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Dual‑Donor‑Induced Crystallinity Modulation Enables 19.23% Efficiency Organic Solar Cells

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Nano-Micro Letters 2025年第3期17卷 376-388页

作者： Anhai Liang yuqing Sun Sein Chung Jiyeong Shin Kangbo Sun Chaofeng Zhu Jingjing zhao Zhenmin zhao yufei Zhong Guangye Zhang Kilwon Cho Zhipeng Kan Center On Nanoenergy Research Institute of Science and Technology for Carbon Peak&NeutralitySchool of Physical Science&TechnologyGuangxi UniversityNanning 530004People’s Republic of China Department of Chemical Engineering Pohang University of Science and TechnologyPohang 37673South Korea College of New Materials and New Energies Shenzhen Technology UniversityShenzhen 518118People’s Republic of China Zhejiang Engineering Research Center for Fabrication and Application of Advanced Photovoltaic Materials School of Materials Science and EngineeringNingboTech UniversityNingbo 315100People’s Republic of China State Key Laboratory of Featured Metal Materials and Life-Cycle Safety for Composite Structures Nanning 530004People’s Republic of China

Trap-assisted charge recombination is one of the primary limitationsof restricting the performance of organic solar cells. However, effectivelyreducing the presence of traps in the photoactive layer remains ***, wide bandgap polymer donor PTzBI-dF is demonstrated as an effectivemodulator for enhancing the crystallinity of the bulk heterojunction active layerscomposed of D18 derivatives blended with y6, leading to dense and orderedmolecular packings, and thus, improves photoluminescence quenching *** a result, the photovoltaic devices exhibit reduced trap-assisted charge recombinationlosses, achieving an optimized power conversion efficiency of over 19%.Besides the efficiency enhancement, the devices comprised of PTzBI-dF as athird component simultaneously attain decreased current leakage, improved chargecarrier mobilities, and suppressed bimolecular charge recombination, leading toreduced energy losses. The advanced crystalline structures induced by PTzBI-dFand its characteristics, such as well-aligned energy level, and complementaryabsorption spectra, are ascribed to the promising performance *** findings suggest that donor phase engineering is a feasible approach to tuning the molecular packings in the active layer, providingguidelines for designing effective morphology modulators for high-performance organic solar cells.

关键词： Trap-assisted charge recombination Photoluminescence Miscibility Current leakage Power conversion efficiency

Channel pruning on frequency response

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Science China(Information Sciences) 2025年第1期68卷 159-170页

作者： Hang LIN yifan PENG Lin BIE Chenggang yAN Xibin zhao yue GAO School of Software Tsinghua University School of Automation Hangzhou Dianzi University

Network pruning has a significant role in reducing network parameters and accelerating the inference time of the network. Some existing methods prune the network based on the frequency of the data, and finally obtain a sub-network with high accuracy. However, according to our experimental analysis, different frequencies of information in the data contribute differently to the accuracy of the model, and using this information directly for pruning without making a selection will lead to incorrect results. We believe that pruning should retain the convolutional kernels in the network that process important information, while those kernels that process unimportant information should be removed. In this paper, we first investigate the meaning of each frequency band information in the spectrum and their contribution to the prediction accuracy of the network,and according to these results, we propose a new pruning method based on frequency response(PFR). Our PFR finds and removes the convolutional kernels in the network that specialize in processing unimportant information, resulting in a compact neural network model. PFR obtains significant experimental results on different datasets, for example, a 56.0% raduction of float points operations(FLOPs) on Res Net-50 and only 0.37% of Top-1 accuracy degradation on the Image Net dataset.

关键词： deep learning model compression filter pruning channel pruning frequency response

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Constructing Donor–Acceptor‑Linked COFs Electrolytes to Regulate Electron Density and Accelerate the Li^(+)Migration in Quasi‑Solid‑State Battery

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Nano-Micro Letters 2025年第1期17卷 456-471页

作者： Genfu zhao Hang Ma Conghui Zhang yongxin yang Shuyuan yu Haiye Zhu yongjiang Sun Hong Guo School of Materials and Energy International Joint Research Center for Advanced Energy Materials of Yunnan ProvinceYunnan UniversityKunming 650091People’s Republic of China yunnan yuntianhua Co. LtdR&D CenterKunming 650228People’s Republic of China Southwest United Graduate School Kunming 650091People’s Republic of China

Regulation the electronic density of solid-state electrolyte by donor–acceptor(D–A)system can achieve highly-selective Li^(+)transportation and conduction in solid-state Li metal *** study reports a high-performance solid-state electrolyte thorough D–A-linked covalent organic frameworks(COFs)based on intramolecular charge transfer *** other reported COFbased solid-state electrolyte,the developed concept with D–A-linked COFs not only achieves electronic modulation to promote highly-selective Li^(+)migration and inhibit Li dendrite,but also offers a crucial opportunity to understand the role of electronic density in solid-state Li metal *** introduced strong electronegativity F-based ligand in COF electrolyte results in highlyselective Li^(+)(transference number 0.83),high ionic conductivity(6.7×10^(-4)S cm^(−1)),excellent cyclic ability(1000 h)in Li metal symmetric cell and high-capacity retention in Li/LiFePO_(4)cell(90.8%for 300 cycles at 5C)than substituted C-and N-based *** is ascribed to outstanding D–A interaction between donor porphyrin and acceptor F atoms,which effectively expedites electron transferring from porphyrin to F-based ligand and enhances Li^(+)***,we anticipate that this work creates insight into the strategy for accelerating Li^(+)conduction in high-performance solid-state Li metal batteries through D–A system.

关键词： Electronic modulation engineering Donor-acceptor-linked covalent organic frameworks Quasi-solid-state Li metal battery

Differential distribution of PINK1 and Parkin in the primate brain implies distinct roles

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Neural Regeneration Research 2025年第4期20卷 1124-1134页

作者： yanting Liu Wei Huang Jiayi Wen Xin Xiong Ting Xu Qi Wang Xiusheng Chen Xianxian zhao Shihua Li Xiaojiang Li Weili yang Guangdong Key Laboratory of Non-human Primate Research Key Laboratory of CNS Regeneration(Ministry of Education)Guangdong-Hongkong-Macao CNS Regeneration Institute of Jinan UniversityJinan UniversityGuangzhouGuangdong ProvinceChina

The vast majority of in vitro studies have demonstrated that PINK1 phosphorylates Parkin to work together in mitophagy to protect against neuronal ***,it remains largely unclear how PINK1 and Parkin are expressed in mammalian *** has been difficult to address because of the intrinsically low levels of PINK1 and undetectable levels of phosphorylated Parkin in small *** this issue is critical for elucidating the in vivo roles of PINK1 and ***,we showed that the PINK1 kinase is selectively expressed as a truncated form(PINK1–55)in the primate *** the present study,we used multiple antibodies,including our recently developed monoclonal anti-PINK1,to validate the selective expression of PINK1 in the primate *** found that PINK1 was stably expressed in the monkey brain at postnatal and adulthood stages,which is consistent with the findings that depleting PINK1 can cause neuronal loss in developing and adult monkey ***1 was enriched in the membrane-bound fractionations,whereas Parkin was soluble with a distinguishable *** double staining experiments showed that PINK1 and Parkin did not colocalize under physiological conditions in cultured monkey astrocytes,though they did colocalize on mitochondria when the cells were exposed to mitochondrial *** findings suggest that PINK1 and Parkin may have distinct roles beyond their well-known function in mitophagy during mitochondrial damage.

关键词： neurodegeneration Parkin Parkinson’s disease PINK1 subcellular distribution

EVOLUTION OF SINGLE ELLIPTIC VORTEX RINGS

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Acta Mechanica Sinica 1997年第1期13卷 17-25页

作者： zhao, y Shi, XG Department of Mechanics and Engineering Science Peking University The State Key Laboratory for Turbulence Research Beijing China

The evolution of single elliptic vortex rings for initial aspect ratio (AR) = 2,4,6 has been studied. The incompressible Navier-Stokes equations are solved by a dealiased pseudo-spectral method with 64(3) grid points in a periodic cube. We find that there are three kinds of vortex motion as AR increases and bifurcation occurs at certain AR. The processes of advection, interaction and decay of vortex ring are discussed. Numerical results coincide with experiments and other authors' numerical simulation.

关键词： elliptic vortex ring pseudo-spectral method bifurcation vortex reconnection

Equivariant PT-symmetric real Chern insulators

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Frontiers of physics 2020年第1期15卷 63-69,F0004页

作者： y.X.zhao National laboratory of solid state microstructures and department of physics nanjing universitynanjing 210093china Collaborative innovation center of advanced microstructures nanjing universitynanjing 210093china

It was understood that Chern insulators cannot be realized in the presence of PT *** this paper,we reveal a new class of PT-symmetric Chern insulators,which has internal degrees of freedom forming real representations of a symmetry group with a complex endomorphism *** a generalization to the conventional 2n-dimensional Chern insulators with integer n≥1,these PT-symmetric Chern insulators have the n-th complex Chern number as their topological invariant,and have a Z classification given by the equivariant orthogonal K ***,in a fairly different sense,there exist ubiquitously Chern insulators with *** generalizing the Thouless charge pump argument,we find that,for a PT-symmetric Chern insulator with Chern number *** are equally many v flavors of coexisting left-and right-handed chiral *** modes with opposite chirality are complex conjugates to each other as complex representations of the internal symmetry group,but are not *** the physical dimensionality d=2,the PT-symmetric Chern insulators may be realized in artificial systems including photonic crystals and periodic mechanical systems.

关键词： topological insulator Chern insulator

Optimizing Emergency Logistics for the Offsite Hazardous Waste Management

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Journal of Systems Science and Systems Engineering 2019年第6期28卷 747-765页

作者： Jiahong zhao Ginger y.Ke School of Civil and Transportation Engineering Guangdong University of TechnologyGuangzhou 510006China Faculty of Business Administration Memorial University of NewfoundlandSt.John'sNewfoundland and LabradorCanada A1B 3X5

Hazardous wastes pose increasing threats to people and environment during the processes of offsite collection,storage,treatment,and disposal.A novel game theoretic model,including two levels,is developed for the corresponding optimization of emergency logistics,where the upper level indicates the location and capacity problem for the regulator,and the lower level reflects the allocation problem for the emergency *** from other works in the literature,we focus on the issue of multi-quality coverages (full and partial coverages) in the optimization of facility location and *** be specific,the regulator decides the location plan and the corresponding capacity of storing emergency groups for multiple types of hazmats,so to minimizes the total potential environmental risk posed by incident sites;while the commander minimizes the total costs to provide an efficient allocation *** solve the bi-level programming model,two solution techniques,namely a KKT condition approach and a heuristic model,are designed and *** proposed model and solution techniques are then applied to a hypothetical case and a real-world case to demonstrate the practicality and provide managerial insights.

关键词： Bi-level programming hazardous material time-based risk assessment multi-quality covering model KKT heuristic technique

Sun's Log-concavity Conjecture on the Catalan–Larcombe–French Sequence

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Acta Mathematica Sinica,English Series 2016年第5期32卷 553-558页

作者： James J.y.zhao Center for Applied Mathematics Tianjin University

Let {Pn},n≥0 denote the Catalan-Larcombe-French sequence, which naturally came from the series expansion of the complete elliptic integral of the first kind. In this paper, we prove the strict log-concavity of the sequence { n√Pn}n≥1, which was originally conjectured by Z. W. Sun. We also obtain the strict log-concavity of the sequence {n√Vn}n≥1, where {Vn}n≥0 is the Fennessey-Larcombe- French sequence arising from the series expansion of the complete elliptic integral of the second kind.

关键词： The Catalan-Larcombe-French sequence the Fennessey-Larcombe-French sequence logconcavity three-term recurrence relation

Regularity of atomic nuclei with random interactions： sd bosons

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Frontiers of physics 2018年第6期13卷 197-211页

作者： y. M. zhao School of Physics and Astronomy Shanghai Jiaotong University Shanghai 200240 China

Atomic nuclei are complex systems with gigantic configuration spaces, therefore truncations of model spaces are indispensable. Due to the short-range nature of the nuclear interactions, one may resort to a truncation by using coherent nucleon-pairs which are conveniently further simplified as bosons, such as sd bosons. The discovery of the spin-zero ground state dominance with random two-body interactions led to a series of studies on regular structure for sd bosons in the presence of random interactions, and this review article summarizes studies along this line in last two decades. We concentrate on various patterns exhibited in sd boson systems, and demonstrate that many random samples which were thought to be noisy exhibit very regular patterns, some of which are interpreted in terms of the V（5）, O（6）, O（6）, SU（3）, and SU（3） dynamical symmetries of the sd interacting boson model.

关键词： regularity random interactions sd bosons