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A non-peptide-based chymotrypsin-targeted long-wavelength emission fluorescent probe with large Stokes shift and its application in bioimaging

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Chinese Chemical Letters 2024年第10期35卷 430-436页

作者： Chuanfeng Fan Jian Gao yingkai Gao Xintong Yang Gaoning Li Xiaochun Wang Fei Li jin Zhou Haifeng Yu yi Huang jin Chen yingying Shan Li Chen Key Laboratory of Optic-electric Sensing and Analytical Chemistry for Life Science MOEShandong Provincial Key Laboratory of Biochemical EngineeringQingdao Nucleic Acid Rapid Detection Engineering Research CenterCollege of Marine Science and Biological EngineeringQingdao University of Science and TechnologyQingdao266042China School of Chemistry and Life Science Anshan Normal UniversityLiaoning Key Laboratory of Development and Utilization for Natural Products Active MoleculesAnshan114007China Biomedical Analysis Center Army Medical UniversityChongqing 400038China School of Pharmacy Weifang Medical UniversityWeifang 261053China College of Chemistry Baicheng Normal UniversityBaicheng 137000China

As a hydrolase,chymotrypsin(CHT)is involved in many physiological activities,and its abnormal activity is closely related to diabetes,pancreatic fibrosis,chronic pancreatitis and pancreatic *** this work,an innovative long-wavelength emission fluorescent probe TCF-CHT was designed and synthesized for the high specificity detection of CHT,which utilized TCF-OH and a mimetic peptide substrate 4-bromobutyryl as chromogenic group and recognition group,***-CHT exhibited excellent selectivity and eye-catching sensitivity(8.91 ng/m L)towards CHT,“off-on”long-wavelength emission at 670 nm and large Stokes shift(140 nm).Furthermore,the successful fulfillment and perfect performance in imaging endogenous CHT in complex organisms(P815 cells,HepG2 cells,zebrafish and tumor-bearing mice)verified its potential as a powerful tool for the recognition of CHT in complicated biological environments.

关键词： Chymotrypsin Fluorescent probe Long-wavelength emission Large Stokes shift Bioimaging

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Root-derived long-distance signals trigger ABA synthesis and enhance drought resistance in Arabidopsis

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Journal of Genetics and Genomics 2024年第7期51卷 749-761页

作者： Qian-Qian Liu jin-Qiu Xia Jie Wu yi Han Gui-Quan Zhang Ping-Xia Zhao Cheng-Bin Xiang Division of Life Sciences and Medicine Division of Molecular&Cell BiophysicsHefei National Science Center for Interdisciplinary Sciences at the MicroscaleUniversity of Science and Technology of ChinaThe Innovation Academy of Seed DesignChinese Academy of SciencesHefeiAnhui 230027China College of Life Sciences Anhui Agricultural UniversityHefeiAnhui 230036China College of Agronomy South China Agricultural UniversityGuangzhouGuangdong 510642China School of Biology and Basic Medical Sciences Soochow UniversitySuzhouJiangsu 215123China

Vascular plants have evolved intricate long-distance signaling mechanisms to cope with environmental stress,with reactive oxygen species(ROS)emerging as pivotal systemic signals in plant stress ***,the exact role of ROS as root-to-shoot signals in the drought response has not been *** this study,we reveal that compared with wild-type plants,ferric reductase defective 3(frd3)mutants exhibit enhanced drought resistance concomitant with elevated NINE-CIS-EPOXYCAROTENOID DIOXYGENASE 3(NCED3)transcript levels and abscisic acid(ABA)contents in leaves as well as increased hydrogen peroxide(H_(2)O_(2))levels in roots and *** experiments distinctly illustrate that drought resistance can be conferred by the frd3 rootstock regardless of the scion genotype,indicating that long-distance signals originating from frd3 roots promote an increase in ABA levels in ***,the drought resistance conferred by the frd3 mutant rootstock is weakened by the CAT2-overexpressing scion,suggesting that H_(2)O_(2)may be involved in long-distance ***,the results of comparative transcriptome and proteome analyses support the drought resistance phenotype of the frd3 *** together,our findings substantiate the notion that frd3 root-derived long-distance signals trigger ABA synthesis in leaves and enhance drought resistance,providing new evidence for root-to-shoot long-distance signaling in the drought response of plants.

关键词： frd3 Drought resistance Root-to-shoot long-distance signals Reactive oxygen species(ROS) H_(2)O_(2) Iron ABA

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Electrostatic Encapsulation of Cobalt Ions into Crystalline Framework Derived Polymer Aerogel:Ultra-light,Pressure Resistant,Hydrophobic,Photothermal Conversion,Heat Insulation and Infrared Stealth

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Chinese Journal of Polymer Science 2024年第7期42卷 946-957,I0007页

作者： yi-Fan Kang jin-Lu Tang Ming Song Wei Wang Jia-Cheng Ma Zhan-You Ji Tong Liu Wen-Huan Huang China Key Laboratory of Chemical Additives for China National Light Industry College of Chemistry and Chemical EngineeringShaanxi University of Science and TechnologyXi’an710021China College of New Energy Xi’an Shiyou UniversityXi’an710065China Xi’an Key Laboratory of Functional Supramolecular Structure and Materials College of Chemistry and Materials ScienceNorthwest UniversityXi’an710127China

A variety of electromagnetic wave absorption materials(EMWAs)have been reported,but the integration of powder materials and multifunctional devices should be investigated in-depth to adapt to practical ***,carbon-coated cobalt composites were prepared by adsorbing magnetic metal cations into an anionic crystalline framework through an electrostatic encapsulate *** reflection loss(RL_(min))of-40.49 d B and effective absorption bandwidth(EAB)of 5.36 GHz(RL<-10 d B,10.4-15.76 GHz)was achieved with an optimal radar cross section(RCS)reduction of 34.9 dB·m^(2) for the sample *** commercial applications,Co@CN-4 was integrated into sodium carboxymethyl cellulose(CMC)aerogel to create an ultra-lightweight composite aerogel that is compressive resistant and heat-holding while also having photothermal conversion *** hydrophobic modification makes it more widely *** study provides a new strategy for EWAMs to integrate versatility and improve their application prospects.

关键词： Electrostatic incorporation Magnetic nanoparticle Co@CN composites Electromagnetic wave absorbing Metal-organic framework

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Upcycling of Poly(butylene adipate-co-terephthalate)into Dual Covalent Adaptable Networks through Chain Breaking-Crosslinking Strategy

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Chinese Journal of Polymer Science 2024年第10期42卷 1505-1513,I0011页

作者： Bin-Bo Wang Rong Huang Xin Wang Tao Jiang yi Wang Shuai Du Fa-Lin Li jin Zhu Song-Qi Ma Key Laboratory of Synthetic and Biological Colloids Ministry of EducationSchool of Chemical and Material EngineeringJiangnan UniversityWuxi214122China Key Laboratory of Bio-based Polymeric Materials Technology and Application of Zhejiang Province Divisions of Polymers and CompositesNingbo Institute of Materials Technology and EngineeringChinese Academy of SciencesNingbo315201China University of Chinese Academy of Sciences Beijing100049China

Poly(butylene adipate-co-terephthalate)(PBAT),a widely studied biodegradable material,has not effectively addressed the problem of plastic *** into consideration the cost-effectiveness,upcycling PBAT should take precedence over direct composting *** present work adopts a chain breaking-crosslinking strategy,upcycling PBAT into dual covalent adaptable networks(CANs).During the chainbreaking stage,the ammonolysis between PBAT and polyethyleneimine(PEI)established the primary crosslinked ***,styrene maleic anhydride copolymer(SMA)reacted with the hydroxyl group,culminating in the formation of dual covalent adaptable *** contrast to PBAT,the PBAT-dual-CANs exhibited a notable Young's modulus of 239 MPa,alongside an inherent resistance to creep and *** to catalysis from neighboring carboxyl group and excess hydroxyl groups,the PBAT-dual-CANs exhibited fast stress ***,they could be recycled through extrusion and hot-press reprocessing,while retaining their *** straightforward strategy offers a solution for dealing with plastic waste.

关键词： Poly(butylene adipate-co-terephthalate) Dynamic crosslinked networks Chain breaking-crosslinking strategy Upcycle Recycle

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Riemann-Hilbert Problem and Multiple High-order Poles Solutions of the Focusing MKdV Equation with Nonzero Boundary Conditions

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Acta Mathematicae Applicatae Sinica 2024年

作者： Zi-yi WANG Shou-fu TIAN jin-jie YANG School of Mathematics China University of Mining and Technology

The focusing modified Korteweg-de Vries (mKdV) equation with multiple high-order poles under the nonzero boundary conditions is first investigated via developing a Riemann-Hilbert(RH) approach. We begin with the asymptotic property, symmetry and analyticity of the Jost solutions, and successfully construct the RH problem of the focusing mKdV equation. We solve the RH problem when 1/S11(k) has a single highorder pole and multiple high-order poles. Furthermore, we derive the soliton solutions of the focusing mKdV equation which corresponding with a single high-order pole and multiple high-order poles, respectively. Finally,the dynamics of one-and two-soliton solutions are graphically discussed.

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Data collection of wireless sensor network based on trajectory optimization of laser-charged UAV

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High-Confidence Computing 2024年第2期4卷 116-128页

作者： Chuanwen Luo Jian Zhang jin Qian yi Hong Zhibo Chen Yunan Hou Xiujuan Zhang Yuqing Zhu School of Information Science and Technology Beijing Forestry UniversityBeijing 100083China Engineering Research Center for Forestry-Oriented Intelligent Information Processing of National Forestry and Grassland Administration Beijing 100083China College of Information Engineering Taizhou UniversityTaizhou 225300China School of Computer Science Qufu Normal UniversityRizhao 276826China Research Center of Applied Mathematics and Machine Intelligence Zhejiang LabHangzhou 311121China Department of Computer Science California State UniversityCA 90032USA

Unmanned Aerial Vehicle(UAV)can be used as wireless aerial mobile base station for collecting data from sensors in UAV-based Wireless Sensor Networks(WSNs),which is crucial for providing seamless services and improving the performance in the next generation wireless ***,since the UAV are powered by batteries with limited energy capacity,the UAV cannot complete data collection tasks of all sensors without energy replenishment when a large number of sensors are deployed over large monitoring *** overcome this problem,we study the Real-time Data Collection with Lasercharging UAV(RDCL)problem,where the UAV is utilized to collect data from a specified WSN and is recharged using Laser Beam Directors(LBDs).This problem aims to collect all sensory data from the WSN and transport it to the base station by optimizing the flight trajectory of UAV such that realtime data performance is ensured It has been proven that the RDCL problem is *** address this,we initially focus on studying two sub-problems,the Trajectory Optimization of UAV for Data Collection(TODC)problem and the Charging Trajectory Optimization of UAV(CTO)problem,whose objectives are to find the optimal flight plans of UAV in the data collection areas and charging areas,*** we propose an approximation algorithm to solve each of them with the constant ***,we present an approximation algorithm that utilizes the solutions obtained from TODC and CTO problems to address the RDCL ***,the proposed algorithm is verified by extensive simulations.

关键词： Wireless sensor networks Laser-charged UAV Trajectory optimization Data collection

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Liquid lens based holographic camera for real 3D scene hologram acquisition using end-to-end physical model-driven network

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Light(Science & Applications) 2024年第3期13卷 488-497页

作者： Di Wang Zhao-Song Li yi Zheng You-Ran Zhao Chao Liu jin-Bo Xu yi-Wei Zheng Qian Huang Chen-Liang Chang Da-Wei Zhang Song-Lin Zhuang Qiong-Hua Wang School of Instrumentation and Optoelectronic Engineering Beihang UniversityBeijing 100191China School of Optical-Electrical and Computer Engineering University of Shanghai for Science and TechnologyShanghai 200093China

With the development of artificial intelligence,neural network provides unique opportunities for holography,such as high fidelity and dynamic *** to obtain real 3D scene and generate high fidelity hologram in real time is an urgent ***,we propose a liquid lens based holographic camera for real 3D scene hologram acquisition using an end-to-end physical model-driven network(EEPMD-Net).As the core component of the liquid camera,the first 10 mm large aperture electrowetting-based liquid lens is proposed by using specially fabricated *** design of the liquid camera ensures that the multi-layers of the real 3D scene can be obtained quickly and with great imaging *** EEPMD-Net takes the information of real 3D scene as the input,and uses two new structures of encoder and decoder networks to realize low-noise phase *** comparing the intensity information between the reconstructed image after depth fusion and the target scene,the composite loss function is constructed for phase optimization,and the high-fidelity training of hologram with true depth of the 3D scene is realized for the first *** holographic camera achieves the high-fidelity and fast generation of the hologram of the real 3D scene,and the reconstructed experiment proves that the holographic image has the advantage of low *** proposed holographic camera is unique and can be used in 3D display,measurement,encryption and other fields.

关键词： calculation solution holographic

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Establishment of microneurovascular units in alginate hydrogel microspheres to reveal the anti-hypoxic effect of salidroside

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Journal of Pharmaceutical Analysis 2024年第6期14卷 926-929页

作者： Shiyu Chen Yuxuan Li yingrui Zhang Hongren Yao Tong Xu yi Zhang jin-Ming Lin Xian-Li Meng State Key Laboratory of Southwestern Chinese Medicine Resources Innovative Institute of Chinese Medicine and PharmacyChengdu University of Traditional Chinese MedicineChengdu611137China Beijing Key Laboratory of Microanalytical Methods and Instrumentation Department of ChemistryKey Laboratory of Bioorganic Phosphorus Chemistry&Chemical Biology(Ministry of Education)Tsinghua UniversityBeijing100084China School of Ethnic Medicine Chengdu University of Traditional Chinese MedicineChengdu611137China

Microneurovascular units(mNVUs),comprising neurons,micro-glia,and blood-brain barrier(BBB)endothelial cells,are pivotal to the central nervous system and are associated with cerebral hypoxia and brain *** hypoxia triggers microglial overactivity,causing inflammation,neuronal injury,and disruption of the BBB[1].Salidroside(Sal),a key compound in Tibetan medicine Rhodiola crenulata,mitigates hypoxia-induced metabolic disorders and neuronal damage by preserving mitochondrial function[2].

关键词： injuries preserving Tibetan

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Highly efficient room temperature phosphorescent liquid crystalline polymer optical waveguides for advanced optoelectronics

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Science China Chemistry 2024年第10期67卷 3450-3457页

作者： Jie Li Yan Guan Wei Xia jin-Kang Chen Jiang Huang yi Chen Qi Lin Er-Qiang Chen He-Lou Xie Key Laboratory of Environmentally Friendly Chemistry and Application of Ministry of Education and Key Laboratory of Advanced Functional Polymer Materials of CollegesUniversities of Hunan Province and College of ChemistryXiangtan UniversityXiangtan 411105China School of Physics and Optoelectronics Xiangtan UniversityXiangtan 411105China Beijing National Laboratory for Molecular Sciences Key Laboratory of Polymer Chemistry and Physics of Ministry of EducationCollege of Chemistry and Molecular EngineeringPeking UniversityBeijing 100871China

Active organic optical waveguide materials(OOWMs)incorporating room temperature phosphorescence(RTP)hold significant promise for diverse applications in photonic and optoelectronic *** this potential,realizing active RTP optical waveguides with large-sized ordered structures and minimal light loss remains a formidable *** address this issue,we present a groundbreaking thermoplastic active OOWM with low light loss,leveraging room temperature phosphorescent liquid crystalline polymer(LCP).This innovative material can be easily synthesized through the copolymerization of phosphorescent and liquid crystalline *** resulting RTP copolymer exhibits a nematic liquid crystal phase with a phosphorescence lifetime of approximately 0.15 ms and an afterglow duration of around 1 *** the excellent processability of LCP,we successfully produce meter-scale fibers via melt *** RTP LCP fibers,characterized by a high orientation of mesogens along the fiber axis,demonstrate superior light confinement and efficient light conduction compared to unoriented samples,resulting in a low optical loss coefficient of 0.13 dB/***,the thermal responsiveness of the RTP LCP optical waveguide enables its use as a photo *** pioneering work paves the way for the design of new OOWMs tailored for advanced photonics and optoelectronics devices.

关键词： room temperature phosphorescence liquid crystalline polymer active optical waveguide

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Spatial structural characteristics of the Deda ancient landslide in the eastern Tibetan Plateau:Insights from Audio-frequency Magnetotellurics and the Microtremor Survey Method

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China Geology 2024年第2期7卷 188-202页

作者： Zhen-dong Qiu Chang-bao Guo yi-ying Zhang Zhi-hua Yang Rui-an Wu yi-qiu Yan Wen-kai Chen Feng jin Institute of Geomechanics Chinese Academy of Geological SciencesBeijing 100081China Faculty of Engineering China University of GeosciencesWuhan 430074China Key Laboratory of Active Tectonics and Geological Safety Ministry of Natural ResourcesBeijing 100081China Research Center of Neotectonism and Crustal Stability China Geological SurveyBeijing 100081China China Water Resources Beifang Investigation Design and Research Co.Ltd.Tianjin 300222China

It is of crucial importance to investigate the spatial structures of ancient landslides in the eastern Tibetan Plateau’s alpine canyons as they could provide valuable insights into the evolutionary history of the landslides and indicate the potential for future *** study examines the Deda ancient landslide,situated in the Chalong-ranbu fault zone,where creep deformation suggests a complex underground *** integrating remote sensing,field surveys,Audio-frequency Magnetotellurics(AMT),and Microtremor Survey Method(MSM)techniques,along with engineering geological drilling for validation,to uncover the landslide’s spatial feature *** research indicates that a fault is developed in the upper part of the Deda ancient landslide,and the gully divides it into Deda landslide accumulation zoneⅠand Deda landslide accumulation zoneⅡin *** distinctive geological characteristics detectable by MSM in the shallow subsurface and by AMT in deeper *** findings include the identification of two sliding zones in the Deda I landslide,the shallow sliding zone(DD-I-S1)depth is approximately 20 m,and the deep sliding zone(DD-I-S2)depth is 36.2-49.9 *** sliding zone(DD-Ⅱ-S1)depth of the DedaⅡlandslide is 37.6-43.1 m.A novel MSM-based method for sliding zone identification is proposed,achieving less than 5%discrepancy in depth determination when compared with drilling *** results provide a valuable reference for the spatial structural analysis of large-deepseated landslides in geologically complex regions like the eastern Tibetan Plateau.

关键词： Ancient landslide Remote sensing Audio-frequency Magnetotellurics(AMT) Microtremor Survey Method(MSM) Geological drilling engineering Spatial structure Tibetan Plateau Geological hazard survey engineering

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