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Correlation analysis of interstitial maturity and prognosis of colorectal cancer:Meta-analysis

World Journal of Gastrointestinal Oncology 2024年第6期16卷 2816-2825页

作者： Zhen-Jun Liu xu-wen zhang Qi-Qi Liu Shao-Zhao Wang Department of Gastrointestinal Surgery Feicheng People's HospitalFeicheng 271600Shandong ProvinceChina Department of Hepatobiliary Surgery Feicheng People's HospitalFeicheng 271600Shandong ProvinceChina Department of Gastrointestinal Surgery Peking University Shenzhen HospitalShenzhen 518036Guangdong ProvinceChina Department of Anorectal Word Central Hospital Affiliated Shandong First Medical UniversityJinan 250013Shandong ProvinceChina

BACKGROUND To investigate the relationship between interstitial maturity and prognosis of colorectal *** To examine the correlation between interstitial maturity and the prognosis of colorectal *** The paper database PubMed,EMBASE,Cochranelibrary,Springerlink,CNKI,and Wanfang database were searched until December 2023."tumor stroma maturity""desmoplastic stroma reaction""desmoplastic reaction""stroma reaction""degree of stroma reaction""stroma classification""stroma density""colorectal cancer""colon cancer""rectal cancer""prognosis"were searched for the search *** system assessors independently screened the literature quality according to the inclusion exclusion criteria,Quality evaluation and data extraction were performed for the included literatures,and meta-analysis was performed for randomized control trials included at using Review Manager 5.2 *** Finally,data of 9849 patients with colorectal cancer from 19 cosets in 15 literatures were included,including 4339 patients with mature type(control group),3048 patients with intermediate type(intermediate group)and 2456 patients with immature type(immature group).The results of meta-analysis showed:Relapse-free survival[hazard ratio(HR)=2.66,95%confidence interval(CI):2.30-3.08;P<0.00001],disease-free survival(HR=3.68,95%CI:2.33-5.81;P<0.00001)and overall survival(HR=1.70,95%CI:1.53-1.87;P<0.00001)were significantly lower than those in mature group(control group);relapse-free survival(HR=1.36,95%CI:1.17-1.59;P<0.0001)and disease-free survival rate(HR=1.85,95%CI:1.53-2.24;P<0.0001)was significantly lower than the mature group(control group).CONCLUSION There is the correlation between tumor interstitial maturity and survival prognosis of colorectal cancer,and different degrees of tumor interstitial maturity have a certain impact on the quality of life of colorectal cancer patients.

关键词： Colorectal tumor Survival prognosis Tumor interstitial maturity Systematic review Meta-analysis

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基于3,6-二氯噻吩并[3,2-b]噻吩的共轭聚合物的直接芳基化缩聚合成及其半导体性质

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高分子学报 2024年第1期55卷 36-47页

作者：林琳琳张栩文石毅博邓云峰耿延候天津大学材料科学与工程学院天津300350 天津大学-新加坡国立大学福州联合学院天津大学国际校区福州350205

以β位氯代的噻吩衍生物3,6-二氯噻吩并[3,2-b]噻吩(2ClTT)为C-H单体、溴代噻吩取代吡咯并吡咯二酮(DPPC14-Br)或溴代异靛蓝(IIDC14-Br)为C-Br单体,采用直接芳基化缩聚(DArP)合成了共轭聚合物DPP-2ClTT和IID-2ClTT.氯原子的引入可大幅... 详细信息

以β位氯代的噻吩衍生物3,6-二氯噻吩并[3,2-b]噻吩(2ClTT)为C-H单体、溴代噻吩取代吡咯并吡咯二酮(DPPC14-Br)或溴代异靛蓝(IIDC14-Br)为C-Br单体,采用直接芳基化缩聚(DArP)合成了共轭聚合物DPP-2ClTT和IID-2ClTT.氯原子的引入可大幅提高并噻吩α-C-H键的反应活性,理论计算表明,2ClTT的直接芳基化反应活性与文献报道的高活性氯代联噻吩C-H单体的活性相当.此外,利用氯原子较强的电负性,可以降低聚合物的前线轨道能级,DPP-2ClTT和IID-2ClTT的HOMO/LUMO能级分别为-5.35/-3.66 eV和-5.88/-3.73 eV.由于具有合适的HOMO和LUMO能级以及离域的HOMO和LUMO轨道,以DPP-2ClTT为活性层制备的有机薄膜晶体管(OTFT)表现出双极传输特性,最高电子和空穴迁移率分别为1.36和0.89 cm^(2)/V/s. IID-2ClTT具有较低的HOMO能级以及较为定域的HOMO轨道,因而该聚合物在OTFT器件中表现出n型传输特性,最高电子迁移率为0.029 cm^(2)/V/s.相比于IID-2ClTT,DPP-2ClTT高的电子迁移率可归因于其好的骨架平面性、有序的分子堆积以及优异的薄膜形貌.

关键词：共轭聚合物直接芳基化缩聚噻吩衍生物载流子迁移率有机薄膜晶体管

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Distributed dynamic task allocation for unmanned aerial vehicle swarm systems:A networked evolutionary game-theoretic approach

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Chinese Journal of Aeronautics 2024年第6期37卷 182-204页

作者： Zhe zhang Ju JIANG Haiyan xu wen-An zhang College of Automation Engineering Nanjing University of Aeronautics and AstronauticsNanjing 211106China College of Economics and Management Nanjing University of Aeronautics and AstronauticsNanjing 211106China College of Information Engineering Zhejiang University of TechnologyHangzhou 310023China

Task allocation is a key aspect of Unmanned Aerial Vehicle(UAV)swarm collaborative *** an continuous increase of UAVs’scale and the complexity and uncertainty of tasks,existing methods have poor performance in computing efficiency,robustness,and realtime allocation,and there is a lack of theoretical analysis on the convergence and optimality of the *** paper presents a novel intelligent framework for distributed decision-making based on the evolutionary game theory to address task allocation for a UAV swarm system in uncertain scenarios.A task allocation model is designed with the local utility of an individual and the global utility of the ***,the paper analytically derives a potential function in the networked evolutionary potential game and proves that the optimal solution of the task allocation problem is a pure strategy Nash equilibrium of a finite strategy ***,a PayOff-based Time-Variant Log-linear Learning Algorithm(POTVLLA)is proposed,which includes a novel learning strategy based on payoffs for an individual and a time-dependent Boltzmann *** former aims to reduce the system’s computational burden and enhance the individual’s effectiveness,while the latter can ensure that the POTVLLA converges to the optimal Nash equilibrium with a probability of *** simulation results show that the approach is optimal,robust,scalable,and fast adaptable to environmental changes,even in some realistic situations where some UAVs or tasks are likely to be lost and increased,further validating the effectiveness and superiority of the proposed framework and algorithm.

关键词： Task allocation Unmanned Aerial Vehicles(UAV) Game theory Log-linear learning Distributed optimization algorithm

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3-Methylcyclohexanone Processed n-Channel Organic Thin-Film Transistors Based on a Conjugated Polymer Synthesized by Direct Arylation Polycondensation

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Chinese Journal of Polymer Science 2023年第5期41卷 824-831,I0012页

作者： Dong-Sheng Yan xu-wen zhang Zhong-Li Wang Chen-Hui xu Yi-Bo Shi Yun-Feng Deng Yang Han Yan-Hou Geng School of Materials Science and Engineering and Tianjin Key Laboratory of Molecular Optoelectronic Science Tianjin Universityand Collaborative Innovation Center of Chemical Science and Engineering(Tianjin)Tianjin 300072China State Key Laboratory of Separation Membranes and Membrane Processes Tianjin Key Laboratory of Advanced Fibers and Energy StorageSchool of Material Science and EngineeringTiangong UniversityTianjin 300387China Joint School of National University of Singapore and Tianjin University International Campus of Tianjin UniversityFuzhou 350207China

The solubility of a direct arylation polycondensation(DArP)synthesized conjugated polymer,i.e.,poly(3,6-bis(furan-2-yl)-2,5-bis(4-tetradecyloctadecyl)-pyrrolo[3,4-c]pyrrole-1,4(2H,5H)-dione-alt-1,2-bis(3,4-d ifl uorothien-2-yl)ethene)(PFuD PP-4FTVT),in variou s organic solvents was *** polymer is soluble in 3-methylcyclohexanone(3-MC),a green solvent from peppermint oil,besides other solvents such as anisole,cyclopentyl methyl ether(CPME)and o-dichlorobenzene(o-DCB),*** on the Hansen solu bility parameters(HSP)analysis,3-MC is identified as a"marginal solvent"of *** morphology of the spin-coated films with 3-MC as the solvent strongly correlated with the solution preparation *** a 3-MC solution aged for 3 h at 70℃,n-channel organic thin-film transistors(OTFTs)with electron mobility(μe)above 1 cm^(2)·V^(-1)·s^(-1) and current on/off ratio(Ion/Ioff)higher than 105 were fabricated by *** is the first report on high mobility conjugated polymers for OTFTs processible with natu rally occurred green solvent.

关键词： Conjugated polymers Organic thin-film transistors Electron mobility Green solvent Direct arylation polycondensation

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Study on metal recovery process and kinetics of oxidative leaching from spent LiFePO_(4)Li-batteries

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Chinese Journal of Chemical Engineering 2024年第4期68卷 94-102页

作者： Xiaoming zhang wen Xie Xiaolei Zhou wenjie zhang Jiawei wen Xin Wang Guoyong Huang Shengming xu College of New Energy and Materials China University of PetroleumBeijing 102249China State Key Laboratory of Heavy Oil Processing College of Chemical EngineeringChina University of PetroleumBeijing 102249China Beijing Spacecrafts Beijing 100094China Ganfeng Lithium Group Co. Ltd.Xinyu 338000China Institute of Nuclear and New Energy Technology Tsinghua UniversityBeijing 100084China Beijing Key Laboratory of Fine Ceramics Tsinghua UniversityBeijing 100084China

A green environmental protection and enhanced leaching process was proposed to recover all elements from spent lithium iron phosphate(LiFePO_(4)) lithium *** order to reduce the influence of Al impurity in the recovery process,NaOH was used to remove *** impurity removal,the spent LiFePO_(4) cathode material was used as raw material under the H_(2)SO_(4) system,and the pressure oxidation leaching process was adopted to achieve the preferential leaching of *** E-pH diagram of the Fe-P-Al-H_(2)O system can determine the stable region of each element in the recovery process of spent LiFePO_(4)*** the optimal conditions(500 r·min^(-1),15 h,363.15 K,0.4 MPa,the liquid-solid ratio was 4:1 ml·g^(-1)and the acid-material ratio was 0.29),the leaching rate of Li was 99.24%,Fe,Al,and Ti were 0.10%,2.07%,and 0.03%,*** Fe and P were precipitated and recovered as FePO_(4)·2H_(2)*** kinetic analysis shows that the process of high-pressure acid leaching of spent LiFePO_(4) materials depends on the surface chemical *** the life cycle assessment(LCA)of the spent LiFePO_(4) whole recovery process,eight midpoint impact categories were selected to assess the impact of recovery *** results can provide basic environmental information on production process for recycling industry.

关键词： Spent LiFePO_(4)Li-batteries Oxidative leaching Kinetic study Life cycle assessment

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Magnetic and luminescent properties of bifunctional composite Fe_(3)O_(4)@Y_(2)O_(2)S:Eu^(3+)

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Journal of Rare Earths 2024年第8期42卷 1568-1576,I0006页

作者： Zhiqi Liang Zhili zhang Liu Li wen xu Decai Li School of Mechanical Electronic and Control EngineeringBeijing Jiaotong UniversityBeijing100044China Beijing Key Laboratory of Flow and Heat Transfer of Phase Changing in Micro and Small Scale Beijing100044China State Key Laboratory of Tribology Tsinghua UniversityBeijing100084China

As a kind of non-destructive testing method,magnetic particle inspection is widely used in the fields of aviation and high-speed *** properties of magnetic fluorescent bifunctional composites,such as fluorescence intensity and magnetic properties,have increasing demands in magnetic particle *** earth compounds offer potential as novel materials for fluorescent magnetic bifunctional composites due to their excellent optical properties and extremely narrow emission *** this work,the rare earth fluorescent material Y_(2)O_(2)S:Eu^(3+) was synthesized by solid-state reaction ***_(3)O_(4)nanoparticles prepared by hydrothermal method were uniformly coated on the Y_(2)O_(2)S:Eu^(3+) particles through physical adsorption of *** obtained Fe_(3)O_(4)@Y_(2)O_(2)S:Eu^(3+) exhibits dark red color under the ultraviolet *** additio n,X-ray diffractio n,morphology,photoluminescence and hyste resis loop of Fe_(3)O_(4)@Y_(2)O_(2)S:Cu^(3+) were *** luminescence mechanism of Y_(2)O_(2)S:Eu^(3+) is described in detail Fe_(3)O_(4)@Y_(2)O_(2)S:Cu^(3+) displays good paramagnetism and has a good controllability under a magnetic *** magnetic particle inspection of Fe_(3)O_(4)@Y_(2)O_(2)S:Eu^(3+) was performed using a 4-pole electromagnet and a test piece *** magnetic fluorescent bifunctional composite presented in this work can be applied for non-destructive testing.

关键词： Bifunctional material Fe_(3)O_(4) Y_(2)O_(2)S:Eu^(3+) Luminescence Solid-state reaction Rare earths

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DeepCRBP:improved predicting function of circRNA-RBP binding sites with deep feature learning

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Frontiers of Computer Science 2024年第2期18卷 235-237页

作者： Zishan xu Linlin SONG Shichao LIU wen zhang College of Informatics Huazhong Agricultural UniversityWuhan 430070China

1 Introduction Recently,there is growing evidence that it is essential to predict the interactions between circRNAs and RBP binding sites for diagnosing diseases and providing a potential target to treat diseases[1].Many studies have predicted the binding sites of circRNA-RBPs by using deep learning methods based on the sequence information of circRNAs for each ***,many methods focus on diversified view of sequence encoding for improving the performance of the predictive models.

关键词： learning Deep function

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Design study of charge-stripping scheme of heavy ion beams for HIAF-BRing

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Nuclear Science and Techniques 2024年第5期35卷 30-41页

作者： Jun-Jie zhang Zhi-You xu Jin-Quan zhang wen-wen Ge Liang-Ting Sun Huan-Yu Zhao Institute of Modern Physics Chinese Academy of SciencesLanzhou 730000China School of Nuclear Science and Technology University of Chinese Academy of SciencesBeijing 100049China

Charge strippers play an essential role in heavy-ion accelerators by stripping the projectile ions to higher charge states to enhance the acceleration efficiency downstream of the *** the high-energy mode of the booster ring(BRing)of the high-intensity heavy-ion accelerator facility,the pre-accelerated ions from the iLinac will be stripped by a carbon foil to higher charge states and then injected into the *** key parameters of the stripper and stripped ions were calculated,and the influence of stripping on the beam quality was *** get high stripping efficiencies,the foil thicknesses and resultant charge state distributions for the typical ions were determined by the code *** equilibrium thickness was obtained for the U beam,while the stripper thicknesses for the Xe and Kr beams were determined based on a compromise between the stripped charge states and the stripping *** energy loss,energy straggling,and emittance growth due to stripping have a non-negligible impact on the transport of the stripped beams and the injection of the ***,these parameters were simulated by *** addition,the foil’s temperature evolution,which greatly affects the foil lifetime,was simulated by *** maximum temperature of the foil bombarded by the U and Xe beams with the nominal parameters will exceed the safe value in terms of the impact of evaporation on the foil’s *** the foil temperature constraint,the highest tolerable beam intensity and the injected ion number into the ring were derived for different beam *** results of this paper will present important reference data for the optimization design and commissioning of the beamline and injection to the BRing for the stripped ions.

关键词： High-intensity heavy-ion accelerator facility Charge stripper Energy spread Thermal analysis Emittance growth Injection turns

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Robust Information Hiding Based on Neural Style Transfer with Artificial Intelligence

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Computers, Materials & Continua 2024年第5期79卷 1925-1938页

作者： Xiong zhang Minqing zhang xu AnWang wen Jiang Chao Jiang Pan Yang College of Cryptography Engineering Engineering University of People’s Armed PoliceXi’an710086China Key Laboratory of People’s Armed Police for Cryptology and Information Security Xi’an710086China Key Laboratory of CTC&Information Engineering(Engineering University of People’s Armed Police) Ministry of EducationXi’an710086China Staff Department of People’s Armed Police Ningxia Corps Yinchuan750000China

This paper proposes an artificial intelligence-based robust information hiding algorithm to address the issue of confidential information being susceptible to noise attacks during *** algorithm we designed aims to mitigate the impact of various noise attacks on the integrity of secret information during *** method we propose involves encoding secret images into stylized encrypted images and applies adversarial transfer to both the style and content features of the original and embedded *** process effectively enhances the concealment and imperceptibility of confidential information,thereby improving the security of such information during transmission and reducing security ***,we have designed a specialized attack layer to simulate real-world attacks and common noise scenarios encountered in practical *** adversarial training,the algorithm is strengthened to enhance its resilience against attacks and overall robustness,ensuring better protection against potential *** results demonstrate that our proposed algorithm successfully enhances the concealment and unknowability of secret information while maintaining embedding ***,it ensures the quality and fidelity of the stego *** method we propose not only improves the security and robustness of information hiding technology but also holds practical application value in protecting sensitive data and ensuring the invisibility of confidential information.

关键词： Information hiding neural style transfer robustness

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New strategies for asymmetric photocatalysis: asymmetric organocatalytic/photoredox relay catalysis for efficient synthesis of polycyclic compounds containing vicinal amino alcohols

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Science China Chemistry 2024年第3期67卷 945-952页

作者： Jia-Lu zhang wen-Bo He Xiu-Qin Hu Peng-Fei xu State Key Laboratory of Applied Organic Chemistry College of Chemistry and Chemical EngineeringLanzhou UniversityLanzhou 730000China State Key Laboratory of Veterinary Etiological Biology College of Veterinary MedicineLanzhou UniversityLanzhou Veterinary Research InstituteChinese Academy of Agricultural SciencesLanzhou 730000China MOE Frontiers Science Center for Rare Isotopes Lanzhou UniversityLanzhou 730000China

An asymmetric catalytic strategy in photocatalysis utilizing a chirality-induced approach through an organocatalytic/photoredox relay catalysis strategy is successfully achieved for the rapid construction of polycyclic compounds containing vicinal amino alcohols in a one-pot protocol. This methodology facilitates the efficient synthesis of diverse substituted polycyclic tetrahydroquinoline and benzofuran-derived vicinal amino alcohols, each containing five consecutive chiral centers, with high yields,excellent diastereoselectivities and enantioselectivities(up to 95% yield, >20:1 dr and 98% ee), under mild reaction conditions driven by sequential bifunctional squaramide organocatalyst-catalyzed [4+2] annulation and photocatalyst-catalyzed ketyl radical addition cyclization reaction process. Furthermore, investigations into the stereoselectivity mechanism and high-resolution mass spectrometry(HRMS) experiments on free radical trapping have provided evidence for elucidating the detailed mechanism of chirality-induced processes and chiral intermediate conversions in this procedure.

关键词： enantioselective photocatalysis asymmetric organocatalytic/photocatalysis relay catalysis five consecutive chiral centers chirality-induced strategy chirality vicinal amino alcohols

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