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Catechol-Formaldehyde Resin Coated CdS Core-Shell Composite as Robust Photocatalyst for Long-Term Sustainable Artificial Photosynthesis of H_(2)O_(2)

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Chinese Journal of Chemistry 2024年第17期42卷 1975-1985页

作者： Yuexin xiang Zhinan xia Wanchao Hu Cuiyan tong yang xiao Changli Lu Institute of Chemistry Northeast Normal UniversityChangchunJilin130024China

Catechol-formaldehyde resin(CFR)is very attractive for H_(2)O_(2) production via the catalytic ***,the H2O2 formation is accompanied by the oxidation of catechol groups to o-benzoquinone groups on CFR,which will cause irreversible damage to CFR and greatly limit its long-term stable catalytic ***,CdS/CFR composite photocatalyst with a core-shell structure was synthesized by hydrothermal *** photogenerated electrons of Cds are used as a powerful driving force for the reversible redox conversion between catechol groups and o-benzoquinone groups on the CFR.

关键词： Hydrogen peroxide Photocatalysis Catechol-formaldehyde resin Cds Core-shell structures Oxygen reduction reaction Charge transfer Heterogeneous catalysis

Market Equilibrium Based on Cloud-edge Collaboration

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CSEE Journal of Power and Energy Systems 2024年第1期10卷 96-104页

作者： tong Cheng Haiwang Zhong Qing xia the State Key Laboratory of Power Systems the Department of Electrical EngineeringTsinghua UniversityBeijing 100084China

Market participants can only bid with lagged information disclosure under the existing market mechanism,which can lead to information asymmetry and irrational market behavior,thus influencing market *** promote rational bidding behavior of market participants and improve market efficiency,a novel electricity market mechanism based on cloudedge collaboration is proposed in this *** market information,called residual demand curve,is published to market participants in real-time on the cloud side,while participants on the edge side are allowed to adjust their bids according to the information disclosure prior to closure *** proposed mechanism can encourage rational bids in an incentive-compatible way through the process of dynamic equilibrium while protecting participants’*** paper further formulates the mathematical model of market equilibrium to simulate the process of each market participant’s strategic bidding behavior towards equilibrium.A case study based on the IEEE 30-bus system shows the proposed market mechanism can effectively guide bidding behavior of market participants,while condensing exchanged information and protecting privacy of participants.

关键词： Cloud-edge collaboration market mechanism residual demand curve strategic bidding

Development of high-power microwave mechanical integrated continuous mining device

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Journal of Rock Mechanics and Geotechnical Engineering 2024年第9期16卷 3365-3377页

作者： xia-Ting Feng Feng Lin Jiuyu Zhang Chengxiang yang Yuntan Ao Tianyang tong Key Laboratory of Ministry of Education on Safe Mining of Deep Metal Mines Northeastern UniversityShenyang110819China Key Laboratory of Liaoning Province on Deep Engineering and Intelligent Technology Northeastern UniversityShenyang110819China

This article introduces a high-power microwave mechanical integrated continuous mining device,which can achieve synchronous cutting of hard rocks by microwave and *** device includes a cutting system,a rotary translation system,a loading system,a high-power microwave system,and a control and monitoring *** technology of“master-slave follow-up”disc cutter alternating side cutting of rock was proposed,which could improve the effectiveness of rock *** integrated structure of a microwave-cut system was then proposed,and synchronous motion of the microwave-cut system and adjustment of the loading system could be *** automatic adjustment technology of the microwave working distance was developed to dynamically control the optimal microwave working *** basic functions of the equipment were verified by *** comparing the two types of disk cutters,it is found that the master-slave follow-up disk cutter can improve significantly the dust removal effect and rock breaking efficiency in rock breaking process versus the conventional large disc *** tests of slate with or without microwave were conducted using a master-slave follow-up disk *** results show that the cutting patterns of slates change from intermittent chunks(without microwave irradiation)to persistent debris(with microwave irradiation),and the cutting speed is significantly improved(170%).The development of the device provides a scientific basis for changing the conventional mining technology of metal mines and realizing the mechanical continuous mining in hard metal mines.

关键词： Hard metal mine Microwave machinery Continuous mining Master-slave follow-up disc cutter

Interaction mechanism of cyanide with pyrite during the cyanidation of pyrite and the decyanation of pyrite cyanide residues by chemical oxidation

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International Journal of Minerals,Metallurgy and Materials 2024年第9期31卷 1996-2005页

作者： Wenwen Han Hongying yang Linlin tong Key Laboratory for Ecological Metallurgy of Multimetallic Mineral(Ministry of Education) Northeastern UniversityShenyang 110819China School of Metallurgy Northeastern UniversityShenyang 110819China

The toxic cyanides in cyanide residues produced from cyanidation process for gold extraction are harmful to the *** is one of the main minerals existing in cyanide *** this work,the interaction of cyanide with pyrite and the decyanation of pyrite cyanide residue were *** revealed that high pH value,high cyanide concentration,and high pyrite dosage promoted the interaction of cyanide with *** cyanidation of pyrite was pseudo-second-order with respect to *** decyanation of pyrite cyanide residue by Na_(2)SO_(3)/air oxidation was *** cyanide removal efficiency was 83.9% after 1 h of reaction time under the optimal conditions of pH value of 11.2,SO_(3)^(2-) dosage of 22 mg·g^(-1),and air flow rate of 1.46 L·min^(-1).X-ray photoelectron spectroscopy analysis of the pyrite samples showed the formation of Fe(Ⅲ)and FeSO_(4) during the cyanidation *** cyanide that adsorbed on the pyrite surface after cyanidation mainly existed in the forms of free cyanide(CN^(-))and ferrocyanide(Fe(CN)_(6)^(4-)),which were effectively removed by Na_(2)SO_(3)/air *** the decyanation process,air intake promoted pyrite oxidation and weakened cyanide adsorption on the pyrite *** study has practical significance for gold enterprises aiming to mitigate the environmental impact related to cyanide residues.

关键词： pyrite cyanide decyanation sodium sulfite/air oxidation cyanide residue

Quantum Tunneling Enhanced Hydrogen Desorption from Graphene Surface: Atomic versus Molecular Mechanism

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Chinese Physics Letters 2024年第8期41卷 58-68页

作者： yangwu tong Yong yang Science Island Branch of Graduate School University of Science and Technology of ChinaHefei 230026China Key Lab of Photovoltaic and Energy Conservation Materials Institute of Solid State PhysicsHFIPSChinese Academy of SciencesHefei 230031China

We study the desorption mechanism of hydrogen isotopes from graphene surface using first-principles calculations,with focus on the effects of quantum *** low temperatures,quantum tunneling plays a dominant role in the desorption process of both hydrogen monomers and *** the case of dimer desorption,two types of mechanisms,namely the traditional one-step desorption in the form of molecules(molecular mechanism),and the two-step desorption in the form of individual atoms(atomic mechanism),are studied and *** the ortho-dimers,the dominant desorption mechanism is found to switch from the molecular mechanism to the atomic mechanism above a critical temperature,which is∼300K and 200K for H and D,respectively.

关键词： desorption quantum mechanism

Intelligent Reflecting Surface-Aided Secure and Covert Communications

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China Communications 2024年第9期21卷 1-10页

作者： Zhou xiaobo Jiang Yong xia Tingting xia Guiyang Shen tong School of Information and Artificial Intelligence Anhui Agricultural UniversityAnhui 230036China

This work employs intelligent reflecting surface(IRS)to enhance secure and covert communication *** formulate an optimization problem to jointly design both the reflection beamformer at IRS and transmit power at transmitter Alice in order to optimize the achievable secrecy rate at Bob subject to a covertness *** first develop a Dinkelbach-based algorithm to achieve an upper bound performance and a high-quality *** reducing the overhead and computational complexity of the Dinkelbach-based scheme,we further conceive a low-complexity algorithm in which analytical expression for the IRS reflection beamforming is derived at each *** result shows that the devised low-complexity algorithm is able to achieve similar secrecy rate performance as the Dinkelbach-based *** examination also shows that introducing an IRS into the considered system can significantly improve the secure and covert communication performance relative to the scheme without IRS.

关键词： covert communications intelligent reflecting surface physical layer security reflection beamforming

Preparation of Self-limiting Heating Cables with Excellent Processability, Mechanical Properties and PTC Effect via Thermal and Electrical Treatments

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Chinese Journal of Polymer Science 2024年第4期42卷 511-520页

作者： Tian-Hao yang tong Wu Qiang Fu State Key Laboratory of Polymer Materials Engineering College of Polymer Science and EngineeringSichuan UniversityChengdu610065China State Key Laboratory of Polymer Materials Engineering Polymer Research Institute of Sichuan UniversityChengdu610065China

Polymer/conductive filler composites have been widely used for the preparation of self-limiting heating cables with the positive temperature coefficient (PTC) effect. The control of conductive filler distribution and network in polymer matrix is the most critical for performance of PTC materials. In order to compensate for the destruction of the filler network structure caused by strong shearing during processing, an excessive conductive filler content is usually added into the polymer matrix, which in turn sacrifices its processability and mechanical properties. In this work, a facile post-treatment of the as-extruded cable, including thermal and electrical treatment to produce high-density polyethylene (HDPE)/carbon black (CB) cable with excellent PTC effect, is developed. It is found for the as-extruded sample, the strong shearing makes the CB particles disperse uniformly in HDPE matrix, and 25 wt% CB is needed for the formation of conductive paths. For the thermal-treated sample, a gradually aggregated CB filler structure is observed, which leads to the improvement of PTC effect and the notable reduction of CB content to 20 wt%. It is very interesting to see that for the sample with combined thermal and electrical treatment, CB particles are agglomerated and oriented along the electric field direction to create substantial conductive paths, which leads to a further decrease of CB content down to 15 wt%. In this way, self-limiting heating cables with excellent processability, mechanical properties and PTC effect have simultaneously been achieved.

关键词： Self-limiting heating cables Positive temperature coefficient Thermal treatment Electrical treatment

Carbon fiber reinforced liquid crystalline elastomer composites:a dual exploration in strength augmentation and transformation flexibility through 4D printing

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International Journal of Smart and Nano Materials 2024年第2期15卷 312-329页

作者： Yuliang xia.tong Mu Yanju Liu Jinsong Leng Centre for Composite Materials and Structures Harbin Institute of Technology(HIT)HarbinPeople's Republic of China Department of Astronautical Science and Mechanics Harbin Institute of Technology(HIT)HarbinPeople's Republic of China

Liquid Crystal Elastomers(LCEs)are renowned for their reversible deformation ***,enhancing their mechanical strength while retaining such flexibility has posed a considerable *** overcome this,we utilized 4D printing to develop an innovative composite of LCE with carbon fiber fabric(LCEC).This approach has notably increased the tensile strength of LCE by eightfold,all the while maintaining its exceptional capacity for reversible *** adjusting the alignment angle between carbon fiber and the LCE printing direction from 0°to 90°,the LCEC demonstrates an array of new deformation patterns,including bending,twisting,wrapping,and S-shaped transformations,which are distinct from pure LCE *** study unveils that LCE composites exhibit deformation processes markedly different from their pure material counterparts,with the ability of pure LCE to sustain tensile strains exceeding 1900%.These findings,previously undocumented and unexplored,represent a substantial contribution to the field of smart *** finite element analysis,we explored the carbon fiber and LcE matrix dynamics,revealing bending mechanics in *** combined experimental and simulation approach yields crucial insights for crafting durable,high-strength LCECs with diverse deformational properties,advancing smart material technology.

关键词： Liquid crystal elastomer composites 4D printing Smart materials

Predicted Critical State Based on Invariance of the Lyapunov Exponent in Dual Spaces

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Chinese Physics Letters 2024年第1期41卷 68-76页

作者：刘通夏旭 Department of Applied Physics School of ScienceNanjing University of Posts and TelecommunicationsNanjing 210003China Academy of Mathematics and System Sciences Chinese Academy of SciencesBeijing 100190China

Critical states in disordered systems,fascinating and subtle eigenstates,have attracted a lot of research ***,the nature of critical states is difficult to describe quantitatively,and in general,it cannot predict a system that hosts the critical *** propose an explicit criterion whereby the Lyapunov exponent of the critical state should be 0 simultaneously in dual spaces,namely the Lyapunov exponent remains invariant under the Fourier *** this criterion,we can exactly predict a one-dimensional quasiperiodic model which is not of self-duality,but hosts a large number of critical ***,we perform numerical verification of the theoretical prediction and display the self-similarity of the critical *** to computational complexity,calculations are not performed for higher dimensional ***,since the description of extended and localized states by the Lyapunov exponent is universal and dimensionless,utilizing the Lyapunov exponent of dual spaces to describe critical states should also be ***,we conjecture that some kind of connection exists between the invariance of the Lyapunov exponent and conformal invariance,which can promote the research of critical phenomena.

关键词： state exponent critical