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Acta Metallurgica Sinica(English Letters) 2024年第2期37卷 255-265页

作者： x.Y.Yue S.Y.Peng x.Zhang C.n.He Y.Z.Tian Key Laboratory for Anisotropy and Texture of Materials(Ministry of Education) School of Materials Science and EngineeringNortheastern UniversityShenyang110819China School of Materials Science and Engineering and Tianjin Key Laboratory of Composite and Functional Materials Tianjin UniversityTianjin300350China Research Centre for Metallic Wires Northeastern UniversityShenyang110819China

A Cu-10wt%Fe composite was prepared through hot-pressed sintering,and the material was subsequently solution *** hot-pressed sintered and solution treated materials were rolled and *** precipitation behavior and performance changes were systematically studied by using scanning electron microscopy and transmission electron *** contrast to the hot-pressed sintered specimen,the solution treatment significantly affects the thermal stability and properties of the Cu-10wt%Fe *** Cu-10wt%Fe composite was prepared after solid solution,cold rolling and aging at 773 K for 1 h,and it obtained excellent tensile strength of 494 MPa,uniform elongation of 16.3%,electrical conductivity of 51.1%IACS and softening temperature of 838 *** for the distinct difference in thermal stability and properties between hot-pressed sintered and solution treated specimens were *** findings provide a theoretical basis for designing high-performance Cu-based in-situ composites by post treatment.

关键词： Cu-Fe composite Hot-pressed sintering Thermal stability Strength Electrical conductivity

An intelligent active probing and trace-back scheme for IoT anomaly detection

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Digital Communications and networks 2024年第1期10卷 168-181页

作者： Luying wang Lingyi Chen neal n.xiong Anfeng Liu Tian wang Mianxiong Dong School of Computer Science and Engineering Central South UniversityChangsha 410083China Department of Computer Science and Mathematics Sul Ross State UniversityAlpineTX 79830USA Artificial Intelligence and Future networks Beijing Normal University&UICZhuhai 519087China Department of Information and Electronic Engineering Muroran Institute of TechnologyMuroran 050-8585Japan

Due to their simple hardware,sensor nodes in IoT are vulnerable to attack,leading to data routing blockages or malicious tampering,which significantly disrupts secure data *** Intelligent Active Probing and Trace-back Scheme for IoT Anomaly Detection(APTAD)is proposed to collect integrated IoT data by recruiting Mobile Edge Users(MEUs).(a)An intelligent unsupervised learning approach is used to identify anomalous data from the collected data by MEUs and help to identify anomalous nodes.(b)Recruit MEUs to trace back and propose a series of trust calculation methods to determine the trust of nodes.(c)The last,the number of active detection packets and detection paths are designed,so as to accurately identify the trust of nodes in IoT at the minimum cost of the network.A large number of experimental results show that the recruiting cost and average anomaly detection time are reduced by 6.5 times and 34.33%respectively,while the accuracy of trust identification is improved by 20%.

关键词： Anomaly detection Internet of things Integrating data collection Mobile edge users Intelligent

On Existence of the Even L_(p)Gaussian Minkowski Problem for p>n

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Chinese Annals of Mathematics,Series B 2024年第2期45卷 179-192页

作者： Hejun wang School of Mathematics and Statistics Shandong Normal UniversityJi'nan 250014China

This paper concerns the even L_(p)Gaussian Minkowski problem in n-dimensional Euclidean space R^(n).The existence of the solution to the even L_(p)Guassian Minkowski problem for p>n is obtained.

关键词： Convex body Existence L_(p)Gaussian surface area measure The even L_(p)Gaussian Minkowski problem

Vacancy defect MoSeTe embedded in n and F co-doped carbon skeleton for high performance sodium ion batteries and hybrid capacitors

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Journal of Energy Chemistry 2024年第3期90卷 652-664,I0014页

作者： Dehui Yang Wentao Guo Fei Guo Jiaming Zhu Gang wang Hui wang Guanghui Yuan Shenghua Ma Beibei wang State Key Laboratory of Photon-Technology in Western China Energy International Collaborative Center on Photoelectric Technology and Nano Functional MaterialsInstitute of Photonics&Photon-TechnologyNorthwest UniversityXi’an 710127ShannxiChina Key Laboratory of Synthetic and natural Functional Molecule Chemistry(Ministry of Education) College of Chemistry&Materials ScienceNorthwest UniversityXi’an 710127ShannxiChina School of Chemistry and Chemical Engineering Ankang Research Centre of New Nano-materials Science and TechnologyShaanxi University Innovation Research Institute of Advanced Energy Storage Materials and Battery Technology for Future IndustrializationAnkang UniversityAnkang 725000ShannxiChina

Sodium-ion batteries(SIBs) and hybrid capacitors(SIHCs) have garnered significant attention in energy storage due to their inherent advantages,including high energy density,cost-effectiveness,and enhanced ***,developing high-performance anode materials to improve sodium storage performa nce still remains a major ***,a facile one-pot method has been developed to fabricate a hybrid of MoSeTe nanosheets implanted within the n,F co-doped honeycomb carbon skeleton(MoSeTe/n,F@C).Experimental results demonstrate that the incorporation of large-sized Te atoms into MoSeTe nanosheets enlarges the layer spacing and creates abundant anion vacancies,which effectively facilitate the insertion/extraction of na^(+) and provide numerous ion adsorption sites for rapid surface capacitive ***,the heteroatoms n,F co-doped honeycomb carbon skeleton with a highly conductive network can restrain the volume expansion and boost reaction kinetics within the *** anticipated,the MoSeTe/n,F@C anode exhibits high reversible capacities along with exceptional cycle *** coupled with na_(3)V_(2)(PO_(4))_(3)@C(nVPF@C) to form SIB full cells,the anode delivers a reversible specific capacity of 126 mA h g^(-1) after 100 cycles at 0.1 A g^(-1).Furthermore,when combined with AC to form SIHC full cells,the anode demonstrates excellent cycling stability with a reversible specific capacity of50 mA h g^(-1) keeping over 3700 cycles at 1.0 A g^(-1).In situ xRD,ex situ TEM characterization,and theoretical calculations(DFT) further confirm the reversibility of sodium storage in MoSeTe/n,F@C anode materials during electrochemical reactions,highlighting their potential for widespread practical *** work provides new insights into the promising utilization of advanced transition metal dichalcogenides as anode materials for na^(+)-based energy storage devices.

关键词： MoSeTe n F co-doped honeycomb carbon skeleton Sodium-ion batteries Sodium-ion hybrid capacitor

An ultra-porous g-C_(3)n_(4) micro-tube coupled with Mx.ne(Ti_(3)C_(2)Tx.nanosheets for efficient degradation of organics under natural sunlight

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Journal of Environmental Sciences 2024年第3期137卷 258-270页

作者： Zongyang Ya Qiyou wang Jingjin Cai Peng wang x.nyu Jiang Zhiyin Cai Shanglin xiang Tingwei wang Dongyu Cai College of Materials Science&Engineering Nanjing Tech University30 South PuZhu RoadNanjing 211816China Key Laboratory of Flexible Electronics(KLOFE)&Institute of Advanced Materials(IAM) Jiangsu National Synergetic Innovation Center for Advanced Materials(SICAM)Nanjing Tech University30 South PuZhu RoadNanjing 211816China

It remains as a challenge for realizing efficient photo-responsive catalysts towards largescale degradation of organic pollutants under natural *** work reports a new pore engineering strategy for creating ultra-porous g-C_(3)n_(4) micro-tubes with an unprecedentedly high specific surface area of 152.96 m^(2)/*** is mainly associated with releasing internal vapor pressure in the autoclave where the hydrothermal treatment of the urea/melamine mixture is *** by microscopic observation,porosity measurement and spectroscopic characterization,it is found that releasing the pressure at halfway of hydrothermal process is vital for forming exfoliated rod-like precursors and the de-aggregation of these rods presents substantial benefits on the production of mesopores on g-C_(3)n_(4) microtubes during the calcination of *** offers a large number of reactive sites required by photocatalytic *** these micro-tubes with Ti_(3)C_(2)T_(x) nanosheets via electrostatic interaction yields a 1D/2D heterojunction with a close interfacial *** addition of metallically conductive Ti_(3)C_(2)T_(x) nanosheets accelerates the separation between electrons and holes,and also enhances the light *** these merits of structural design lead to forming a group of highly efficient catalysts demonstrating an excellent photocatalytic degradation rate of k=0.0560 min^(-1)for RhB dyes under 100 mW/cm~2 visible light radiation that micks sunlight *** laboratory valuation is further supported by an outdoor test that shows a fast degradation rate of 0.0744 min^(-1)under natural sunlight.

关键词： Carbon nitride Mx.ne Heterojunction Photocatalysis

A cascade of in situ conversion of bicarbonate to CO_(2) and CO_(2) electroreduction in a flow cell with a ni-n-S catalyst

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Journal of Energy Chemistry 2024年第1期88卷 183-193,I0005页

作者： Linghui Kong Min wang Yongxiao Tuo Shanshan Zhou Jinxiu wang Guangbo Liu xuejing Cui Jiali wang Luhua Jiang nanomaterials and Electrocatalysis Laboratory College of Materials Science and EngineeringQingdao University of Science and TechnologyQingdao 266042ShandongChina State Key Laboratory of Heavy Oil Processing College of New EnergyChina University of Petroleum(East China)Qingdao 266580ShandongChina

Combination of CO_(2) capture using inorganic alkali with subsequently electrochemical conversion of the resultant HCO_(3)^(-)to high-value chemicals is a promising route of low cost and high *** electrochemical reduction of HCO_(3)^(-)is challenging due to the inaccessible of negatively charged molecular groups to the electrode ***,we adopt a comprehensive strategy to tackle this challenge,i.e.,cascade of in situ chemical conversion of HCO_(3)^(-)to CO_(2) and CO_(2) electrochemical reduction in a flow *** a tailored ni-n-S single atom catalyst(SACs),where sulfur(S)atoms located in the second shell of ni center,the CO_(2)electroreduction(CO_(2)ER)to CO is *** experimental results and density functional theory(DFT)calculations reveal that the introduction of S increases the p electron density of n atoms near ni atom,thereby stabilizing^(*)H over n and boosting the first proton coupled electron transfer process of CO_(2)ER,i.e.,^(*)+e^(-)+^(*)H+^(*)CO_(2)→^(*)*** a result,the obtained catalyst exhibits a high faradaic efficiency(FE_(CO)~98%)and a low overpotential of 425 mV for CO production as well as a superior turnover frequency(TOF)of 47397 h^(-1),outcompeting most of the reported ni *** importantly,an extremely high FECOof 90%is achieved at 50 mA cm^(-2)in the designed membrane electrode assembly(MEA)cascade electrolyzer fed with liquid *** work not only highlights the significant role of the second coordination on the first coordination shell of the central metal for CO_(2)ER,but also provides an alternative and feasible strategy to realize the electrochemical conversion of HCO_(3)^(-)to high-value chemicals.

关键词： S doped ni-n-C single atom catalysts CO_(2)electrochemical reduction DFT calculations Membrane electrode assembly Reduction of bicarbonate

Soil and microbial C:n:P stoichiometries play vital roles in regulating P transformation in agricultural ecosystems:A review

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Pedosphere 2024年第1期34卷 44-51页

作者： Guanglei CHEn Jiahui YUAn Shenqiang wang Yuting LIAnG Dengjun wang Yiyong ZHU Yu wang State Key Laboratory of Soil and Sustainable Agriculture Changshu National Agro-Ecosystem Observation and Research StationInstitute of Soil ScienceChinese Academy of SciencesNanjing 210008China School of Life Sciences Jiangsu Normal UniversityXuzhou 221000China School of Fisheries Aquacultureand Aquatic SciencesAuburn UniversityAuburn AL 36849USA Jiangsu Collaborative Innovation Center for Solid Organic Waste Resource Utilization College of Resources and Environmental ScienceNanjing Agricultural UniversityNanjing 210095China

Stoichiometry plays a crucial role in biogeochemical cycles and can modulate soil nutrient availability and functions. In agricultural ecosystems,phosphorus(P) fertilizers(organic or chemical) are often applied to achieve high crop yields. However, P is readily fixed by soil particles, leading to low P use efficiency. Therefore, understanding the role of carbon:nitrogen:P stoichiometries of soil and microorganisms in soil P transformation is of great significance for P management in agriculture. This paper provides a comprehensive review of the recent research on stoichiometry effect on soil P transformation in agricultural ecosystems. Soil microorganisms play an important role in the transformation of soil non-labile inorganic P to microbial biomass P by regulating microbial biomass stoichiometry. They also mobilize soil unavailable organic P into available P by changing ecoenzyme stoichiometry. Organic materials, such as manure and straw, play an important role in promoting the transformation of insoluble P into available P as well. Additionally, periphytic biofilms can reduce P loss from rice field ecosystems. Agricultural stoichiometries are different from those of natural ecosystems and thereby should receive more attention due to the influences of anthropogenic factors. Therefore, it is necessary to conduct further stoichiometry research on the soil biochemical mechanisms underlying P transformation in agricultural ecosystems. In conclusion, understanding stoichiometry impact on soil P transformation is crucial for P management in agricultural ecosystems.

关键词： ecoenzyme microbial biomass microbial community microorganism P availability periphytic biofilm soil P transformation

Asymmetric copolyimide membranes fabricated by nonsolvent-induced phase separation for He/CH_(4) and He/n_(2) separation

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Frontiers of Chemical Science and Engineering 2024年第4期18卷 97-106页

作者： Ying Li Lu wang Junyan xie Yong Dai xuehong Gu xuerui wang State Key Laboratory of Materials-Oriented Chemical Engineering College of Chemical EngineeringNanjing Tech UniversityNanjing 211816China Quzhou Membrane Material Innovation Institute Quzhou 324000China

Membrane gas separation is considered an energy-saving technique to extract He from natural gas due to no phase change and room temperature ***,the membrane performance was strongly limited by the trade-off between permeance and ***,novel 4,4′-(hexafluoroisopropylidene)diphthalic anhydride(6FDA)-2,2′-bis(3-amino-4-hydroxyphenyl)hexafluoropropane(APAF)-5-amino-2-(4-aminobenzene)benzimidazole(BIA)asymmetric membranes with a thickness of 300 nm were successfully prepared by the non-solvent induced phase separation *** membrane performance was modulated by regulating dope solution compositions(e.g.,tetrahydrofuran and polymer concentration).The ideal He/CH_(4) selectivity was 124 and the optimized He permeance reached 87 GPU,beyond the current upper ***/CH_(4) selectivity was 75 and He permeance was 73 GPU for the binary mixture feed containing 0.2 mol%*** membrane showed good resistance to CO_(2) and C_(2)H_(6),which are the typical impurities in natural *** 6FDA-APAF-BIA membranes have good stability(>160 h),which can provide great potential in He extraction from natural gas.

关键词： He separation membrane natural gas copolyimide

High-frequency magnetic properties of biphase Ce_(2)Fe_(17)n_(3)/α-Fe microflakes with easy-plane anisotropy

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Journal of Rare Earths 2024年第1期42卷 110-115,I0004页

作者： Ke wang Hang Zhang Yuandong Huang Zhibiao xu Fashen Li Tao wang Key Laboratory for Magnetism and Magnetic Materials of MOE Lanzhou UniversityLanzhou730000China Key Laboratory of Special Function Materials and Structure Design Ministry of EducationLanzhou UniversityLanzhou730000China

Soft magnetic composites(SMCs)are effective as magnetic powder cores in an *** to high saturation magnetization,large magnetocrystalline anisotropy and high operating frequency of M(metal)-RE(rear earth)soft magnetic composites,it is possible to miniaturize inductor cores by reducing total loss,especially eddy current loss and excess loss at high *** this article,the characteristics of Ce_(2)Fe_(17)n_(3)/α-Fe(CFn/F)loss per volume and effective permeability reaching a high frequency of 3 MHz are *** biphase CFn/F composite exhibits a high permeability of 16 at 70 MHz,which is two times greater than that of pure Ce_(2)Fe_(17)n_(3)(CFn)*** total loss is as low as 545 mW/cm^(3)at 3 MHz and 6 *** direct current(DC)-bias properties have a percent of permeability exceeding 65% at H=7960 A/*** phenomenon indicates that our material has a higher working frequency and lower core loss than other materials;the biphase CFn/F structure is a promising and efficient approach for developing the miniaturized radio frequency(RF)inductor core.

关键词： High frequency Soft magnetic composites Easy-plane anisotropy Permeability spectra Core loss Rare earths

Computational design of bimetallic Tm_(2)@g-C_(9)n_(4)electrocatalysts for enhanced CO reduction toward C_(2)products

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Chinese Chemical Letters 2024年第7期35卷 484-490页

作者： Jiajun wang Guolin Yi Shengling Guo Jianing wang Shujuan Li Ke xu Weiyi wang Shulai Lei Tianjin Key Laboratory of Structure and Performance for Functional Molecules College of ChemistryTianjin Normal UniversityTianjin 300387China Department of Chemical Physics&Hefei national Laboratory for Physical Sciences at Microscale University of Science and Technology of ChinaHefei 230026China Hubei Key Laboratory of Low Dimensional Optoelectronic Materials and Devices Hubei University of Arts and ScienceXiangyang 441053China Hubei Longzhong Laboratory Xiangyang 441053China

Electrochemical CO reduction(ECOR)as a potential strategy for producing valuable chemicals and fuels has captured substantial ***,the currently available electrocatalysts suffer from poor selectivity and low Faradaic efficiency,limiting their industrial ***,we systematically investigate the potential of homonuclear bimetallic electrocatalysts,Tm_(2)@C_(9)n_(4)(TM=Fe,Co,ni,and Cu),for the ECOR through extensive density functional theory *** findings suggest that all four proposed monolayers exhibit exceptional stability,making them highly suitable for experimental synthesis and practical ***,these transition-metal dual atoms anchored on C_(9)n_(4)monolayers show great potential in facilitating the production of high-value C_(2)products,such as C_(2)H_(5)OH and C_(2)H_(4),due to the significantly low limiting potentials(-0.06~-0.46 V)and small kinetic energy barriers(0.54–1.08 eV)for the CO coupling ***,with the exception of ni_(2)@C_(9)n_(4),these bimetallic catalysts demonstrate the impressive suppression of the competitive hydrogen evolution reaction(HER),leading to a high selectivity for C_(2)products in *** predictions would accelerate the development of high-performance C_(9)n_(4)-based dual-atom catalysts for the ECOR.

关键词： C_(9)n_(4)monolayer Double-atom catalysts CO electroreduction Multi-carbon products Density functional theory