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Polysulfide regulation by defect-modulated Ta_(3)N_(5-x) electrocatalyst toward superior room-temperature sodium-sulfur batteries

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Science Bulletin 2024年第2期69卷 197-208页

作者： Zhen Zhang Dan Luo Jun Chen Chuyin Ma Matthew Li Haoze Zhang Renfei Feng Rui Gao Haozhen Dou Aiping yu Xin Wang Zhongwei Chen Department of Chemical Engineering Waterloo Institute for NanotechnologyUniversity of WaterlooWaterloo N2L 3G1Canada Dalian Institute of Chemical Physics Chinese Academy of SciencesDalian 116023China South China Academy of Advanced Optoelectronics&International Academy of Optoelectronics at Zhaoqing South China Normal UniversityGuangzhou 510006China Chemical Sciences and Engineering Division Argonne National LaboratoryLemont 60439USA Canadian Light Source Saskatoon S7N 2V3Canada

Resolving low sulfur reaction activity and severe polysulfide dissolution remains challenging in metalsulfur *** by a theoretical prediction,herein,we strategically propose nitrogenvacancy tantalum nitride(Ta3N5-x)impregnated inside the interconnected nanopores of nitrogendecorated carbon matrix as a new electrocatalyst for regulating sulfur redox reactions in roomtemperature sodium-sulfur *** a pore-constriction mechanism,the nitrogen vacancies are controllably constructed during the nucleation of *** defect manipulation on the local environment enables well-regulated Ta 5d-orbital energy level,not only modulating band structure toward enhanced intrinsic conductivity of Ta-based materials,but also promoting polysulfide stabilization and achieving bifunctional catalytic capability toward completely reversible polysulfide ***,the interconnected continuous Ta3N5-x-in-pore structure facilitates electron and sodium-ion transport and accommodates volume expansion of sulfur species while suppressing their shuttle *** to these attributes,the as-developed Ta3N5-x-based electrode achieves superior rate capability of 730 mAh g-1 at 3.35 A g-1,long-term cycling stability over 2000 cycles,and high areal capacity over 6 mAh cm-2 under high sulfur loading of 6.2 mg *** work not only presents a new sulfur electrocatalyst candidate for metal-sulfur batteries,but also sheds light on the controllable material design of defect structure in hopes of inspiring new ideas and directions for future research.

关键词： Tantalum nitride Nitrogen defects Sodium-sulfur batteries Electrocatalysts Polysulfide conversion

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The MYC2-PUB22-JAZ4 module plays a crucial role in jasmonate signaling in tomato

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Molecular Plant 2024年第4期17卷 598-613页

作者： Shaofang Wu Chaoyi Hu Changan Zhu Yanfen Fan Jie Zhou Xiaojia Xia Kai Shi Yanhong Zhou Christine H.Foyer Jingquan yu Department of Horticulture Zijingang CampusZhejiang UniversityHangzhou 310058China Hainan Institute Zhejiang UniversityYazhou Bay Science and Technology CitySanya 572025China College of Horticulture Northwest Agriculture&Forestry UniversityXianyang 712100China School of Biosciences College of Life and Environmental SciencesUniversity of BirminghamEdgbaston B152TTUK Key Laboratory of Horticultural Plants Growth and Development Agricultural Ministry of ChinaZhejiang UniversityHangzhou 310058China

Jasmonates(JAs),a class of lipid-derived stress hormones,play a crucial role across an array of plant physiological processes and stress *** JA signaling is thought to rely predominantly on the degradation of specific JAZ proteins by SCF^(COI1),it remains unclear whether other pathways are involved in the regulation of JAZ protein ***,we report that PUB22,a plant U-box type E3 ubiquitin ligase,plays a critical role in the regulation of plant resistance against Helicoverpa armigera and other JA responses in *** COI1 physically interacts with JAZ1/2/5/7,PUB22 physically interacts with JAZ1/3/4/***22 ubiquitinates JAZ4 to promote its degradation via the 26S proteasome ***,we observed that pub22 mutants showreduced resistance to ***,whereas jaz4 single mutants and jaz1 jaz3 jaz4 jaz6 quadruple mutants have enhanced *** hypersensitivity of pub22 mutants to herbivores could be partially rescued by JAZ4 ***,we found that expression of PUB22 can be transcriptionally activated by MYC2,thus forming a positive feedback circuit in JA *** noticed that the PUB22-JAZ4 module also regulates other JA responses,including defense against ***,inhibition of root elongation,and anthocyanin *** together,these results indicate that PUB22 plays a crucial role in plant growth and defense responses,together with COI1-regulated JA signaling,by targeting specific JAZs.

关键词： PUB22 JAZ COI1 MYC2 JA signaling Solanum lycopersicum

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地铁杂散电流引起变压器直流偏磁抑制方法

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电网技术 2024年第4期48卷 1700-1710,I0085页

作者：程新翔喻锟曾祥君倪砚茹唐雨杭韩炜智能电网运行与控制湖南省重点实验室(长沙理工大学) 湖南省长沙市410114 国网山西省太原供电公司山西省太原市030000

针对城市地铁运行时泄漏的杂散电流会引起沿线变压器直流偏磁问题,提出一种基于碳化硅PiN二极管的偏磁抑制方法。首先,建立杂散电流分布模型并采集现场地电位实测数据,明晰了地铁运行下城区整体大地电位的数值分布特点。然后利用碳化硅... 详细信息

针对城市地铁运行时泄漏的杂散电流会引起沿线变压器直流偏磁问题,提出一种基于碳化硅PiN二极管的偏磁抑制方法。首先,建立杂散电流分布模型并采集现场地电位实测数据,明晰了地铁运行下城区整体大地电位的数值分布特点。然后利用碳化硅PiN二极管在直流电压和故障电流下的电压阻断能力及电流导通特性,提出了基于碳化硅PiN二极管的变压器直流偏磁抑制电路结构与工作流程。最后基于PSCAD/EMTDC仿真平台搭建了城市电网110kV变电站主变直流偏磁仿真模型,验证了偏磁抑制方法故障电流导通能力和偏磁直流抑制效果。仿真结果表明:电网故障时,偏磁抑制方法瞬时导通,继电保护迅速动作跳闸;变压器实施偏磁抑制后,中性点直流电流被阻隔,磁滞回线、一次侧绕组电流及励磁电流畸变率降低,直流偏磁得到有效抑制。

关键词：杂散电流地表电位变压器直流偏磁碳化硅二极管偏磁抑制

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中空多壳层结构TiN修饰隔膜对锂硫电池性能的增强

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科学通报 2024年第16期69卷 2298-2307页

作者：徐伟毕如一杨梅王江艳于然波王丹中国科学院过程工程研究所生化工程国家重点实验室北京100190 北京科技大学冶金与生态工程学院北京100083 中国科学院大学化学工程学院北京100049 生物药制备与递送重点实验室(中国科学院) 北京100190

锂硫电池(lithium-sulfur(Li-S)batteries)具有远高于锂离子电池的理论比容量.然而,硫的导电性差,充放电过程中体积变化剧烈,其放电中间产物易溶于电解液并穿过隔膜,造成穿梭效应,导致锂硫电池的实测比容量低、循环寿命短.本文设计构筑... 详细信息

锂硫电池(lithium-sulfur(Li-S)batteries)具有远高于锂离子电池的理论比容量.然而,硫的导电性差,充放电过程中体积变化剧烈,其放电中间产物易溶于电解液并穿过隔膜,造成穿梭效应,导致锂硫电池的实测比容量低、循环寿命短.本文设计构筑了中空多壳层结构氮化钛(TiNHoMS),作为锂硫电池隔膜修饰材料,有效解决了上述难题.氮化钛具有优异的导电性,能够催化硫和多硫化锂的氧化还原转化.HoMS具有多个壳层和多层内部空腔,能提供多重空间阻隔和丰富的多硫化锂吸附位点,从而有效抑制穿梭效应,并且能够缩短电子/离子传输路径.得益于此,采用三壳层TiNHoMS修饰隔膜的锂硫电池性能显著提高,远优于采用未修饰隔膜电池的性能.测试结果表明,在1 C电流下,初始比容量由642 mAh/g提高到1134 mAh/g,而且300次循环后比容量仍保持在792 mAh/g.通过一系列电化学表征分析发现,TiNHoMS提高了隔膜对电解液的浸润性,催化了硫正极的氧化还原反应,抑制了多硫化锂的穿梭效应,从而有效地提高了锂硫电池的比容量和循环稳定性.

关键词：中空多壳层结构氮化钛隔膜修饰锂硫电池穿梭效应

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Eco-friendly calcium alginate microspheres enable enhanced profile control and oil displacement

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Petroleum Science 2024年第3期21卷 1928-1943页

作者： Xiao-Han Zhang Chang-Jing Zhou yuan-Xiang Xiao Bo Hui Yong-Gang Xie yu-Bin Su Xin-Ru Li Jie Huang Mao-Chang Liu International Research Center for Renewable Energy State Key Laboratory of Multiphase Flow in Power EngineeringXi'an Jiaotong UniversityXi'an710049ShaanxiPR.China Shaanxi Key Laboratory of Advanced Stimulation Technology for Oil&Gas Reservoirs School of Petroleum EngineeringXi'an Shiyou UniversityXi'an 710065ShaanxiPR.China Oil&Gas Technology Research Institute Changqing Oilfield Branch CompanyPetroChinaXi'an710021ShaanxiPR China Suzhou Academy of Xi'an Jiaotong University Suzhou215123JiangsuPR China

Polymer microspheres(PMs),such as polyacrylamide,have been widely applied for enhanced oil recovery(EOR),yet with environmental ***,we report a microfluid displacement technology containing a bio-based eco-friendly material,i.e.,calcium alginate(CaAlg)microspheres for *** dominant mechanisms responsible for EOR over Ca Alg fluid have been verified,including the microscopic oil displacement efficacy augmented by regulating capillary force(determined by the joint action of interfacial tension and wettability between different phases)and macroscopic sweep volume increment through profile control and mobility ratio *** comprehensive effectiveness can be further impacted when the CaAlg microsphere is embellished ulteriorly by using appropriate amount of sodium dodecyl sulfonate(SDS).The core flooding and nuclear magnetic resonance(NMR)tests demonstrate that CaAlg-SDS microsphere can balance the interphase property regulation(wettability alteration and IFT reduction)and rheology properties,enabling simultaneous profile control and oil *** introduction of SDS will have a negative impact on rheological properties,which is not favored for *** results show that the involvement of 4-m M SDS will provide the best behavior,with an EOR rate of 34.38%.This cost-effective and environmentally-friendly bio-microspherebased microfluidic displacement technology is expected to achieve“green”oil recovery in future oilfield exploitation.

关键词： Calcium alginate microspheres Wettability Interfacial tension Rheology Viscoelasticity Enhanced oil recovery(EOR)

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Network pharmacology-based exploration of molecular mechanisms underlying therapeutic effects of Jianpi Huatan Quyu recipe on chronic heart failure with spleen Qi deficiency syndrome

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World Journal of Cardiology 2024年第7期16卷 422-435页

作者： Si-Qi Li Dong-yu Min Jun-Wen Jiang Xiao-Ying Li Xu-Na Yang Wen-Bo Gu Jia-Hui Jiang Li-Hao Chen Han Nan Ze-yu Chen Second Department of Cardiology The Affiliated Hospital of Liaoning University of Traditional Chinese MedicineShenyang 110000Liaoning ProvinceChina

BACKGROUND Chronic heart failure is a complex clinical *** Chinese herbal compound preparation Jianpi Huatan Quyu recipe has been used to treat chronic heart failure;however,the underlying molecular mechanism is still not *** To identify the effective active ingredients of Jianpi Huatan Quyu recipe and explore its molecular mechanism in the treatment of chronic heart *** The effective active ingredients of eight herbs composing Jianpi Huatan Quyu recipe were identified using the Traditional Chinese Medicine Systems Pharmacology Database and Analysis *** target genes of chronic heart failure were searched in the Genecards *** target proteins of active ingredients were mapped to chronic heart failure target genes to obtain the common drugdisease targets,which were then used to construct a key chemical componenttarget network using Cytoscape 3.7.2 *** protein-protein interaction network was constructed using the String *** Ontology and Kyoto Encyclopedia of Genes and Genomes enrichment analyses were performed through the Metascape ***,our previously published relevant articles were searched to verify the results obtained via network *** A total of 227 effective active ingredients for Jianpi Huatan Quyu recipe were identified,of which quercetin,kaempferol,7-methoxy-2-methyl isoflavone,formononetin,and isorhamnetin may be key active ingredients and involved in the therapeutic effects of TCM by acting on STAT3,MAPK3,AKT1,JUN,MAPK1,TP53,TNF,HSP90AA1,p65,MAPK8,MAPK14,IL6,EGFR,EDN1,FOS,and other *** pathways identified by KEGG enrichment analysis include pathways in cancer,IL-17 signaling pathway,PI3K-Akt signaling pathway,HIF-1 signaling pathway,calcium signaling pathway,cAMP signaling pathway,NF-kappaB signaling pathway,AMPK signaling pathway,*** studies on Jianpi Huatan Quyu recipe suggested that this Chinese compound preparation can regulate the TNF-α,IL-6,MAPK

关键词： Jianpi Huatan Quyu recipe Traditional Chinese medicine Chronic heart failure Data mining Network pharmacology Bioinformatics Spleen Qi deficiency syndrome

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Enhanced visible-light photocatalytic hydrogen evolution using two-dimensional carbon nitride sheets with the removal of amine groups

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Chinese Chemical Letters 2024年第2期35卷 446-450页

作者： yu Zhang Liting Wu Shaopeng Wang Dingyi Yang Huan Liang Yizhang Wu Jian Hao Youqing Wang Jianke Liu Yong Wang Department of Physics Shaanxi University of Science and TechnologyXi'an 710021China School of Advanced Materials and Nanotechnology Academy of Advanced Interdisciplinary ResearchXidian UniversityXi'an 710126China The State Key Discipline Laboratory of Wide Band Gap Semiconductor Technology Xidian UniversityXi'an 710126China Collaborative Innovation Center of Advanced Microstructures National Laboratory of Solid State MicrostructuresNanjing UniversityNanjing 210093China State Key Laboratory of High-Efficiency Utilization of Coal and Green Chemical Engineering Ningxia UniversityYinchuan 750021China

Two-dimensional(2D)carbon nitride sheets(CNs)with atomically thin structures are regarded as one of the most promising materials for solar energy ***,due to their substantially enlarged bandgap caused by the strong quantum size effect and their incomplete polymerisation with a large number of non-condensed surface amino groups,the practical applicability of CNs in photocatalysis is *** this study,CNs with broad visible-light absorption were synthesised using a 5-min fast thermal *** removal of uncondensed amine groups reduces the bandgap of CNs from 3.06 eV to 2.60 eV,increasing their absorption of visible ***,the CNs were distorted after annealing,which can differentiate the spatial positions of electrons and holes,enhancing the visible-light absorption *** a result,when exposed to visible light,the photocatalytic hydrogen production activity of atomically thin 2D CNs rose by 8.38 *** research presents a dependable and speedy method for creating highly effective visible-light photocatalysts with narrowed bandgaps and improved visible-light absorption.

关键词： 2D carbon nitride sheets Rapid thermal annealing DFT calculations Visible-light absorption visible-light photocatalysis

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玉米穗腐病的抗性鉴定与抗性基因定位研究进展

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黑龙江农业科学 2024年第7期 97-107页

作者：侯萌王巍赵韦陈钰黑龙江省农业科学院玉米研究所黑龙江哈尔滨150086

玉米是我国第一大粮食作物,其生长过程中易受多种病害影响,其中穗腐病是常见病害之一,会造成玉米产量损失和品质下降。该病害致病菌种类繁多、致病机理复杂。从经济、安全、有效的角度,抗病育种无疑是最佳选择。因此,围绕玉米种质资源... 详细信息

玉米是我国第一大粮食作物,其生长过程中易受多种病害影响,其中穗腐病是常见病害之一,会造成玉米产量损失和品质下降。该病害致病菌种类繁多、致病机理复杂。从经济、安全、有效的角度,抗病育种无疑是最佳选择。因此,围绕玉米种质资源对穗腐病的鉴定评价和抗病位点发掘进行总结,对加快抗病育种具有一定的促进作用。本文从玉米穗腐病的危害和防治、国内外穗腐病优势致病菌、我国各区域优势致病菌、国内外已鉴定的抗穗腐病资源,以及通过连锁分析和全基因组关联分析方法定位出的抗病位点进行了综述,并对玉米穗腐病的抗性育种进行展望,为今后开展玉米穗腐病相关研究提供参考。

关键词：玉米穗腐病抗性鉴定抗性定位

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Nanoindentation behavior and creep-induced cracking of long-term crept austenitic steel at 650℃

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Journal of Iron and Steel Research International 2024年第2期31卷 464-474页

作者： Zhen Zhang yu-hang Duan Shuai Wang Jin-shan Chen An-zhe Wang Xiang-yang Mao yuan-ji Shi Jie Zhang Ming Liu Zheng-fei Hu School of Materials Science and Engineering Nanjing Institute of TechnologyNanjing211167JiangsuChina Jiangsu Key Laboratory of Advanced Structural Materials and Application Technology Nanjing211167JiangsuChina Jiangsu Wind Power Engineering Technology Center Nanjing210023JiangsuChina Nanjing Vocational University of Industry Technology Nanjing210023JiangsuChina Baoshan Iron&Steel Co. Ltd.Shanghai201900China Fujian Provincial Key Laboratory of Terahertz Functional Devices and Intelligent Sensing School of Mechanical Engineering and AutomationFuzhou UniversityFuzhou350116FujianChina School of Materials Science and Engineering Tongji UniversityShanghai201804China

The grain boundary(GB)damage of long-term crept HR3C(25Cr–20Ni–Nb–N)austenitic steel with solid solution state was investigated by nanoindentation test accompanied with in-situ electron back-scattered *** corresponding microstructure was characterized by scanning electron microscopy and transmission electron *** show that the increase in nanoindentation hardness at the GBs and triple grain junctions may be related to the dislocation accumulation and carbide growth during the *** M23C6 and dislocations piling-up at the GB accelerate the nucleation and coalescence of creep cavity along the *** nanoindentation hardness in grains varies with orientation of the stress *** orientation difference of neighbor grains may induce local high geometrically necessary dislocation densities and strain gradients near the GB,consequently causing stress concentration and subsequent crack growth at specific GBs.

关键词： Austenitic steel Creep Nanoindentation Grain orientation Creep-induced cracking

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Wheel-legged In-pipe Robot with a Bioinspired Hook and Dry Adhesive Attachment Device

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Journal of Bionic Engineering 2024年第3期21卷 1208-1222页

作者： Yahong Liu Yi Sun Kai Cao Shutao Wu Xiaofeng Xu Qingfei Han Shikun Wen Huan Shen Guangming Chen Jiajun Xu Zhiwei yu Aihong Ji Lab of Locomotion Bioinspiration and Intelligent Robots College of Mechanical and Electrical EngineeringNanjing University of Aeronautics and AstronauticsNanjing 210016China State Key Laboratory of Mechanics and Control for Aerospace Structures Nanjing University of Aeronautics and AstronauticsNanjing 210016China

In-pipe robots have been widely used in pipes-with smooth inner ***,current in-pipe robots face challenges in terms of moving past obstacles and climbing in marine-vessel pipeline systems,which are affected by marine biofouling and electrochemical *** paper takes inspiration from the dual-hook structure of Trypoxylus dichotomus’s feet and gecko‑like dry adhesives,proposing an in-pipe robot that is capable of climbing on rough and smooth pipe *** combination of the bioinspired hook and dry adhesives allows the robot to stably attach to rough or smooth pipe inwalls,while the wheel-leg hybrid mechanism provides better conditions for obstacle *** paper explores the attachment and obstacle-surmounting mechanisms of the ***,motion strategies for the robot are devised based on different pipe structural *** experiments showed that this robot can adapt to both smooth and rough pipe environments simultaneously,and its motion performance is superior to conventional driving *** robot’s active turning actuators also enable it to navigate through horizontally or vertically oriented 90°bends.

关键词： In-pipe robot Bioinspired attachment device Wheel-legged robot Mechanical design

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