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Mercury transportation in soil via using gypsum from flue gas desulfurization unit in coal-fired power plant

Journal of Environmental Sciences 2013年第9期25卷 1858-1864页

作者： Kelin Wang william orndorff Yan Cao Weiping Pan Institute for Combustion Science and Environmental Technology Western Kentucky University

The mercury flux in soils was investigated, which were amended by gypsums from flue gas desulphurization （FGD） units of coal- fired power plants. Studies have been carried out in confined greenhouses using FGD gypsum treated soils. Major research focus is uptakes of mercury by plants, and emission of mercury into the atmosphere under varying application rates of FGD gypsum, simulating rainfall irrigations, soils, and plants types. Higher FGD gypsum application rates generally led to higher mercury concentrations in the soils, the increased mercury emissions into the atmosphere, and the increased mercury contents in plants （especially in roots and leaves）. Soil properties and plant species can play important roles in mercury transports. Some plants, such as tall fescue, were able to prevent mercury from atmospheric emission and infiltration in the soil. Mercury concentration in the stem of plants was found to be increased and then leveled off upon increasing FGD gypsum application. However, mercury in roots and leaves was generally increased upon increasing FGD gypsum application rates. Some mercury was likely absorbed by leaves of plants from emitted mercury in the atmosphere.

关键词： flue gas desulphurization gypsums soils mercury emissions mercury uptakes mercury infiltration greenhouse tests

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Mercury adsorption characteristics of HBr-modified fly ash in an entrained-flow reactor

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Journal of Environmental Sciences 2015年第7期27卷 156-162页

作者： Yongsheng Zhang Lilin Zhao Ruitao Guo Na Song Jiawei Wang Yan Cao william orndorff Wei-ping Pan Key Laboratory of Condition Monitoring and Control for Power Plant Equipment Ministry of Education North China Electric Power University Institute for Combustion Science and Environmental Technology Western Kentucky University

In this study, the mercury adsorption characteristics of HBr-modified fly ash in an entrained-flow reactor were investigated through thermal decomposition methods. The results show that the mercury adsorption performance of the HBr-modified fly ash was enhanced significantly. The mercury species adsorbed by unmodified fly ash were Hg Cl2,Hg S and Hg O. The mercury adsorbed by HBr-modified fly ash, in the entrained-flow reactor,existed in two forms, Hg Br2 and Hg O, and the HBr was the dominant factor promoting oxidation of elemental mercury in the entrained-flow reactor. In the current study, the concentration of Hg Br2 and Hg O in ash from the fine ash vessel was 4.6 times greater than for ash from the coarse ash vessel. The fine ash had better mercury adsorption performance than coarse ash, which is most likely due to the higher specific surface area and longer residence time.

关键词： Mercury Modified fly ash Entrained-flow reactor Thermal decomposition

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