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Nano Research 2024年第7期17卷 6087-6094页

作者： Mao Qian Yakun Tang Lang liu Yue Zhang xiaohui li JiaJia Chen State Key Laboratory of Chemistry and Utilization of Carbon Based Energy Resources Xinjiang UniversityUrumqi 830017China State Key Laboratory of Physical Chemistry of Solid Surfaces Xiamen UniversityXiamen 361005China

The diffusion and loss of lithium polysulfides(liPSs)in lithium-sulfur batteries(LSBs)reduce the sulfur utilization rate and the catalytic conversion efficiency of sulfur species,resulting in early battery ***_(2)ZnTi_(3)O_(8)(LZTO),characterized by its stable spinel structure,exhibits high li+conductivity and holds great potential as an effective adsorbent for *** study proposes a collaborative design concept of LZTO host–separator modifier,which offers a complementary and matching approach in the cathode side,effectively addressing the challenges associated with dissolution and inadequate conversion of *** functional theory(DFT)calculation substantiates the pronounced chemical affinity of LZTO towards *** importantly,the high efficiency ion transport channels are achieved in separator coating due to the presence of the LZTO ***,the catalytic efficacy of LZTO is validated through meticulous analysis of symmetric batteries and Tafel ***,the LZTO host–separator modifier-based cell displays satisfactory rate capability(1449 and 1166 mAh·g^(−1)at 0.1 and 0.5 C)and an impressively capacity(606 mAh·g^(−1)after 500 cycles at 1 C).The coordinated strategy of host–separator modifier is supposed to have wide applications in LSBs.

关键词： li_(2)ZnTi_(3)O_(8) lithium-sulfur batteries host-separator modifier catalytic conversion diffusion and loss of liPSs

REFINEMENTS OF THE NORM OF TWO ORTHOGONAL PROJECTIONS

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Acta Mathematica Scientia 2024年第4期44卷 1229-1243页

作者： xiaohui li Meiqi liU Chunyuan DENG School of Mathematics Science South China Normal UniversityGuangzhou 510631China

In this paper,some refinements of norm equalities and inequalities of combination of two orthogonal projections are *** use certain norm inequalities for positive contraction operator to establish norm inequalities for combination of orthogonal projections on a Hilbert ***,we give necessary and sufficient conditions under which the norm of the above combination of o`rthogonal projections attains its optimal value.

关键词： norm orthogonal projection positive operator spectral block operator valued matrix

Cobalt-doped TiO_(2)@C hierarchical nanocomposites derived from Ti_(3)C_(2) MXene as cathodes for hybrid magnesium-lithium batteries

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Nano Research 2024年第1期17卷 253-261页

作者： xiaohui li Yakun Tang Lang liu Yue Zhang Yang Gao Mao Qian Wenjie Ma State Key Laboratory of Chemistry and Utilization of Carbon Based Energy Resources College of ChemistryXinjiang UniversityUrumqi 830017China

TiO_(2)has been explored in hybrid magnesium-lithium batteries(HMLBs)due to the advantages of low self-discharge and small volume expansion during ion ***,how to improve the inherently low ionic and electrical conductivity of TiO_(2)is the problem that needs to be *** this work,a smart strategy is adopted to prepare cobalt-doped TiO_(2)@C(Co^(4+)-TiO_(2)@C)hierarchical nanocomposite derived from Co(II)(OH)n@*** with TiO_(2)@C(without cobalt doping),Co^(4+)-TiO_(2)@C shows the highest specific capacity(154.7 mAh·g^(-1)at 0.1 A·g^(-1)after 200 cycles)and extraordinary rate performance in *** excellent electrochemical performance of Co4+-TiO_(2)@C is ascribed to the synergistic effect of the hierarchical structure and *** experimental results and density functional theory(DFT)calculation reveal that the cobalt-doping has effectively improved the electronic conductivity and reduced the li+migration *** work provides a new insight to design TiO_(2)-based cathode materials with high-performance in HMLBs.

关键词： Ti_(3)C_(2)MXene TiO_(2) hybrid magnesium-lithium batteries hierarchical structure cobalt-doping

Insertion sequence transposition activates antimycobacteriophage immunity through an Isr2-silenced lipid metabolism gene island

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mlife 2024年第1期3卷 87-100页

作者： Yakun li Yuyun Wei Xiao Guo xiaohui li lining Lu lihua Hu Zheng-Guo He State Key Laboratory for Conservation and Utilization of Subtropical Agro-Bioresources Guangxi Research Center for Microbial and Enzyme Engineering TechnologyCollege of Life Scienceand TechnologyGuangxi UniversityNanningChina

Insertion sequences(ISs)exist widely in bacterial genomes,but their roles in the evolution of bacterial antiphage defense remain to be ***,we report that,under the pressure of phage infection,the IS1o96 transposition of Mycobacterium smegmatis into the Isr2 gene can occur at high frequencies,which endows the mutant mycobacterium with a broad-spectrum antiphage ***2 functions as a negative regulator and directly silences expression of a gene island composed of 11 lipid metabolism-related *** complete or partial loss of the gene island leads to a significant decrease of bacteriophage adsorption to the mycobacterium,thus defending against phage ***,a phage that has evolved mutations in two tail-filament genes can re-escape from the Isr2 inactivation-triggered host *** study uncovered a new signaling pathway for activating antimycobacteriophage immunity by Is transposition and provided insight into the natural evolution of bacterial antiphage defense.

关键词： antiphage defense bacteriophage gene island insertion sequence mycobacteria

Carbon enhanced nucleophilicity of Na_(3)V_(2)(PO_(4))_(3):A general approach for dendrite-free zinc metal anodes

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Journal of Energy Chemistry 2024年第4期91卷 203-212页

作者： Sijun Wang lingzi Hu xiaohui li Dan Qiu Shunhang Qiu Qiancheng Zhou Wenwen Deng Xiaoying Lu Ze Yang Ming Qiu Ying Yu Institute of Nanoscience and Nanotechnology School of Physical Science and TechnologyCentral China Normal UniversityWuhan 430079HubeiChina School of Material Science and Engineering Suzhou University of Science and TechnologySuzhou 215000JiangsuChina Faculty of Science and Technology Technological and Higher Education Institute of Hong KongHong KongChina

Zincophilic property and high electrical conductivity are both very important parameters to design novel Zn anode for aqueous Zn-ion batteries(AZIBs).However,single material is difficult to exhibit zincophilic property and high electrical conductivity at the same ***,originating from theoretical calculation,a zincophilic particle regulation strategy is proposed to address these limitations and carbon coated Na_(3)V_(2)(PO_(4))_(3)is taken as an example to be a protective layer on zinc metal(NVPC@Zn).Na_(3)V_(2)(PO_(4))_(3)(NVP)is a common cathode material for Zn-ion batteries,which is *** materials not only offer an electron pathway to help Zn deposition onto NVPC surface,but also enhance the zinc nucleophilicity of Na_(3)V_(2)(PO_(4))_(3).Hence,this hybrid coating layer can tune zinc deposition and resist side reactions such as hydrogen generation and Zn metal ***,a symmetrical battery with NVPC@Zn electrode displays highly reversible plating/stripping behavior with a long cycle lifespan over 1800 h at2 mA cm^(-2),much better than carbon and Na_(3)V_(2)(PO_(4))_(3)solely modified Zn *** the Na_(3)V_(2)(PO_(4))_(3)is replaced with zincophobic Al2O3or zincophilic V2O3,the stability of the modified zinc anodes is also *** strategy expands the option of zincophilic materials and provides a general and effective way to stabilize the Zn electrode.

关键词： Zinc-ion batteries Zinc anode Carbon enhanced nucleophilicity Zincophilic particle regulation

XMe - Xiamen Molecular Electronics Code:An Intelligent and Open-Source Data Analysis Tool for Single-Molecule Conductance Measurements

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Chinese Journal of Chemistry 2024年第3期42卷 317-329页

作者： Zhichao Pan Gang Dong Chi Shang Ruihao li Tengyang Gao Luchun lin Huicong Duan xiaohui li Jie Bai Yilin Lai Wenfeng Wu Jia Shi Junyang liu Wenjing Hong State Key Laboratory of Physical Chemistry of Solid Surfaces College of Chemistry and Chemical Engineering & Institute of Artificial IntelligenceXiamen UniversityXiamenFujian361005 China School of Artificial Intelligence Guilin University of Electronic TechnologyGuilinGuangxi541004 China

Charge transport characterization of single-molecule junctions is essential for the fundamental research of single-molecule physical chemistry and the development towards single-molecule electronic devices and circuits. Among the single-molecule conductance characterization techniques,the single-molecule break junction technique is widely used in tens of worldwide research laboratories which can generate a large amount of experimental data from thousands of individual measurement cycles. However,data interpretation is a challenging task for researchers with different research backgrounds,and the different data analysis approaches sometimes lead to the misunderstanding of the measurement data and even reproducibility issues of the measurement. It is thus a necessity to develop a user-friendly all-in-one data analysis tool that automatizes the basic data analysis in a standard and widely accepted way. In this work,we present the XMe Code (Xiamen Molecular Electronics Code),an intelligent all-in-one data analysis tool for the comprehensive analysis of single-molecule break junction data. XMe code provides end-to-end data analysis that takes in the original experimental data and returns electronic characteristics and even charge transport mechanisms. We believe that XMe Code will promote the transparency of the data analysis in single-molecule electronics and the collaborations among scientists with different research backgrounds.

关键词： Molecular electronics Single-molecule studies Break junction Data science Software

Dietary sodium acetate and sodium butyrate attenuate intestinal damage and improve lipid metabolism in juvenile largemouth bass(Micropterus salmoides) fed a high carbohydrate diet by reducing endoplasmic reticulum stress

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Animal Nutrition 2024年第1期16卷 443-456页

作者： liulan Zhao liangshun Cheng Yifang Hu xiaohui li Yihui Yang Jin Mu lianfeng Shen Guojun Hu Kuo He Haoxiao Yan Qiao liu Song Yang College of Animal Science and Technology Sichuan Agricultural University

High-carbohydrate(HC) diets decrease the intestinal levels of sodium acetate(SA) and sodium butyrate(SB) and impair the gut health of largemouth bass; however, SA and SB have been shown to enhance immunity and improve intestinal health in farmed animals. Thus, the present study was to investigate the effects of dietary SA and SB on HC diet-induced intestinal injury and the potential mechanisms in juvenile largemouth bass. The experiment set five isonitrogenous and isolipidic diets, including a lowcarbohydrate diet(9% starch)(LC), a high carbohydrate diet(18% starch)(HC), and the HC diet supplemented with 2 g/kg SA(HCSA), 2 g/kg SB(HCSB) or a combination of 1 g/kg SA and 1 g/kg SB(HCSASB).The feeding experiment was conducted for 8 weeks. A total of 525 juvenile largemouth bass with an initial body weight of 7.00 ± 0.20 g were used. The results showed that dietary SA and SB improved the weight gain rate and specific growth rate (Pliorated serum parameters(alkaline phosphatase, acid phosphatase, glutamate transaminase, and glutamic oxaloacetic transaminase)(Plipolysis(P<0.05). In summary, this study demonstrated that dietary SA and SB attenuated HC-induced intestinal damage and reduced excessive intestinal fat deposition in largemouth bass.

关键词： Sodium acetate Sodium butyrate High carbohydrate diet Endoplasmic reticulum stress Intestine health lipid metabolism

The compatibly large nonlinear optical effect and high laser-induced damage threshold in a thiophosphate CsInP_(2)S_(7)constructed with[P_(2)S_(7)]^(4-)and[InS_(6)]^(9-)

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Chinese Chemical Letters 2024年第1期35卷 533-536页

作者： Mengjia Luo xiaohui li Xingxing Jiang Zheshuai lin Zhengyang Zhou Nanchang Key Laboratory of Photoelectric Conversion and Energy Storage Materials Nanchang Institute of TechnologyNanchang 330099China Shanghai Institute of Ceramics Chinese Academy of SciencesShanghai 200050China Functional Crystals Lab Technical Institute of Physics and ChemistryChinese Academy of SciencesBeijing 100190China Institute of Experimental Physics Free University BerlinBerlin D-14195Germany

It is challenging to cooperatively improve the nonlinear optical(NLO)efficiency and the laser-induced damage threshold(liDT).This work reports a novel IR NLO materials CsInP_(2)S_(7)(CIPS)designed by combination the strategies of alkali metals substitution and microscopic NLO units PS4 introduction based on AgGaS_(2).CIPS was composed of strongly distorted[InS_(6)]^(9-)octahedra and[P_(2)S_(7)]4-dimers constructed by corner-sharing[PS_(4)]^(3-),which increase the NLO efficiency and decrease thermal expansion anisotropy *** with AgGaS_(2),CIPS exhibited strong phase matchable NLO response ca.1.1×AGS@2.1μm,high liDT ca.20.8×AgGaS_(2),and IR transparency up to 15.3μ*** analysis and theoretical investigation confirmed that large SHG effect and ultrahigh liDT of CIPS originated from the synergistic contribution of[InS_(6)]^(9-)octahedra and[P_(2)S_(7)]*** results indicate that CIPS is a promising NLO candidate in the mid-IR region,and this study provides a new approach for developing potential NLO-liDT compatible materials.

关键词： Infrared nonlinear optics materials A novel thiophosphate Structure design Structure-activity relationship High laser-induced damage threshold

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自动化决策拒绝权的属性、功能与限度

法学 2024年第7期 15-30页

作者：李晓辉中国政法大学比较法学研究院

自动化决策拒绝权作为个人信息权利的一种具体形式,是赋予数据主体在一定条件下拒绝自动化决策并要求人工干预下的二次决策的权利。在自动化决策广泛应用并暴露出现实风险的情况下,自动化决策拒绝权成为制衡算法权力的重要手段。欧盟《... 详细信息

自动化决策拒绝权作为个人信息权利的一种具体形式,是赋予数据主体在一定条件下拒绝自动化决策并要求人工干预下的二次决策的权利。在自动化决策广泛应用并暴露出现实风险的情况下,自动化决策拒绝权成为制衡算法权力的重要手段。欧盟《一般数据保护条例》机制并未对该权利发挥预期的规范效果。我国《个人信息保护法》确认了自动化决策拒绝权,应在明确该权利私法上形成权属性的基础上,强调其功能上的救济性和制衡性,将人工干预下的二次决策理解为一种实现程序正义的机制。自动化决策拒绝权的适用例外和结果导向划定了其作为算法正义矫正机制的限度。

关键词：算法权力制衡自动化决策拒绝权《个人信息保护法》《一般数据保护条例》

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局部编织技术的编织原理与应用

毛纺科技 2024年第3期52卷 44-50页

作者：范友红李小辉东华大学服装与艺术设计学院上海200051 东华大学现代服装设计与技术教育部重点实验室上海200051 同济大学上海国际设计创新研究院上海200080

为了对局部编织的创新设计提供理论与技术支持,基于SDS-ONE APEX3岛精服装设计系统以纬平针为地组织设计局部编织花样色码,主要从编织与休止针数变化的角度介绍局部编织技术的编织原理,提出不加不减局部编织、减针局部编织与加针局部编... 详细信息

为了对局部编织的创新设计提供理论与技术支持,基于SDS-ONE APEX3岛精服装设计系统以纬平针为地组织设计局部编织花样色码,主要从编织与休止针数变化的角度介绍局部编织技术的编织原理,提出不加不减局部编织、减针局部编织与加针局部编织的工艺设计方法,并在电脑横机上编织出织片小样,进一步阐述局部编织技术在二维平面的嵌花色块拼接、镂空肌理的孔眼效应、三维立体的凹凸造型以及结构轮廓成形编织方面的应用。通过对比分析花样色码与织片小样,指出局编加减针规则与先后顺序、吊目方式、色纱组合等因素对局编织片外观的影响,对局部编织技术在针织创意花型开发与成形编织方面的应用具有指导意义。

关键词：局部编织编织原理花样色码吊目电脑横机