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An Organic Small Molecule as a Solid Additive in Non-Fullerene Organic Solar Cells with Improved Efficiency and Operational Stability

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Chinese Journal of Polymer Science 2023年第2期41卷 194-201页

作者： Yi-Nuo Yang xiao-Ming Li Shi-Jie Wang xiao-peng duan Yun-Hao Cai xiao-Bo Sun Dong-Hui Wei Wei Ma Yan-Ming Sun School of Chemistry Beihang UniversityBeijing100191China State Key Laboratory for Mechanical Behavior of Materials Xi’an Jiaotong UniversityXi’an710049China The College of Chemistry and Molecular Engineering Zhengzhou UniversityZhengzhou450001China

The use of additive is an effective approach to optimize the active layer morphology and improve the power conversion efficiency(PCE)of organic solar cells(OSCs).However,residual solvent additives always lead to undesirably compromise the stability of *** this work,an organic small molecule BBT-Cl was designed and used as a novel solid additive to partly replace solvent additive to fabricate highperformance *** synergistic effect of the dual additives on the optical property,morphology and photovoltaic characteristics of the PM6:Y6 based non-fullerene OSCs have been systematically *** introduction of BBT-Cl could effectively enhance the crystallinity of the blend and promote charge extraction and ***,the OSCs processed by the dual additives exhibit a high PCE of 17.73%,which is obviously higher than OSCs with CN additive(16.48%).Meanwhile,BBT-Cl based dual additives treatment has also been successfully introduced into another two non-fullerene OSCs to verify its general ***,20%PCE aging is significantly prolonged from 720 min to 2880 min for the devices proceeded with the dual *** work highlights the great potential of solid additive in the fabrication of efficient OSCs with excellent stability.

关键词： Organic solid additive Morphology Dual additives Organic solar cells Operational stability

Accurate Distinction of Weak and Strong AC Grids for Emerging Hierarchical-Infeed LCC-UHVDC Systems

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CSEE Journal of Power and Energy Systems 2024年第2期10卷 772-777页

作者： Hao xiao Xianzhong duan Yi Zhang Department of Electrical and Computer Engineering University of ManitobaWinnipeg R3T 2N2ManitobaCanada State Key Laboratory of Advanced Electromagnetic Engineering and Technology Hubei Electric Power Security and High Efficiency Key LaboratorySchool of Electrical and Electronic EngineeringHuazhong University of Science and TechnologyWuhan 430074HubeiChina RTDS Technologies Inc. Winnipeg R3T 2E1ManitobaCanada

Distinction of weak and strong AC grids for emerging hierarchical-infeed LCC-UHVDC systems is important for planning and operation departments. However, accuracy of earlier distinction methods is limited as they were developed by empirical reasoning without rigorous theoretical analysis. Hence in this letter, hierarchical-infeed interactive effective short-circuit ratio (HIESCR) index is first used for strength evaluation of HIDC systems with complex inter-inverter interactions considered. Boundary HIESCR (BHIESCR) is also introduced in the proposed distinction method of weak and strong AC grids. That is, weak (or strong) AC grids are, respectively, identified when HIESCR is less (or greater) than BHIESCR. Second, it is shown BHIESCR remains almost unchanged as 3.0 versus various system parameters and rated operation variables based on rigorous theoretical analysis. This salient feature makes the proposed method more accurate than earlier methods. Finally, the proposed method is validated by simulations based on the PSCAD/EMTDC program.

关键词： Hierarchical-Infeedinteractive effective short-circuit ratio hierarchical-infeed LCC-UHVDC systems inter-inverter interactions strong AC grids weak AC grids

Prediction and scheduling of multi-energy microgrid based on BiGRU self-attention mechanism and LQPSO

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Global Energy Interconnection 2024年第3期7卷 347-361页

作者： Yuchen duan peng Li Jing Xia School of Automation and Intelligence Beijing Jiaotong UniversityBeijing 100044P.R.China Goldwind Science&Technology Co.Ltd. Beijing 100176P.R.China

To predict renewable energy sources such as solar power in microgrids more accurately,a hybrid power prediction method is presented in this ***,the self-attention mechanism is introduced based on a bidirectional gated recurrent neural network(BiGRU)to explore the time-series characteristics of solar power output and consider the influence of different time nodes on the prediction ***,an improved quantum particle swarm optimization(QPSO)algorithm is proposed to optimize the hyperparameters of the combined prediction *** final proposed LQPSO-BiGRU-self-attention hybrid model can predict solar power more *** addition,considering the coordinated utilization of various energy sources such as electricity,hydrogen,and renewable energy,a multi-objective optimization model that considers both economic and environmental costs was constructed.A two-stage adaptive multi-objective quantum particle swarm optimization algorithm aided by a Lévy flight,named MO-LQPSO,was proposed for the comprehensive optimal scheduling of a multi-energy microgrid *** algorithm effectively balances the global and local search capabilities and enhances the solution of complex nonlinear *** effectiveness and superiority of the proposed scheme are verified through comparative simulations.

关键词： Microgrid Bidirectional gated recurrent unit Self-attention Lévy-quantum particle swarm optimization Multi-objective optimization

High-throughput screening of single-atom catalysts confined in monolayer black phosphorus for efficient nitrogen reduction reaction

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Nano Research 2024年第4期17卷 2360-2367页

作者： xiao-Yan Li Manyi duan pengfei Ou Department of Electrical and Computer Engineering University of TorontoTorontoOntario M5S 1A4Canada School of Physics and Electronic Engineering Sichuan Normal UniversityChengdu 610101China Department of Chemistry Northwestern UniversityEvanstonIL 60208USA

The discovery of metal-nitrogen centers as the active sites for electrolysis has aroused significant interest in utilizing single-atom catalysts for nitrogen reduction reaction(NRR).Properly designed nanostructured catalysts that strongly interact with nitrogen molecules(N_(2))can promote adsorption and activation,thereby resulting in efficient catalysts with high stability,activity,and *** this study,using density functional theory calculations,we selected monolayer black phosphorus(BP)as the substrate and screened a series of single-atom transition metals confined in tri-coordinated and tetra-coordinated active centers(without and with N dopants)to electro-catalyze *** a result,we have identified two promising candidates(Hf_(1)-N_(1)P_(2)-1 and Tc_(1)-N_(4)),which exhibit not only low overpotentials of 0.56 and 0.49 V but also high thermodynamic and electrochemical stability,as well as good selectivity towards NRR over the competing hydrogen evolution *** also demonstrate the ability of Hf_(1)-N_(1)P_(2)-1 and Tc_(1)-N_(4) to activate and hydrogenate N_(2) by donating electrons and regulating charge *** study not only predicts new BP-based promising catalysts but also provides guidance for the rational design of high-performance NRR electrocatalysts under ambient conditions.

关键词： N_(2) electroreduction reaction single-atom catalysts black phosphorus density functional theory high-throughput calculations

Joint Sample Position Based Noise Filtering and Mean Shift Clustering for Imbalanced Classification Learning

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Tsinghua Science and Technology 2024年第1期29卷 216-231页

作者： Lilong duan Wei Xue Jun Huang xiao Zheng School of Computer Science and Technology Anhui University of TechnologyMaanshan 243032China Institute of Artificial Intelligence Hefei Comprehensive National Science CenterHefei 230088China

The problem of imbalanced data classification learning has received much *** classification algorithms are susceptible to data skew to favor majority samples and ignore minority *** weighted minority oversampling technique(MWMOTE)is an effective approach to solve this problem,however,it may suffer from the shortcomings of inadequate noise filtering and synthesizing the same samples as the original minority *** this end,we propose an improved MWMOTE method named joint sample position based noise filtering and mean shift clustering(SPMSC)to solve these ***,in order to effectively eliminate the effect of noisy samples,SPMsC uses a new noise filtering mechanism to determine whether a minority sample is noisy or not based on its position and distribution relative to the majority *** that MWMOTE may generate duplicate samples,we then employ the mean shift algorithm to cluster minority samples to reduce synthetic replicate ***,data cleaning is performed on the processed data to further eliminate class *** on extensive benchmark datasets demonstrate the effectiveness of SPMsC compared with other sampling methods.

关键词： imbalanced data classification oversampling noise filtering clustering

Injury and protection of spiral ganglion neurons

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Chinese Medical Journal 2024年第6期137卷 651-656页

作者： Beilei duan Kevin A.peng Line Wang Department of Otorhinolaryngology Head and Neck SurgeryBeijing Friendship HospitalCapital Medical UniversityBeijing 100050China Department of Neurotology House ClinicLos AngelesCA 90017USA

Cochlear spiral ganglion neurons(SGNs)are bipolar ganglion cells and are the first neurons in the auditory transduction *** transmit complex acoustic information from hair cells to second-order sensory neurons in the cochlear nucleus for sound *** to SGNs causes largely irreversible hearing impairment because these neurons are highly differentiated cells and cannot regenerate,making treatment of sensorineural hearing loss(SNHL)arising from SGN injury *** exposed to ototoxic drugs or damaging levels of noise or when there is loss of neurotrophic factors(NTFs),aging,and presence of other factors,SGNs can be irreversibly damaged,resulting in *** has been found that NTFs and stem cells can induce regeneration among dead spiral ganglion *** this paper,we summarized the present knowledge regarding injury,protection,and regeneration of SGNs.

关键词： Spiral ganglion Injury Protection Auditory hair cell Ototoxic drugs Aminoglycosides Presbycusis

CPL-active hybrid copper(Ⅰ) halides enabled by cation inclusion with chiral crown-ether

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Science China Chemistry 2024年第10期67卷 3283-3290页

作者： peng Fan Li-Xuan Cai xiao-Fang duan Fan Yin Chen-Chen Li Zhong-Hua Deng xiao-Zhen Li Qing-Fu Sun College of Chemistry and Materials Science Fujian Normal University State Key Laboratory of Structural Chemistry Fujian Institute of Research on the Structure of MatterChinese Academy of Sciences Fujian College University of Chinese Academy of Sciences Strait Institute of Flexible Electronics (Future Technologies) Fujian Key Laboratory of Flexible ElectronicsFujian Normal University and Strait Laboratory of Flexible Electronics

Chiral hybrid metal halides with high photoluminescence quantum yield（PLQY） and superior dissymmetry factor(glum) are promising candidates for circularly polarized luminescence（CPL） emitting ***,it is a great challenge to achieve both high glumand large ***,we report a new supramolecular strategy to fabricate chiral hybrid Cu（Ⅰ）-halides with nearunity quantum yields and intense CPL *** dissymmetry factor can be dramatically modulated by tuning the hostguest *** to the chirality and variable conformations of the host-guest complexes,a series of chiral[G@LR/S]2Cu4I6have been *** incorporation of different cations within the chiral LR/Shosts leads to variations of packing modes along the c-axis and different extent of distortions in the[Cu4I6]*** them,[H3O@LR/S]+cations are stacked based on Van der Waals interactions and hierarchically self-assemble into a right/left-handed helix in[H3O@LR/S]2Cu4I6,which results in a high glumof-7×10-3and a large PLQY of 96.92%.Notably,[G@LR/S]2Cu4I6shows promising applications in single-component white light emitting diodes（WLEDs）,exhibiting a maximum dissymmetry factor of -1.2×*** effective host-guest complexation and oriented hierarchical self-assembly provide an effective strategy for the development of high-performance CPL materials.

关键词： host-guest interaction circularly polarized luminescence copper iodide cluster hierarchical self-assembly chirality

Crystalline-amorphous M@MN_x(M=Co,Fe,Ni)encapsulated in nitrogen-doped carbon for enhanced efficient and durable hydrogen evolution reaction

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Rare Metals 2024年第4期43卷 1547-1556页

作者： Yang Yang xiao-Chuan duan Shao-Hui Guo Xian-Ming Zhang College of Materials Science and Engineering College of ChemistryKey Laboratory of Interface Science and Engineering in Advanced MaterialsTaiyuan University of TechnologyYuci030600China

Developing earth-abundant electrocatalysts for hydrogen evolution reaction(HER)is important for the sustainable energy ***,efficient and stable heterocatalysts consisting of crystalline-amorphous M@MN_(x)(M=Co,Fe,Ni)encapsulated in N-doped carbon layers supported with N-doped graphene sheets(denoted as M@MN_(x)@NC-NG)are synthesized by facile hydrothermal reaction and nitridation *** the nitriding process,metal ions in M(tzbc)_2(H_(2)O)_4(tzbc=4-(1H-1,2,4-triazol-1-yl)benzoic acid)complexes are reduced to crystalline M cores,accompanied by the formation of amorphous MN_(x)shells;the tzbc ligands are insitu carbonized to form outermost N-doped carbon(NC)layers that connect with inner MN_(x)via M-N-C motifs inherited from the complex precursors and inhibit the transition of MN_(x)from amorphous to crystalline *** Co@CoN_(x)@NC-NG catalyst exhibits excellent HER activity with small overpotentials of 45 and 64 mV at a cathode current density of 10 mA·cm^(-2)and low Tafel slopes of 40 and 85 mV·dec^(-1)in 0.5 mol·L^(-1)H_(2)SO_4 and1.0 mol·L^(-1)KOH electrolytes,*** Co@CoN_(x)@NC-NG retains 97%of the initial overpotential after 100,000 s in both acidic and alkaline *** outstanding HER performance originates from the crystalline-amorphous Co@CoN_(x)that redistributes electrons around the heterointerfaces,facilitating the conversion process of H^(+)/H_(2)O to hydrogen and thereby promoting HER *** outermost NC layers serve as the armor of Co@CoN_(x),and graphene nanosheets act as carriers of egg-like Co@CoN_(x)@NC and conduction paths for electron shuttles,ensuring stable and continuous electrocatalytic hydrogen production.

关键词： Hydrogen evolution reaction Electrocatalysts Iron group metals Heterojunction Crystalline-amorphous structure

An Improved Iterated Greedy Algorithm for Solving Rescue Robot Path Planning Problem with Limited Survival Time

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Computers, Materials & Continua 2024年第7期80卷 931-947页

作者： xiaoqing Wang peng duan Leilei Meng Kaidong Yang School of Computer Science Liaocheng UniversityLiaocheng252000China Shandong Key Laboratory of Optical Communication Science and Technology School of Physics Science and Information TechnologyLiaocheng UniversityLiaocheng252059China

Effective path planning is crucial for mobile robots to quickly reach rescue destination and complete rescue tasks in a post-disaster *** this study,we investigated the post-disaster rescue path planning problem and modeled this problem as a variant of the travel salesman problem(TSP)with life-strength *** address this problem,we proposed an improved iterated greedy(IIG)***,a push-forward insertion heuristic(PFIH)strategy was employed to generate a high-quality initial ***,a greedy-based insertion strategy was designed and used in the destruction-construction stage to increase the algorithm’s exploration ***,three problem-specific swap operators were developed to improve the algorithm’s exploitation ***,an improved simulated annealing(SA)strategy was used as an acceptance criterion to effectively prevent the algorithm from falling into local *** verify the effectiveness of the proposed algorithm,the Solomon dataset was extended to generate 27 instances for ***,the proposed IIG was compared with five state-of-the-art *** parameter analysiswas conducted using the design of experiments(DOE)Taguchi method,and the effectiveness analysis of each component has been verified one by *** results indicate that IIGoutperforms the compared algorithms in terms of the number of rescue survivors and convergence speed,proving the effectiveness of the proposed algorithm.

关键词： Rescue robot path planning life strength improved iterative greedy algorithm problem-specific swap operators