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Two-dimensional bimetallic selenium-containing metal-organic frameworks and their calcinated derivatives as electrocatalysts for overall water splitting

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Frontiers in Energy 2024年第3期18卷 378-389页

作者： Zhao-ting SHANG Tang-ming LI Bing-qian HU Min LIU wang-ting lu Fan YU Yun ZHENG Key Laboratory of Optoelectronic Chemical Materials and Devices of Ministry of Education College of Optoelectronic Materials and TechnologyJianghan UniversityWuhan 430056China Institute of New Energy Materials and Engineering School of Materials Science and EngineeringFuzhou UniversityFuzhou 350108China Department of Chemical Engineering University of WaterlooWaterlooOntario N2L 3G1Canada

The use of two-dimensional(2D)layered metal-organic frameworks(MOFs)as self-sacrificial templates has been proven to be a successful method to create high-efficiency Selenium(Se)-containing electrocatalysts for overall water ***,two strategies are then utilized to introduce Se element into the Co–Fe MOF,one being the etching of as-prepared MOF by SeO_(2) solution,and the other,the replacing of SCN−with SeCN−as the construction *** electrochemical activity of the pristine 2D MOF and their calcinated derivatives for catalyzing the hydrogen evolution reaction(HER)and oxygen evolution reaction(OER)is evaluated and further *** is found that the effect of introducing Se on improving electrochemical catalytic activity is significant for the HER ***,the calcinated derivative in the replacing method exhibits an overpotential of 235 mV for HER and 270 mV for OER at a current density of 10 mA/*** comparing the two methods of introducing Se element into MOF,similar electrocatalytic activity can be achieved on the their calcinated *** high electrochemical performance of 2D CoFe-MOF derivatives may be resulted from the unique 2D hierarchical porous structure and strong synergistic effect between different components in the material.

关键词： 2D MOF selenium(Se)-containing materials hydrogen evolution reaction(HER) oxygen evolution reaction(OER)

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数字农业发展对缩小城乡居民收入差距的作用机制与实践路径

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税务与经济 2024年第4期 83-90页

作者：郭修平王鲁婷王艳华吉林农业大学经济管理学院

数字农业是农业现代化发展的高级形态，能够提升农民创收能力、优化农业农村发展环境、均衡城乡资源分布、完善收入分配机制，对缩小城乡居民收入差距发挥积极作用。在实现共同富裕的战略目标下，发展数字农业缩小城乡居民收入差距的重... 详细信息

数字农业是农业现代化发展的高级形态，能够提升农民创收能力、优化农业农村发展环境、均衡城乡资源分布、完善收入分配机制，对缩小城乡居民收入差距发挥积极作用。在实现共同富裕的战略目标下，发展数字农业缩小城乡居民收入差距的重点任务包括催生农业发展新动能、发展乡村数字新基建、重塑城乡经济地理和构建发展成果共享机制。因此，我国应立足于数字经济发展特征，提升数字农业创新活力，构建数字农业农村标准体系，强化数字信息服务功能，建立数据风险防控体系，以促进农民增产增收，优化农业资源空间配置，打造城乡发展利益共同体。

关键词：数字农业城乡居民收入差距共同富裕

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贵州栽培种铁皮石斛遗传多样性分析

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时珍国医国药 2024年第4期35卷 992-995页

作者：任得强王廷璐李梅陈春伶贵州中医药大学药学院贵州1贵阳550025

目的研究贵州栽培种铁皮石斛的遗传多样性,可为种质资源利用及遗传改良提供参考。方法利用简单重复序列间区(Inter-simple sequence repeats,ISSR)、简单重复序列(simple sequence repeat,SSR)分子标记技术,对贵州20份分别来自浙江、云... 详细信息

目的研究贵州栽培种铁皮石斛的遗传多样性,可为种质资源利用及遗传改良提供参考。方法利用简单重复序列间区(Inter-simple sequence repeats,ISSR)、简单重复序列(simple sequence repeat,SSR)分子标记技术,对贵州20份分别来自浙江、云南的栽培种的铁皮石斛进行遗传多样性研究,使用NTsys、Popgen32等软件进行遗传分析。结果经筛选得到32对多态性引物,共扩增得到152条清晰的条带,平均每对引物扩增4.75条带,其中多态性条带145条,平均每对引物扩增4.53条多态性条带,其条带的多态率(PPL)为96.05%。经遗传分析,Nei’s基因多样性指数(H)平均值为0.3507,Shannon’s多态性信息指数(I)平均值为0.5219等位基因数(Ne)平均值为1.5992、观测等位基因数(Na)平均值为1.9605,这表明研究所用铁皮石斛具有丰富的遗传变异。聚类分析结果表明,根据来源可将20个贵州栽培种铁皮石斛聚为2类。结论ISSR及SSR分子标记可以有效应用于铁皮石斛遗传多样性分析中,贵州铁皮石斛遗传变异丰富,应加强不同来源的铁皮石斛在系统选育及遗传改良中的合理利用。

关键词：铁皮石斛 ISSR SSR 遗传多样性

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Well-dispersed Sb particles embedded on N-doped carbon nanofibers toward high-performance Li-ion battery

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Rare Metals 2024年第7期43卷 2994-3006页

作者： Ying Li Yi-Han Zhao lu-lu Zhao Peng-Fei wang Ying Xie ting-Feng Yi School of Materials Science and Engineering Northeastern University Key Laboratory of Dielectric and Electrolyte Functional Material Hebei Province School of Resources and MaterialsNortheastern University at Qinhuangdao Key Laboratory of Functional Inorganic Material Chemistry Ministry of EducationSchool of Chemistry and Materials ScienceHeilongjiang University

The alloy-type material Sb is widely used in the anode materials of lithium-ion batteries（LIBs） due to its high theoretical specific ***,its serious volume expansion problem during alloying/dealloying of Li+limits its practical *** this work,C-Sb composite was constructed as anode material of LIBs by electrospinning route for the first time,Sb was introduced into the polyacrylonitrile-based hard carbon and coal tar pitch-based soft carbon composite amorphous carbon fiber with a diameter of 300-600 nm,which realized high cycling *** C-Sb-2（the mass ratio of polyacrylonitrile to Sb source is 1:2） electrode displayed charge capacities of 1098.5,930.3,841.7,753.5,643.9 and 545.8 mAh·g-1at 0.1,0.2,0.3,0.5,1 and 2 A·g-1,*** when the current density returned to 0.1 A·g-1,the charge capacity was 939.3 mAh·g-1,revealing good stability and *** introduction of Sb into the amorphous carbon improved its conductivity and addressed the volume expansion issue of high specific capacity Sb during charge/***-situ XRD analysis confirmed the high reversibility of the C-Sb-2 during charging and *** functional theory（DFT） calculations revealed the gradual enhancement of the interface interaction between SbxLiyand amorphous carbon（AMC） with increasing lithium content,contributing to the anchoring of alloy nanoparticles on the AMC surface and buffering the volume change of the ***,the gradual lithiation of Sb facilitated the electron transfer from SbxLiyto *** findings hold promise for designing lithium storage materials with exceptional performance,highlighting the potential of C-Sb composites as anode materials for efficient next-generation lithium storage.

关键词： Li-ion battery Metallic Sb Carbon Electrospinning Cycling stability

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Tube-based robust reinforcement learning for autonomous maneuver decision for UCAVs

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Chinese Journal of Aeronautics 2024年第7期37卷 391-405页

作者： Lixin wang Sizhuang ZHENG Haiyin PIAO Changqian lu ting YUE Hailiang LIU School of Aeronautical Science and Engineering Beihang UniversityBeijing 100191China Shenyang Aircraft Design&Research Institute Shenyang 110035China

Reinforcement Learning(RL)algorithms enhance intelligence of air combat AutonomousManeuver Decision(AMD)policy,but they may underperform in target combat environmentswith *** enhance the robustness of the AMD strategy learned by RL,thisstudy proposes a Tube-based Robust RL(TRRL)***,this study introduces a tube todescribe reachable trajectories under disturbances,formulates a method for calculating tubes basedon sum-of-squares programming,and proposes the TRRL algorithm that enhances robustness byutilizing tube size as a quantitative ***,this study introduces offline techniques forregressing the tube size function and establishing a tube library before policy learning,aiming toeliminate complex online tube solving and reduce the computational burden during ***,an analysis of the tube library demonstrates that the mitigated AMD strategy achievesgreater robustness,as smaller tube sizes correspond to more cautious *** finding highlightsthat TRRL enhances robustness by promoting a conservative *** effectively balanceaggressiveness and robustness,the proposed TRRL algorithm introduces a“laziness factor”as aweight of ***,combat simulations in an environment with disturbances confirm thatthe AMD policy learned by the TRRL algorithm exhibits superior air combat performance comparedto selected robust RL baselines.

关键词： Air combat Autonomous maneuver decision Robust reinforcement learning Tube-based algorithm Combat simulation

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Pathogen-induced methylglyoxal negatively regulates rice bacterial blight resistance by inhibiting OsCDR1 protease activity

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Molecular Plant 2024年第2期17卷 325-341页

作者： Zheng-Wei Fu Jian-Hui Li Xiang Gao Shi-Jia wang ting-ting Yuan Ying-Tang lu State Key Laboratory of Hybrid Rice College of Life SciencesRenmin Hospital of Wuhan UniversityWuhan UniversityWuhan 430072China Key Laboratory of Biology and Genetic Improvement of OilCrops Ministry of Agriculture and Rural AffairsOilCrops Research Institute of the Chinese Academy of Agricultural SciencesWuhan 430062China

Xanthomonas oryzae ***(Xoo)causes bacterial blight(BB),a globally devastating disease of rice(Oryza sativa)that is responsible for significant crop *** and sugar metabolites are important for pathogen infection,providing energy and regulating events associated with defense responses;howev-er,the mechanisms by which they regulate such events in BB are *** an inevitable sugar metabolite,methylglyoxal(MG)is involved in plant growth and responses to various abiotic stresses,but the underlying mechanisms remain *** and how MG functions in plant biotic stress responses is almost completely ***,we report that the Xoo strain PXO99 induces OsWRKY62.1 to repress transcrip-tion of OsGLY Il genes by directly binding to their promoters,resulting in overaccumulation of *** negatively regulates rice resistance against Pxo99:osglyll2 mutants with higher MG levels are more sus-ceptible to the pathogen,whereas OsGLYIl2-overexpressing plants with lower MG content show greater resistance than the wild *** of OsGLYll2 to prevent excessive MG accumulation confers broad-spectrum resistance against the biotrophic bacterial pathogens Xoo and Xanthomonas oryzae *** and the necrotrophic fungal pathogen Rhizoctonia solani,which causes rice sheath *** evidence shows that MG reduces rice resistance against PXO99 through CONSTITUTIVE DISEASE RESISTANCE 1(OsCDR1).MGmodifies the Arg97 residue of OsCDR1to inhibit its aspartic protease activ-ity,which is essential for OsCDR1-enhanced *** together,these findings illustrate how Xoo promotes infection by hijacking a sugar metabolite in the host plant.

关键词： Oryza sativa bacterial blight OsWRKY62.1 methylglyoxal OsCDR1

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Nanophase separated,grafted alternate copolymer styrene-maleic anhydride as an efficient room temperature solid state lithium ion conductor

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Chinese Chemical Letters 2024年第7期35卷 491-496页

作者： Qian wang ting Gao Xiwen lu Hangchao wang Minggui Xu Longtao Ren Zheng Chang Wen Liu Institute of Science and Technology China Three Gorges CorporationBeijing 100038China State Key Laboratory of Chemical Resource Engineering Beijing Advanced Innovation Center for Soft Matter Science and EngineeringCollege of ChemistryBeijing University of Chemical TechnologyBeijing 100029China

All solid-state lithium metal batteries(ASSLMBs)based on polymer solid electrolyte and lithium metal anode have attracted much attention due to their high energy density and intrinsic ***,the low ionic conductivity at room temperature and poor mechanical properties of the solid polymer electrolyte result in increased polarization and poor cycling stability of the Li metal *** order to improve the ionic conductivity at room temperature while maintaining mechanical strength,we combine the conductivity of short chain polyethylene oxide(PEO)and strength of styrene-maleic anhydride copolymer(SMA)to obtain a grafted block copolymer with nanophase separation structure,which has room temperature ionic conductivity up to 1.14×10^(-4)S/cm and tensile strength up to 1.4 ***||Li symmetric cell can work stably for more than 1500 h under the condition of 0.1 mA/cm^(2).Li||LiFePO_(4)full cells can deliver a high capacity of 151.4 mAh/g at 25℃and 0.2 C/0.2 C charge/discharge conditions,showing 85.6%capacity retention after 400 ***,the all solid state Li||LiFePO_(4)pouch cell shows excellent safety performance under different abuse *** results demonstrate that the nanophase separated,grafted alternate copolymer electrolyte has huge potential for application in Li metal batteries.

关键词： Solid polymer electrolyte All solid-state battery Li metal battery Copolymers Nanophase separation

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Minimalistic approach to left atrial appendage occlusion guided by cardiac computed tomography angiography

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Journal of Geriatric Cardiology 2024年第4期21卷 431-442页

作者： Xian-Sai MENG Qing-Song wang Xin-Yan wang Xu lu Yang MU Jing wang ting-ting SONG Yun-Dai CHEN Tao CHEN Jun GUO Graduate School of Chinese PLA Medical College BeijingChina Senior Department of Cardiology the Sixth Med-ical CenterChinese PLA General HospitalBeijingChina

OBJECTIVE To assess the feasibility and safety of the minimalistic approach to left atrial appendage occlusion(LAAO) guided by cardiac computed tomography angiography(CCTA).METHODS Ninety consecutive patients who underwent LAAO, with or without CCTA-guided, were matched(1:2). Each step of the LAAO procedure in the computed tomography(CT) guidance group(CT group) was directed by preprocedural CT planning. In the control group, LAAO was performed using the standard method. All patients were followed up for 12 months, and device surveillance was conducted using *** A total of 90 patients were included in the analysis, with 30 patients in the CT group and 60 matched patients in the control group. All patients were successfully implanted with Watchman devices. The mean ages for the CT group and the control group were 70.0 ± 9.4 years and 68.4 ± 11.9 years(P = 0.52), respectively. The procedure duration(45.6 ± 10.7 min vs. 58.8 ± 13.0 min,P < 0.001) and hospital stay(7.5 ± 2.4 day vs. 9.6 ± 2.8 day, P = 0.001) in the CT group was significantly shorter compared to the control group. However, the total radiation dose was higher in the CT group compared to the control group(904.9 ± 348.0 m Gy vs.711.9 ± 211.2 m Gy, P = 0.002). There were no significant differences in periprocedural pericardial effusion(3.3% vs. 6.3%, P = 0.8) between the two groups. The rate of postprocedural adverse events(13.3% vs. 18.3%, P = 0.55) were comparable between both groups at 12 months *** CCTA is capable of detailed LAAO procedure planning. Minimalistic LAAO with preprocedural CCTA planning was feasible and safe, with shortened procedure time and acceptable increased radiation and contras consumption. For patients with contraindications to general anesthesia and/or transesophageal echocardiography, this promising method may be an alternative to conventional LAAO.

关键词： anesthesia matched approach

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Joint Optimization of Resource Allocation and Trajectory Based on User Trajectory for UAV-Assisted Backscatter Communication System

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China Communications 2024年第2期21卷 197-209页

作者： Peizhong Xie Junjie Jiang ting Li Yin lu School of Communication and Information Engineering Nanjing University of Posts and TelecommunicationsNanjing 210003China Key Lab of Broadband Wireless Communication and Sensor Network Technology(Nanjing University of Posts and Telecommunications) Ministry of EducationNanjing 210003China

The Backscatter communication has gained widespread attention from academia and industry in recent years. In this paper, A method of resource allocation and trajectory optimization is proposed for UAV-assisted backscatter communication based on user trajectory. This paper will establish an optimization problem of jointly optimizing the UAV trajectories, UAV transmission power and BD scheduling based on the large-scale channel state signals estimated in advance of the known user trajectories, taking into account the constraints of BD data and working energy consumption, to maximize the energy efficiency of the system. The problem is a non-convex optimization problem in fractional form, and there is nonlinear coupling between optimization *** iterative algorithm is proposed based on Dinkelbach algorithm, block coordinate descent method and continuous convex optimization technology. First, the objective function is converted into a non-fractional programming problem based on Dinkelbach method,and then the block coordinate descent method is used to decompose the original complex problem into three independent sub-problems. Finally, the successive convex approximation method is used to solve the trajectory optimization sub-problem. The simulation results show that the proposed scheme and algorithm have obvious energy efficiency gains compared with the comparison scheme.

关键词： energy efficiency joint optimization UAV-assisted backscatter communication user trajectory

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Collective Molecular Machines: Multidimensionality and Reconfigurability

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Nano-Micro Letters 2024年第8期16卷 309-340页

作者： Bin wang Yuan lu Department of Chemical Engineering Tsinghua UniversityBeijing 100084People’s Republic of China Key Laboratory of Industrial Biocatalysis Ministry of EducationTsinghua UniversityBeijing 100084People’s Republic of China

Molecular machines are key to cellular activity where they are involved in converting chemical and light energy into efficient mechanical *** the last 60 years,designing molecular structures capable of generating unidirectional mechanical motion at the nanoscale has been the topic of intense *** progress has been made,attributed to advances in various fields such as supramolecular chemistry,biology and nanotechnology,and ***,individual molecular machines are only capable of producing nanometer work and generally have only a single *** order to address these problems,collective behaviors realized by integrating several or more of these individual mechanical units in space and time have become a new *** this review,we comprehensively discuss recent developments in the collective behaviors of molecular *** particular,collective behavior is divided into two *** is the appropriate integration of molecular machines to efficiently amplify molecular motions and deformations to construct novel functional *** other is the construction of swarming modes at the supramolecular level to perform nanoscale or microscale *** discuss design strategies for both modes and focus on the modulation of features and ***,in order to address existing challenges,the idea of transferring experience gained in the field of micro/nano robotics is presented,offering prospects for future developments in the collective behavior of molecular machines.

关键词： Molecular machines Collective control Collective behaviors DNA Biomolecular motors

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