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Journal of Rare Earths 2024年第3期42卷 586-599,I0006页

作者： Zhen Li Wei zhao Kedong Yu Ning Guo Guangchun xiao Zhiming Wang Hui Zhang College of Mechanical Engineering Qilu University of Technology(Shandong Academy of Sciences)Jinan250353China Shandong Institute of Mechanical Design and Research Jinan250031China

The effects of Y_(2)O_(3) on the microstructure, microhardness, wear resistance, high-temperature oxidation resistance, hot corrosion resistance, and electrochemical corrosion behaviour of CoCrFeNiTiNb high entropy alloy coatings formed on Ti-6Al-4V alloy surfaces were studied. The results show that the addition of Y_(2)O_(3) changes the proportion of the phase but does not change its type. The average grain size is only 1/4.7 of that of the high entropy alloy(HEA) coating, and the fine-grained strengthening leads to increases in the microhardness and wear resistance of 21.8% and 26.9%, respectively. The addition of Y_(2)O_(3) enhances the denseness and bonding properties of the oxide and corrosion product layers, reducing the oxidation and hot corrosion rates by 60.3% and 40.3%, respectively. The addition of Y_(2)O_(3) doubles the corrosion resistance which is attributed to the refinement of the grains, the increased proportion of HCP and TiN, and the weakening of galvanic coupling corrosion.

关键词： Laser cladding High entropy alloy coatings Rare earths Wear properties High temperature properties Electrochemical corrosion

Progress on the application of graphene-based composites toward energetic materials:A review

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Defence Technology（防务技术） 2024年第1期31卷 95-116页

作者： Ting Zhang xiaoming Gao Jiachen Li Libai xiao Hongxu Gao Fengqi zhao Haixia Ma College of Chemistry&Chemical Engineering Yan'an UniversityYan'an 716000ShaanxiPR China School of Chemical Engineering Northwest UniversityXi'an 710069ShaanxiPR China Xi'an Modern Chemistry Research Institute Xi'an 710065ShaanxiPR China

Carbon material is an important additive in energetic *** is a monolayer carbon material in which carbon atoms are arranged in two-dimensional honeycomb structure,who has special optical,electrical,and mechanical ***,the application of graphene-based composites in energetic materials has received extensive *** review mainly summarizes the applications of graphene and graphene-based nanomaterials in energetic *** effects of these materials on the thermal stability,sensitivity,mechanical property,ignition and combustion of energetic materials were ***,the progress of functionalized modification of graphene has been summarized,including covalent bonding modification and doping *** studies show that graphenebased materials exhibit excellent performances and might emerge as promising candidate for energetic materials.

关键词： Graphene Desensitization Thermal decomposition Catalytic combustion Energetic materials

Thylakoid engineered M2 macrophage for sonodynamic effect promoted cell therapy of early atherosclerosis

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Nano Research 2024年第4期17卷 2919-2928页

作者： Guanghao Wu Changwen Mu Qianru zhao Yao Lei ran Cheng Weidong Nie Jiamin Qu Yuping Dong Ruili Yang Haiyan Xie State Key Laboratory of Natural and Biomimetic Drugs School of Pharmaceutical SciencesChemical Biology CenterPeking UniversityBeijing 100191China School of Materials Science and Engineering Beijing Institute of TechnologyBeijing 100081China School of Life Science Beijing Institute of TechnologyBeijing 100081China School of Stomatology Peking UniversityBeijing 100081China

Atherosclerosis is the most common cause of cardiovascular diseases that contribute to the major morbidity worldwide,but still lacking of effective treatment ***,a hybrid cell is constructed for the sonodynamic effect promoted cell therapy of early atherosclerosis by fusing M2 macrophages with thylakoid(TK)*** systemic administration,the obtained TK-M2 actively accumulates in the early atherosclerotic plaques,wherein M2 macrophages relieve the cholesterol accumulation and the inflammation in the foam ***,the TK membranes decorated on the M2 macrophages exhibit both type I and type II sonodynamic effects under ultrasound(US)activation,inducing the direct apoptosis of foam *** cooperation of M2 and TK leads to significant outcome in eliminating atherosclerotic plaques without obvious side-effects,providing a new avenue for atherosclerosis treatment.

关键词： atherosclerosis thylakoid ultrasound M2 macrophage

Distribution of oxide inclusions in H13 castings under super-gravity field with multi-stage rotation speeds

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Journal of Iron and Steel Research International 2024年第1期31卷 121-133页

作者： Shao-ying Li xiao-jun Xi Xing-ming zhao Han-jie Guo Jing Guo School of Metallurgical and Ecological Engineering University of Science and Technology Beijing(USTB)Beijing100083China Beijing Key Laboratory of Special Melting and Preparation of High-End Metal Materials Beijing100083China Beijing Beiye Functional Materials Corporation Beijing100192China Shandong Tianwu Forming Technology Co. Ltd.Liaocheng252024ShandongChina

The 42 kg industrial H13 castings were prepared by different super-gravity fields with multi-rotation speeds,and the distribution of oxide inclusions in the castings was *** addition,the inward movement Reynolds number and inward movement time of oxide inclusions as well as the solidification time of molten steel at different positions in the castings were calculated to clarify the removal mechanism of oxide inclusions in super-gravity *** results show that the large size(i.e.,greater than 10μm)oxide inclusions are mainly concentrated in the inner and outer parts of the super-gravity castings with constant rotation speed(500 r min^(-1))and five-stage rotation speeds(500,600,750,850,and 950 r min^(-1)),respectively,while there are no large oxide inclusions in the super-gravity castings with three-stage rotation speeds(500,600,and 750 r min^(-1)).Although an increase in the particle size of inclusion and the rotation speed in super-gravity field is conducive to the increase in the inward movement Reynolds number of oxide inclusions and reduction in the inward movement time of oxide inclusions,it will reduce the local solidification time of molten *** the range of the rotation speed studied,the super-gravity field with three-stage rotation speeds has the best effect on the removal of inclusions in H13 molten steel.

关键词： Distribution Oxide inclusion H13 casting Super-gravity field Rotation speed

Detection method of forward-scatter signal based on Rényi entropy

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Journal of Systems Engineering and Electronics 2024年第4期35卷 865-873页

作者： ZHENG Yuqing AI xiaofeng YANG Yong zhao Feng xiao Shunping State Key Laboratory of Complex Electromagnetic Environment Effects on Electronics and Information System National University of Defense TechnologyChangsha 410073China

The application scope of the forward scatter radar(FSR)based on the Global Navigation Satellite System(GNSS)can be expanded by improving the detection ***,the forward-scatter signal model when the target crosses the baseline is ***,the detection method of the for-ward-scatter signal based on the Rényi entropy of time-fre-quency distribution is proposed and the detection performance with different time-frequency distributions is ***-tion results show that the method based on the smooth pseudo Wigner-Ville distribution(SPWVD)can achieve the best ***,combined with the geometry of FSR,the influence on detection performance of the relative distance between the target and the baseline is ***,the proposed method is validated by the anechoic chamber measurements and the results show that the detection ability has a 10 dB improvement compared with the common constant false alarm rate(CFAR)detection.

关键词： forward scatter radar(FSR) Global Navigation Satellite System(GNSS) time-frequency distribution Rényi entropy signal detection

An all-in-one FeO_(x)-rGO sponge fabricated by solid-phase microwave thermal shock for water evaporation and purification

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Journal of Environmental Sciences 2024年第4期138卷 671-683页

作者： Youkun Sun Xiuwen zhao Xueling Song Jinchen Fan Junhe Yang Yingchun Miao Shuning xiao School of Materials and Chemistry University of Shanghai for Science and TechnologyShanghai 200093China College of Chemistry and Environmental Science Qujing Normal UniversityQujing 655011China Prytula Igor Collaborate Innovation Center for Diamond Shanghai Jian Qiao UniversityShanghai 201306China

Developing high-efficiency photothermal seawater desalination devices is of significant importance in addressing the shortage of *** much effort made into photothermal materials,there is an urgent need to design a rapidly synthesized photothermal evaporator for the comprehensive purification of complex ***,we report on all-in-one FeOx-rGO photothermal sponges synthesized via solid-phase microwave thermal *** narrow band gap of the semiconductor material Fe_(3)O_(4) greatly reduces the recombination of electron-hole pairs,enhancing non-radiative relaxation light *** abundantπorbitals in rGO promote electron excitation and thermal vibration between the *** of the surface hydrophilicity and hydrophobicity promotes salt resistance while simultaneously achieving the purification of various complex polluted *** optimized GFM-3 sponge exhibitedan enhanced photothermal conversion rate of 97.3% and a water evaporation rate of 2.04 kg/(m^(2)·hr),showing promising synergistic water purification *** findings provide a highly efficient photothermal sponge for practical applicationsof seawater desalination and purification,as well as develop a super-rapid processing methodology for evaporation devices.

关键词： Desalination Photothermal device Microwave synthesis Water purification FeO_(x)-rGO

Biomineralization and mineralization using microfluidics:A comparison study

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Journal of Rock Mechanics and Geotechnical Engineering 2024年第2期16卷 661-669页

作者： Yang xiao Xiang He Guoliang Ma Chang zhao Jian Chu Hanlong Liu Key Laboratory of New Technology for Construction of Cities in Mountain Area Chongqing UniversityChongqing400045China State Key Laboratory of Coal Mine Disaster Dynamics and Control Chongqing UniversityChongqing400045China School of Civil Engineering Chongqing UniversityChongqing400045China School of Civil and Environmental Engineering Nanyang Technological UniversitySingapore

Biomineralization through microbial process has attracted great attention in the field of geotechnical engineering due to its ability to bind granular materials,clog pores,and seal *** minerals formed by biomineralization are generally the same as that by mineralization,their mechanical behaviors show a significant *** study aims to figure out the differences between biomineralization and mineralization processes by visualizing and tracking the formation of minerals using *** biomineralization and mineralization processes occurred in the Y-shaped sandcontaining microchip that mimics the underground sand *** from different areas in the reaction microchannel of microchips were captured to directly compare the distribution of *** size and numbers from different reaction times were measured to quantify the differences between biomineralization and mineralization processes in terms of crystal *** showed that the crystals were precipitated in a faster and more uncontrollable manner in the mineralization process than that in the biomineralization process,given that those two processes presented similar precipitation *** addition,a more heterogeneous distribution of crystals was observed during the biomineralization *** precipitation behaviors were further explained by the classical nucleation crystal growth *** present microfluidic tests could advance the understanding of biomineralization and provide new insight into the optimization of biocementation technology.

关键词： Microbially induced carbonate precipitation (MICP) Biocementation Crystal Calcium carbonate Nucleation

Stromal thrombospondin 1 suppresses angiogenesis in oral submucous fibrosis

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International Journal of Oral Science 2024年第1期16卷 163-172页

作者： xiao Yang Hui zhao Rui Li Yang Chen Zhi Xu Zhengjun Shang State Key Laboratory of Oral&Maxillofacial Reconstruction and Regeneration Key Laboratory of Oral Biomedicine Ministry of EducationHubei Key Laboratory of StomatologySchool&Hospital of StomatologyWuhan UniversityWuhanChina Department of Oral and Maxillofacial-Head and Neck Oncology School of Stomatology–Hospital of StomatologyWuhan UniversityWuhanChina Department of Stomatology Union HospitalTongji Medical CollegeHuazhong University of Science and TechnologyWuhanChina

A decline in mucosal vascularity is a histological hallmark of oral submucous fibrosis (OSF), a premalignant disease that is largely induced by betel quid chewing. However, the lack of available models has challenged studies of angiogenesis in OSF. Here, we found that the expression of thrombospondin 1 (THBS1), an endogenous angiostatic protein, was elevated in the stroma of tissues with OSF. Using a fibroblast-attached organoid (FAO) model, the overexpression of THBS1 in OSF was stably recapitulated in vitro. In the FAO model,treatment with arecoline, a major pathogenic component in areca nuts, enhanced the secretion of transforming growth factor (TGF)-β1 by epithelial cells, which then promoted the expression of THBS1 in fibroblasts. Furthermore, human umbilical vein endothelial cells (HUVECs)were incorporated into the FAO to mimic the vascularized component. Overexpression of THBS1 in fibroblasts drastically suppressed the sprouting ability of endothelial cells in vascularized FAOs (v FAOs). Consistently, treatment with arecoline reduced the expression of CD31in v FAOs, and this effect was attenuated when the endothelial cells were preincubated with neutralizing antibody of CD36, a receptor of THBS1. Finally, in an arecoline-induced rat OSF model, THBS1 inhibition alleviated collagen deposition and the decline in vascularity in vivo. Overall, we exploited an assembled organoid model to study OSF pathogenesis and provide a rationale for targeting THBS1.

关键词： angiogenesis elevated endogenous

Analysis of destructive effect of Zn on carbon brick and way of Zn into carbon brick

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Journal of Iron and Steel Research International 2024年第6期31卷 1344-1354页

作者： Peng-bo Liu Shu-sen Cheng Yu-qing Xue xiao-man Cheng zhao Liu University of Science and Technology Beijing Beijing 100083China Ministry of Ironmaking Shangdong Taishan Steel Group Co.Ltd.Taian 271000ShandongChina

The service life of a blast furnace depends largely on the degree of damage to the carbon brick in the *** brick and ramming material in the hearth of a 1780 m3 blast furnace after shutdown were sampled and *** was found that the substances in the cracks of the carbon brick near and above the taphole were ZnO and Zn_(2)SiO_(4),whereas the substances in the cracks of the carbon brick below the taphole were *** reaction of Zn with CO,SiO_(2),and Fes generates ZnO,Zn_(2)SiO_(4),and ZnS,resulting in volume expansion,which is an important reason for the cracking of carbon ***,several obvious Zn vapor flow channels were found in the ramming material,through which Zn vapor could enter the carbon brick,causing damage to the carbon *** the compactness of the ramming material is beneficial to preventing Zn vapor from entering the carbon brick through the voids in the ramming material,reducing the destructive effect of Zn on the carbon brick and further extending the service life of the blast furnace.

关键词： Zn Blast furnace Carbon brick Ramming material Crack

Defect chemistry for extrinsic doping in ductile semiconductor α-Ag_(2)S

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Journal of Materiomics 2024年第6期10卷 1270-1278页

作者： Hexige Wuliji Kunpeng zhao Huirong Jing Runxin Ouyang Yu Yang Tian-ran Wei Hong Zhu Xun Shi State Key Laboratory of Metal Matrix Composites School of Materials Science and EngineeringShanghai Jiao Tong UniversityShanghai200240China University of Michigan-Shanghai Jiao Tong University Joint Institute Shanghai Jiao Tong UniversityShanghai200240China State Key Laboratory of High Performance Ceramics and Superfine Microstructure Shanghai Institute of CeramicsChinese Academy of SciencesShanghai200050China

As a new type of inorganic ductile semiconductor,silver sulfide(α-Ag_(2)S)has garnered a plethora of interests in recent years due to its promising applications in flexible ***,the lack of detailed defect calculations and chemical intuition has largely hindered the optimization of material's *** this study,we systematically investigate the defect chemistry of extrinsic doping inα-Ag_(2)S using first-principles *** computationally examine a broad suite of 17 dopants and find that all aliovalent elements have extremely low doping limits(<0.002%)in α-Ag_(2)S,rendering them ineffective in tuning the electron *** contrast,the isovalent elements Se and Te have relatively high doping limits,being consistent with the experimental *** the dopant Se or Te itself does not provide additional electrons,its introduction has a significant impact on the band gap,the band-edge position,and especially the formation energy of Ag interstitials,which effectively improve the electron concentrations by 2–3 orders of *** size effects of Se and Te doping are responsible for the more favorable Ag interstitials in Ag_(2)S_(0.875)Se_(0.125) and Ag_(2)S_(0.875)Te_(0.125) with respect to pristine *** work serves as a theoretical foundation for the rational design of Ag_(2)S-based functional materials.

关键词： Defect chemistry Extrinsic doping Thermoelectric Silver sulfide First-principles