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Laser-assisted synthesis of cobalt@N-doped carbon nanotubes decorated channels and pillars of wafer-sized silicon as highly efficient three-dimensional solar evaporator

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Chinese Chemical Letters 2021年第10期32卷 3090-3094页

作者： Yiwei Zhao Haifeng Yuan Xiaofei Zhang Guobin Xue Jiebin Tang Yuke Chen Xiaoli Zhang weijia zhou Hong Liu State Key Laboratory of Crystal Materials Shandong UniversityJi’nan 250100China Collaborative Innovation Center of Technology and Equipment for Biological Diagnosis and Therapy in Universities of Shandong Institute for Advanced Interdisciplinary Research(iAIR)University of JinanJi’nan 250022China School of Materials Science and Engineering Zhengzhou UniversityZhengzhou 450001China

The Co@NCNTs/Si pillars with channels is assemble to a suitable pure water gathering device,which is applied in seawater desalination and sewage purification to produce pure water by utilizing solar ***-efficiency utilization of solar energy to generate water vapor is popular,recyclable,and environmentally friendly for seawater desalination and sewage purification,helping to alleviate the global water shortage ***,we report an efficient and simple method to prepare a threedimensional(3 D) evaporator for steam generation by harnessing the power of the *** evaporation is composed of one-dimensional(1 D) cobalt embedded and nitrogen doped carbon nanotubes(Co@NCNTs) and 3 D silicon pillars array structure(Si pillars).The Co@NCNTs/Si pillars shows a wide light absorption range provided by carbon nanotubes and a long light absorption path because of the silicon *** surface temperature of the sample rises rapidly in 1.5 min and exceed 80C under solar illumination of one *** water evaporation can be high as 1.21 kg m^(-2) h^(-1) under one sun irradiation(1 kW/m^(2)) with the energy efficiency up to 82.4%.This scalable Co@NCNTs/Si pillars can prepare pure water from seawater and sewage,where the removal rate of ions in seawater and pollutants in sewage is similar to 100%.Based on our research,this multistage three-dimensional structure is a simple and efficient novel photothermal material for extensive seawater desalination and sewage purification.

关键词： Laser process Carbon nanotubes Silicon pillars Photothermal conversion Water evaporation

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Chromium phosphide nanoparticles embedded in porous nitrogen-/phosphorus-doped carbon as efficient electrocatalysts for a nitrogen reduction reaction

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Carbon Energy 2022年第2期4卷 237-245页

作者： Jiayuan Yu Bin Chang Wanqiang Yu Xiao Li Dufu Wang Zhinian Xu Xiaoli Zhang Hong Liu weijia zhou Institute for Advanced Interdisciplinary Research(IAIR) Shandong Collaborative Innovation Center of Technology and Equipements for Biological Diagnosis and TherapyUniversity of JinanJinanChina Shandong Best Environmental Technology Co.Ltd. JinanChina School of Materials Science and Engineering Zhengzhou UniversityZhengzhouChina State Key Laboratory of Crystal Materials Shandong UniversityJinanChina

The resource recovery of heavy metals from effluent has significant environmental implications and potential commercial *** phosphide nanoparticles embedded in a nitrogen-/phosphorus-doped porous carbon matrix(CrP/NPC)are synthesized via a consecutive Cr^(6+)leachate treatment and resource recovery *** testing shows that CrP/NPC shows excellent nitrogen reduction reaction(NRR)performance,which yields the highest NH_(3) production rate of 22.56μg h^(−1) mg^(−1)_(cat).and Faradaic efficiency(16.37%)at−0.5 V versus the reversible hydrogen electrode in a 0.05M Na_(2)SO_(4) aqueous solution,as well as robust catalytic *** isotopic experiments using ^(15)N^(2) as a nitrogen source confirm that the detected NH_(3) is derived from the NRR ***,density functional theory(DFT)calculations show that the electron deficiency environment of the Cr site can significantly reduce the barrier of the NRR process and promote the formation of intermediate species.

关键词： biosynthesis carbon-based materials chromium phosphide leachate treatment nitrogen reduction reaction resource recovery

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A biomimetic liver cancer on-a-chip reveals a critical role of LIPOCALIN-2 in promoting hepatocellular carcinoma progression

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Acta Pharmaceutica Sinica B 2023年第11期13卷 4621-4637页

作者： Peiliang Shen Yuanyuan Jia weijia zhou Weiwei Zheng Yueyao Wu Suchen Qu Shiyu Du Siliang Wang Huilian Shi Jia Sun Xin Han Jiangsu Key Laboratory for Pharmacology and Safety Evaluation of Chinese Materia Medica School of Medicine&Holistic Integrative MedicineJiangsu Joint International Research Laboratory of Chinese Medicine and Regenerative MedicineNanjing University of Chinese MedicineNanjing 210023China Department of Pharmacy Nanjing Drum Tower HospitalThe Affiliated Hospital of Nanjing University Medical SchoolNanjing 210008China Nanjing Medical Center for Clinical Pharmacy Nanjing 210008China Department of Infectious Diseases Jiangsu Province Hospital of Chinese MedicineAffiliated Hospital of Nanjing University of Chinese MedicineNanjing 210023China

Hepatic stellate cells(HSCs)represent a significant component of hepatocellular carcinoma(HCC)microenvironments which play a critical role in tumor progression and drug ***-ona-chip technology has provided a powerful in vitro platform to investigate the crosstalk between activated HSCs and HCC cells by mimicking physiological architecture with precise spatiotemporal *** we developed a tri-cell culture microfluidic chip to evaluate the impact of HSCs on HCC *** analysis revealed activated HSCs contributed to endothelial invasion,HCC drug resistance and natural killer(NK)cell *** array and RNA sequencing analysis were combined to indicate the iron-binding protein LIPOCALIN-2(LCN-2)as a key factor in remodeling tumor microenvironments in the ***-2 targeted therapy demonstrated robust anti-tumor effects both in vitro 3D biomimetic chip and in vivo mouse model,including angiogenesis inhibition,sorafenib sensitivity promotion and NK-cell cytotoxicity *** together,the microfluidic platform exhibited obvious advantages in mimicking functional characteristics of tumor microenvironments and developing targeted therapies.

关键词： HCC-on-a-chip model Hepatic stellate cells Tumor microenvironment Endothelial invasion Sorafenib resistance NK cell Exhaustion LIPOCALIN-2 Personalized anti-cancer therapies

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Waste-yeast biomass as nitrogen/phosphorus sources and carbon template:Environment-friendly synthesis of N,P-Mo_(2)C nanoparticles on porous carbon matrix for efficient hydrogen evolution

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Chinese Chemical Letters 2022年第6期33卷 3231-3235页

作者： Jiayuan Yu Wanqiang Yu Bin Chang Xiao Li Jin Jia Dufu Wang Zhinian Xu Xiaoli Zhang Hong Liu weijia zhou Collaborative Innovation Center of Technology and Equipment for Biological Diagnosis and Therapy in Universities of Shandong Institute for Advanced Interdisciplinary Research(iAIR)University of JinanJi'nan 250022China Shandong Best Environmental Technology Co. Ltd.Ji'nan 250J01 China School of Materials Science and Engineering Zhengzhou UniversityZhengzhou 450001China State Key Laboratory of Crystal Materials Shandong UniversityJi'nan 250100China

Tailor-made advanced electrocatalysts with high active and stable for hydrogen evolution reaction(HER)play a key role in the development of hydrogen ***,a N,P-co-doped molybdenum carbide confined in porous carbon matrix(N,P-Mo_(2)C/NPC)with a hierarchical structure is prepared by a resources recovery *** N,P-Mo_(2)C/NPC compound exhibits outstanding HER activity with a low overpotential of 84 mV to achieve 10 mA/cm^(2),and excellent stability in alkaline *** electrochemical measurements confirm that the enhanced HER activity of N,P-Mo_(2)C/NPC is ascribe to the synergy of N,P-codoped and porous carbon *** functional theory calculations further reveal that the electron density of active sites on Mo_(2)C can be regulated by the N/P doping,leading to optimal H adsorption *** this work,the proof-of-concept resource utilization,a microorganism derived molybdenum carbide electrocatalyst for HER is fabricated,which may inaugurate a new way for designing electrocatalysts by the utilization of solid waste.

关键词： Hydrogen evolution reaction Molybdenum carbide Non-metal doping Resource utilization Solid waste management

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Green and large-scale production of ammonia:Laser-driven pyrolysis of nitrogen-enriched biomass

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SusMat 2023年第4期3卷 533-542页

作者： Yue Li Tong Wu Yujie Wang Jiawei Li Wanqiang Yu Guixiang Zhang Bin Chang Lili Zhao Hong Liu weijia zhou Institute for Advanced Interdisciplinary Research(iAIR) School of Chemistry and Chemical EngineeringUniversity of JinanJinanChina KAUST Catalysis Center(KCC) King Abdullah University of Science and Technology(KAUST)ThuwalKingdom of Saudi Arabia State Key Laboratory of Crystal Materials Shandong UniversityJinanChina

As a vital chemical,ammonia(NH3)plays an irreplaceable role in many fields such as chemical synthesis and energy *** renewable biomass can be converted into biofuels,but its nitrogen resources are underused ***-driven pyrolysis is envisaged to debuts as a bridge to connect them to realize the direct conversion from nitrogen-rich biomass into *** pulsed laser-induced local-transient thermal effect recognized the biological nitrogen resources conversion,such as cheap and plentiful yeasts,to small gaseous molecules and achieved spectacular ammonia production rate up to 260.4 mg/h,an order of magnitude higher performance than thermochemical ammonia ***,the tiny hot point generated by a low-energy laser(20W)guarantees the whole ammonia synthesis reaction systemis in amild environment of low temperature and normal ***,the remaining solid residue after laser-driven pyrolysis also can be further exploited as a highly active catalyst for electrocatalytic nitrate reduction reaction(NIRR).

关键词： ammonia synthesis laser pyrolysis local temperature field nitrogen-enriched biomass wastes recycling

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Dielectric response of ANb_(2)O_(6)(A = Zn, Co, Mn, Ni) columbite niobates: From microwave to terahertz

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Journal of Advanced Ceramics 2024年第8期13卷 1189-1197页

作者： weijia Luo Shun Wang Siyong Zheng Jining Li Menglong Wang Yongzheng Wen ingxia Li Ji zhou State Key Laboratory of New Ceramics and Fine Processing School of Materials Science and EngineeringTsinghua UniversityBeijing 100084China Institute of Laser and Optoelectronics School of Precision Instrument and Opto-Electronics EngineeringTianjin UniversityTianjin 300072China Shandong Inspur Artificial Intelligence Research Institute Co. Ltd.Jinan 250013China School of Microelectronics Tianjin UniversityTianjin 300072China

In the upcoming 6-generation(6G)revolution,the achievement of low power consumption has become a key objective in research concerning terahertz *** an important component of passive devices,there are very few low-loss dielectric ceramics in the terahertz *** elucidate the mechanism of loss and promote the application of microwave dielectric ceramics for future 6G technology(covering microwave and terahertz frequencies),the terahertz responses of ANb_(2)O_(6)(A=Zn,Co,Mn,and Ni)columbite niobates were *** influences of magnetic loss on the Qxf values in the microwave range with different transition metal ions in the A-site were reasonably ***,due to the weakened magnetic relaxation properties in the terahertz range,the samples all exhibited low loss and approximate transparency,especially for MnNb_(2)O_(6) and NiNb_(2)O_(6)(tano<0.01 and absorption coefficient<10 cm^(-1) below 1.2 THz),which subverted the definition of traditional low-loss microwave dielectric ***,based on Mie theory,we designed a prototypical broadband metamaterial reflector to validate the applicability of the ANb_(2)O_(6) system in the terahertz band,which is highly important for the development of terahertz ceramic-based passive devices.

关键词： columbite niobates terahertz response transition metal ions magnetic loss ceramic-based metamaterials

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Applications of MXenes in human-like sensors and actuators

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Nano Research 2023年第4期16卷 5767-5795页

作者： Jinbo Pang Songang Peng Chongyang Hou Xiao Wang Ting Wang Yu Cao weijia zhou Ding Sun Kai Wang Mark H.Rümmeli Gianaurelio Cuniberti Hong Liu Institute for Advanced Interdisciplinary Research(iAIR) Collaborative Innovation Center of Technology and Equipment for Biological Diagnosis and Therapy in Universities of ShandongUniversity of JinanJinan 250022China Institute for Materials Science and Max Bergmann Center of Biomaterials Technische Universität DresdenDresden 01069Germany Center for Advancing Electronics Dresden Technische Universität DresdenDresden 01069Germany Dresden Center for Computational Materials Science Technische Universität DresdenDresden 01062Germany Dresden Center for Intelligent Materials(GCL DCIM) Technische Universität DresdenDresden 01062Germany High-Frequency High-Voltage Device and Integrated Circuits R&D Center Institute of MicroelectronicsChinese Academy of SciencesBeijing 100029China Key Laboratory of Microelectronic Devices&Integrated Technology Institute of MicroelectronicsChinese Academy of SciencesBeijing 100029China Shenzhen Key Laboratory of Nanobiomechanics Shenzhen Institute of Advanced TechnologyChinese Academy of SciencesShenzhen 518055China State Key Laboratory of Biobased Material and Green Papermaking Qilu University of TechnologyShandong Academy of SciencesJinan 250353China School of Bioengineering Qilu University of TechnologyShandong Academy of ScienceJinan 250353China Key Laboratory of Modern Power System Simulation and Control&Renewable Energy Technology(Ministry of Education) Northeast Electric Power UniversityJilin 132012China School of Electrical Engineering Northeast Electric Power UniversityJilin 132012China School of Electrical Engineering Weihai Innovation Research InstituteQingdao UniversityQingdao 266000China School of Electrical and Computer Engineering Jilin Jianzhu UniversityChangchun 130118China Institute for Complex Materials Leibniz Institute for Solid State and Materials Research Dresden(IFW Dresden)20 Helmholtz StrasseDresden 01069Germany College of Energy Soochow Institute for Energy and Materials Innovations Soochow UniversitySuzhou 215006China Key L

Human beings perceive the world through the senses of sight,hearing,smell,taste,touch,space,and *** first five senses are prerequisites for people to *** sensing organs upload information to the nervous systems,including the brain,for interpreting the surrounding ***,the brain sends commands to muscles reflexively to react to stimuli,including light,gas,chemicals,sound,and ***,as an emerging two-dimensional material,has been intensively adopted in the applications of various sensors and *** this review,we update the sensors to mimic five primary senses and actuators for stimulating muscles,which employ MXene-based film,membrane,and composite with other functional ***,a brief introduction is delivered for the structure,properties,and synthesis methods of ***,we feed the readers the recent reports on the MXene-derived image sensors as artificial retinas,gas sensors,chemical biosensors,acoustic devices,and tactile sensors for electronic ***,the actuators of MXene-based composite are ***,future opportunities are given to MXene research based on the requirements of artificial intelligence and humanoid robot,which may induce prospects in accompanying healthcare and biomedical engineering applications.

关键词： MXenes sensors actuators gas sensors biosensors tactile sensors sound sensors artificial retina

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Thermo-Flow Performances for the Main-Auxiliary Integrated Natural Draft Dry Cooling System

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Journal of Thermal Science 2024年第3期33卷 1010-1025页

作者： ZHANG Zongyang HOU Yichen zhou Hanyu JIA He CHEN Lei KONG Yanqiang WANG weijia YANG Lijun DU Xiaoze Key Laboratory of Power Station Energy Transfer Conversion and System of Ministry of Education School of Energy Power and Mechanical EngineeringNorth China Electric Power UniversityBeijing102206China

Recently,natural draft dry cooling system with the main-auxiliary integrated air-cooled heat exchangers in the up and lower layers,has drawn attention to the electric power *** research firstly develops two physical models for the integrated cooling system,namely Case A and Case *** Case A,the main air-cooled heat exchanger is arranged in the upper layer and the auxiliary air-cooled heat exchanger arranged in the lower layer,while in Case B,the two heat exchanger systems are arranged in the opposite *** then,directing at the engineering TMCR and TRL 1 working conditions,the unit-local-overall thermo-flow characteristics of Case A and Case B are obtained and compared by numerical *** findings show that,for the auxiliary air-cooled exchanger,Case A has obviously higher cooling performances than Case B,with the difference varying from 5.46%to 7.55%.Whereas,for the main air-cooled exchanger,Case B shows the recovered cooling performances,with the difference changing from 1.15%to 2.99%.Case A is preferably recommended to the engineering application in consideration of more strict cooling demand of the auxiliary cooling ***,this research will provide some theoretical guidelines for the design and construction of the main-auxiliary integrated natural draft dry cooling system.

关键词： integrated dry cooling system main air-cooled heat exchanger auxiliary air-cooled heat exchanger upper layer and lower layer thermo-flow performances

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Emerging Internet of Things driven carbon nanotubes-based devices

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Nano Research 2022年第5期15卷 4613-4637页

作者： Shu Zhang Jinbo Pang Yufen Li Feng Yang Thomas Gemming Kai Wang Xiao Wang Songang Peng Xiaoyan Liu Bin Chang Hong Liu weijia zhou Gianaurelio Cuniberti Mark HRümmeli Collaborative Innovation Center of Technology and Equipment for Biological Diagnosis and Therapy in Universities of Shandong Institute for Advanced Interdisciplinary Research(iAIR)University of JinanJinan 250022China Department of Chemistry Guangdong Provincial Key Laboratory of CatalysisSouthern University of Science and TechnologyShenzhen 518055China Leibniz Institute for Solid State and Materials Research Dresden P.O.Box 270116Dresden D-01171Germany State Key Laboratory of Crystal Materials Center of Bio&Micro/Nano Functional MaterialsShandong University27 Shandanan RoadJinan 250100China School of Electrical Engineering Qingdao UniversityQingdao 266071China Shenzhen Institutes of Advanced Technology Chinese Academy of Sciences 1068 Xueyuan AvenueShenzhen University TownShenzhen 518055China High-Frequency High-Voltage Device and Integrated Circuits R&D Center Institute of MicroelectronicsChinese Academy of SciencesBeijing 100029China Key Laboratory of Microelectronic Devices&Integrated Technology Institute of MicroelectronicsChinese Academy of SciencesBeijing 100029China School of Chemistry and Chemical Engineering University of JinanJinan 250022China College of Energy Soochow Institute for Energy and Materials InnovationsSoochow UniversitySuzhou 215006China Key Laboratory of Advanced Carbon Materials and Wearable Energy Technologies of Jiangsu Province Soochow UniversitySuzhou 215006China Centre of Polymer and Carbon Materials Polish Academy of SciencesM.Curie Sklodowskiej 34Zabrze 41-819Poland Institute of Environmental Technology(CEET) VSB-Technical University of Ostrava17.Listopadu 15Ostrava 70833Czech Republic Dresden Center for Computational Materials Science Technische Universität DresdenDresden 01062Germany Dresden Center for Intelligent Materials(GCL DCIM) Technische Universität DresdenDresden 01062Germany Institute for Materials Science and Max Bergmann Center of Biomaterials Technische Universität DresdenDresden 01069Germany Center for Advancing Electronics D

Carbon nanotubes(CNTs)have attracted great attentions in the field of electronics,sensors,healthcare,and energy *** emerging applications have driven the carbon nanotube research in a rapid ***,the structure control over CNTs has inspired an intensive research vortex due to the high promises in electronic and optical device ***,this in-depth review is anticipated to provide insights into the controllable synthesis and applications of high-quality ***,the general synthesis and post-purification of CNTs are briefly ***,the state-of-the-art electronic device applications are discussed,including field-effect transistors,gas sensors,DNA biosensors,and pressure ***,the optical sensors are delivered based on the *** addition,energy applications of CNTs are discussed such as thermoelectric energy ***,future opportunities are proposed for the Internet of Things(IoT)oriented sensors,data processing,and artificial intelligence.

关键词： carbon nanotubes electronics sensors electronic skins Internet of Things artificial intelligence

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Applications of 2D-Layered Palladium Diselenide and Its van der Waals Heterostructures in Electronics and Optoelectronics

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Nano-Micro Letters 2021年第9期13卷 292-343页

作者： Yanhao Wang Jinbo Pang Qilin Cheng Lin Han Yufen Li Xue Meng Bergoi Ibarlucea Hongbin Zhao Feng Yang Haiyun Liu Hong Liu weijia zhou Xiao Wang Mark HRummeli Yu Zhang Gianaurelio Cuniberti Institute of Marine Science and Technology Shandong UniversityQingdao 266237People’s Republic of China College of Energy Soochow Institute for Energy and Materials Innovations Soochow UniversitySuzhou 215006People’s Republic of China Key Laboratory of Advanced Carbon Materials and Wearable Energy Technologies of Jiangsu Province Soochow UniversitySuzhou 215006People’s Republic of China Centre of Polymer and Carbon Materials Polish Academy of SciencesM.Curie Sklodowskiej 3441-819 ZabrzePoland Institute for Complex Materials IFW Dresden 20 Helmholtz Strasse01069 DresdenGermany Institute of Environmental Technology VŠB-Technical University of Ostrava 17.listopadu 15Ostrava 70833Czech Republic Collaborative Innovation Center of Technology and Equipment for Biological Diagnosis and Therapy in Universities of Shandong Institute for Advanced Interdisciplinary Research(iAIR)University of JinanShandongJinan 250022People’s Republic of China State Key Laboratory of Crystal Materials Center of Bio and Micro/Nano Functional MaterialsShandong University27 Shandanan RoadJinan 250100People’s Republic of China Department of Chemistry Guangdong Provincial Key Laboratory of Catalytic ChemistrySouthern University of Science and TechnologyShenzhenGuangdong 518055People’s Republic of China State Key Laboratory of Advanced Materials for Smart Sensing GRINM Group Co.Ltd.Xinwai Street 2Beijing 100088People’s Republic of China Shenzhen Institutes of Shenzhen Institutes of Advanced Technology Chinese Academy of Sciences1068 Xueyuan AvenueShenzhen University TownShenzhen 518055People’s Republic of China Institute for Materials Science and Max Bergmann Center of Biomaterials Technische Universität Dresden01069 DresdenGermany Center for Advancing Electronics Dresden Technische Universität Dresden01069 DresdenGermany Dresden Center for Computational Materials Science Technische Universität Dresden01062 DresdenGermany Dresden Center for Intelligent Materials(GCL DCIM) Technische Universität Dresden01062 Dr

The rapid development of two-dimensional(2D)transition-metal dichalcogenides has been possible owing to their special structures and remarkable *** particular,palladium diselenide(PdSe_(2))with a novel pentagonal structure and unique physical characteristics have recently attracted extensive research ***,tremendous research progress has been achieved regarding the physics,chemistry,and electronics of PdSe_(2).Accordingly,in this review,we recapitulate and summarize the most recent research on PdSe_(2),including its structure,properties,synthesis,and ***,a mechanical exfoliation method to obtain PdSe_(2) nanosheets is introduced,and large-area synthesis strate-gies are explained with respect to chemical vapor deposition and metal ***,the electronic and optoelectronic properties of PdSe_(2) and related hetero-structures,such as field-effect transistors,photodetectors,sensors,and thermoelec-tric devices,are ***,the integration of systems into infrared image sensors on the basis of PdSe_(2) van der Waals heterostructures is ***,future opportunities are highlighted to serve as a general guide for physicists,chemists,materials scientists,and ***,this com-prehensive review may shed light on the research conducted by the 2D material community.

关键词： Palladium diselenide nTMDC Synthesis Field-effect transistors Photodetectors Sensors

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