China

Hydrogen is a renewable and clean energy,and photocatalytic water splitting for hydrogen evolution technology is a promising technical means to solve the development *** this study,the ternary composite Co_(8)POM@MXene–CdS hybrid catalyst was constructed and used for photocatalytic hydrogen *** the condition of AM 1.5G simulated sunlight,the photocatalytic H_(2) evolution rate of the ternary composite was 8.13 mmol g^(−1) h^(−1),which was more than 25 times higher than that of the bare *** means of synchronous illumination X-ray photoelectron spectroscopy(SI-XPS)and density functional theory(DFT)calculations,it was proved that the loading of MXene and Co_(8)POM improved the photogenerated carrier separation and immigration efficiency on *** photogenerated electrons transfer from CdS to ***_(8)POM containing the{Co_(4)O_(3)}quasi-cubane,as an oxidation co-catalyst,accepts photogenerated holes from CdS to catalyze the oxidation reaction of TEOA,which improves the photocatalytic hydrogen production activity and the stability of CdS.

关键词： CdS polyoxometalates MXene hybrid catalyst photocatalytic hydrogen evolution

Forming limit and failure behavior of fiber metal laminates under low-constraint conditions

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Chinese Journal of Aeronautics 2025年第1期38卷 638-653页

作者： yao WANG Feng ding yong LI yunhua ZHANG Sifa ZHENG Libin ZHAO Ning HU School of Mechanical Engineering Hebei University of TechnologyTianjin 300401China Suzhou Automotive Research Institute(Xiangcheng) Tsinghua UniversitySuzhou 215134China State Key Laboratory of Reliability and Intelligence Electrical Equipment Hebei University of TechnologyTianjin 300130China School of Mechanical Engineering and Automation Beihang UniversityBeijing 100191China Henan Benjie Technology Co. Ltd.Zhengzhou 450003China Key Laboratory of Advanced Intelligent Protective Equipment Technology Ministry of EducationTianjin 300401China Key Laboratory of Hebei Province on Scale-span Intelligent Equipment Technology Hebei University of TechnologyTianjin 300401China

Fiber Metal Laminates(FMLs),as high-performance composite materials,demonstrate exceptional potential in a wide range of applications,such as aeronautical and astronautical ***,the traditional cured FMLs possess complex interlayer stresses and low forming limits,restricting further promotion and application of ***-constraint FMLs exhibit a lower forming resistance and better formability due to no curing during the forming process;however,the formation mechanism and response are not *** paper presents the Forming Limit Diagram(FLD)of low-constraint GLARE(glass fiber reinforced aluminum laminates)based on the forming limit test,and compares it with the conventionally cured laminates to evaluate the differences in the forming *** addition,combined with the analysis of failure mechanism and micro-deformation mechanism of specimens,the influence of different temperatures(20–80℃)and forming states(width)on the deformation performance of laminates is further *** results reveal that the forming limit curve of low-constraint laminates shifts up with the increase of temperature,the forming limit initially increases with the increase of width,then followed by a gradual decrease,and the maximum principal strain of low-constraint laminates is increased by 29% at 80℃ compared to 20℃.The cured laminate has a principal strain range of 0–0.02,while the low-constraint laminates have a principal strain range of 0.03–*** with cured laminates,low-constraint laminates possess a higher forming limit due to the improvement in deformable degree between layers by resin flow and fiber slippage,which enhances their *** study is expected to serve as a reference for establishing forming limit criteria and optimizing forming schemes for low-constraint laminates.

关键词： Fiber Metal Laminates(FMLs) GLARE Low-constraint state Forming limit Failure mechanism

Advances in synaptic PET imaging and intervention with synapse-targeted small-molecular drugs for dementia diagnosis and therapy

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Fundamental Research 2025年第1期5卷 63-71页

作者： Xiuhong Lu Bin Ji Gang Huang Hong ding Shanghai Key Laboratory of Molecular Imaging Jiading District Central Hospital Affiliated Shanghai University of Medicine and Health SciencesShanghai 201318China School of pharmacy Shanghai University of Medicine and Health SciencesShanghai 201318China Department of Radiopharmacy and Molecular Imaging School of pharmacyFudan UniversityShanghai 201203China

Dementia is characterized by synaptic and neuronal dysfunction in disease-specific brain *** failure of dementia clinical trials with therapeutic drugs targeting abnormal protein aggregates has caused researchers to shift their focus to synaptic functions and increased the importance of clinically available imaging for synaptic density and the development of synapse-targeted *** density imaging with positron emission tomography(PET)tracer enables non-invasive detection of synaptic loss and hence investigates the association with other neuropathological events exemplified by disease-specific abnormal protein *** studies have reviewed the progress of synaptic density imaging;however,to our knowledge,there is no article yet that summarizes the research progress of multimodal imaging of synaptic density tracers combined with other dementia ***,synaptic function intervention for dementia therapy has not yet been *** this review,first we detail the progress of synaptic density imaging including tracer development and preclinical/clinical application,followed by a discussion of multimodal imaging of synaptic density tracers combined with classic dementia biomarkers in the clinical research ***,we briefly summarize the synapse-targeted drugs for dementia therapy.

关键词： Synaptic density imaging Synaptic vesicle protein 2A Dementia Multimodal imaging UCB-J Positron emission tomography

Upper bound stability analysis of tiered geosynthetic-reinforced soil wall

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Journal of Rock Mechanics and Geotechnical Engineering 2025年第1期17卷 556-572页

作者： Chengzhi Xiao Xiangsheng Meng Shan Gao Luqiang ding School of Civil and Transportation Engineering Hebei University of TechnologyTianjin300401China

The tiered geosynthetic-reinforced soil (GRS) walls have been increasingly applied in the high and steep retaining soil structures. However, very little is known about the design method for the tiered GRS wall in practice. This study is aimed at proposing an upper-bound stability analysis method of a tiered GRS wall. The proposed method was firstly validated by the existing results from the centrifuge test and the numerical method, and then a parametric study was performed to investigate the effects of the cohesionless backfill friction angle φ1 and the wall geometric parameters including the offset distance, the total wall height, the batter angle δ, the number of tiers n, and wall height ratio of adjacent tiers on the dimensionless equivalent earth pressure coefficient KT. The analysis results demonstrated that as the φ1 increases, the shear strength of backfill is enhanced and thus the KT or the total reinforcement tensile force decreases, and the KT decreases with the increase of the offset distance at the initial stage and then becomes stable when it reaches a certain critical value. For a fixed offset distance, the KT or the total reinforcement tensile force decreases with the increase of the δ. For the two-tiered GRS walls having the offset distance less than the critical value, the wall with the smaller wall height ratio has a larger KT. Further, the variation of the location of the critical failure surfaces of tiered GRS walls was presented in this study with the variation of the φ1 and the wall geometry.

关键词： Geosynthetics Tiered GRS walls Offset distance Upper bound theorem Internal stability