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Utilization of DTAB as a collector for the reverse flotation separation of quartz from fluorapatite

International Journal of Minerals,Metallurgy and Materials 2022年第3期29卷 446-454页

作者： Wenbiao Liu wenxuan huang Feng Rao Zhanglei Zhu Yongming Zheng Shuming Wen Faculty of Land and Resource Engineering Kunming University of Science and TechnologyKunming 650093China School of Zijin Mining Fuzhou UniversityFuzhou 350108China State Key Laboratory of Complex Nonferrous Metal Resources Clean Utilization Kunming University of Science and TechnologyKunming 650093China R&D center Yunnan Yuntianhua Co.Ltd.Kunming 650228China College of Chemistry and Chemical Engineering Xi’an University of Science and TechnologyXi’an 710054China

Reverse flotation desilication is an indispensable step for obtaining high-grade fluorapatite. In this work, dodecyltrimethylammoni- um bromide (DTAB) is recommended as an efficient collector for the reverse flotation separation of quartz from fluorapatite. Its collectivity for quartz and selectivity for fluorapatite were also compared with figures corresponding to the conventional collector dodecylamine hydrochlor- ide (DAC) via microflotation experiments. The adsorption behaviors of DTAB and DAC on minerals were systematically investigated with surface chemical analyses, such as contact angle determination, zeta potential detection, and adsorption density measurement. The results re- vealed that compared to DAC, DTAB displayed a similar and strong collectivity for quartz, and it showed a better selectivity (or worse col- lectivity) for fluorapatite, resulting in a high-efficiency separation of the two minerals. The surface chemical analysis results showed that the adsorption ability of DTAB on the quartz surface was as strong as that of DAC, whereas the adsorption amount of DTAB on the fluorapatite surface was much lower than that of DAC, which is associated with the flotation performance. During the floatation separation of the actual ore, 8wt% fluorapatite with a higher grade can be obtained using DTAB in contrast to DAC. Therefore, DTAB is a promising collector for the high-efficiency purification and sustainable utilization of valuable fluorapatite recourses.

关键词： fluorapatite desilication dodecyltrimethylammonium bromide adsorption

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Construction of ground-state preserving sparse lattice models for predictive materials simulations

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npj Computational Materials 2017年第1期3卷 203-211页

作者： wenxuan huang Alexander Urban Ziqin Rong Zhiwei Ding Chuan Luo Gerbrand Ceder Department of Material Science and Engineering Massachusetts Institute of TechnologyCambridgeMAUSA Department of Materials Science and Engineering UC BerkeleyBerkeleyCAUSA Institute of Computing Technology Chinese Academy of SciencesBeijing 100190China Materials Science Division Lawrence Berkeley National LaboratoryBerkeleyCAUSA

First-principles based cluster expansion models are the dominant approach in ab initio thermodynamics of crystalline mixtures enabling the prediction of phase diagrams and novel ground ***,despite recent advances,the construction of accurate models still requires a careful and time-consuming manual parameter tuning process for ground-state preservation,since this property is not guaranteed by *** this paper,we present a systematic and mathematically sound method to obtain cluster expansion models that are guaranteed to preserve the ground states of their reference *** method builds on the recently introduced compressive sensing paradigm for cluster expansion and employs quadratic programming to impose constraints on the model *** robustness of our methodology is illustrated for two lithium transition metal oxides with relevance for Li-ion battery cathodes,i.e.,Li_(2x)Fe_(2(1−x))O_(2) and Li_(2x)Ti_(2(1−x))O_(2),for which the construction of cluster expansion models with compressive sensing alone has proven to be *** demonstrate that our method not only guarantees ground-state preservation on the set of reference structures used for the model construction,but also show that out-of-sample ground-state preservation up to relatively large supercell size is achievable through a rapidly converging iterative *** method provides a general tool for building robust,compressed and constrained physical models with predictive power.

关键词： cluster preserving thermodynamics

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New insights into different surfactants’impacts on sludge fermentation:Focusing on the particular metabolic processes and microbial genetic traits

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Frontiers of Environmental Science & Engineering 2022年第8期16卷 221-234页

作者： Jingyang Luo Shiyu Fang wenxuan huang Feng Wang Le Zhang Fang Fang Jiashun Cao Yang Wu Dongbo Wang Key Laboratory of Integrated Regulation and Resource Development on Shallow Lakes Ministry of EducationHohai UniversityNanjing 210098China College of Environment Hohai UniversityNanjing 210098China State Key Laboratory of Pollution Control and Resource Reuse School of Environmental Science and EngineeringTongji UniversityShanghai 200092China College of Environmental Science and Engineering Hunan UniversityChangsha 410082China

Surfactants were expected to exhibit positive effects on the waste activated sludge(WAS)***,the systematic comparison of different categories of surfactants on the WAS fermentation and the functional mechanisms,especially microbial metabolic traits,have not yet been precisely *** study revealed the positive effects of different surfactants on the volatile fatty acid(VFA)production,which followed the order of alkyl polysaccharides(APG)>sodium dodecylbenzene sulfonate(SDBS)>hexadecyl trimethyl ammonium bromide(HTAB).Mechanistic exploration found that the presence of different surfactants improved solubilization and hydrolysis steps,and then contributed to the subsequent acidification with different *** functional microorganisms associated with VFA generation were enriched in surfactant-conditioned *** analysis further indicated that the key genes involved in the particular process of VFA generation were *** simultaneous bioavailable substrate improvement,functional bacterial enrichment,and metabolic activity upregulation induced by different surfactants jointly contributed to VFA promotion during WAS *** study could provide a comprehensive realization of surfactants’impacts on theWAS fermentation process,and more importantly,it reminded the public to discern the distinct interplaying effects induced by different chemicals in regulating the WAS disposal and resource recovery.

关键词： Waste activated sludge(WAS) Volatile fatty acids(VFA) Surfactant types Functional microorganisms Metabolic activity upregulation

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Linkages of volatile fatty acids and polyhexamethylene guanidine stress during sludge fermentation:Metagenomic insights of microbial metabolic traits and adaptation

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Chinese Chemical Letters 2023年第6期34卷 172-177页

作者： Feng Wang Wei Du wenxuan huang Shiyu Fang Xiaoshi Cheng Leiyu Feng Jiashun Cao Jingyang Luo Yang Wu Key Laboratory of Integrated Regulation and Resource Development on Shallow Lakes Ministry of EducationHohai UniversityNanjing 210098China College of Environment Hohai UniversityNanjing 210098China State Key Laboratory of Pollution Control and Resource Reuse School of Environmental Science and EngineeringTongji UniversityShanghai 200092China

The massive use of polyhexamethylene guanidine(PHMG),as a typical bactericidal agent,raised environmental concerns to the *** work comprehensively revealed the hormesis effects of PHMG occurred in waste activated sludge(WAS)on the generation of volatile fatty acids(VFAs)during anaerobic *** low level of PHMG(100 mg/g TSS)significantly promoted the VFAs generation(1283 mg COD/L,compared with 337 mg COD/L in the control)via synchronously facilitating the solubilization,hydrolysis,and acidification steps but inhibiting *** analysis showed that the functional anaerobe(i.e.,Bacteroides,Macellibacteroide and Parabacteroide)and corresponding genetic expressions responsible for extracellular hydrolysis(i.e.,clp P),membrane transport(i.e.,ffh and gsp F),intracellular substrates metabolism(i.e.,ald and paa F)and VFAs biosynthesis(i.e.,ACACA and FASN)were enhanced in the optimal presence of ***,the anaerobic species could respond and adapt to low PHMG stimuli via quorum sensing(i.e.,cqs A,rpf C and rpf G),and thus maintain the high microbial metabolic ***,they were unable to tolerate the toxicity of excessive PHMG,resulting in the extremely low VFAs *** work enlightened the effects of emerging pollutants on WAS fermentation at the genetic levels,and provided guidance on the WAS treatment and resource recovery.

关键词： Polyhexamethylene guanidine(PHMG) Waste activated sludge(WAS) Volatile fatty acids(VFAs) Metabolic pathways Adaptive mechanisms

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Mechanisms of allicin exposure for the sludge fermentation enhancement:Focusing on the fermentation processes and microbial metabolic traits

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Journal of Environmental Sciences 2022年第5期34卷 253-264页

作者： Feng Wang Jingyang Luo Shiyu Fang wenxuan huang Yunqi Zhang Le Zhang Xiaoshi Cheng Wei Du Fang Fang Jiashun Cao Yang Wu Key Laboratory of Integrated Regulation and Resource Development on Shallow Lakes Ministry of EducationHohai UniversityNanjing 210098China College of Environment Hohai UniversityNanjing 210098China State Key Laboratory of Pollution Control and Resource Reuse School of Environmental Science and EngineeringTongji UniversityShanghai 200092China

As a frequently used product with antimicrobial activity,consumed allicin might be dis-charged and concentrated in waste-activated sludge(WAS).However,the influence of al-licin(as an exogenous pollutant)on WAS fermentation has not been clearly *** study aimed to disclose the impacts of allicin on volatile fatty acid(VFA)generation dur-ing WAS *** results showed that the appropriate presence of allicin(10 mg/g TSS)significantly enhanced the VFA yield(1894 versus 575 mg COD/L in the control)with increased acetate proportion(24.3%).Further exploration found that allicin promoted WAS solubilization,hydrolysis and acidification *** analysis revealed that the key genes involved in extracellular hydrolysis metabolism(i.e.,CAZymes),mem-brane transport(i.e.,gtsA and ytfT),substrate metabolism(i.e.,yhdR and pfkC)and fatty acid synthesis(i.e.,accA and accD)were all highly *** also induced the bacteria to produce more signalling molecules and regulate cellular functions,thereby enhancing the microbial adaptive and regulatory capacity to the unfavourable ***,the variations in fermentative microbes and their contributions to the upregulation of func-tional genes(i.e.,ytfR,gltL,INV,iolD and pflD)for VFA generation were ***,the simultaneous stimulation of functional microbial abundances and metabolic activities contributed to VFA production in allicin-conditioned reactors.

关键词： Allicin Waste activated sludge(WAS) Anaerobic fermentation Metagenomic analysis Functional genes

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Pollutant emissions from biomass burning:A review on emission characteristics,environmental impacts,and research perspectives

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Particuology 2024年第2期85卷 296-309页

作者： Ke Jiang Ran Xing Zhihan Luo wenxuan huang Fan Yi Yatai Men Nan Zhao Zhaofeng Chang jinfeng Zhao Bo Pan Guofeng shen College of Urban and Environmental Sciences Peking UniversityBeijing100871China Beijing Key Lab Plant Resources Research and Development Beijing Technology and Business UniversityBeijing100048China College of Ecology and Environment Zhengzhou UniversityZhengzhou450001China Facultyof Environmental Sciences and Engineering Kunming University of Science and TechnologyYunnan Provincial Key Laboratoryof Soil Carbon Sequestration and Pollution ControlKunming650500China Institute of Carbon Neutrality Peking UniversityBeijing100871China

Biomass is one most abundant resource on the earth providing important energies in support of so-cioeconomic development in many *** of biomass fuels comprises to nearly 10%of the total energy from anthropogenic combustion processes:however,as the burning is usually incomplete,this process yields products of incomplete combustion posing consequently significant impacts on air quality,human health,and climate ***,we analyzed spatiotemporal characteristics in intentional and unintentional biomass burning from different sectors,discussed impacts of biomass burning emissions on indoor and outdoor air quality,and consequent influences on human *** global total con-sumption amount of biomass including both natural and anthropogenic sources was approximately 7900 Tg in 2019,with significantly large regional and sectorial discrepancies among ***,anthropogenic biomass burning amounts increased gradually,but notably in some developing countries like China residential consumption of biomass fuels,as one large sector of biomass use,decreased over *** biomass consumption needs to be accurately *** are relatively rich datasets of pollutant emission factors from biomass burning,including laboratory and field tests,but still large variations exit and contribute substantially to the uncertainty in emission *** pri-mary PM2.5,black carbon and organic carbon emissions from biomass burning were about 51,4.6,and 29 Tg,respectively,contributing to nearly 70%,55%,and 90%of the total emission from all sources,and emissions from the residential sector and open fires are major *** carbon emissions from biomass burning attracts growing interests but available studies adopted different methodologies challenging the comparability of those *** burning emissions polluted not only ambient air but more severely indoor air quality,adversely affecting human *** studies that should be emphasiz

关键词： Biomass burning Carbonaceous aerosol Emission Air quality Human health

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Chinese Chemical Letters 2023年第4期34卷 396-401页

作者： Jingyang Luo Yuxiao Li wenxuan huang Feng Wang Shiyu Fang Xiaoshi Cheng Qian Feng Fang Fang Jiashun Cao Yang Wu Key Laboratory of Integrated Regulation and Resource Development on Shallow Lakes Ministry of EducationHohai UniversityNanjing 210098China College of Environment Hohai UniversityNanjing 210098China State Key Laboratory of Pollution Control and Resource Reuse School of Environmental Science and EngineeringTongji UniversityShanghai 200092China

The distinct influences of cephalosporins(CEPs, i.e., cefamandole nafate and cefpirome sulfate) affiliated to different generations on the volatile fatty acids(VFAs) production and antibiotic resistance genes(ARGs) fates during waste activated sludge(WAS) fermentation were unveiled. The presence of CEPs mainly exhibited negative effects on the total VFAs production(5%–15% reduction), especially the cefamandole nafate, which is quite different to previous understanding. Further investigation revealed that the CEPs contributed to the solubilization and hydrolysis but inhibited the acidification process by affecting the functional microbial populations(i.e., Tissierella) and general microbial metabolic activities(i.e., pyruvate metabolism and VFAs biosynthesis). In addition, CEPs(especially the cefpirome sulfate)caused the propagation of ARGs(i.e., bla TEM, tet X and mex F) during WAS fermentation. CEPs enhanced the cell membrane permeability to promote the antibiotics mechanism of efflux pump and the horizontal transfer of ARGs. Also, the CEPs altered the regulatory systems(i.e., two component system) and microbial populations associated with ARGs, resulting in the proliferation of specific ARGs. Overall, the dissimilarity of different CEPs impacts on the WAS fermentation for VFAs production and ARGs variations enlightened the diverse environmental behaviors of anthropogenic pollutants and evoked the caution of ecological risks.

关键词： Wasteactivated sludge(WAS) Cephalosporins(CEPs) Volatilefattyacids(VFAs) Antibiotic resistancegenes(ARGs) Geneticexpressions

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MALE STERILITY 3 encodes a plant homeodomain-finger protein for male fertility in soybean

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Journal of Integrative Plant Biology 2022年第5期64卷 1076-1086页

作者： Jingjing Hou Weiwei Fan Ruirui Ma Bing Li Zhihui Yuan wenxuan huang Yueying Wu Quan Hu Chunjing Lin Xingqi Zhao Bao Peng Limei Zhao Chunbao Zhang Lianjun Sun State Key Laboratory of Agrobiotechnology Beijing Key Laboratory for Crop Genetic Improvementand College of Agronomy and BiotechnologyChina Agricultural UniversityBeijing 100193China Soybean Research Institute the National Engineering Research Center for SoybeanJilin Academy of Agricultural SciencesChangchun 130033China Jiamusi Branch of Heilongjiang Academy of Agricultural Sciences Jiamusi 154007China

Male-sterile plants are used in hybrid breeding to improve yield in soybean(Glycine max(L.)Merr.).Developing the capability to alter fertility under different environmental conditions could broaden germplasm resources and simplify hybrid ***,molecular mechanisms potentially underlying such a system in soybean were ***,using positional cloning,we identified a gene,MALE STERILITY 3(MS3),which encodes a nuclear-localized protein containing a plant homeodomain(PHD)-finger domain.A spontaneous mutation in ms3 causing premature termination of MS3 translation and partial loss of the *** analysis indicated that MS3 knockout resulted in nonfunctional pollen and no selfpollinated pods,and RNA-seq analysis revealed that MS3 affects the expression of genes associated with carbohydrate ***,the fertility of mutant ms3 can restore under longd *** mutant could thus be used to create a new,more stable photoperiod-sensitive genic male sterility line for two-line hybrid seed production,with significant impact on hybrid breeding and production.

关键词： fertility restoration male sterililty PHD-finger photoperiod soybean

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RP-3航空煤油替代燃料简化-优化反应动力学建模

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上海交通大学学报 2017年第12期51卷 1409-1414页

作者：黄文宣陈方刘洪黄小彬上海交通大学航空航天学院上海200240

针对传统化学反应机理简化方法无法兼顾精度和计算量的问题,提出了耦合化学反应机理简化和优化方法(CROM).应用CROM成功实现了对RP-3航空煤油3组分替代燃料详细化学反应机理的简化和优化,得到包含47组分、94反应的优化机理.采用优化机理... 详细信息

针对传统化学反应机理简化方法无法兼顾精度和计算量的问题,提出了耦合化学反应机理简化和优化方法(CROM).应用CROM成功实现了对RP-3航空煤油3组分替代燃料详细化学反应机理的简化和优化,得到包含47组分、94反应的优化机理.采用优化机理,数值模拟了RP-3航空煤油在激波管和对冲火焰装置中的燃烧过程,并将模拟结果与文献实验值和文献计算值进行对比验证.结果表明,该优化机理能够准确预测RP-3航空煤油的点火延迟时间和火焰传播速度,且比文献的化学反应机理规模更小、计算效率更高,具有较高的工程应用价值.

关键词： RP-3航空煤油替代燃料反应动力学机理机理简化机理优化

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基于光注入法布里-珀罗激光器的窄带可调谐微波光子滤波器

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中国激光 2017年第10期44卷 162-169页

作者：王文轩陶继黄龙南京信息职业技术学院通信学院江苏南京210023 南京大学现代工程与应用科学学院江苏南京210093

基于光注入法布里-珀罗(F-P)激光器的波长选择性放大理论,设计并实现了一种窄带可调谐的单通带微波光子滤波器(MPF)。通过改变注入锁定参数,研究了注入锁定参数对中心频率、插入损耗和带外抑制比等性能指标的影响,以及波长功率放大与腔... 详细信息

基于光注入法布里-珀罗(F-P)激光器的波长选择性放大理论,设计并实现了一种窄带可调谐的单通带微波光子滤波器(MPF)。通过改变注入锁定参数,研究了注入锁定参数对中心频率、插入损耗和带外抑制比等性能指标的影响,以及波长功率放大与腔模红移的关系。实验结果表明,通过合理调节注入功率比、主从激光器失谐频率和偏置电流,可以获得带外抑制比为27.9dB、3dB带宽为275 MHz和调谐范围为9~32GHz的MPF。所提结构可以应用于高频、宽带可调谐的滤波选频和光电振荡。

关键词：光通信光学器件微波光子滤波器注入锁定法布里-珀罗激光器波长选择性放大

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