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Boosting hydrocarbon conversion via Cu-doping induced oxygen vacancies on CeO2 in CO2 electroreduction

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journal of Energy Chemistry 2025年第1期100卷 66-76页

作者： Lei Xue Tong Shi Chenhui Han Heng Zhang Fenrong Liu Haorun Li yan Wang Xiaojun Gu Shanghong zeng Inner Mongolia Key Laboratory of Chemistry and Physics of Rare Earth Materials School of Chemistry and Chemical Engineering Inner Mongolia University State Key Laboratory of Coal Conversion Institute of Coal Chemistry Chinese Academy of Sciences Institute of Catalysis Department of Chemistry Zhejiang University National Key Laboratory of Baiyunobo Rare Earth Resource Research and Comprehensive Utilization Baotou Research Institute of Rare Earths

Conversion of CO2back to hydrocarbons is the most direct way of closing the“carbon cycle”,and its significance is further enlarged if this process is driven by renewable energies such as ***,precisely controlling the product selectivity towards hydrocarbons against the competitive hydrogen evolution remains challenging,especially for Cu-based ***,we report a novel defect engineering strategy,by which Cu-doping-induced oxygen vacancies on CeO2nanorods were effectively created,with adjustable vacancy/Cu *** resulting optimum catalyst shows up to 79% catalytic current density to hydrocarbons （excluding CO）,with 49% faradaic efficiency to *** and density functional theory unveil that the ratio between oxygen vacancy and Cu affects significantly the formation of*CHO and activation of H2O,which leads to the following deep hydrogenation to *** findings may spur new insights for designing and developing more controllable chemical process relevant to CO2utilization.

关键词： Oxygen vacancy Hydrocarbon production Reaction mechanism

Glutamatergic CyLD deletion leads to aberrant excitatory activity in the basolateral amygdala:association with enhanced cued fear expression

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Neural Regeneration Research 2025年第11期20卷 3259-3272页

作者： Huidong Li Faqin Li Zhaoyi Chen Erwen Wu Xiaoxi Dai Danni Li Haojie An Shiyi zeng Chunyan Wang Li yang Cheng Long School of Life Sciences South China Normal UniversityGuangzhouGuangdong ProvinceChina School of Life Sciences Guangzhou UniversityGuangzhouGuangdong ProvinceChina Guangdong Provincial Key Laboratory of Major Obstetric Diseases The Third Affiliated Hospital of Guangzhou Medical UniversityGuangzhouGuangdong ProvinceChina South China Normal University-Panyu Central Hospital joint Laboratory of Translational Medical Research Panyu Central HospitalGuangzhouGuangdong ProvinceChina

Neuronal activity,synaptic transmission,and molecular changes in the basolateral amygdala play critical roles in fear ***(CyLD)is a deubiquitinase that negatively regulates the nuclear factor kappa-B *** is well studied in non-neuronal cells,yet underinvestigated in the brain,where it is highly *** studies have shown involvement of CyLD in the remodeling of glutamatergic synapses,neuroinflammation,fear memory,and anxiety-and autism-like ***,the precise role of CyLD in glutamatergic neurons is largely ***,we first proposed involvement of CyLD in cued fear *** next constructed transgenic model mice with specific deletion of Cyld from glutamatergic *** results show that glutamatergic CyLD deficiency exaggerated the expression of cued fear in only male ***,loss of CyLD in glutamatergic neurons resulted in enhanced neuronal activation,impaired excitatory synaptic transmission,and altered levels of glutamate receptors accompanied by over-activation of microglia in the basolateral amygdala of male ***,our study suggests a critical role of glutamatergic CyLD in maintaining normal neuronal,synaptic,and microglial *** may contribute,at least in part,to cued fear expression.

关键词： basolateral amygdala cued fear expression cylindromatosis deubiquitinase glutamate receptor 1 glutamatergic neuron microglial activation N-methyl-D-aspartate receptor 1 neuronal activation synaptic transmission

SNOEK-Kê-K■STER PEAK OF INTERNAL FRICTION IN Fe-P-N ALLOyS

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Acta Metallurgica Sinica(English Letters) 1998年第1期11卷 12-18页

作者： y.y.Che G.y.zeng y.C.Xu j.W ji Northeastern Univ Shenyang China

The internal friction and precipitate phases of the deformed Fe-P-N alloys have been investigated. It has been found that the ratio of depends on the content of P and the relation holds if the content of N is lower than *** and the content of P is lower than ***. It shows that the intercept K2 is related to the presence of the atomic pairs and clusters of P in the alloy matrix.

关键词： internal friction Fe-P-N alloy

Improved mechanical properties and strengthening mechanism with the altered precipitate orientation in magnesium alloys

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journal of Magnesium and Alloys 2022年第5期10卷 1256-1267页

作者： y.j.Wan y.zeng y.C.Dou D.C.Hu X.y.Qian Q.zeng K.X.Sun G.F.Quan Key Laboratory of Advanced Technologies of Materials Ministry of EducationSchool of Material Science and EngineeringSouthwest Jiaotong UniversityChengdu 610031China College of Materials Science and Engineering Sichuan University of Science and EngineeringZigong 643000China Department of Materials The University of ManchesterOxford RoadManchester M139PLUnited Kingdom

Aging prior to twinning deformation was proposed to alter the precipitate orientation of the plate-shapedβ-MgAlfrom(0002)basal planes(named basal plates)to■prismatic planes(named prismatic plates)in AZ31 Mg *** experimental results showed that the compressive yield strength(CyS)of the sample containing prismatic plates increased 40 MPa and the compression ratio raised by 22%compared to that containing basal *** underlying strengthening mechanism was analyzed via a yield strengthen(yS)model with a function of grain size,precipitate characters(size,oritention,fraction)and Schmid factor(SF).It revealed that the improvement of CyS was mainly attributed to the altered precipitate orientation and refined grain size produced by twinning ***,the prismatic plates always have a stronger hardening effect on basal slip than basal plates under the same varites of precipitate diameter and ***,the decreased CRSS ratio of prismatic slip to basal slip revealed that the activity of non-basal slip in Mg alloy might be *** activated slip systems provided more mobile dislocations,contributing to the large compression ratio of the Mg rolled sheet with prismatic plates.

关键词： Precipitate orientation Precipitation strengthening Grain boundary strengthening yield strength model

ON THE DyNAMIC CHARACTERISTICS OF MOULD-FILLING UNDER COUNTERGRAVITy

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Acta Metallurgica Sinica(English Letters) 1997年第5期10卷 409-414页

作者： zeng, j.M. Gu, H. Zhou, y.H. Guangxi Univ Nanning China

In this paper, the mathematical models for mould-filling under countergravity are derived on the basis of the principle of momentum. Dynamic processes of mould-filling are observed on a perspex model by means of high speed photography. The results indicate that the mould-filling under countergravity can be described by the second order nonlinear differential equations characterized by damping oscillations. The velocity oscillations amplify as the pressuring speed increases if the pressure differential functions are of the same type. On the other hand, if the functions are of different type, then the velocity oscillations depend upon whether the functions progressively increase or decrease. Velocity oscillations can be diminished dramatically by increasing the local damping within the gating system.

关键词： casting mould-filling dynamics

PHOTOCATALyTIC PERFORMANCE OF PLASMA SPRAyED TiO_2-ZnFe_2O_4 COATINGS

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Acta Metallurgica Sinica(English Letters) 2005年第3期18卷 363-368页

作者： y.zeng j.T.Liu W.j.Qian j.H.Gao ShanghaiInstituteofCeramics TheChineseAcademyofSciencesShanghai200050China

A novel TiO2-ZnFe2O4 coating is prepared by plasma spraying. The effects of spra ying parameters and the composition of powders on the microstructure, surface mo rphology and photo-absorption of plasma sprayed coatings are studied. The photoc atalytic efficiency of the as-sprayed coatings is evaluated through the photo mi neralization of methylene blue. It was found that TiO2 coatings can decompose me thylene blue under the illumination of ultraviolet rays, and the degrading effic iency is improved with an increase in the content of FeTiO3 in the coatings. How ever, the presence of large amount of ZnFe2O4 compound will substantially lower the photocatalytic efficiency of the TiO2-ZnFe2O4 coatings for the unfavorable p hoto-excited electron-hole transfer process.

关键词： plasma spraying photocatalytic activity TiO2 ZnFe2O4

Structure Heterogeneity in Metallic Glass: Modeling and Experiment

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journal of Materials Science & Technology 2014年第6期30卷 560-565页

作者： H.B.Ke j.F.zeng C.T.Liu y.yang Centre for Advanced Structural Materials Department of Mechanical and Biomedical EngineeringCity University of Hong Kong

Despite the great efforts dedicated to metallic glasses （MGs）, their structure still remains a mystery to be understood. With comparison to the existing mjciomechanical models, such as the free-volume and shear transformation zone （STZ） models, we first discuss in this article our recently proposed ＇core-shell＇ model, which contains a solid-like matrix and liquid-like inclusions. This serves as the theoretical basis to understand the structural heterogeneity in MGs in our analytical framework. After that, a scanning ultrafast nanoindentation technique is used to map out the structure heterogeneity in a Zr-based bulk metallic glass （BMG）. With these ongoing research efforts, we hope that more research work could be stimulated in the pursuit of the structure-property relation in MGs.

关键词： Metallic glass Structure heterogeneity Nanoindentation Core-shell model

MICROSTRUCTURE AND INCLUSION CHARACTERIZATION IN THE SIMULATED COARSE-GRAIN HEAT AFFECTED ZONE WITH LARGE HEAT INPUT OF A Ti-Zr-MICROALLOyED HSLA STEEL

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Acta Metallurgica Sinica(English Letters) 2005年第2期18卷 96-106页

作者： y.T.Chen X.Chen Q.F.Ding j.zeng TechnologyCenter WuhanIronandSteel（group）CooperationWuhan430080China

The microstructure and the characteristics of the inclusions embedded in ferrite matrix in simulated coarse-grain heat affected zone (CGHAZ) of a Ti-Zr-treated high strength low alloy (HSLA) steel have been investigated. The microstructure of the simulated CGHAZ dominantly consisted of intragranular acicular ferrite (IAF) combining with a small amount of polygonal ferrite (PF), widmanst tten ferrite (WF), bainite ferrite (BF), pearlite and martensite-austenite (M-A) islands. The PF, WF and BF were generally observed at the prior austenite grain boundaries and the interlocking acicular ferrite was usually found intragranularly. It was found that the inclusions were composed of Ti2O3, ZrO2, Al2O3 locating at the center of the particles and MnS lying on the surface layer of the inclusions. The intragranular complex inclusions promoted the acicular ferrite formation and the refinement of microstructure whilst those at prior austenite grain boundaries caused PF formation on the inclusions. The simulated CGHAZ consisting of such complicated microstructure exhibited desired mechanical properties.

关键词： microalloyed HSLA steel heat affected zone microstructure mechanical property inclusion acicular ferrite titanium zirconium

Correlation of chromosomal polysomy with overexpression of c-myc and c-erbB-2 in primary nasopharyngeal carcinoma: Tissue microarray study

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Chinese Science Bulletin 2002年第3期47卷 217-220页

作者： Zhang, Lj yan, j Liang, QW Huang, Bj zeng, yX Fang, y Sun yat Sen Univ Med Sci Canc Ctr Canc Inst Guangzhou 510060 Peoples R China

Many genes may be involved in nasopharyn-geal carcinoma (NPC) development and progression. Several known oncogenes, including c-myc and c-erb-B2, have been shown to have structural alteration and aberrant expression in NPC. Here, we constructed a tissue microarray to deter-mine the status of c-myc and c-erbB-2 oncogenes at the DNA and protein levels using interphase fluorescence in situ hy-bridization (FISH) and immunohistochemistry (IHC) and to define the diagnostic, prognostic importance of the genetic changes. Results showed that amplification of c-myc and c-erbB-2 was not found in NPC. Polysemy 8 and 17 were observed in 43%-50% and 20%-27% of NPC tumors, respectively. Overexpressions of c-myc and c-erbB-2 onco-proteins were detected in 53.6% and 54.5% cases of NPC with polysomy 8 and 17, respectively. There was no signifi-cant correlation between c-myc and c-erbB-2 staining and the clinical stage. But overexpression of c-erbB-2 was associ-ated with polysemy 17 in NPC. These findings suggest that

关键词： nasopharyngeal carcinoma c-myc c-erbB-2 tissue mi-croarray chromosomal polysomy.