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Polyethylenimine-modified graphene quantum dots promote endothelial cell proliferation

Regenerative Biomaterials 2024年第2期3卷 137-146页

作者： Qirong Xu chen Li Xiangyan Meng Xinghong Duo Yakai Feng School of Chemistry and Chemical Engineering Qinghai University for NationalitiesXining 810007PR China Key Laboratory of National Ethnic Affairs Commission of Resource Chemistry and Ecological Environment Protection on Qinghai-Tibet Plateau Xining 810007PR China institute of Disaster and Emergency Medicine Tianjin UniversityTianjin 300072PR China School of Chemical Engineering and Technology Tianjin UniversityTianjin 300350PR China Key Laboratory of Systems Bioengineering(Ministry of Education) Tianjin UniversityTianjin 300072PR China

Endothelial cell proliferation plays an important role in angiogenesis and treatment of related *** aim of this study was to evaluate the effect of polyethylenimine(PEI)-modified graphene quantum dots(GQDs)gene vectors on endothelial cell *** GQDs-cationic polymer gene vectors were synthesized by amidation reaction,and used to deliver pzNF580 gene to Human umbilical vein endothelial cells(HUVECs)for promoting their *** chemical modification of GQDs can ad-just gene vectors'surface properties and charge distribution,thereby enhancing their interaction with gene molecules,which could effectively compress the pzNF580 *** CCK-8 assay showed that the cell viability was higher than 80%at higher vector concentration(40μg/mL),demonstrating that the GQDs-cationic polymer gene vectors and their gene complex nanoparticles(NPs)having low *** results of the live/dead cell double staining assay were consistent with those of the CCK-8 assay,in which the cell viability of the A-GQDs/pzNF580(94.38±6.39%),C-GQDs-PEI-polylactic acid-co-polyacetic acid(PLGA)/pzNF580(98.65±6.60%)and N-GQDs-PEI-PLGA/pzNF580(90.08±1.60%)groups was significantly higher than that of the Lipofectamine 2000/pzNF580(71.98±3.53%)positive treatment *** results of transfection and western blot experiments showed that the vector significantly enhanced the delivery of plasmid to HUVECs and increased the expression of pzNF580 in *** addition,the gene NPs better promote endothelial cell migration and *** cell migration rate and proliferation ability of C-GQDs-PEI-PLGA/pzNF580 and N-GQDs-PEI-PLGA/pzNF580 treatment groupS were higher than those of Lipofectamine 2000/pDNA treatment *** GQDs possess the potential to serve as efficient gene *** tightly bind gene molecules through charge and other non-covalent interactions,significantly improving the effciency of gene delivery and ensuring the smooth release of genes with

关键词： graphene quantum dots polyethylenimine zNF580 gene endothelial cell proliferation

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A review of solid-state lithium metal batteries through in-situ solidification

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Science China Chemistry 2024年第1期67卷 67-86页

作者： Pan Xu zong-Yao Shuang chen-zi zhao Xue Li Li-zhen Fan Aibing chen Haoting chen Elena Kuzmina Elena Karaseva Vladimir Kolosnitsyn Xiaoyuan zeng Peng Dong Yingjie zhang Mingpei wang Qiang zhang Beijing Key Laboratory of Green Chemical Reaction Engineering and Technology Department of Chemical EngineeringTsinghua UniversityBeijing 100084China National and Local Joint Engineering Laboratory for Lithium-ion Batteries and Materials Preparation Technology Key Laboratory of Advanced Battery Materials of Yunnan ProvinceFaculty of Metallurgical and Energy EngineeringKunming University of Science and TechnologyKunming 650093China Institute of Advanced Materials and Technology University of Science and Technology BeijingBeijing 100083China College of Chemical and Pharmaceutical Engineering Hebei University of Science and TechnologyShijiazhuang 050018China Ordos Carbon Neutral Research and Application Co. Ltd.Ordos City 017010China Ufa Institute of Chemistry UFRC RAS Ufa 450054Russia Institute for Carbon Neutrality Tsinghua UniversityBeijing 100084China Shanxi Research Institute for Clean Energy Tsinghua UniversityTaiyuan 030032China

High-energy-density lithium metal batteries are the next-generation battery systems of choice,and replacing the flammable liquid electrolyte with a polymer solid-state electrolyte is a prominent conduct towards realizing the goal of high-safety and high-specific-energy ***,the inherent intractable problems of poor solid-solid contacts between the electrode/electrolyte and the growth of Li dendrites hinder their practical *** in-situ solidification has demonstrated a variety of advantages in the application of polymer electrolytes and artificial interphase,including the design of integrated polymer electrolytes and asymmetric polymer electrolytes to enhance the compatibility of solid–solid contact and compatibility between various electrolytes,and the construction of artificial interphase between the Li anode and cathode to suppress the formation of Li dendrites and to enhance the high-voltage stability of polymer *** review firstly elaborates the history of in-situ solidification for solid-state batteries,and then focuses on the synthetic methods of solidified ***,the recent progress of in-situ solidification technology from both the design of polymer electrolytes and the construction of artificial interphase is summarized,and the importance of in-situ solidification technology in enhancing safety is ***,prospects,emerging challenges,and practical applications of in-situ solidification are envisioned.

关键词： in-situ solidification polymer electrolyte artificial solid electrolyte interphase rechargeable lithium metal batteries dendrite-free lithium metal anode

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Privacy Preserving Algorithm for Spectrum Sensing in Cognitive Vehicle Networks

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Chinese Journal of Electronics 2024年第1期33卷 30-42页

作者： Hongning LI Tonghui HU Jiexiong chen Xiuqiang wU Qingqi PEI Guangzhou Institute of Technology Xidian University Guangzhou CEPREI Shaanxi Key Laboratory of Blockchain and Secure Computing

The scarcity of spectrum resources fails to meet the increasing throughput demands of vehicular networks. There is an urgent need to maximize the utilization of spectrum bands in mobile networks. To ascertain the availability of spectrum bands, users should engage in wireless channel sensing and collaboration. However, spectrum sensing data always involves users’ privacy, such as their location. This paper first introduces sensing trajectory inference attack in cognitive vehicular networks and then proposes a data confusion-based privacy-preserving algorithm and a cryptonym array-based privacy-preserving aggregation scheme for spectrum sensing in cognitive vehicular networks. Unlike existing methods, the proposed schemes transmit confused data during the aggregation process. This deliberate obfuscation makes it almost impossible to infer users’ location from the transmitted data. The analysis demonstrates the resilience of the proposed schemes against sensing trajectory inference attack.

关键词： Privacy Data privacy wireless sensor networks Authentication Data aggregation Throughput Inference algorithms

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Model Parameters Identification and Backstepping Control of Lower Limb Exoskeleton Based on Enhanced whale Algorithm

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Chinese Journal of Mechanical Engineering 2024年第2期37卷 100-114页

作者： Yan Shi Jiange Kou zhenlei chen Yixuan wang Qing Guo School of Automation Science and Electrical Engineering Beihang UniversityBeijing 100191China School of Aeronautics and Astronautics University of Electronic Science and Technology of ChinaChengdu 611731China

Exoskeletons generally require accurate dynamic models to design the model-based controller conveniently under the human-robot interaction ***,due to unknown model parameters such as the mass,moment of inertia and mechanical size,the dynamic model of exoskeletons is difficult to ***,an enhanced whale optimization algorithm(EwOA)is proposed to identify the exoskeleton model ***,the periodic excitation trajectories are designed by finite Fourier series to input the desired position demand of exoskeletons with mechanical physical *** a backstepping controller based on the identified model is adopted to improve the human-robot wearable comfortable performance under cooperative ***,the proposed Model parameters identification and control are verified by a two-DOF exoskeletons *** knee joint motion achieves a steady-state response after 0.5 ***,the position error of hip joint response is less than 0.03 rad after 0.9 *** addition,the steady-state human-robot interaction torque of the two joints is constrained within 15 N·*** research proposes a whale optimization algorithm to optimize the excitation trajectory and identify model ***,an enhanced mutation strategy is adopted to avoid whale evolution’s unsatisfactory local optimal value.

关键词： Parameter identification Enhanced whale optimization algorithm(EwOA) Backstepping Human-robot interaction Lower limb exoskeleton

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In vivo real-time monitoring delayed administration of M2 macrophages to enhance healing of tendon by NIR-II fluorescence imaging

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Nano Research 2024年第5期17卷 4379-4390页

作者： Yuzhou chen Mo chen chengxuan Yu Huizhu Li Liman Sai Nguyen T.K.Thanh Yueming wang Yan wo Jian zhang Xing Yang Evgenii L.Guryev Andrei V.zvyagin Hao De Min Tang Shiyi chen Yunxia Li Yuefeng Hao Sijia Feng Jun chen Sports Medicine Institute of Fudan University Department of Sports MedicineHuashan HospitalFudan UniversityShanghai 200040China Department of Orthopedic Surgery Xinhua Hospital Affiliated to Shanghai Jiao Tong University School of MedicineShanghai 200092China Department of Bone and Joint Surgery Department of OrthopedicsRenji HospitalSchool of MedicineShanghai Jiao Tong UniversityShanghai 200001China Department of Physics Shanghai Normal UniversityShanghai 200234China Biophysics Group Department of Physics and AstronomyUniversity College LondonLondon WC1E 6BTUK UCL Healthcare Biomagnetic and Nanomaterials Laboratories London W1S 4BSUK Department of Anatomy and Physiology School of MedicineShanghai Jiao Tong UniversityShanghai 200025China Department of Orthopedics Affiliated Suzhou Hospital of Nanjing Medical UniversitySuzhou 215500China Institute of Biology and Biomedicine Lobachevsky State University of Nizhny NovgorodNizhny Novgorod 603950Russia Mathematical Institute University of OxfordOxford OX26GGUK Institute of Natural Sciences School of MathematicsShanghai Jiao Tong UniversityShanghai 200240China

The administration time is a critical but long-neglected point in cell therapy based on macrophages because the incorrect time of macrophage administration could result in diverse outcomes regarding the same macrophage *** this work,the second near-infrared(NIR-II)fluorescence imaging in vivo tracking of M2 macrophages during a pro-healing therapy in the mice model of rotator cuff injury revealed that the behavior of administrated macrophages was influenced by the timing of their *** delayed cell therapy(DCT)group had a longer retention time of injected M2 macrophages in the repairing tissue than that in the immediate cell therapy(ICT)*** Keller-Segel model and histological analysis further demonstrated that DCT altered the chemotaxis of M2 macrophages and improved the healing outcome of the repaired structure in comparison with *** results offer a possible explanation of previous conflicting results on reparative cell therapy and provoke reconsideration of the timing of these therapies.

关键词： macrophage cell therapy NIR-II in vivo imaging delayed therapy tendon healing

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Carrier transport barrier in AlGaN-based deep ultraviolet LEDs on offcut sapphire substrates

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Chinese Optics Letters 2024年第2期22卷 148-158页

作者：陈秋爽陈荔陈聪高歌郭炜叶继春 Ningbo Institute of Materials Technology and Engineering Ningbo 315201China University of Chinese Academy of Sciences Beijing 100049China

AlGaN-based light-emitting diodes(LEDs)on offcut substrates enhance radiative emission via forming carrier localization centers in multiple quantum wells(MQws).This study introduces the carrier transport barrier concept,accessing its impact on the quantum efficiency of LEDs grown on different offcut sapphire substrates.A significantly enhanced internal quantum efficiency(IQE)of 83.1%is obtained from MQws on the 1°offcut sapphire,almost twice that of the controlled 0.2°offcut ***,1°offcut LEDs have higher turn-on voltage and weaker electroluminescence than 0.2°*** calculations demonstrate the existence of a potential barrier on the current path around the step-induced Ga-rich ***-rich stripes reduce the turn-on voltage but restrict sufficient driving current,impacting LED performance.

关键词： carrier localization step-bunching potential barrier offcut substrate DUV LEDs

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Pairing nitroxyl radical and phenazine with electron-withdrawing/-donating substituents in “water-in-ionic liquid” for high-voltage aqueous redox flow batteries

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Green Energy & Environment 2024年第4期9卷 713-722页

作者： zhifeng Huang Rolf Hempelmann Yiqiong zhang Li Tao Ruiyong chen Transfercenter Sustainable Electrochemistry Saarland University and KIST Europe66125SaarbruckenGermany State Key Laboratory of Chem/Bio-Sensing and Chemometrics College of Chemistry and Chemical Engineering Hunan University Changsha410082HunanChina College of Materials Science and Engineering Changsha University of Science and Technology Changsha410114HunanChina Materials Innovation Factory Department of ChemistryUniversity of LiverpoolLiverpoolL697ZDUnited Kingdom

Aqueous redox-active organic materials-base electrolytes are sustainable alternatives to vanadium-based electrolyte for redoxﬂow batteries(RFBs)due to the advantages of high ionic conductivity,environmentally benign,safety and low ***,the underexplored redox properties of organic materials and the narrow thermodynamic electrolysis window of water(1.23 V)hinder their wide ***,seeking suitable organic redox couples and aqueous electrolytes with a high output voltage is highly suggested for advancing the aqueous organic *** this work,the functionalized phenazine and nitroxyl radical with electron-donating and electron-withdrawing group exhibit redox potential of-0.88 V and 0.78 V ***,respectively,in“water-in-ionic liquid”supporting *** spectra reveal that the activity of water is largely suppressed in“water-in-ionic liquid”due to the enhanced hydrogen bond interactions between ionic liquid and water,enabling an electrochemical stability window above 3 V.“water-in-ionic liquid”supporting electrolytes help to shift redox potential of nitroxyl radical and enable the redox activity of functionalized *** assembled aqueous RFB allows a theoretical cell voltage of 1.66 V and shows a practical discharge voltage of 1.5 V in the“water-in-ionic liquid”***,capacity retention of 99.91%per cycle is achieved over 500 charge/discharge cycles.A power density of 112 mw cm^(-2) is obtained at a current density of 30 mA cm^(-2).This work highlights the importance of rationally combining supporting electrolytes and organic molecules to achieve high-voltage aqueous RFBs.

关键词： Aqueous redoxﬂow batteries water-in-ionic liquid electrolytes High-voltage aqueous batteries Organic redox-active materials

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Microstructure development of Ti scaffold by laser powder bed fusion with chemical polishing and its mechanical properties,biocompatibility

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Biosurface and Biotribology 2024年第2期10卷 52-62页

作者： Changfu Lu Jing chen Teng Ma Yuxin chen Da zeng Yiliang Gan Youwen Yang Double Medical Technology Inc. XiamenChina Institute of Additive Manufacturing Jiangxi University of Science and TechnologyNanchangChina Key Laboratory of Construction Hydraulic Robots of Anhui Higher Education Institutes Tongling UniversityTonglingChina College of Engineering and Applied Science Nanjing UniversityNanjingChina

Titanium(Ti)dental scaffolds are widely used in dental prosthetics due to their excellent mechanical properties and ***,conventional Ti scaffolds manufactured through machining often do not fit perfectly with the bone defect *** powder bed fusion(LPBF)technology enables the personalised manufacturing of custom-made Ti scaffolds.A custom-made Ti scaffold was prepared using LPBF and its surface roughness was improved through chemical *** enhance the surface roughness,a nitric acid mixed solution with a specific composition of HF:HNO_(3):C_(3)H_(6)O_(3)=2:2:3 was *** polishing mechanism was investigated by adjusting the F/Ti ratio to control the formation and dissolution of the oxide *** a result,the surface of the Ti scaffold after polishing exhibited a smooth and flat appearance compared to the LPBF part,with a reduced surface roughness(Ra)of 1.23±0.19μ*** custom-made Ti scaffold also demonstrated favourable mechanical properties,with a bending strength of 335.18±33.62 MPa and stiffness of 2.13±0.21 ***,in vitro cell tests confirmed the excellent biocompatibility of the custom-made Ti *** authors present a feasible strategy for the further clinical application of custom-made Ti scaffolds,offering enhanced surface properties and addressing the limitations of conventional machining methods.

关键词： additive manufacturing dental material property surface roughness

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MMP-9 deficiency accelerates the progress of periodontitis

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Genes & Diseases 2024年第5期11卷 117-121页

作者： Chun-Yan wan Yixin Yin Xiaoyan Li Meng Meng Liu Graham Goldman Li-An wu Feng wang Dao-Shu Luo zhuo chen wen-An Xu Stephen chen Mary MacDougall Merry L.Lindsey zhi chen Shuo chen Department of Endodontics The Affiliated Hospital of Qingdao UniversitySchool of StomatologyQingdao UniversityQingdaoShandong 266003China Department of Developmental Dentistry School of DentistryThe University of Texas Health Science Center at San AntonioSan AntonioTX 78229USA Oral Implantology Center Jinan Stomatological HospitalJinanShandong 250001China Department of Endodontics School and Hospital of StomatologyCheeloo College of MedicineShandong Key Laboratory of Oral Tissue RegenerationShandong Engineering Laboratory for Dental Materials and Oral Tissue RegenerationShandong UniversityJinanShandong 250012China Department of Pediatric Dentistry School of StomatologyThe Fourth Military Medical UniversityXi’anShaanxi 710032China Laboratory of Clinical Applied Anatomy Department of Human AnatomySchool of Basic Medical SciencesFujian Medical UniversityFuzhouFujian 350108China Key Laboratory for Oral Biomedical Research of zhejiang Province Affiliated Hospital of StomatologyMedical CollegeZhejiang UniversityHangzhouZhejiang 310027China Department of Stomatology Nanfang HospitalSouthern Medical UniversityGuangzhouGuangdong 510515China UBC Faculty of Dentistry University of British ColumbiaVancouverBC V6T 1Z3Canada School of Graduate Studies and Research Meharry Medical College and Research BiologistResearch Service Nashville VA Medical CenterNashvilleTN 37208USA State Key Laboratory Breeding Base of Basic Science of Stomatology(Hubei-MOST) Key Laboratory for Oral Biomedicine of Ministry of Education(KLOBM)School and Hospital of StomatologyWuhan UniversityWuhanHubei 430079China

Periodontitis is a chronic inflammatory disease caused by periodontopathic bacteria that affects periodontal support tissues.1 If left untreated,it results in loss of periodontal attachment and alveolar bone *** one-half of adults in the United States older than 30 years have periodontal disease.2 Though the disease is initiated by bacterial infection,it activates host defense systems that eventually lead to the degradation of the *** periodontitis,the disease progress involves further production of pro-inflammatory mediators such as cytokines,proteolytic enzymes like matrix metalloproteinases(MMPs),and their inhibitors.

关键词： period eventually untreated

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Comprehensive,Continuous,and Vertical Measurements of Seawater Constituents with Triple-Field-of-View High-Spectral-Resolution Lidar

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Research 2024年第2期2023卷 191-201页

作者： Kai zhang Yatong chen Hongkai zhao zhongping Lee Emmanuel Boss Iwona Stachlewska Davide Dionisi Cedric Jamet Paolo D.Girolamo Aleksey Malinka chengchong Jiang Hongda wu Lingyun wu Feitong chen Xiaolei zhu Nanchao wang Chuxiao chen Qun Liu Lan wu Yudi zhou weibiao chen Dong Liu Ningbo Research Institute State Key Laboratory of Modern Optical InstrumentationCollege of Optical Science and EngineeringZhejiang UniversityHangzhou 310027China zJU-Hangzhou Global Scientific and Technological lnnovation Center Zhejang UniversityHangzhou 311200China Donghai Laboratory.zhoushan 316021 China State Key Lab of Marine Environmental Science College of Ocean and Earth SciencesXiamen UniversityXiamen 361102China School of Marine Sciences University of MaineOronoME 04469-5741USA Faculty of Physics University of WarsawWarsaw 02093Poland institute of Marine Sciences Italian National Research CouncilRome 00133Italy Universitédu Littoral Cote d'Opale CNRSUniv.LilleIRDUMR 8187-LOG-Laboratoire d'Oceanologie et de GéosciencesWimereux F-6293 Francen Institute Scuola di Ingegneria Universita della BasilicataPotenza 85100Italy Institute of Physics National Academy of Sciences of BelarusMinsk 220072Belarus Key Laboratory of Space Laser Communication and Detection Technology Shanghai lnstitute of Optics and Fine MechanicsChinese Academy of SciencesShanghai 201800China Inteligent Optics&Photonics Research Center Jiaxing Research Institute Zhejiang UniversityJiaxing 314000China Jiaxing Key Laboratory of Photonic Sensing&Intelligent Imaging Jiaxing 314000China

Measuring the characteristics of seawater constituent is in great demand for studies of marine ecosystems and ***,existing techniques based on remote sensing or in situ samplings present various tradeoffs with regard to the diversity,synchronism,temporal-spatial resolution,and depth-resolved capacity of their data ***,we demonstrate a novel oceanic triple-field-of-view(FOV)high-spectral-resolution lidar(HSRL)with an iterative retrieval *** technique provides,for the first time,comprehensive,continuous,and vertical measurements of seawater absorption coefficient,scattering coefficient,and slope of particle size distribution,which are validated by simulations and field ***,it depicts valuable application potentials in the accuracy improvement of seawater classification and the continuous estimation of depth-resolved particulate organic carbon *** triple-FOV HSRL with high performance could greatly increase the knowledge of seawater constituents and promote the understanding of marine ecosystems and biogeochemistry.

关键词： lidar Vertical seawater

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