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Water-Driven Malleable,Weldable and Eco-Friendly Recyclable Carbon Fiber Reinforced Dynamic Composites

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Chinese Journal of Chemistry 2024年第5期42卷 516-522页

作者： Ping Yu Qirui Huang Yi wang wan Peng Zichen Jia Haiyue wang Juanjuan Ma Chunyu wang Xuzhou Yan School of Environmental and Chemical Engineering Jiangsu Key Laboratory of Function Control Technology for Advanced MaterialsJiangsu Ocean UniversityLianyungangJiangsu222005 China School of Chemistry and Chemical Engineering Frontiers Science Center for Transformative MoleculesShanghai Jiao Tong UniversityShanghai200240 China

Traditional carbon fiber-reinforced polymers based on thermoset matrix have been extensively used in the fields of wind turbine blades,automotive sector,and aerospace,among many ***,there is still a major challenge of recycling those polymers due to the high cost and adverse impacts on the *** this work,we apply a polyimine network as matrix,which possess considerable tensile and thermal properties,to prepare the carbon fiber reinforced polyimine materials with trifluoromethyl diphenoxybenzene units(CFRFP)using a prepreg-based compression molding *** CFRFP can be reshaped or reprocessed by heat or with water rapidly,and exhibited multifunction,including welding,chemical recycling,*** unique findings gained from our study will facilitate the manufacturing capability and enrich the types of fiber-reinforced composites.

关键词： Dynamic chemistry Green chemistry Fiber-reinforced composites Fluoropolyimine Welding Reshaping Recycling Renewable resources

Testing the first law of black hole mechanics with gravitational waves

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Science China(Physics,Mechanics & Astronomy) 2024年第10期Mechanics & Astronomy) .卷 80-86页

作者： Chao-wan-Zhen wang Jin-Bao Zhu Guo-Qing Huang Fu-Wen Shu Department of Physics Nanchang University Center for Relativistic Astrophysics and High Energy Physics Nanchang University GCAP-CASPER Physics DepartmentBaylor University

The successful observation of gravitational waves has provided humanity with an additional method to explore the universe, particularly black holes. In this study, we utilize data from LIGO and Virgo gravitational wave observations to test the first law of black hole mechanics, employing two different approaches. We consider the secondary compact object as a perturbation to the primary black hole before the merger, and the remnant black hole as a stationary black hole after the merger. In the pre-merger and post-merger analysis, our results demonstrate consistency with the first law, with an error level of approximate 25% at a68% credibility level for GW190403 051519. In the full inspiral-merger-ringdown analysis, our results show consistency with the first law of black hole mechanics, with an error level of about 6% at a 68% credibility level and 10% at a 95% credibility level for GW191219 163120. Additionally, we observe that the higher the mass ratio of the gravitational wave source, the more consistent our results are with the first law of black hole mechanics. Overall, our study sheds light on the nature of compact binary coalescence and their implications for black hole mechanics.

关键词： gravitational waves black hole mechanics data analysis ringdown

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Efficient stochastic parallel gradient descent training for on-chip optical processor

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Opto-Electronic Advances 2024年第4期7卷 5-15页

作者： Yuanjian wan Xudong Liu Guangze Wu Min Yang Guofeng Yan Yu Zhang Jian wang Wuhan National Laboratory for Optoelectronics and School of Optical and Electronic Information Huazhong University of Science and TechnologyWuhan 430074China Optics Valley Laboratory Wuhan 430074China

In recent years,space-division multiplexing(SDM)technology,which involves transmitting data information on multiple parallel channels for efficient capacity scaling,has been widely used in fiber and free-space optical communication *** enable flexible data management and cope with the mixing between different channels,the integrated reconfig-urable optical processor is used for optical switching and mitigating the channel ***,efficient online train-ing becomes intricate and challenging,particularly when dealing with a significant number of *** we use the stochastic parallel gradient descent(SPGD)algorithm to configure the integrated optical processor,which has less com-putation than the traditional gradient descent(GD)*** design and fabricate a 6×6 on-chip optical processor on silicon platform to implement optical switching and descrambling assisted by the online training with the SPDG ***,we apply the on-chip processor configured by the SPGD algorithm to optical communications for optical switching and efficiently mitigating the channel crosstalk in SDM *** comparison with the traditional GD al-gorithm,it is found that the SPGD algorithm features better performance especially when the scale of matrix is large,which means it has the potential to optimize large-scale optical matrix computation acceleration chips.

关键词： optical communications optical signal processing channel descrambling optical neural network chip silicon photonics

Electrochemical synthesis of trimetallic nickel-iron-copper nanoparticles via potential-cycling for high current density anion exchange membrane water-splitting applications

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Journal of Energy Chemistry 2024年第2期89卷 535-542,I0012页

作者： Ziqi Zhang Sheng wan Hanbo wang Jinghan He Ruige Zhang Yuhang Qi Haiyan Lu State Key Laboratory of Inorganic Synthesis and Preparative Chemistry College of ChemistryJilin UniversityChangchun 130012JilinChina

Hydrogen is known for its elevated energy density and environmental compatibility and is a promising alternative to fossil *** water electrolysis utilizing renewable energy sources has emerged as a means to obtain high-purity ***,electrocatalysts used in the process are fabricated using conventional wet chemical synthesis methods,such as sol-gel,hydrothermal,or surfactantassisted approaches,which often necessitate intricate pretreatment procedures and are vulnerable to post-treatment ***,this study introduces a streamlined and environmentally conscious one-step potential-cycling approach to generate a highly efficient trimetallic nickel-iron-copper electrocatalyst in situ on nickel *** synthesized material exhibited remarkable performance,requiring a mere 476 mV to drive electrochemical water splitting at 100 mA cm^(-2)current density in alkaline ***,this material was integrated into an anion exchange membrane watersplitting device and achieved an exceptionally high current density of 1 A cm^(-2)at a low cell voltage of2.13 V,outperforming the noble-metal benchmark(2.51 V).Additionally,ex situ characterizations were employed to detect transformations in the active sites during the catalytic process,revealing the structural transformations and providing inspiration for further design of electrocatalysts.

关键词： Electrocatalytic water splitting Hydrogen evolution reaction Oxygen evolution reaction Electrochemical synthesis Anion exchange membrane

Multi-layer network embedding on scc-based network with motif

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Digital Communications and Networks 2024年第3期10卷 546-556页

作者： Lu Sun Xiaona Li Mingyue Zhang Liangtian wan Yun Lin Xianpeng wang Gang Xu Department of Communication Engineering Institute of Information Science TechnologyDalian Maritime UniversityDalian116026China Key Laboratory of Big Data Intelligent Computing Chongqing University of Posts and TelecommunicationsChongqing400065China Key Laboratory for Ubiquitous Network and Service Software of Liaoning Province DUT School of Software Technology&DUT-RU International School of Information Science and EngineeringDalian University of TechnologyDalian 116620China College of Information and Communication Engineering Harbin Engineering UniversityHarbin 150001China School of Information and Communication Engineering Hainan UniversityHaikou 570228China State Key Laboratory of Millimeter Waves School of Information Science and EngineeringSoutheast UniversityNanjing 210096China

Interconnection of all things challenges the traditional communication methods,and Semantic Communication and Computing(SCC)will become new *** is a challenging task to accurately detect,extract,and represent semantic information in the research of SCC-based *** previous research,researchers usually use convolution to extract the feature information of a graph and perform the corresponding task of node ***,the content of semantic information is quite *** graph convolutional neural networks provide an effective solution for node classification tasks,due to their limitations in representing multiple relational patterns and not recognizing and analyzing higher-order local structures,the extracted feature information is subject to varying degrees of ***,this paper extends from a single-layer topology network to a multi-layer heterogeneous topology *** Bidirectional Encoder Representations from Transformers(BERT)training word vector is introduced to extract the semantic features in the network,and the existing graph neural network is improved by combining the higher-order local feature module of the network model representation network.A multi-layer network embedding algorithm on SCC-based networks with motifs is proposed to complete the task of end-to-end node *** verify the effectiveness of the algorithm on a real multi-layer heterogeneous network.

关键词： Semantic communication and computing Multi-layer network Graph neural network Motif

Cadaverine and putrescine exposure influence carbon and nitrogen cycling genes in water and sediment of the Yellow River

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Journal of Environmental Sciences 2024年第8期142卷 236-247页

作者： wanghong Su Qiaoling Yu Jiawei Yang Qian Han Sijie wang Petr Hedenec Xiaochen wang Ruijun wan-Yan Huan Li School of Public Health Lanzhou UniversityLanzhou 730000China 2 Institute for Tropical Biodiversity and Sustainable DevelopmentUniversity Malaysia Terengganu21030Kuala NerusTerengganuMalaysia State Key Laboratory of Grassland Agro-ecosystems Center for Grassland MicrobiomeCollege of pastoral agriculture science and technology Lanzhou UniversityLanzhou 730000China

The response patterns of microbial functional genes involved in biogeochemical cycles to cadaver decay is a central topic of recent environmental ***,the response mechanisms and pathways of the functional genes associated with the carbon(C)and nitrogen(N)cycling to cadaveric substances such as cadaverine and putrescine remain *** study explored the variation of functional genes associated with C fixation,C degradation and N cycling and their influencing factors under cadaverine,putrescine and mixed *** results showed only putrescine significantly increased the alpha diversity of C fixation genes,while reducing the alpha diversity of N cycling genes in *** the C cycling,the mixed treatment significantly decreased the total abundance of reductive acetyl-CoA pathway genes(i.e.,acsB and acsE)and lig gene linked to lignin degradation in water,while only significantly increasing the hydroxypropionate-hydroxybutylate cycle(i.e.,accA)gene abundance in *** the N cycling,mixed treatment significantly decreased the abundance of the nitrification(i.e.,amoB),denitrification(i.e.,nirS3)genes in water and the assimilation pathway gene(i.e.,gdhA)in *** factors(i.e.,total carbon and total nitrogen)were all negatively associated with the genes of C and N ***,cadaverine and putrescine exposure may inhibit the pathway in C fixation and N cycling,while promoting C *** findings can offer some new insight for the management of amine pollution caused by animal cadavers.

关键词： Carbon cycling Nitrogen cycling Cadaverine Putrescine Pollution management

Novel 2D bifunctional layered rare-earth hydroxides@GO catalyst as a functional interlayer for improved liquid-solid conversion of polysulfides in lithium-sulfur batteries

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Chinese Chemical Letters 2024年第5期35卷 434-440页

作者： Haodong wang Xiaoxu Lai Chi Chen Pei Shi Houzhao wan Hao wang Xingguang Chen Dan Sun CAS Key Laboratory of Design and Assembly of Functional Nanostructures and Fujian Provincial Key Laboratory of Nanomaterials Fujian Institute of Research on the Structure of MatterChinese Academy of SciencesFuzhou 350002China College of Chemistry and Materials Fujian Normal UniversityFuzhou 350007China Xiamen Institute of Rare Earth Materials Haixi InstitutesChinese Academy of SciencesXiamen 361021China School of Microelectronics Hubei UniversityWuhan 430062China Xiamen Key Laboratory of Rare Earth Photoelectric Functional Materials Xiamen 361021China

The detrimental“shuttle effect”of lithium polysulfides(LiPSs)together with sluggish multi-order reaction kinetics are the main drawbacks hindering lithium-sulfur(Li-S)batteries from commercial ***,we first propose the implementability of layered rare-earth hydroxides(LREHs)in Li-S batteries to optimize electrochemical *** this work,a two-dimensional(2D)rare-earth-based composite constructed by the layered gadolinium hydroxy chloride[Gd_(2)(OH)_(5)(H_(2)O)_(n)]Cl nanoplates(LGdH NPs)and graphene oxide(GO)was designed as a sulfur immobilizer for Li-S *** the experimental results and density functional theory(DFT)calculations,it is revealed that the LGdH@GO composite not only provides a strong anchoring of the intermediates during cycling,but also acts as an effective catalyst to accelerate the liquid-solid conversion of *** Li-S batteries assembled by LGdH@GO modified separators delivered a superior rate performance with a specific capacity of 605.34 mAh/g at 5 C,as well as excellent cycle stability with a decay rate of 0.087%over 500 cycles at 2 *** study provided a deep understanding of the mechanism to suppress the“shuttle effect”by the LREHs,and a guide to design effective functional interlayers for high-performance Li-S batteries with excellent electrocatalytic activity.

关键词： Lithium-sulfur batteries Functional separator Layered rare-earth hydroxides Shuttle effect Adsorption Catalysis

Synthesis and potential osteogenic applications of Wnt3a-loaded ZIF-8 nanoparticles

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Chinese Chemical Letters 2024年第3期35卷 399-405页

作者： Hengfei wang Song Chen Zihan He Junyu Chen Zhou Zhu Qianbing wan Jian wang Xibo Pei State Key Laboratory of Oral Diseases National Clinical Research Center for Oral DiseasesDepartment of ProsthodonticsWest China Hospital of StomatologySichuan UniversityChengdu 610041China Chongqing Key Laboratory of Oral Diseases and Biomedical Sciences Chongqing Municipal Key Laboratory of Oral Biomedical Engineering of Higher EducationStomatological Hospital of Chongqing Medical UniversityChongqing 400016China

The Wnt signaling pathway plays a critical role in bone homeostasis,and the related protein therapy strategies have been reported to have great potential in osseointegration;however,they face formidable challenges such as complex external environments and unavoidable protein *** this work,we report a novel approach combining the synthesis of metal–organic frameworks(MOFs)and protein encapsulation in a one-pot process based on zeolitic imidazolate framework-8(ZIF-8)and Wnt3a protein,with improved biomechanical behavior and enhanced protein biological *** combination was designed to enhance the Wnt3a protein function through the improved chemical stability provided by the ZIF-8 ***,the zinc ions contained in the ZIF-8 crystals induced bone homeostasis,further favoring the *** results showed that the Wnt3a protein-loaded ZIF-8 crystals served as efficient drug delivery vehicles to promote osteogenesis,preventing protein *** particular,Wnt3a-loaded ZIF-8 nanoparticles(Wnt3a@ZIF-8 NPs)had higher efficacy on bone marrow mesenchymal stem cells(BMSCs)than ZIF-8 NPs or Wnt3a proteins,contributing to the osteogenesis through ZIF-8 crystals and intracellular Wnt3a proteins released from Wnt3a@ZIF-8 ***,polymerase chain reaction(PCR)analysis showed that the osteogenic pathways were ***,the present one-pot process can open up new avenues to develop signaling protein-delivery systems for applications in protein therapy strategies.

关键词： Metal–organic frameworks Nanoparticle Drug release Osteogenesis Bone defects

Multi-spherical interactions and mechanisms of hydrocarbon enrichment in the Southeast Asian archipelagic tectonic system

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Science China Earth Sciences 2024年第2期67卷 566-583页

作者： Rixiang ZHU Hongjun wang Huajian wang Xiaomei wang Bo wan wang ZHANG Houqin ZHU Yuke LIU Junlai LIU Qingren MENG Fang HAO Zhijun JIN State Key Laboratory of Lithospheric Evolution Institute of Geology and GeophysicsChinese Academy of SciencesBeijing100029China State Key Laboratory of Enhanced Oil and Gas Recovery PetroChina Research Institute of Petroleum Exploration and DevelopmentBeijing100083China School of Earth Sciences and Resources China University of GeosciencesBeijing100083China State Key Laboratory of Deep Oil and Gas China University of Petroleum(East China)Qingdao266580China Institute of Energy Peking UniversityBeijing100871China

Global cooling began since 50 Ma,but a warm climate was maintained in the archipelagic tectonic system in Southeast Asia where a wealth of Cenozoic oil and gas resources was formed and *** the perspective of Earth system,this study analyzes Cenozoic tectonic activities,climatic and environmental evolution,and petroleum enrichment in Southeast Asia,and provides the following insights:(1)Subduction of oceanic plates and the extension of overlying continental lithosphere resulted in widespread volcanic eruptions as well as the formation of rift basins and shallow marine shelves,leading to complex interactions between deep tectonic processes and Earth’s surface including mountains,basins,and seas.(2)Microcontinental accretion and prolonged stay in equatorial low-latitude regions have changed trade winds into monsoons,altered ocean current pathways and flow rates,and profoundly affected rainfall and climate.(3)The archipelagic tectonic system,coupled with a hot and rainy climate,fostered tropical rainforests,mangroves,and phytoplankton,providing abundant organic matter and promoting the development of petroleum resources.(4)Combinations of rift basin development and marine transgression and regression led to an effective superposition of source-reservoir-seal combinations from multiplepetroleum *** deep burial of organic matter and high geothermal gradients facilitated the generation and large-scale accumulation of oil and gas.(5)Multi-spherical(such as atmosphere,biosphere,hydrosphere and lithosphere)interactions on the Earth,which resulted from the convergence of multiple tectonic plates,are believed as the primary driver for exceptional enrichments of Cenozoic oil and gas resources in Southeast *** understandings are significant for developing theories of oil and gas enrichment under the guidance of Earth System *** order to continue making significant oil and gas exploration discoveries in the deep-layers,deep-waters,and unconventio

关键词： Southeast Asia Archipelagic tectonic system Interactions of Earth’s spheres Oil and gas resources Cenozoic