检索结果-南通市图书馆

From waste to wealth:Coal tar residue derived carbon materials as low-cost anodes for potassium-ion batteries

在线全文

学校读者我要写书评

暂无评论

International Journal of Minerals,Metallurgy and Materials 2025年第2期32卷 464-475页

作者： Zhonghua Lu Jun Shen Xin Zhang Lingcong Chao Liang Chen Ding Zhang tao wei Shoudong xu College of Chemical Engineering and Technology Taiyuan University of TechnologyTaiyuan 030024China College of Chemistry Taiyuan University of TechnologyTaiyuan 030024China School of Chemical Engineering and Pharmacy Wuhan Institute of TechnologyWuhan 430205China School of Energy and Power Jiangsu University of Science and TechnologyZhenjiang 212003China

Carbon materials are widely recognized as highly promising electrode materials for various energy storage system *** tar residues(CTR),as a type of carbon-rich solid waste with high value-added utilization,are crucially important for the development of a more sustainable *** this study,we employed a straightforward direct carbonization method within the temperature range of 700-1000℃to convert the worthless solid waste CTR into economically valuable carbon materials as anodes for potassium-ion batteries(PIBs).The effect of carbonization temperature on the microstructure and the potassium ions storage properties of CTR-derived carbons(CTRCs)were systematically explored by structural and morphological characterization,alongside electrochemical performances *** on the co-regulation between the turbine layers,crystal structure,pore structure,functional groups,and electrical conductivity of CTR-derived carbon carbonized at 900℃(CTRC-900H),the electrode material with high reversible capacity of 265.6m Ah·g^(-1)at 50 m A·g^(-1),a desirable cycling stability with 93.8%capacity retention even after 100 cycles,and the remarkable rate performance for PIBs were ***,cyclic voltammetry(CV)at different scan rates and galvanostatic intermittent titration technique(GITT)have been employed to explore the potassium ions storage mechanism and electrochemical kinetics of *** indicate that the electrode behavior is predominantly governed by surface-induced capacitive processes,particularly under high current densities,with the potassium storage mechanism characterized by an“adsorption-weak intercalation”*** work highlights the potential of CTR-based carbon as a promising electrode material category suitable for high-performance PIBs electrodes,while also provides valuable insights into the new avenues for the high value-added utilization of CTR.

关键词： coal tar residue carbon materials anode potassium-ion batteries high value-added

Construction and application of multicomponent fluorescent droplets

在线全文

学校读者我要写书评

暂无评论

Chinese Chemical Letters 2025年第1期36卷 137-146页

作者： wei-tao Dou Qing-Wen Zeng Yan Kang Haidong Jia Yulian Niu Jinglong Wang Lin xu Shanghai Key Laboratory of Green Chemistry and Chemical Processes Shanghai Frontiers Science Center of Molecule Intelligent SynthesesSchool of Chemistry and Molecular EngineeringEast China Normal UniversityShanghai 200062China Shanghai Jahwa United Co. Ltd.Shanghai 200082China Chongqing Key Laboratory of Precision Optics Chongqing Institute of East China Normal UniversityChongqing 401120China

The rapid development of microfluidic technology has led to the evolution of microdroplets from simple emulsion structures to complex multilayered and multicompartmental *** advancements have endowed microdroplets with the capability to contain multiple compartments that remain isolated from one another,enabling them to carry different molecules of ***,researchers can now investigate intricate spatially confined chemical reactions and signal transduction pathways within subcellular ***,modern microdroplets often possess excellent optical transparency,allowing fluorescently labelled,multi-layered,and compartmental droplets to provide detailed insights through real-time,in situ,and dynamic fluorescence ***,this review systematically summarizes current methodologies for preparing multicomponent microdroplets and their applications,particularly focusing on fluorescent ***,it discusses existing critical challenges and outlines future research *** offering a comprehensive overview of the preparation methods and applications of fluorescent microdroplets,this review aims to stimulate the interest of researchers and foster their utilization in more complex and biomimetic environments.

关键词： Fluorescent Microfluidic Fluorescent droplets Multilayered droplets Multicompartmental droplets

A C-type lectin with dual carbohydrate recognition domains functions in innate immune response in Asian corn borer, Ostrinia furnacalis

在线全文

学校读者我要写书评

暂无评论

INSECT SCIENCE 2025年第1期32卷 172-192页

作者： Li, Er-tao Ji, Jia-Yue Kong, wei-Jie Shen, Dong-xu Li, Cai An, Chun-Ju China Agr Univ Coll Plant Protect Dept Entomol Beijing 100193 Peoples R China Shanxi Agr Univ Pomol Inst Jinzhong Shanxi Peoples R China Jiangsu Univ Sci & Technol Sch Biotechnol Jiangsu Key Lab Sericultural Biol & Biotechnol Zhenjiang Jiangsu Peoples R China

C-type lectins (CTLs) act as pattern recognition receptors (PRRs) to initiate the innate immune response in insects. A CTL with dual carbohydrate recognition domains (CRDs) (named immulectin-4 [IML-4]) was selected from the Ostrinia furnacalis transcriptome dataset for functional studies. We cloned the full-length complementary DNA of O. furnacalis IML-4 (OfIML-4). It encodes a 328-residue protein with a Glu-Pro-Asn (EPN) and Gln-Pro-Asp (QPD) motifs in 2 CRDs, respectively. OfIML-4 messenger RNA levels increased significantly upon the bacterial and fungal infection. Recombinant OfIML-4 (rIML-4) and its individual CRDs (rCRD1 and rCRD2) exhibited the binding ability to various microorganisms including Escherichia coli, Micrococcus luteus, Pichia pastoris, and Beauveria bassiana, and the cell wall components including lipopolysaccharide from E. coli, peptidoglycan from M. luteus or Bacillus subtilis, and curdlan from Alcaligenes faecalis. The binding further induced the agglutination of E. coli, M. luteus, and B. bassiana in the presence of calcium, the phagocytosis of Staphylococcus aureus by the hemocytes, in vitro encapsulation and melanization of nickel-nitrilotriacetic acid beads, and a significant increase in phenoloxidase activity of plasma. In addition, rIML-4 significantly enhanced the phagocytosis, nodulation, and resistance of O. furnacalis to B. bassiana. Taken together, our results suggest that OfIML-4 potentially works as a PRR to recognize the invading microorganisms, and functions in the innate immune response in O. furnacalis.

关键词： cellular immunity C-type lectin humoral immunity immulectin Ostrinia furnacalis pattern recognition receptor (PRR)

A polynomial resultant approach to algebraic constructions of extremal graphs

在线全文

维普期刊数据库

学校读者我要写书评

暂无评论

Science China Mathematics 2025年第2期68卷 485-506页

作者： tao Zhang Zixiang xu Gennian Ge Institute of Mathematics and Interdisciplinary Sciences Xidian UniversityXi’an 710071China School of Mathematical Sciences Capital Normal UniversityBeijing 100048China

The Turán problem asks for the largest number of edges ex(n,H)in an n-vertex graph not containing a fixed forbidden subgraph H,which is one of the most important problems in extremal graph ***,the order of magnitude of ex(n,H)for bipartite graphs is known only in a handful of *** particular,giving explicit constructions of extremal graphs is very challenging in this *** this paper,we develop a polynomial resultant approach to the algebraic construction of explicit extremal graphs,which can efficiently decide whether a specified structure exists.A key insight in our approach is the multipolynomial resultant,which is a fundamental tool of computational algebraic *** main results include the matched lower bounds on the Turán number of 1-subdivision of K3,t1and the linear Turán number of the Berge theta hypergraph■_(3,t_(2))^(B).where t_(1)=25 and t_(2)=***,the constant t1improves the random algebraic construction of Bukh and Conlon(2018)and makes the known estimation better on the smallest value of t1concerning a problem posed by Conlon et al.(2021)by reducing the value from a magnitude of 10^(56)to the number 25,while the constant t_(2)improves a result of He and Tait(2019).

关键词： Turan number resultant algebraic construction subdivision Berge theta hypergraph

Analysis of vibration response characteristics of subway station and superstructure with hard combination

在线全文

维普期刊数据库

学校读者我要写书评

暂无评论

Earthquake Engineering and Engineering Vibration 2025年第1期24卷 271-281页

作者： Jia Jinglong xu weiping Liu xu wei Yong Key Laboratory of Transportation Tunnel Engineering Ministry of EducationSchool of Civil EngineeringSouthwest Jiaotong UniversityChengdu 610031China State Key Laboratory of Intelligent Geotechnics and Tunnelling Chengdu 610031China China Railway Eryuan Chongqing Survey and Design Institute Co.Ltd. Chongqing 400023China

The vibration response and noise caused by subway trains can affect the safety and comfort of *** study the dynamic response characteristics of subway stations and superstructures under train loads with a hard combination,a numerical model is developed in this *** indoor model test verified the accuracy of the numerical *** influence laws of different hard combinations,train operating speeds and modes were studied and evaluated *** results show that the frequency corresponding to the peak vibration acceleration level of each floor of the superstructure property is concentrated at 10–20 *** vibration response decreases in the high-frequency parts and increases in the lowfrequency parts with increasing distance from the ***,the factors,such as train operating speed,operating mode,and hard combination type,will affect the vibration of the *** vibration response under the reversible operation of the train is greater than that of the unidirectional *** operating speed of the train is proportional to its vibration *** vibration amplification area appears between the middle and the top of the superstructure at a higher train *** vibration acceleration level will exceed the limit value of relevant regulations,and vibration-damping measures are *** the scope of application,this study provides some suggestions for constructing subway stations and superstructures.

关键词： subway station superstructure vibration response hard combination

Adsorption removal of mercury from flue gas by metal selenide:A review

在线全文

学校读者我要写书评

暂无评论

Journal of Environmental Sciences 2025年第2期148卷 420-436页

作者： Yang Zheng Guoliang Li Yi Xing Wenqing xu tao Yue School of Energy and Environmental Engineering University of Science and Technology BeijingBeijing 100083China State Key Laboratory of Advanced Metallurgy University of Science and Technology BeijingBeijing 100083China CAS Key Laboratory of Green Process and Engineering Institute of Process EngineeringInnovation Academy for Green ManufactureChinese Academy of SciencesBeijing 100190China

Mercury(Hg)pollution has been a global concern in recent decades,posing a significant threat to entire ecosystems and human health due to its cumulative toxicity,persistence,and transport in the *** intense interaction between mercury and selenium has opened up a new field for studying mercury removal from industrial flue gas *** the advantages of good Hg0 capture performance and lowsecondary pollution of the mineral selenium compounds,the most noteworthy is the relatively low regeneration temperature,allowing adsorbent regeneration with low energy consumption,thus reducing the utilization cost and enabling recovery of mercury *** paper reviews the recent progress of mineral selenium compounds in flue gas mercury removal,introduces in detail the different types ofmineral selenium compounds studied in the field ofmercury removal,reviews the adsorption performance of various mineral selenium compounds adsorbents on mercury and the influence of flue gas components,such as reaction temperature,air velocity,and other factors,and summarizes the adsorption mechanism of different fugitive forms of selenium *** on the current research progress,future studies should focus on the economic performance and the performance of different carriers and sizes of adsorbents for the removal of Hg0 and the correlation between the gas-particle flow characteristics and gas phase mass transfer with the performance of Hg0 removal in practical industrial *** addition,it remains a challenge to distinguish the oxidation and adsorption of Hg0 quantitatively.

关键词： Non-conventional pollutants Adsorbents Metal selenides Flue gas Mercury removal

Observer-based event-triggered formation tracking control for second-order multi-agent systems in constrained region

在线全文

维普期刊数据库

学校读者我要写书评

暂无评论

Science China(Information Sciences) 2025年第2期68卷 151-169页

作者： Fenglan SUN Zhonghua xu wei ZHU ■ KURTHS Key Lab of Intelligent Analysis and Decision on Complex Systems School of ScienceChongqing University of Posts and Telecommunications Key Lab of Intelligent Air-Ground Cooperative Control for Universities in Chongqing College of AutomationChongqing University of Posts and Telecommunications Department of Complexity Science Potsdam Institute for Climate Impact Research Institute of Physics Humboldt University of Berlin

In this paper, an event-triggered time-varying formation tracking control for a class of second-order nonlinear multiagent systems(MAS) operating within a constrained region is investigated. To mitigate the negative effects of external unknown disturbance, a novel disturbance observer with performance guarantees is proposed, enabling precise disturbance *** the artificial potential field(APF) method, a repulsive potential function is introduced to prevent inter-agent collisions as well as collisions with environmental obstacles. To reduce continuous communication and frequent system updates, a sliding mode technique is incorporated into the formation tracking controller, utilizing an event-triggered mechanism. The controller is also applicable to the formation control of MAS in switching-constrained regions. The achievement of the specified timevarying geometric formation is rigorously demonstrated through the Lyapunov framework. Numerical simulations are presented to validate the effectiveness of the theoretical results.

关键词： formation tracking control region constraints repulsive potential function event-triggered mechanism

Decentralized Federated Learning Algorithm Under Adversary Eavesdropping

在线全文

同方期刊数据库

学校读者我要写书评

暂无评论

IEEE/CAA Journal of Automatica Sinica 2025年第2期12卷 448-456页

作者： Lei xu Danya xu Xinlei Yi Chao Deng Tianyou Chai tao Yang the State Key Laboratory of Synthetical Automation for Process Industries Northeastern University the Department of Mechanical Engineering University of Victoria Shanghai Institute of Intelligent Science and Technology Tongji University IEEE the Institute of Advanced Technology Nanjing University of Posts and Telecommunications

In this paper, we study the decentralized federated learning problem, which involves the collaborative training of a global model among multiple devices while ensuring data *** classical federated learning, the communication channel between the devices poses a potential risk of compromising private information. To reduce the risk of adversary eavesdropping in the communication channel, we propose TRADE(transmit difference weight) concept. This concept replaces the decentralized federated learning algorithm's transmitted weight parameters with differential weight parameters, enhancing the privacy data against eavesdropping. Subsequently, by integrating the TRADE concept with the primal-dual stochastic gradient descent(SGD)algorithm, we propose a decentralized TRADE primal-dual SGD algorithm. We demonstrate that our proposed algorithm's convergence properties are the same as those of the primal-dual SGD algorithm while providing enhanced privacy protection. We validate the algorithm's performance on fault diagnosis task using the Case Western Reserve University dataset, and image classification tasks using the CIFAR-10 and CIFAR-100 datasets,revealing model accuracy comparable to centralized federated learning. Additionally, the experiments confirm the algorithm's privacy protection capability.

关键词： Adversary eavesdropping decentralized federated learning privacy protection stochastic gradient descent

The association of isocarbophos and isofenphos with different types of glucose metabolism:The role of inflammatory cells

在线全文

同方期刊数据库

学校读者我要写书评

暂无评论

Journal of Environmental Sciences 2025年第1期147卷 322-331页

作者： Jintian Geng Dandan wei Lulu Wang Qingqing xu Juan Wang Jiayu Shi Cuicui Ma Mengzhen Zhao Wenqian Huo tao Jing Chongjian Wang Zhenxing Mao Department of Epidemiology and Biostatistics College of Public HealthZhengzhou UniversityZhengzhou 450001China Department of Occupational and Environmental Health Sciences College of Public HealthZhengzhou UniversityZhengzhou 450001China School of Public Health Tongji Medical CollegeHuazhong University of Science and TechnologyWuhan 430074China

To investigate the associations between isocarbophos and isofenphos with impaired fasting glucose(IFG)and type 2 diabetes mellitus(T2DM),and to assess the mediation roles of inflammation *** were 2701 participants in the case-control study,including 896 patients with T2DM,900 patients with IFG,905 subjects with *** isocarbophos and isofenphos concentrationsweremeasured using gas chromatography and triple quadrupole tandem mass *** linear models were used to calculate the relationships between plasma isofenphos and isocarbophos levels with inflammatory factor levels and *** cell was used as mediators to estimate the mediating effects on the above *** and isofenphos were positively related with T2DM after adjusting for other *** odds ratio(95%confidence interval)(OR(95%CI))for T2DM was 1.041(1.015,1.068)and for IFG was 1.066(1.009,1.127)per unit rise in *** prevalence of T2DM increased by 6.4%for every 1 unit more of ln-isofenphos(OR(95%CI):1.064(1.041,1.087)).Additionally,a 100%rise in ln-isocarbophos was linked to 3.3%higher ln-HOMA2IR and a 0.029 mmol/L higher glycosylated hemoglobin(HbA1c)(95%CI:0.007,0.051).While a 100%rise in ln-isofenphos was linked to increase in ln-HOMA2 and ln-HOMA2IR of 5.8%and 3.4%,***,white blood cell(WBC)and neutrophilic(NE)were found to be mediators in the relationship between isocarbophos and T2DM,and the corresponding proportions were 17.12%and 17.67%,*** and isocarbophos are associated with IFG and T2DM in the rural Chinese population,WBC and NE have a significant role in this relationship.

关键词： Isocarbophos Isofenphos Type 2 diabetes mellitus Inflammatory cells Mediation effect