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Molecular Chaperone-Dependent Polymer Translocation through Nanopores: The Effects of Chaperone Concentration and Chaperone-Polymer Interaction

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Chinese Journal of Polymer Science 2024年第1期42卷 125-132,I0011页

作者： Chang-Sheng Zuo kang wang Li-Zhen Sun Ting-Ting Sun Department of Physics Zhejiang University of Science and TechnologyHangzhou 310023China Department of Applied Physics Zhejiang University of TechnologyHangzhou 310014China

The polymer translocation through a nanopore from a donor space(or named cis side) to a receiver space(trans side) in the chaperone-induced crowded environment has attracted increasing attention in recent years due to its significance in biological systems and technological applications. In this work, we mainly focus on the effects of chaperone concentration and chaperone-polymer interaction on the polymer translocation. By assuming the polymer translocation to be a quasi-equilibrium process, the free energy F of the polymer can be estimated by Rosenbluth-Rosenbluth method and then the translocation time τ can be calculated by Fokker-Plank equation based on the obtained free energy landscape. Our calculation results show that the translocation time can be controlled by independently tuning the chaperone concentration and chaperone-polymer interaction at the cis side or the trans side. There exists a critical chaperone-polymer attraction ε~*=-0.2 at which the volume exclusion and interaction effects of the chaperone can balance each other. Additionally, we also find that at large chaperone-polymer attraction, the translocation time is mainly governed by the diffusion coefficient of the polymer.

关键词： Polymer translocation Rosenbluth-Rosenbluth method Fokker-Plank equation Free energy landscapes

African Bison Optimization Algorithm: A New Bio-Inspired Optimizer with Engineering Applications

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Computers, Materials and Continua 2024年第1期81卷 603-623页

作者： Zhao, Jian wang, kang wang, Jiacun Guo, Xiwang Qi, Liang School of Science University of Science and Technology Liaoning Anshan 114051 China Team of Artificial Intelligence Theory and Application University of Science and Technology Liaoning Anshan 114051 China Department of Computer Science and Software Engineering Monmouth University West Long Branch NJ 07764 United States Information and Control Engineering College Liaoning Petrochemical University Fushun 113000 China Department of Computer Science and Technology Shandong University of Science and Technology Qingdao 266590 China

This paper introduces the African Bison Optimization (ABO) algorithm, which is based on biological population. ABO is inspired by the survival behaviors of the African bison, including foraging, bathing, jousting, mating, and eliminating. The foraging behavior prompts the bison to seek a richer food source for *** bison find a food source, they stick around for a while by bathing behavior. The jousting behavior makes bison stand out in the population, then the winner gets the chance to produce offspring in the mating behavior. The eliminating behavior causes the old or injured bison to be weeded out from the herd, thusmaintaining the excellent individuals. The above behaviors are translated into ABO by mathematical modeling. To assess the reliability and performance of ABO, it is evaluated on a diverse set of 23 benchmark functions and applied to solve five practical engineering problems with constraints. The findings from the simulation demonstrate that ABO exhibits superior and more competitive performance by effectively managing the trade-off between exploration and exploitation when compared with the other nine popular metaheuristics algorithms. © 2024 The Authors.

关键词： Livestock

In situ meso-tetra(4-carboxyphenyl)porphyrin ligand substitution in Hf-MOF for enhanced catalytic activity and stability in photoredox reactions

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Rare Metals 2024年第6期43卷 2682-2694页

作者： Jie Hu Hong-Xin Lao Xiu-Wu Xu Wei-kang wang Le-Le wang Qin-Qin Liu School of Materials Science and Engineering Jiangsu UniversityZhenjiang 212013China College of Chemistry and Materials Engineering Research Center of Carbon NeutralityAnhui Normal UniversityWuhu 241002China Fujian Provincial Key Laboratory of Ecology-Toxicological Effects and Control for Emerging Contaminants Putian UniversityPutian 351100China

Though there are numerous intrinsic merits of metal-organic frameworks(MOFs),low charge separation efficiency has imposed heavy restrictions on their photocatalytic ***,in situ porphyrin ligand substitution,as a strategy for improving the charge separation efficiency and increasing the amounts of active sites,has been designed and realized in a Hf-biphenyl dicarboxylic acid(BPDC)***,a size and geometry matched meso-tetra(4-carboxyphenyl)porphyrin(TCPP)ligand was selected and doped into Hf-BPDC MOF by forming coordinating bonds with Hf centers,forming dualligand Hf-BPDC-TCPP *** resultant Hf-BPDC-TCPP MOF showed significantly improved activity and chemical stability in the photocatalytic H_(2)generation(261μmol·g^(-1)·h^(-1))and tetracycline(TC)degradation reactions(95.8%),which was 48 and 1.47 folds higher than that of the Hf-BPDC *** and electrochemical studies revealed that the introduction of porphyrin ligand could generate a stronger internal electric field for boosting the charge separation and transfer,increase the specific surface area for providing more active sites,and narrow the band gap to enhance the visible light *** in situ ligand substitution method provides a promising approach to build a tunable platform for constructing high-performance MOF photocatalysts.

关键词： Ligand substitution Metal organic frameworks Meso-tetra(4-carboxyphenyl)porphyrin Hydrogen evolution reaction Tetracycline degradation

PVDF/6H-SiC composite fiber films with enhanced piezoelectric performance by interfacial engineering for diversified applications

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Journal of Materials Science & Technology 2024年第3期170卷 238-245页

作者： Linlin Zhou Tao Yang Chunyu Guo kang wang Enhui wang Laipan Zhu Hailong wang Sheng Cao Kuo-Chih Chou Xinmei Hou Institute for Carbon Neutrality University of Science and Technology BeijingBeijing 100083China Beijing Institute of Nanoenergy and Nanosystems Chinese Academy of SciencesBeijing 101400China School of Materials Science Engineering Zhengzhou UniversityZhengzhou 450001China State Key Laboratory of Featured Metal Materials and Life-cycle Safety for Composite Structures Guangxi UniversityNanning 530004China

Piezoelectric silicon carbide(SiC)has been quite attractive due to its superior chemical and physical properties as well as wide potential ***,the inherent brittleness and unsatisfactory piezoelectric response of piezoelectric semiconductors remain the major obstacles to their diversified ***,flexible multifunctional PVDF/6H-SiC composite fiber films are fabricated and utilized to assemble both piezoelectric nanogenerators(PENGs)and stress/temperature/light *** open cir-cuit voltage(V_(oc))and the density of short circuit current(I_(sc))of the PENG based on the PVDF/5 wt%6H-SiC composite fiber films reach 28.94 V and 0.24μA cm^(-2),showing a significant improvement of 240%and 300%compared with that based on the pure PVDF *** effect of 6H-SiC nanoparticles(NPs)on inducing interfacial polarization and stress concentration in composite fiber films is proved by first-principles calculation and finite element *** stress/temperature/light sensors based on the composite fiber film also show high sensitivity to the corresponding *** study shows that the PVDF/6H-SiC composite fiber film is a promising candidate for assembling high-performance energy harvesters and diverse sensors.

关键词： 6H-SiC PVDF Multifunctional composite fiber film Energy harvester Stress/temperature/light sensor

Monitoring seismicity in the southern Sichuan Basin using a machine learning workflow

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Earthquake Research Advances 2024年第1期4卷 59-66页

作者： kang wang Jie Zhang Ji Zhang Zhangyu wang Huiyu Zhu School of Earth and Space Sciences University of Science and Technology of ChinaHefei230026China

Monitoring seismicity in real time provides significant benefits for timely earthquake warning and *** this study,we propose an automatic workflow based on machine learning(ML)to monitor seismicity in the southern Sichuan Basin of *** workflow includes coherent event detection,phase picking,and earthquake location using three-component data from a seismic *** combining Phase Net,we develop an ML-based earthquake location model called Phase Loc,to conduct real-time monitoring of the local *** approach allows us to use synthetic samples covering the entire study area to train Phase Loc,addressing the problems of insufficient data samples,imbalanced data distribution,and unreliable labels when training with observed *** apply the trained model to observed data recorded in the southern Sichuan Basin,China,between September 2018 and March *** results show that the average differences in latitude,longitude,and depth are 5.7 km,6.1 km,and 2 km,respectively,compared to the reference *** Loc combines all available phase information to make fast and reliable predictions,even if only a few phases are detected and *** proposed workflow may help real-time seismic monitoring in other regions as well.

关键词： Earthquake monitoring Machine learning Local seismicity Gaussian waveform Sparse stations

An envelope-based machine learning workflow for locating earthquakes in the southern Sichuan Basin

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Earthquake Research Advances 2024年第2期4卷 45-54页

作者： kang wang Jie Zhang Ji Zhang Zhangyu wang Ziyu Li School of Earth and Space Sciences University of Science and Technology of ChinaHefei230026China

The development of machine learning technology enables more robust real-time earthquake monitoring through automated implementations. However, the application of machine learning to earthquake location problems faces challenges in regions with limited available training data. To address the issues of sparse event distribution and inaccurate ground truth in historical seismic datasets, we expand the training dataset by using a large number of synthetic envelopes that closely resemble real data and build an earthquake location model named ENVloc. We propose an envelope-based machine learning workflow for simultaneously determining earthquake location and origin time. The method eliminates the need for phase picking and avoids the accumulation of location errors resulting from inaccurate picking results. In practical application, ENVloc is applied to several data intercepted at different starting points. We take the starting point of the time window corresponding to the highest prediction probability value as the origin time and save the predicted result as the earthquake location. We apply ENVloc to observed data acquired in the southern Sichuan Basin, China, between September 2018 and March 2019. The results show that the average difference with the catalog in latitude, longitude, depth, and origin time is 0.02°,0.02°, 2 km, and 1.25 s, respectively. These suggest that our envelope-based method provides an efficient and robust way to locate earthquakes without phase picking, and can be used in earthquake monitoring in near-real time.

关键词： Waveform envelope Earthquake location Local seismicity Synthetic data Sparse stations

Efficient piezo-catalytic dye degradation using piezoelectric 6H-SiC under harsh conditions

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Rare Metals 2024年第7期43卷 3173-3184页

作者： Lin-Lin Zhou Tao Yang kang wang Lai-Pan Zhu En-Hui wang Kuo-Chih Chou Hai-Long wang Xin-Mei Hou Institute for Carbon Neutrality University of Science and Technology BeijingBeijing 100083China Institute of Steel Sustainable Technology Liaoning Academy of MaterialsShenyang 110000China Beijing Institute of Nanoenergy and Nanosystems Chinese Academy of SciencesBeijing 101400China School of Materials Science Engineering Zhengzhou UniversityZhengzhou 450001China Beijing Advanced Innovation Center for Materials Genome Engineering Beijing University of Science and TechnologyBeijing 100083China

The development of novel piezoelectric catalysts against harsh conditions is indeed crucial for improving the piezo-catalytic degradation efficiency of colored organic dyes in *** this work,6H-SiC nanoparticles(NPs)are utilized to piezo-catalytic degrade rhodamine B(RhB)and methylene blue(MB)under ultrasonic vibration for the first *** degradation efficiency of RhB and MB reaches 98.8%and 98.7%within 80 *** piezoelectricity of 6H-SiC is comprehensively analyzed by the piezoresponse force microscope(PFM)and finite element method(FEM).The strong oxidizing active free radicals generated by the continuous piezoelectric polarized electric field of 6H-SiC,i.e.,·O_(2)^(-)and·OH,induce the decomposition reactions of colored organic dyes in *** the dyes are proven to degrade to harmless or less-harmful products gradually during the piezo-catalysis process by high-performance liquid chromatography tandem mass spectrometry(HPLC-MS).Moreover,RhB is also decomposed efficiently by 6HSiC NPs under acidic and alkaline *** results prove the feasibility of 6H-SiC for decomposing common water pollutants under harsh conditions and provide a new perspective for water purification.

关键词： Piezo-catalytic degradation 6H-SiC Rhodamine B(RhB) Methylene blue(MB) Harsh conditions

Low Loss and Low EMI Noise Trench IGBT with Shallow Emitter Trench Controlled P-Type Dummy Region

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Chinese Journal of Electronics 2024年第2期33卷 326-335页

作者： Jinping ZHANG Xiaofeng LI Rongrong ZHU kang wang Bo ZHANG State Key Laboratory of Electronic Thin Films and Integrated Devices University of Electronic Science and Technology of China (UESTC) Institute of Electronic and Information Engineering of UESTC in Guangdong

A novel trench insulated gate bipolar transistor（TIGBT） with a shallow emitter trench controlled P-type dummy region（STCP-TIGBT） is *** with the conventional TIGBT with floating P-type dummy region（CFP-TIGBT） and TIGBT with floating P-type dummy region and normally on hole path（HFPTIGBT）,the proposed STCP structure not only speeds up the extraction of excessive holes in the turn-off process but also reduces the Miller plateau charge(Qgc).Therefore,both the power loss and electromagnetic interference（EMI） noise are significantly *** results show that the Qgcof the proposed device is only 501 nC/cm2,which is reduced by 58.5% and 26.4% when compared to the CFP-TIGBT and HFP-TIGBT,*** same on-state voltage drop(Vceon) of 1.02 V,the turn-off loss(Eoff) of the proposed device is 13.49 mJ/cm2,which is 64.6%and 67.6% less than those of the CFP-TIGBT and HFP-TIGBT,***,the reverse recovery dVak/dt of the freewheeling diode at same turn-on loss(Eon) of 31.8 mJ/cm2for the proposed STCP-TIGBT is only 2.15 kV/μs,which is reduced by 91.3% and 57.2% when compared to 24.69 kV/μs and 5.02 kV/μs for the CFP-TIGBT and HFPTIGBT,*** reduced dV/dt significantly suppresses the electromagnetic interference noise generated by the proposed device.

关键词： Insulated gate bipolar transistors Electrodes Annealing Simulation Electromagnetic interference Noise Voltage

Geology and genesis of the Aqishan Pb-Zn deposit,NW China:Insights from mineralogy,geochemistry,and in situ U-Pb geochronology

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Geoscience Frontiers 2024年第5期15卷 489-514页

作者： kang wang Yinhong wang Jun Deng Jiajun Liu Fangfang Zhang Wei Zhang Hui Zhang Wenxin Gu Hong Chen State Key Laboratory of Geological Processes and Mineral Resources and School of Earth Sciences and ResourcesChina University of GeosciencesBeijing 100083China

The unique ore-forming processes and the key factors responsible for formation of skarn deposits are still obscure,and challenges exist in the determination of timing of Pb-Zn skarns owing to lacking suitable mineral *** we present detailed paragenesis,bulk geochemistry,in situ U-Pb dating of zircon and garnet,and garnet oxygen isotopes together with in situ zircon Hf-O isotopes from the newly discovered Aqishan Pb-Zn deposit in the southern Central Asian Orogenic Belt(CAOB),northwest *** comprehensive data set revealed a Late Carboniferous subduction-related distal Pb-Zn skarn system associated with the granitic ***-ore stage garnets are generally subhedral to euhedral with oscillatory zoning and show slightly fractionated rare earth element patterns with positive Eu anomalies that point to an infiltration metasomatism origin under high water/rock *** syn-ore stage sphalerite is typically enriched in Mn and Cd and has moderate Zn/Cd ratios(337–482),with a formation temperature of 265℃to 383℃,which indicate magmatic-hydrothermal *** isocons defined by P_(2)O_(5)decipher that the principal factors for skarn formation were elevated activities of Fe,Ca,and Si species,where remobilization of Pb metals,meanwhile,contributed to ore-forming budgets to mineralizing *** U-Pb dating of zircons from granite porphyry that occurs distal to the skarns and Pb-Zn orebodies shows that these intrusions emplaced at ca.311.3–310.6 Ma,recording the subduction of the Paleo-Tianshan oceanic *** garnets in close textural association with Pb-Zn sulfides yield indistinguishable in situ LA-ICP-MS U-Pb ages of 310.5±4.1 ***-rock geochemistry and in situ zircon Hf-O isotopes(δ^(18)O=4.6‰–6.0‰)indicate that the granite porphyry was derived from partial melting of juvenile crust and influenced by subducted oceanic *** isotope compositions of garnets(δ^(18)O=8.0‰–9.0‰)demonstrate that the equilibrated ore fluids

关键词： In situ U-Pb dating Garnet O isotopes Aqishan Pb-Zn deposit Skarn mineralization Southern CAOB