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Boosted Lithium-Ion Transport Kinetics in n-Type Siloxene Anodes Enabled by Selective Nucleophilic Substitution of Phosphorus

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Nano-Micro Letters 2024年第10期16卷 618-637页

作者： Se In Kim Woong-Ju Kim Jin Gu Kang dong-wan Kim School of Civil Environmental and Architectural EngineeringKorea University02841 SeoulSouth Korea Nanophotonics Research Center Korea Institute of Science and Technology02792 SeoulSouth Korea

Doped two-dimensional(2D)materials hold significant promise for advancing many technologies,such as microelectronics,optoelectronics,and energy ***,n-type 2D oxidized Si nanosheets,namely n-type siloxene(n-SX),are employed as Li-ion battery *** thermal evaporation of sodium hypophosphite at 275℃,P atoms are effectively incorporated into siloxene(SX)without compromising its 2D layered morphology and unique Kautsky-type crystal ***,selective nucleophilic substitution occurs,with only Si atoms being replaced by P atoms in the O_(3)≡Si-H *** resulting n-SX possesses two delocalized electrons arising from the presence of two electron donor types:(i)P atoms residing in Si sites and(ii)H *** doping concentrations are varied by controlling the amount of precursors or their mean free *** at 2000 mA g^(-1),the n-SX electrode with the optimized doping concentration(6.7×10^(19) atoms cm^(-3))delivers a capacity of 594 mAh g^(-1) with a 73%capacity retention after 500 *** improvements originate from the enhanced kinetics of charge transport processes,including electronic conduction,charge transfer,and solid-state *** approach proposed herein offers an unprecedented route for engineering SX anodes to boost Li-ion storage.

关键词： Li-ion battery Two-dimensional N-type siloxene Doping mechanism Kinetics

0^(--) hidden-heavy tetraquark states via QCD sum rules

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Chinese Physics C 2024年第9期48卷 50-59页

作者： Bing-dong wan Hong-Tai Xu Department of Physics Liaoning Normal UniversityDalian 116029China Center for Theoretical and Experimental High Energy Physics Liaoning Normal UniversityDalian 116029China

In this study,we evaluated the mass spectra of the prospective 0^(--) hidden-charm and hidden-bottom tetraquark states in molecular configuration via QCD sum *** our calculation,the nonperturbative condensate contributions are considered up to dimension eight in operator product *** is found that there could exist 4possible 0^(--) hidden-charm tetraquark states with masses(4.68±0.07),(4.22±0.09),(4.53±0.09),and(4.26±0.13) *** corresponding hidden-bottom partners are found lying at(11.04±0.10),(10.71±0.12),(11.09±0.10),and(11.82±0.14) GeV,*** possible tetraquark decay modes were analyzed,which are expected to be measured in BESⅢ,BELLEⅡ,and LHCb experiments.

关键词： exotic hadronic states QCD sum rules tetraquarks

Nanoscale“precision strike”:Tumor microenvironment-responsive smart micelles for efficient targeted drug delivery

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Nano Research 2024年第9期17卷 8360-8367页

作者： dong wan Yarong Song Xiujuan Lu Yanfeng Huang Jianxin Zhang Yonghui Liu Yi Liu Jie Pan School of Chemistry Tiangong UniversityTianjin 300387China School of Chemical Engineering and Technology Tiangong UniversityTianjin 300387China

To address the limitations of conventional nanotechnology-based drug delivery systems,this work developed enzyme and reduction dual-responsive polymeric *** micelles were synthesized with copolymers composed of TPGS_(3350)-PVGLIG-DOX(TPD)and FA-SS-DOX(FSD),which endow them with tumor-targeted drug delivery ***_(3350)contributes to extending the circulation of micelles in body,augmenting their accumulation in tumor tissues via the enhanced permeability and retention(EPR)*** localized the tumor site,matrix metalloproteinase 2(MMP2)cleaves the PVGLIG peptide moiety within the micelles,thereby releasing TPGS_(3350)and exposing the targeting ligand of *** approach enables the subsequent internalization of the micelles by tumor cells through folate receptor-mediated *** internalization,the high intracellular concentration of glutathione(GSH)triggers the reduction of the disulfide bond within the FA-SS-DOX,leading to the release of the anticancer-drug doxorubicin(DOX),which promotes apoptosis in the tumor cells and enhances the efficacy of chemotherapy.

关键词： cancer peptide micelle dual-responsive folate

Porously Reduced 2-Dimensional Bi_(2)O_(2)CO_(3) Petals for Strain-Mediated Electrochemical CO_(2) Reduction to HCOOH

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Energy & Environmental Materials 2024年第1期7卷 215-221页

作者： Won Seok Cho Dae Myung Hong wan Jae dong Tae Hyung Lee Chul Jong Yoo donghwa Lee Ho Won Jang Jong-Lam Lee Department of Materials Science and Engineering Pohang University of Science and Technology(POSTECH)Pohang Gyungbuk 37673Korea Department of Materials Science and Engineering Research Institute of Advanced Materials Seoul National UniversitySeoul 08826Korea

Here we introduce bismuth-based catalysts for the efficient electrochemical reduction of CO_(2)to formic acid(HCOOH),which are composed of petal-shaped Bi_(2)O_(2)CO_(3)(BOC)that spontaneously formed from Bi thin film in aqueous carbonate solution at room *** the electrochemical reduction process,the BOC petals transform to reduced BOC(R-BOC)consisting of individual BOC and Bi *** mismatch between both domains induces biaxial strain at the *** functional theory calculations suggest that the tensile strain on the Bi domain stabilizes the*OCHO intermediate,reducing the thermodynamic barrier toward CO_(2)conversion to *** with the thermodynamic benefit and the unique nanoporous petal-shaped morphology,R-BOC petals have a superior Faradaic efficiency of 95.9%at-0.8 V_(RHE)for the electrochemical conversion of CO_(2)to *** work demonstrates that the spontaneously formed binary phases with desirable lattice strain can increase the activity of bismuth catalysts to the CO_(2)reduction reaction;such a strategy can be applicable in design of various electrocatalysts.

关键词： bismuth carbon dioxide reduction formic acid heterointerfaces strain

Discharge mode and particle transport in radio frequency capacitively coupled Ar/O_(2)plasma discharges

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Chinese Physics B 2024年第9期33卷 451-460页

作者： Zhuo-Yao Gao wan dong Chong-Biao Tian Xing-Zhao Jiang Zhong-Ling Dai Yuan-Hong Song Key Laboratory of Materials Modification by Laser Ionand Electron Beams(Ministry of Education)School of PhysicsDalian University of TechnologyDalian 116024China

Simulations are conducted on capacitively coupled Ar/O_(2)mixed gas discharges employing a one-dimensional fluid coupled with an electron Monte Carlo(MC)*** research explores the impact of different O_(2)ratio and pressures on the discharge characteristics of Ar/O_(2)*** a fixed Ar/O_(2)gas ratio,with the increasing pressure,higher ion densities,as well as a slight increase in electron density in the bulk region can be *** discharge remains dominated by the drift-ambipolar(DA)mode,and the flux of O(3P)at the electrode increases with the increasing pressure due to higher background gas density,while the fluxes of O(1D)and Ardecrease due to the pronounced loss *** the increasing proportion of O_(2),a change in the dominant discharge mode from a mode to DA mode can be detected,and the O_(2)-associated charged particle densities are significantly ***,Ar+density shows a trend of increasing and then decreasing,while for neutral fluxes at the electrode,Arflux decreases,and O(3P)flux increases with the reduced Ar gas proportion,while trends in O(1D)flux show slight *** evolution of the densities of the charged particle and the neutral fluxes under different discharge parameters are discussed in detail using the ionization characteristics as well as the transport ***,more comprehensive understanding of Ar/O_(2)discharge characteristics in this work will provide a valuable reference for the industry.

关键词： Ar/O_(2) mixed gas discharges electron dynamics transport of charged and neutral particles

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中国当代跨界舞蹈创作的多要素关联研究

北京舞蹈学院学报 2024年第1期 140-145页

作者：于宛冬星海音乐学院舞蹈学院广州510500

文章对“荷花奖”当代舞蹈作品创作实践中的跨界现象进行研究,旨在探讨中国当代跨界舞蹈创作的多要素关联现象,深入探讨文化交流与跨界融合在舞蹈创作中的实践、影响及作用。在创新过程中,当代舞蹈艺术不断突破传统框架,融入多元文化元... 详细信息

文章对“荷花奖”当代舞蹈作品创作实践中的跨界现象进行研究,旨在探讨中国当代跨界舞蹈创作的多要素关联现象,深入探讨文化交流与跨界融合在舞蹈创作中的实践、影响及作用。在创新过程中,当代舞蹈艺术不断突破传统框架,融入多元文化元素,使研究者认识到创作实践的发展涉及跨文化、跨媒介及跨领域的多元化创作形式。“文化缝隙”形成于创新技巧和新形式在实践活动中的互动过程。这一概念意味着不同领域、学科和文化间的交融与碰撞,往往能产生独特见解和创新成果。在舞蹈创作实践中,它具有提供新视角、推动跨学科交流、激发文化创新的作用。探讨这些问题有助于推动艺术理论的发展、提高对当代舞蹈艺术的理解,并促进艺术创作与文化交流。

关键词：中国当代舞蹈创作实践跨文化交融互动创新

Returning from the afterlife?Sotorasib treatment for advanced KRAS mutant lung cancer:A case report

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World Journal of Clinical Cases 2024年第25期12卷 5805-5813页

作者： Ming-Xing wang Pei Zhu Yue Shi Qing-Ming Sun wan-Hui dong Department of Medical Oncology Lu’an Hospital of Traditional Chinese Medicine Affiliated to Anhui University of Chinese MedicineLu’an 237000Anhui ProvinceChina Department of Medical Oncology Lu’an Hospital of Traditional Chinese MedicineLu’an 237000Anhui ProvinceChina

BACKGROUND Lung cancer is increasing in incidence worldwide,and targeted therapies are developing at a rapid ***,the KRAS specific gene is strongly associated with non-small cell lung cancer(NSCLC).Adult patients with locally advanced or metastatic NSCLC who have tested positive for the KRAS G12C mutation and have progressed after at least one systemic treatment are treated with *** SUMMARY In this study,we report on an advanced NSCLC with a KRAS G12C *** histological diagnosis indicates stage IVB left lung adenocarcinoma with pelvic and bone metastases,identified as *** circulating tumor DNA analysis,it was possible to determine the mutation abundance of the KRAS gene exon 2,c.34G>Tp.G12C,which was 32.3%.The patient was advised to take sotorasib as part of their *** imaging data were compared before and after ***,clinical reassessments and regular serial blood testing were *** found that the patient’s clinical symptoms significantly improved after receiving sotorasib medication,and there were no notable side effects,such as liver toxicity,during the *** Sotorasib has shown promising clinical efficacy in patients with the KRAS G12c mutation and has no apparent toxic side effects.

关键词： Non-small cell lung cancer Sotorasib KRAS G12C Targeted therapy Advanced carcinoma Case report

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矿山地质灾害评估的方法及其发展趋势

世界有色金属 2024年第3期 211-213页

作者：万朝东甘肃煤田地质局一四六队甘肃平凉744000

为了确保矿山生产的安全性和稳定性,矿山地质灾害评估变得尤为重要。本文首先介绍矿山地质灾害评估的意义,然后详细阐述目前常见的评估方法,包括定性评估、定量评估、模型评估和综合评价方法,最后探讨未来评估方法的发展趋势。

关键词：矿山地质灾害评估方法发展趋势

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花青素对植物反射特性的影响及遥感估算:叶片尺度

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光谱学与光谱分析 2024年第1期44卷 275-282页

作者：梁守真隋学艳王猛王菲韩冬锐王国良李洪忠马万栋山东省农业科学院农业信息与经济研究所山东济南250100 中国科学院深圳先进技术研究院先进计算与数字工程研究所广东深圳518055 生态环境部卫星环境应用中心生态保护红线监管中心北京100029

花青素是植物三大色素之一,与植物的生长发育、生长状态以及生长环境状况密切相关,花青素动态变化对生态环境的监测和预警具有重要意义。对叶片光学特性与色素关系的深入理解是估算色素浓度的前提,然而花青素对叶片光学属性的影响并未... 详细信息

花青素是植物三大色素之一,与植物的生长发育、生长状态以及生长环境状况密切相关,花青素动态变化对生态环境的监测和预警具有重要意义。对叶片光学特性与色素关系的深入理解是估算色素浓度的前提,然而花青素对叶片光学属性的影响并未能得到系统地分析,极大地限制了植物花青素的反演和监测。该研究从机理出发,采用包含花青素参数的新一代植物叶片辐射传输模型PROSPECT-D,结合改进的Sobol’算法,获取输入参数协同变化条件下叶片的光学表现,计算模型参数的全局敏感性指数,全面分析花青素对叶片光学属性的影响,探索花青素的光学敏感波谱区间,在此基础上,以地面实测的叶片波谱和色素数据为样本,发展并探讨叶片尺度花青素的遥感反演方法。结果表明,Sobol’全局敏感性分析结果受样本量变化的影响,总敏感性指数在样本数为3 000时达到稳定;花青素主要影响400~689 nm波谱范围的叶片反射特性,叶片对光子的反射能力随花青素含量的增加而降低;叶绿素、类胡萝卜素与花青素对叶片的反射存在协同作用,在467~589 nm波谱区间,花青素对叶片反射的贡献高于其他参数,花青素总敏感性指数在509 nm处最高(86.64%);基于叶绿素、类胡萝卜素对叶片反射能力的贡献程度,花青素的波谱敏感区间可分为三个部分:467~505 nm(花青素、叶绿素、类胡萝卜素共同影响区)、 506~541 nm(花青素、类胡萝卜素影响区)、 542~589 nm(花青素、叶绿素影响区);叶片花青素含量与敏感区间的高光谱窄波段、波谱指数之间存在显著的线性关系。在所有的窄波段中,样本花青素含量与560 nm的叶片反射率的相关性最好,相关系数为0.948,但由于花青素与叶绿素、类胡萝卜素光谱吸收波段重叠,考虑其他色素干扰的波谱指数ARI、 mARI(Sentinel-2波段参考)与花青素表现出了好的相关性(相关系数分别为0.953 2, 0.953 6),但由于波段设置的差异,不同卫星的波谱指数表现并不一致。该研究可为未来更大范围的花青素遥感估算奠定重要的理论基础。

关键词：花青素敏感性分析辐射传输模型遥感