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Alkali Tolerance of Concrete Internal Curing Agent Based on Sodium Carboxymethyl Starch

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Journal of Wuhan University of Technology(Materials Science) 2024年第1期39卷 82-90页

作者：陈梅花刘荣进 chen Ping JING Daiyan wan Dandan FU Siyuan College of Materials Science and Engineering Guilin University of TechnologyGuilin 541004China Guangxi Engineering and Technology Center for Utilization of Industrial Waste Residue in Building Materials Guilin 541004China Guangxi Maibu New Material Limited Company Guilin 541004China

Internal curing agents (ICA) based on super absorbent polymer have poor alkali tolerance and reduce the early strength of *** alkali tolerate internal curing agent (CAA-ICA) was designed and prepared by using sodium carboxymethyl starch (CMS) with high hydrophilicity,acrylic acid (AA) containing anionic carboxylic group and acrylamide (AM) containing non-ionic amide group as the main raw *** results show that the ratio of CAA-ICA alkali absorption solution is higher than that existing ICA,which solves the low water absorption ratio of the ICA in alkali *** water absorption ratio of CAA-ICA in saturated Ca(OH)_(2) solution is 95.8 g·g^(-1),and the alkali tolerance coefficient is *** application of CAA-ICA in cement-based materials can increase the internal relative humidity and miniaturize the pore *** compressive strength of mortar increases up to 12.95%at 28 d,which provids a solution to overcome the reduction of the early strength.

关键词： alkali tolerance sodium carboxymethyl starch internal curing agent compressive strength

Bending Analysis of Circular Piezoelectric Semiconductor Plates Incorporating Flexoelectricity

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Acta Mechanica Solida Sinica 2024年第4期37卷 613-621页

作者： Liang Sun Zhengguang xiao Chunli Zhang Weiqiu chen Department of Engineering Mechanics Zhejiang UniversityHangzhou310027China Department of Basic Courses Naval University of EngineeringWuhan430033China Huanjiang Laboratory Zhuji311816China

Based on the three-dimensional(3D)basic equations of piezoelectric semiconductors(PSs),we establish a two-dimensional(2D)deformation-polarization-carrier coupling bending model for PS structures,taking flexoelectricity into *** analytical solutions to classical flexure of a clamped circular PS thin plate are *** the derived analytical model,we numerically investigate the distributions of electromechanical fields and the concentration of electrons in the circular PS thin plate under an upward concentrated *** effect of flexoelectricity on the multi-field coupling responses of the circular PS plate is *** obtained results provide theoretical guidance for the design of novel PS devices.

关键词： Piezoelectric semiconductor Plate model Flexoelectricity Multi-field coupling

Atom substitution of the solid-state electrolyte Li_(10)GeP_(2)S_(12)for stabilized all-solid-state lithium metal batteries

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Journal of Energy Chemistry 2024年第1期88卷 28-38,I0002页

作者： Zijing wan xiaozhen chen Ziqi Zhou xiaoliang Zhong xiaobing Luo Dongwei Xu State Key Laboratory of Coal Combustion School of Energy and Power EngineeringHuazhong University of Science and TechnologyWuhan 430074HubeiChina

Solid-state electrolyte Li_(10)GeP_(2)S_(12)(LGPS)has a high lithium ion conductivity of 12 mS cm^(-1)at room temperature,but its inferior chemical stability against lithium metal anode impedes its practical *** all solutions,Ge atom substitution of the solid-state electrolyte LGPS stands out as the most promising solution to this interface problem.A systematic screening framework for Ge atom substitution including ionic conductivity,thermodynamic stability,electronic and mechanical properties is utilized to solve *** fast screening,an enhanced model Dop Net FC using chemical formulas for the dataset is adopted to predict ionic ***,Li_(10)SrP_(2)S_(12)(LSrPS)is screened out,which has high lithium ion conductivity(12.58 mS cm^(-1)).In addition,an enhanced migration of lithium ion across the LSr PS/Li interface is ***,compared to the LGPS/Li interface,LSrPS/Li interface exhibits a larger Schottky barrier(0.134 eV),smaller electron transfer region(3.103?),and enhanced ability to block additional electrons,all of which contribute to the stabilized *** applied theoretical atom substitution screening framework with the aid of machine learning can be extended to rapid determination of modified specific material schemes.

关键词： Atom substitution Solid-state electrolyte Machine learning Stabilized interface

Revolution in thermoelectric cooling using PbSe thermoelectrics by grid plainification

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Science China Materials 2024年第5期67卷 1672-1673页

作者： xiao-Lei Shi Qingfeng Liu Zhi-Gang chen School of Chemistry and Physics ARC Research Hub in Zero-emission Power Generation for Carbon Neutralityand Centre for Materials ScienceQueensland University of TechnologyBrisbaneQueensland4000Australia State Key Laboratory of Materials-Oriented Chemical Engineering College of Chemical EngineeringNanjing Tech UniversityNanjing211816China

Thermoelectric materials and devices enable direct conversion between heat and electricity,holding potential applications in thermoelectric power generation,localized cooling,and electronic thermal management[1].Howev... 详细信息

关键词： enable thermoelectric constrained

A Quarterly High RFM Mining Algorithm for Big Data Management

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Computers, Materials & Continua 2024年第9期80卷 4341-4360页

作者： Cuiwei Peng Jiahui chen Shicheng wan Guotao Xu School of International Education Guangdong University of TechnologyGuangzhou510006China School of Computer Science and Technology Guangdong University of TechnologyGuangzhou510006China Business Administration South China University of TechnologyGuangzhou510641China Guangzhou Institute of Technology Xidian UniversityGuangzhou710071China

In today’s highly competitive retail industry,offline stores face increasing pressure on *** hope to improve their ability in shelf management with the help of big data *** this,on-shelf availability is an essential indicator of shelf data management and closely relates to customer purchase ***(recency,frequency,andmonetary)patternmining is a powerful tool to evaluate the value of customer ***,the existing RFM patternmining algorithms do not consider the quarterly nature of goods,resulting in unreasonable shelf availability and difficulty in *** solve this problem,we propose a quarterly RFM mining algorithmfor On-shelf products named *** algorithmmines the high recency,high frequency,and high monetary patterns and considers the period of the on-shelf goods in quarterly *** conducted experiments using two real datasets for numerical and graphical analysis to prove the algorithm’s *** with the state-of-the-art RFM mining algorithm,our algorithm can identify more patterns and performs well in terms of precision,recall,and F1-score,with the recall rate nearing 100%.Also,the novel algorithm operates with significantly shorter running times and more stable memory usage than existing mining ***,we analyze the sales trends of products in different quarters and seasonal *** analysis assists businesses in maintaining reasonable on-shelf availability and achieving greater profitability.

关键词： Data mining recency pattern high-utility itemset RFM pattern mining on-shelf management

Permeable carbon fiber based thermoelectric film with exceptional EMI shielding performance and sensor capabilities

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Journal of Advanced Ceramics 2024年第8期13卷 1119-1131页

作者： Junjie Zhu Chuan Sun wanlin Feng Mengran chen Peng-An Zong Chunlei wan College of Materials Science and Engineering Nanjing Tech UniversityNanjing 211800China Nationai Innovation Institute of Defense Technology Academy of Military Sciences of the People's Liberation Army of ChinaBeijing 100089China Institute of Nuclear Physics and Chemistry Innovation Research Team for Advanced CeramicsChina Academy of Engineering PhysicsMianyang 621900China State Key Laboratory of New Ceramics and Fine Processing School of Materials Science and EngineeringTsinghua UniversityBeijing 100084China

Thermoelectric(TE)technologies offer a promising approach for directly converting skin heat into electricity for wearable *** p-type Sb2Tes and n-type BizTes as top-performing materials at room temperature,their rigid inorganic structure,with ultralow moisture permeability,poses challenges in warm and humid conditions,fostering bacterial growth and potential skin *** address this issue,we developed a cross-linked core-shell structure by electrodepositing Sb_(2)Te_(3)(Bi_(2)Te_(3))onto carbon fiber(CF).This architecture significantly improved the electrical conductivity and the Seebeck coefficient,resulting in a remarkable 300-fold increase in the power factor compared to that of pure *** CF/Sb_(2)Te_(3) and CF/Bi2Te films demonstrated optimal power factors of 450 and 121μW·m^(-1)·K^(-2),***,the fabricated films exhibited outstanding moisture permeability,over 3000 g·m^(-2)·d^(-1),exceptional electromagnetic interference shielding efficiency approaching 93 dB,and versatility as sensors for language assistance and respiratory *** attributes underline their broad applicability,emphasizing their suitability for human health protection in diverse scenarios.

关键词： thermoelectric(TE) carbon fiber(CF) Bi_(2)Te_(3) electrodeposition moisture permeability electromagnetic interference shielding

Wall temperature effects on the stability of leeward vortices of a blunt inclined cone

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Acta Mechanica Sinica 2024年第7期40卷 29-42页

作者： Ligeng Zhang Bingbing wan Siwei Dong Jianqiang chen Xi chen State Key Laboratory of Aerodynamics Mianyang 621000China

Streamwise vortex instability is one of the most potent mechanisms for the transition of the three-dimensional boundary *** using the global stability analysis methods,stability characteristics of the leeward vortex over a blunt cone with an angle of attack under a typical wind tunnel condition are studied and are compared to the case with a smaller wall temperature ratio(corresponding to a flight condition).The vortical structure features inward and outward vortices,similar to that in the flight *** the flight condition,the outward vortices appear stronger than the inward vortices,resulting in stronger outer-mode *** the inner mode is heavily stabilized compared to the flight condition,it can still radiate apparent *** acoustic sources are computed based on Lighthill's acoustic analogy,showing that the entropy term measuring the deviation from the isentropic relation is *** Mack second mode is shown to most likely trigger the transition in the flight condition,it is absent in the wind tunnel condition,and a shear-layer mode turns out to be the most dangerous ***,the instability frequencies and growth rates of the wind tunnel case are much smaller than those of the flight case,indicating that wall heating may stabilize the leeward vortices.

关键词： Instability of streamwise vortices Hypersonic boundary layer flow Spatial BiGlobal method PSE3D method

Nitrite-catalyzed economic and sustainable bromocyclization of tryptamines/tryptophols to access hexahydropyrrolo[2,3-b]indoles/tetrahydrofuroindolines in batch and flow

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Chinese Chemical Letters 2024年第7期35卷 247-252页

作者： xiao xiao Biao chen Jia-Wei Li Jun-Bo Zheng Xu wang Hang Zhao Fen-Er chen Institute of Pharmaceutical Science and Technology Collaborative Innovation Center of Yangtze River Delta Region Green PharmaceuticalsZhejiang University of TechnologyHangzhou 310014China College of Chemistry and Chemical Engineering Jiangxi Normal UniversityNanchang 330022China Engineering Center of Catalysis and Synthesis for Chiral Molecules Department of ChemistryFudan UniversityShanghai 200433China Shanghai Engineering Center of Industrial Asymmetric Catalysis for Chiral Drugs Shanghai 200433China

A highly efficient and concise bromocyclization has been successfully achieved,in which tryptamine/tryptophol derivates can be transformed to valuable HPI/TFI scaffolds with economic and green ***,a controllable cascade transformation of bromocyclization and aromatic bromination has also been smoothly achieved to form dibrominated HPIs and *** could be successfully scaled up under both the batch process and a continuous flow *** most remarkable peculiarity of our process over all previous methods is that the generated water is the major ***,successful application of this new protocol has been demonstrated by the pharmaceutical and natural products syntheses.

关键词： Tryptamines and tryptophols Nitrite Economic and sustainable bromocyclization HPI and TFI structures Bath and flow

Extraction of Valuable Metals from Titanium-bearing Blast Furnace Slag by Acid Leaching

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Journal of Wuhan University of Technology(Materials Science) 2024年第2期39卷 376-385页

作者：刘燕 chen Xuegui MAO Shuaidong xiao Yadong LI Jiacong School of Metallurgy Northeastern UniversityShenyang 110819China Key Laboratory of Ecological Metallurgy of Multi-metal Intergrown Ores of Ministry of Education Shenyang 110819China

To realize the resource utilization of the valuable metals in the titanium-containing blast furnace slag,the process route of “hydrochloric acid leaching-electrolysis-carbonization and carbon dioxide capture-preparation of calcium carbonate” was *** this study,the influences of process conditions on the leaching rates of calcium,magnesium,aluminum,and iron and the phases of the leaching residue were investigated for the leaching *** experimental results show that the HCl solution could selectively leach the elements from the titanium-containing blast furnace *** better leaching conditions are the HCl solution concentration of 4 mol/L,the leaching time of 30 min,the ratio of liquid volume to solid gas of 10 mL/g,and the stirring paddle speed of 300 r/*** the conditions,the leaching rates of calcium,magnesium,aluminum,and iron can reach 85.87%,73.41%,81.35%,and 59.08%,and the leaching rate of titanium is 10.71%.The iron and the aluminum are removed from the leachate to obtain iron-aluminum water purification agents,and the magnesium is removed from the leachate to obtain magnesium *** leaching residue phase is dominated by perovskite,followed by magnesium silicate and tricalcium aluminate,and the titaniumrich material could be obtained from the leaching residue by desiliconization.

关键词： titanium-containing blast furnace slag acid leaching valuable metals comprehensive utilization