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Unraveling post-growth mechanisms of monolayer CsPbBr3 nanocubes:Laser-enhanced transformations and cathodoluminescence-electron microscopy correlations

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journal of Energy Chemistry 2025年第1期100卷 146-156页

作者： Mingxing Li xiaoge wang xiaofan Cao Zhiqun He Chunjun Liang Mingxing Chen jing ju Fangtian You Key Laboratory of Luminescence and Optical Information Ministry of Education Institute of Optoelectronic Technology Beijing Jiaotong University Beijing National Laboratory for Molecular Sciences (BNLMS) College of Chemistry and Molecular Engineering Peking University

Lead-halide perovskite nanoparticles（LHP NPs） are highly promising materials for next-generation displays and solid-state lighting due to their exceptional optical properties. However, their inherent instability presents a significant challenge. Recent advances have demonstrated that optoelectronic devices based on monolayer nanoparticle films exhibit both high luminescence efficiency and long-term *** research demonstrates that mobility limitations and anisotropic alignments in CsPbBr3nanocube monolayer films are key to their stabilization, hindering spontaneous growth through face-to-face fusion and resulting in the formation of connecting necks in a diagonal direction. Introducing laser irradiation confirmed this by significantly accelerating nanocubes growth, increasing mobility, and enhancing local structural ordering, leading to larger and more regularly shaped nanosheets. Fourier transform infrared spectroscopy and energy dispersive spectroscopy line-scan analyses indicated that laser irradiation did not disrupt the ligand structure. Transmission electron microscopy and correlative cathodoluminescence electron microscopy revealed the effects of post-growth and heterogeneous structures, including enhanced luminescence and inhomogeneous intensity in the nanosheets. These findings deepen the understanding of the post-growth mechanism of monolayer nanoparticles and the structure-emission correlation and highlight the unique role of laser irradiation in directing the formation of well-defined and regular nanostructures.

关键词： Post-growth mechanism Heterogeneous structure Single-particle spectroscopy Laser irradiation

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INFLUENCE OF HOT DEFORMATION ON CONTINUOUSCOOLING BAINITIC TRANSFORMATION IN A LOWCARBON STEEL

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Acta Metallurgica Sinica(English Letters) 1998年第2期11卷 121-127页

作者： Z.D.wang j.B.Qu x.H.Liu G.D.wang Northeastern Univ Shenyang China

The influence of hot deformation conditions on continuous cooling bainitic transformation has been investigated for a low carbon microalloyed steel. The CCT diagrams show that deformation in unrecrpstallized austcnite ation can accelerate transformation process. Bainitic transformation in intermediate transformation temperature region is prominent, and the proeutectoid polygonal ferrite transformation at evelated high temperature is suppressed. According to optical and TEM analyses, low carbon bainitic ferrite is characterized by granular and lathlike ferrite, based on the cooling rate and deformation conditions. For nondeformation, groaps of coarse parallel ferrite lath form from the prior austenite grain boundaries with the same crystallographic orientation. For heavy deformaton, cell structure within the austenite grains due to the high dislocation density formed, which provides more nucleation sites for bainite ferrite. So deformation can discontinue the growth of ferrite laths and decrease the length of ferrite laths.

关键词： bainite continuous cooling transformation low carbon steel deformation

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Effect of environments and normal loads on tribological properties of nitrided Ni(45)(FeCoCr)(40)(AlTi)(15)high-entropy alloys

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journal of Materials Science & Technology 2020年第7期42卷 85-96页

作者： L.W.Lan x.j.wang R.P.Guo H.j.Yang j.W.Qiao Research Center for High-Entropy Alloys College of Materials Science and EngineeringTaiyuan University of TechnologyTaiyuan030024China

The tribological properties of nitrided Ni(45)(FeCoCr)(40)(AlTi)(15)high-entropy alloys(HEAs)were investigated in air and simulated acid rain under different normal loads(5,7,10,and 12 N)at ambient *** results revealed that as-cast HEAs were only composed of FCC phase,while the volume fraction of FCC phase in the nitrided alloys was significantly ***,the hard phases of AIN,CrN,Fe4 N,and TiN phases were formed in the nitrided *** thickness of the nitriding layer was about 8.4μ*** hardness increased from 8.7 GPa in as-cast alloys to 14.5 GPa in the nitrided *** addition,under the same conditions,the friction coefficient of the nitrided alloys was higher than that of as-cast alloys,but the wear rate was generally lower than that of as-cast ***,the wear rate of the nitrided alloys was the lowest in acid rain due to the lubrication,cleaning,and cooling in the liquid *** air,dominating wear mechanisms in as-cast and nitrided alloys were abrasive,delamination,and adhesive ***,the wear mechanism of as-cast and nitrided alloys in acid rain was mainly abrasive and corrosion wears.

关键词： Abrasive wear Hardness Corrosive wear Microstructure Wear mechanism

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Sediment loads response to climate change:A preliminary study of eight large Chinese rivers

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International journal of Sediment Research 2013年第1期28卷 1-14页

作者： x.x.LU L.S.RAN S.LIU T.jIANG S.R.ZHANG j.j.wang Department of Geography National University of Singapore117570Singapore Global Change and Watershed Management Center Yunnan University of Finance and EconomicsYunnan National Climate Centre China Meteorological AdministrationBeijingChina College of Water Sciences Beijing Normal UniversityChina

Climate change characterized by increasing temperature is able to affect precipitation regime and thus surface ***,the manner in which river sediment loads respond to climate change is not well understood,and related assessment regarding the effect of climate change on sediment loads is *** present a quantitative estimate of changes in sediment loads(from 1.5 Gt yr-1pre-1990 to 0.6 Gt yr-1from 1991-2007) in response to climate change in eight large Chinese *** the past decades,precipitation change coupled with rising temperatures has played a significant role in influencing the sediment delivery dynamics,although human activities, such as reservoir construction,water diversion,sand mining and land cover change,are still the predominant forces. Lower precipitation coupled with rising temperatures has significantly reduced sediment loads delivered into the sea in semi-arid climates(4-61%).In contrast,increasingly warmer and wetter climates in subtropical zones has yielded more sediment(0.4-11%),although the increase was offset by human *** results indicate that,compared with mechanical retention by reservoirs,water reduction caused by climate change or human withdrawals has contributed more sediment reduction for the rivers with abundant sediment supply but limited transport capacity(e.g.,the Huanghe).Furthermore,our results indicate that every 1%change in precipitation has resulted in a 1.3%change in water discharge and a 2%change in sediment *** addition,every 1%change in water discharge caused by precipitation has led to a 1.6%change in sediment loads,but the same percentage of water discharge change caused largely by humans would only result in a 0.9%change in sediment *** figures can be used as a guideline for evaluating the responses of sediment loads to climate change in similar climate zones because future global warming will cause dramatic changes in water and sediment in river basins worldwide at rates previou

关键词： Sediment load Climate change Human activity Water withdrawal Chinese rivers

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In situ digital testing method for quality assessment of soft soil improvement with polyurethane

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journal of Rock Mechanics and Geotechnical Engineering 2024年第5期16卷 1732-1748页

作者： x.F.wang C.j.wang W.V.Yue Z.j.Zhang Z.Q.Yue Department of Civil Engineering China University of Geosciences (Beijing)BeijingChina Department of Water Science and Engineering Zhengzhou UniversityZhengzhouChina Department of Geotechnical Engineering Tongji UniversityShanghaiChina Department of Civil Engineering The University of Hong KongChina

This study purposes an in situ testing method on quality assessment of soil *** drilling data includes the spatial distribution and in situ strength of untreated and treated soil along three different drillholes measured by on-site drilling monitoring *** factual drilling data can characterize the degree of soil improvement by penetration injection with permeable *** from on-site drilling monitoring shows that the linear zones represent constant drilling speeds shown in the plot of drill bit advancement *** drilling time,which indicates the spatial distributions of soil *** soil profile at the study site is composed of four layers,which includes fill,untreated silty clay,treated silty clay,and mucky *** results of soil profile are verified by the parallel site *** constant drilling speeds profile the coring-resistant strength of drilled *** comparing with the untreated silty clay,the constant drilling speeds of the treated silty clay have been decreased by 13.0-62.8%.Two drilling-speed-based indices of 61.2%and 65.6%are proposed to assess the decreased average drilling speed and the increased in situ strength of treated silty *** tests,*** compressive strength(UCS)test,have been performed with core sample to investigate and characterize in situ strength by comparing that with drilling *** show that the average predicted strengths of treated silty clay are 2.4-6.9 times higher than the average measured strength of untreated silty *** UCS-based indices of 374.5%and 344.2%verified the quality assessment(QA)results by this new in situ *** method provides a cost-effective tool for quality assessment of soil improvement by utilizing the digital drilling data.

关键词： Drilling process monitoring system Hydraulic rotary drilling process Constant drilling speed Soil improvement Quality assessment

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Effect of grain size on fatigue cracking at twin boundaries in a CoCrFeMnNi high-entropy alloy

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journal of Materials Science & Technology 2020年第4期39卷 1-6页

作者： A.G.wang x.H.An j.Gu x.G.wang L.L.Li W.L.Li M.Song Q.Q.Duan Z.F.Zhang x.Z.Liao School of Aerospace Mechanical&Mechatronic EngineeringThe University of Sydne0ySydneyAustralia State Key Laboratory of Powder Metallurgy Central South UniversityChangsha 410083China Materials Fatigue and Fracture Division Institute of Metal ResearchChinese Academy of SciencesShenyang 110016China Max-Planck-Institut für Eisenforschung Max-Planck-Stra?e 140237 DüsseldorfGermany

The fatigue cracking behavior at twin boundaries(TBs)in a Co Cr Fe Mn Ni high-entropy alloy with three different grain sizes was systematically investigated under low-cycle *** of grain size,the change from slip band cracking to TB cracking occurred with increasing the difference in the Schmid factors(DSF)between matrix and ***,the required critical DSF for the transition of the dominant cracking mode decreases with decreasing grain size due to the reduced slip band spacing that increases the impingement sites on the TBs and facilitates the coalescence of defects and voids to initiate TB cracks.

关键词： High-entropy alloy Fatigue cracking Twin boundary Slip band Grain size

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A fast numerical method of introducing the strengthening effect of residual stress and strain to tensile behavior of metal matrix composites

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journal of Materials Science & Technology 2021年第28期87卷 167-175页

作者： j.F.Zhang x.x.Zhang H.Andrä Q.Z.wang B.L.xiao Z.Y.Ma Shi-changxu Innovation Center for Advanced Materials Institute of Metal ResearchChinese Academy of SciencesShenyang 110016China University of Chinese Academy of Sciences Beijing 100049China Fraunhofer Institute for Industrial Mathematics Fraunhofer-Platz 1Kaiserslautern 67663Germany

Thermal residual stress and strain(TRSS)in particle reinforced metal matrix composites(PRMMCs)are believed to cause strengthening effects,according to previous ***,the representative volume element(RVE)based computational homogenization technique was used to study the tensile deformation of PRMMCs with different particle aspect ratios(AR).The influence of TRSS was assessed quantitatively via comparing simulations with or without the cooling *** was found that the strengthening effect of TRSS was affected by the particle *** the average strengthening effect of TRSS,a fast method of introducing the strengthening effect of TRSS to the tensile behavior of PRMMCs was *** new method has reduced the computational cost by a factor *** effect of TRSS on continuous fiber-reinforced metal matrix composite was found to have a softening-effect during the entire tensile deformation process because of the pre-yield effect caused by the cooling process.

关键词： Metal matrix composites(MMC) Finite element analysis(FEA) Representative volume element(RVE) Residual stress and strain Aspect ratio

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Mechanical property and structural changes by thermal cycling in phase-separated metallic glasses

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journal of Materials Science & Technology 2021年第19期78卷 144-154页

作者： Y.Tang H.B.xiao x.D.wang Q.P.Cao D.x.Zhang j.Z.jiang International Center for New-Structured Materials(ICNSM) Laboratory of New-Structured MaterialsState Key Laboratory of Silicon Materialsand School of Materials Science and EngineeringZhejiang UniversityHangzhou310027China State Key Laboratory of Modem Optical Instrumentation Zhejiang UniversityHangzhou.310027China

Nondestructive cryogenically thermal cycling has been a simple but effective treatment to enhance mechanical properties of glassy ***,how the structural heterogeneities on nanometer scales are affected by thermal cycling is still an ***,we report the response of spatial heterogeneities in three selected Ti_(41)Zr_(25)Be_(28)Fe_(6),Zr_(56)Co_(14)Cu_(14)Al_(16)and Zr_(42)Y_(14)Co_(22)Al_(22)(at.%)metallic glasses(MGs)with different compositions to the thermal cycling,which show significantly different structure and properties after the same treatments and could be ascribed to the joint contribution of relaxation and rejuvenation induced by thermal *** rejuvenation is initially prevailed in a Zr-Y-containing MG,whereas the relaxation is dominant in a Cu-Co-containing MG,both eventually entering into a dynamic equilibrium *** employing nanometer-scale structural models,the intrinsic correlation between the spatial heterogeneity and thermal cycling is *** discovery could provide the fundamental understanding of the role of spatial heterogeneity in influencing the macroscopic properties of MGs via thermal cycling and help design high-performance glassy materials by tailoring their atomic structures with suitable thermal treatments.

关键词： Thermal cycling Metallic glass Spatial heterogeneity Relaxation Rejuvenation

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Review on Hydrogen Embrittlement of Press-hardened Steels for Automotive Applications

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Acta Metallurgica Sinica(English Letters) 2023年第7期36卷 1123-1143页

作者： Z.wang Q.Lu Z.H.Cao H.Chen M.x.Huang j.F.wang General Motors China Science Lab Shanghai201206China Department of Mechanical Engineering The University of Hong KongPokfulam RoadHong Kong999077China Key Laboratory for Advanced Materials of Ministry of Education School of Materials Science and EngineeringTsinghua UniversityBeijing100084China

Press-hardened steel(PHS)with an ultimate tensile strength(UTS)of 1500 MPa has been widely used in automotive body-in-white in the last two decades,due to its ultra-high strength and excellent formability that is achieved by hot stamping ***,the application of PHS with UTS exceeding 1500 MPa in automotive industry could be deferred due to the increased risk of hydrogen *** reduce this kind of risk,recent research efforts have been focused on various ways to optimize the microstructure of *** present review intends to summarize these efforts,to highlight present solutions to address hydrogen embrittlement,and to shed light on directions for future *** influence of microstructure on the hydrogen embrittlement of PHS has been discussed in terms of both the steel substrate and the surface *** substrate part covers the influence of martensite,carbides,inclusions,and retained austenite,while the surface part covers decarburization and oxidation,pre-coating,and trimming.

关键词： Hot stamping Press-hardened steels Coating-free Hydrogen embrittlement Fracture Al-Si coating

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Effect of Mo Addition on Microstructural Characteristics in a Re-containing Single Crystal Superalloy

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journal of Materials Science & Technology 2015年第2期31卷 143-147页

作者： x.G.Liu L.wang L.H.Lou j.Zhang Superalloys Division Institute of Metal ResearchChinese Academy of Sciences Shenyang National Laboratory for Materials Science Institute of Metal ResearchChinese Academy of Sciences

The effect of Mo addition on microstructural characteristics of a nickel-base single crystal superalloy containing 4 wt% Re was investigated. The γ/γ’ partitioning ratios determined by energy dispersive spectrometer attached to a transmission electron microscope showed that the addition of Mo enhanced the partitioning of Re,W and Cr in the g matrix while decreased the concentration of Ta in the matrix. Synchrotron radiation diffraction was adopted to measure the γ/γ’ lattice misfit at room temperature. The results indicated that Mo addition changed the γ/γ’ lattice misfit towards larger negative as well as increased the tetragonal distortion of the γ lattice. Additionally,Mo addition led to microstructural instability and altered the precipitation behavior of topologically close-packed phases during 1100 C exposure. Instead of precipitating directly from the matrix,the μ phase was observed to be converted from the α phase which precipitated preferentially as a metastable intermediate in the alloy with high Mo content.

关键词： Superalloy Molybdenum Microstructure Partitioning

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