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The surface electron transfer strategy promotes the hole of PDI release and enhances emerging organic pollutant degradation

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Journal of Semiconductors 2024年第10期45卷 84-91页

作者： Yunchuan Yang Dongyu wang Jisheng geng jun Liu jun wang State Key Laboratory of Environmental−Friendly Energy Materials School of Materials and ChemistrySouthwest University of Science and TechnologyMianyang 621010China Tianfu Institute of Research and Innovation Southwest University of Science and TechnologyChengdu 610213China Guangdong−Hong Kong Joint Laboratory for Water Security Center for Water ResearchAdvanced Institute of Natural SciencesBeijing Normal University at ZhuhaiZhuhai 519087China

In semiconductor photocatalysts,the easy recombination of photogenerated carriers seriously affects the application of photocatalytic materials in water *** solve the serious problem of electron−hole pair recombination in perylene diimide(PDI)organic semiconductors,we loaded ferric hydroxyl oxide(FeOOH)on PDI materials,successfully prepared novel FeOOH@PDI photocatalytic materials,and constructed a photo-Fenton *** system was able to achieve highly efficient degradation of BPA under visible light,with a degradation rate of 0.112 min^(−1)that was 20 times higher than the PDI system,and it also showed universal degradation performances for a variety of emerging organic pollutants and anti-interference *** mechanism research revealed that the FeOOH has the electron trapping property,which can capture the photogenerated electrons on the surface of PDI,effectively reducing the compounding rate of photogenerated carriers of PDI and accelerating the iron cycling and H2O2 activation on the surface of FeOOH at the same *** work provides new insights and methods for solving the problem of easy recombination of carriers in semiconductor photocatalysts and degrading emerging organic pollutants.

关键词： perylene diimide organic semiconductors emerging pollutants surface electron transfer strategy photo-Fenton

Artemordins A-S, Cadinane-Type Sesquiterpenoid Dimers from Artemisia ordosica and Their Antihepatoma Activities

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Chinese Journal of Chemistry 2024年第13期42卷 1493-1508页

作者： Yuan wang Tian-Ze Li Yun-Bao Ma Chang-An geng Yong-Cui wang Ji-jun Chen State Key Laboratory of Phytochemistry and Plant Resources in West China Kunming Institute of BotanyChinese Academy of SciencesKunmingYunnan 650201China University of Chinese Academy of Sciences Beijing 100049China

Nineteen new cadinane-involving sesquiterpenoid dimers,artemordins A-S(1-—19),together with 13 known SDs(20-32)were isolated from Artemisia *** structures and absolute configurations were established by comprehensive spectral analyses,X-ray single crystal diffraction,theoretical ECD,and NMR ***,artemordins A-F(1—6)were the first examples of two cadinane units constructed by unprecedented C-3−C-15′or C-3−C-13′single bond with an oxido-rearranged 6/5/6/6 fused ring system;artemordins G-K(7-11)were biogenetically connected by[4+2]cycloaddition reaction and artemordins G-J(7-10)possessed a novel 5/6/6/6/6/6/5-heptacyclic fused ring *** L-S(12-19)were formed by esterification,which involved three different types of *** assay suggested that the most active compounds,artemordins B and H(2 and 8),exhibited inhibitory activities on three hepatoma cell lines with IC50 values of 26.9 and 25.1μmol/L(HepG2),29.5 and 18.3μmol/L(Huh7),19.7 and 15.7μmol/L(SK-Hep-1).

关键词： Artemisia ordosica Artemordins A-s Cadinane-type sesquiterpenoid dimers Antihepatoma activities Terpenoids Natural products Cytotoxicity

Point defects in 2-D liquid crystals with a singular potential:Profiles and stability

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Science China Mathematics 2024年第11期67卷 2515-2540页

作者： Zhiyuan geng Wei wang Basque Center for Applied Mathematics School of Mathematical Sciences Zhejiang University

We study radial symmetric point defects with degree k/2 in the 2-D disk or R2in the Q-tensor framework with a singular bulk energy,which is defined by Bingham ***,we obtain the existence of solutions for the profiles of radial symmetric point defects with degree k/2 in the 2-D disk or ***,we prove that the solution is stable for |k| = 1 and unstable for |k| > *** identities are derived and utilized throughout the proof of existence and stability/instability.

关键词： radial symmetric point defects singular bulk potential Bingham closure stability

Muscovite^(40)Ar/^(39)Ar isotopic dating of pegmatite veins in the Bieyesamas rare metal deposit in the Altay Mountain,Xinjiang,northwestern China

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China Geology 2024年第3期7卷 589-591页

作者： geng-biao Qiao Ping wang Xiao-hong wang jun-lu Chen Key Laboratory for the Study of Focused Magmatism and Giant Ore Deposits Ministry of Natural ResourcesXi’an 710119China Northwest China Center for Geoscience Innovation Xi’an Center of China Geological SurveyXi’an 710119China Petroleum Exploration and Development Research Institute of PetroChina Changqing Oilfield Company Xi’an 710086China

*** The Altay Orogenic Belt in Xinjiang,China is located in the west of the Central Asian Orogenic Belt and in the transition zone between the Siberian Plate and the Kazakhstan-junggar Plate,extending approximately 500 km in northern Xinjiang,China(Fig.1a).The Altay Orogenic Belt has undergone two-way accretion of the Paleozoic crust and the Meso-Cenozoic intracontinental orogeny,leading to the formation of large numbers of intermediate-acid *** than 100000 pegmatite veins have been discovered in the intermediate-acid intrusions,and they constitute an important rare metal metallogenic belt of China(Fig.1b).

关键词： Xinjiang dating isotopic

Remarkable Wear Resistance in a Complex Concentrated Alloy with Nanohierarchical Architecture and Composition Undulation

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Research 2024年第1期2023卷 403-416页

作者： Yushan geng Wenyuan Chen Hui Tan jun Cheng Shengyu Zhu jun Yang Weimin Liu State Key Laboratory of Solid Lubrication Lanzhou Institute of Chemical PhysicsChinese Academy of SciencesLanzhou 730000PR China Center of Materials Science and Optoelectronics Engineering University of Chinese Academy of SciencesBeijing 100049PR China Shandong Laboratory of Yantai Advanced Materials and Green Manufacturing Yantai 264000PR China

Sustained wear damages on the sliding surfaces of alloys are generally the culprit responsible for the failure of various mechanical *** by high-entropy effects,here we deliberately deploy nanohierarchical architecture with composition undulation in a Ni50(AlNbTiV)_(50) complex concentrated alloy,which yields ultralow wear rate within the order of 10^(−7) to 10^(−6) mm^(3)/Nm between room temperature and 800℃.Such remarkable wear resistance heretofore represents one of the highest wear resistance reported for the bulk alloys or composites,and originates from the multi-type adaptive friction interface protection governed by intrinsically nano-coupled grains and *** cooperative heterostructure releases gradient frictional stress in stages upon wear at room temperature through the coexistence of multiple deformation pathways while activating a dense nanocrystalline glaze layer upon wear at 800℃ to minimize adhesive and oxidative *** work uncovers a practical avenue for tailoring wear properties with multicomponent heterostructures over a wide temperature range.

关键词： wear alloys friction

Review of the Low-Lying Excited Baryons∑*(1/2-)

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Chinese Physics Letters 2024年第10期41卷 31-37页

作者： En wang Li-Sheng geng Jia-jun Wu Ju-jun Xie and Bing-Song Zou School of Physics Zhengzhou UniversityZhengzhou 450001China Guangxi Key Laboratory of Nuclear Physics and Nuclear Technology Guangxi Normal UniversityGuilin 541004China School of Physics Beihang UniversityBeijing 102206China Peng Huanwu Collaborative Center for Research and Education Beihang UniversityBeijing 100191China Beijing Key Laboratory of Advanced Nuclear Materials and Physics Beihang UniversityBeijing 102206China Southern Center for Nuclear-Science Theory(SCNT) Institute of Modern PhysicsChinese Academy of SciencesHuizhou 516000China School of Physics University of Chinese Academy of SciencesBeijing 100049China Institute of Modern Physics Chinese Academy of SciencesLanzhou 730000China School of Nuclear Sciences and Technology University of Chinese Academy of SciencesBeijing 101408China Department of Physics Tsinghua UniversityBeijing 100084China CAS Key Laboratory of Theoretical Physics Institute of Theoretical PhysicsChinese Academy of SciencesBeijing 100190China

Strong empirical and phenomenological indications exist for large sea-quark admixtures in the low-lying excited *** the low-lying excited baryon∑*(1/2-)is important for determining the nature of the low-lying excited... 详细信息

关键词： excited quark determining

Microstructure and texture evolution of Cu-Cr-Co-Ti alloys during the two-stage cryorolling

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Rare Metals 2024年第9期43卷 4535-4547页

作者： Jia-jun Zhang Long-Jian Li Zhi-Feng Liu Zong-Ning Chen En-Yu Guo Hui-jun Kang Ren-geng Li Tong-Min wang Key Laboratory of Solidification Control and Digital Preparation Technology(Liaoning Province) School of Materials Science and EngineeringDalian University of TechnologyDalian 116024China Center of Hyper-Gravity Experimental and Interdisciplinary Research Zhejiang UniversityHangzhou 310058China Ningbo Institute of Dalian University of Technology Ningbo 315000China Key Laboratory for Light-Weight Materials Nanjing Tech UniversityNanjing 210009China

This study entailed an investigation of the mechanical properties,microstructural and texture orientation evolutions of Cu-Cr-Co-Ti alloys prepared via twostage cryorolling and intermediate aging *** this end,X-ray diffraction and electron backscatter diffraction were *** results indicate that the two-stage cryorolling and intermediate aging treatments led to the development of profuse twin bundles and significantly enhanced the mechanical *** initial cryorolling led to coplanar slip and developed a strong Y({111})orientation,accelerating the formation of Goss({011})orientation and a Brass-type *** intermediate aging treatment relieved the restriction on dislocation slip and reoriented the grains toward the Copper({112})and Z({111})*** Z orientation,with a relatively high volume fraction,dominated the *** cryorolling intensified twinning and shear banding,transforming the Copper-type shear bands into Brass-type shear bands with rhomboidal prism *** areas inside the Brasstype shear bands exhibited a Y orientation,and the areas outside the shear bands exhibited a stable Brass-type *** evident decrease in the weighted Schmid factors demonstrated that the two-stage cryorolling and intermediate aging treatment can modify the texture evolution and aid the design of high-performance Cu alloys.

关键词： Copper alloys Two-stage cryorolling Macrotexture evolution Electron backscatter diffraction Schmid factor

The Ω(2012) as a Hadronic Molecule

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Chinese Physics Letters 2024年第8期41卷 13-16页

作者： Ju-jun Xie Li-Sheng geng Institute of Modern Physics Chinese Academy of SciencesLanzhou 730000China School of Nuclear Sciences and Technology University of Chinese Academy of SciencesBeijing 101408China Southern Center for Nuclear-Science Theory(SCNT) Institute of Modern PhysicsChinese Academy of SciencesHuizhou 516000China School of Physics Beihang UniversityBeijing 102206China Beijing Key Laboratory of Advanced Nuclear Materials and Physics Beihang UniversityBeijing 102206China Peng Huanwu Collaborative Center for Research and Education Beihang UniversityBeijing 100191China

Recently,a new excited baryon state,Ω(2012),was observed in the invariant mass spectra of𝐾K^(-)■^(0) and K_(S)^(0)■^(-)by the Belle *** state has a narrow width(∼6 MeV)compared to other baryon states with a similar ***,we provide a mini-review on the Ω(2012)state from the molecular perspective,where it appears to be a dynamically generated state with spin-parity 3/2^(−)from the coupled-channels interactions of the K■(1530)and ηΩ in s-wave and K■ in𝑑***,alternative explanations for the Ω(2012)resonance are also discussed.

关键词： wave. invariant state

Intelligent Small Sample Defect Detection of Concrete Surface Using Novel Deep Learning Integrating Improved YOLOv5

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IEEE/CAA Journal of Automatica Sinica 2024年第2期11卷 545-547页

作者： Yongming Han Lei wang Youqing wang Zhiqiang geng IEEE College of Information Science and Technology Beijing University of Chemical TechnologyBeijing 100029 Engineering Research Center of Intelligent PSE Ministry of Education in ChinaBeijing 100029China

Dear Editor,This letter presents an intelligent small sample defect detection of concrete surface using novel deep learning integrating the improved YOLOv5 based on the Wasserstein GAN(WGAN)enhancement *** proposed method is capable of producing top-notch data sets to address the issues of insufficient samples and substandard quality.

关键词： concrete integrating algorithm