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High temperature superconductor Na2B2H stabilized by hydrogen intercalation under ambient pressure

Science China(Physics,Mechanics & Astronomy) 2024年第11期Mechanics & Astronomy) .卷 145-152页

作者： wendi Zhao Defang Duan Zhengtao Liu Zihao huo Shumin Guo Decheng An Maosheng Miao Tian Cui State Key Laboratory of Superhard Materials Key Laboratory of Material Simulation Methods & Software of Ministry of Education College of Physics Jilin University Department of Chemistry and Biochemistry California State University Department of Earth Science University of California institute of High Pressure Physics School of Physical Science and Technology Ningbo University

Hydrogenated metal borides have attracted much attention due to their potential high-temperature superconductivity. Here, we propose a new strategy for hydrogen intercalation tuning the stability and superconductivity of the boron honeycomb sublattice,and predict an unprecedented layered compound Na2B2H, w.ich hosts excellent superconductivity. Strikingly, the superconducting transition temperature（Tc） of Na2B2H reaches 42 K at ambient pressure. The Tcvalue can be further increase to 63 K under 5% biaxial tensile strain. The excellent superconductivity originates from the strong electron-phonon coupling between theσ-bonding bands near the Fermi level and the B-B stretching optical E modes. The interstitial electron localization and crystal orbitals of the H-intercalated Na ion layer well match the boron honeycomb lattice and act as a chemical template to stabilize the B layer. Furthermore, the introduction of hydrogen tuned the Fermi level, and the coupling vibration of Na and H ions effectively enhanced the dynamic stability of the structure. Na2B2H represents a new family of layered high-temperature superconductors,and the strategy of stabilizing the honeycomb boron sublattice via chemical template hosts great potential for application to more layered compounds.

关键词： superconductivity hydrogenation metal borides electron-phonon coupling

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Relationship between postoperative rehabilitation style, gastrointestinal function, and inflammatory factor levels in children with intussusception

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world Journal of Gastrointestinal Surgery 2024年第8期16卷 2640-2648页

作者： Xue-Yan w.i Hong-Chang huo Xin Li Su-Li Sun Jun Zhang Department of Outpatient Shijiazhuang Maternal and Child Health HospitalShijiazhuang 050090Hebei ProvinceChina Department of Pediatric Surgery Shijiazhuang Maternal and Child Health HospitalShijiazhuang 050090Hebei ProvinceChina Department of Nursing Shijiazhuang Maternal and Child Health HospitalShijiazhuang 050090Hebei ProvinceChina

BACKGROUND intussusception occurs in children and progresses *** not treated in time,it may lead to secondary complications such as intestinal perforation,w.ich affect the quality of life and health of *** is the most common clinical treatment and has a good ***,the postoperative prognosis of children with intussusception has a correlation with the postoperative rehabilitation ***,in this study,we explored the relationship between postopera-tive rehabilitation,gastrointestinal function,and the expression of inflammatory factors in children with *** medical records of 18 children who were admitted to our hospital for intussusception surgery between October 2022 and May 2024 were retrospectively *** patients were divided into the routine nursing group(n=6)and rehabilitation training group(n=12)according to the postoperative rehabilitation *** general data,gastrointestinal function,and inflammatory factor levels of the two groups were statistically *** correlation analysis of gastrointestinal function,inflammatory factors,and postoperative rehabil-itation was *** we found no significant intergroup differences in sex,age,or disease course(P>0.05).The times to first defecation,bowel sound recovery,and anal exhaust were shorter and inflammatory factor levels were lower in the rehabilitation training group than in the routine nursing group(Pion analysis showed that gastrin and motilin levels were positively correlated with postoperative rehabilitation(Pinterleukin(iL)-2,iL-4,iL-6,iL-10,high-sensitivity C-reactive protein,and tumor necrosis factor-αlevels were negatively correlated with postoperative rehabilitation(Pintestinal function was positively correlated(Pinflammatory factors were negatively correlated with postoperative recovery time(PiON we found a positive correlation between gastrointe

关键词： Children with intussusception Postoperative rehabilitation mode Gastrointestinal function inflammatory factors

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Chiral multiple-resonance thermally activated delayed fluorescence materials based on chiral spiro-axis skeleton for efficient circularly polarized electroluminescence

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Science China Chemistry 2024年第7期67卷 2257-2264页

作者： Shi-Quan Song Xiao Han Zhong-Zhong huo Ching-Fai Yip Xian-Fang Hong Meng-Ning Ding You-Xuan Zheng State Key Laboratory of Coordination Chemistry Jiangsu Key Laboratory of Advanced Organic MaterialsSchool of Chemistry and Chemical EngineeringNanjing UniversityNanjing 210023China Key Laboratory of Mesoscopic Chemistry of Ministry of Education School of Chemistry and Chemical EngineeringNanjing UniversityNanjing 210023China

Chiral luminescence materials have potential applications in the field of three-dimensional displays due to their circularly polarized luminescence(CPL)***,the further development of circularly polarized organic light-emitting diodes(CP-OLEDs)needs to meet the requirements of high efficiency,high color purity,low cost,and high dissymmetry factor(gPLor gEL),chiral multiple resonance thermally activated delayed fluorescence(MR-TADF)materials are considered as candidates in these ***,based on a pair of chiral spirofluorene precursors,two pairs of high-performance chiral MR-TADF emitters((R/S)-p-Spiro-DtBuCzB and(R/S)-m-Spiro-DtBuCzB)are developed,w.ich exhibit strong emissions peaking at 491 and 502 nm in toluene with full-width at half-maximum values of 25 and 33 nm,*** addition,small singlet–triplet energy gaps of 0.15 and 0.10 eV with high absolute photoluminescence efficiencies of 95.0%and 96.7%are observed for p-Spiro-DtBuCzB and m-Spiro-DtBuCzB molecules,*** based on p-Spiro-DtBuCzB and m-Spiro-DtBuCzB display high maximum external quantum efficiencies of 29.6%and 33.8%,*** importantly,CP-OLEDs present symmetric circularly polarized electroluminescence spectra with|gEL|factors of 3.36×10^(-4)and 7.66×10^(-4)for devices based on(R/S)-p-Spiro-DtBuCzB and(R/S)-m-Spiro-DtBuCzB enantiomers,respectively.

关键词： chiral spiro-axis skeleton-based material multiple resonance thermally activated delayed fluorescence circularly polarized electroluminescence dissymmetry factor external quantum efficiency

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A nitric oxide-triggered hydrolysis reaction to construct controlled self-assemblies with complex topologies

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Science China Chemistry 2024年第4期67卷 1289-1299页

作者： wenzhuo Chen Yuping Tang Shuai Chen Zipei Chen Jia He Hongbin huo Juan Zhang Jiajia Li Fei Yan w.i Tian Laboratory of Shaanxi Administration of Traditional Chinese Medicine for TCM Compatibility Shaanxi Key Laboratory of Chinese Medicine Fundamentals and New Drugs ResearchCollege of PharmacyShaanxi University of Chinese MedicineXianyang 712046China Shaanxi Key Laboratory of Macromolecular Science and Technology Xi’an Key Laboratory of Hybrid Luminescent Materials and Photonic DeviceMOE Key Laboratory of Material Physics and Chemistry under Extraordinary ConditionsSchool of Chemistry and Chemical EngineeringNorthwestern Polytechnical UniversityXi’an 710072China Department of Polymeric Materials School of Materials Science and EngineeringTongji UniversityShanghai 201804China

Hydrolysis reactions are capable of directing the non-equilibrium assembly of biomolecular scaffolds to realize sophisticated structures and functions in natural ***,utilizing the proper hydrolysis reactions to construct controlled assemblies with complex topologies is still an arduous challenge in artificial systems and needs to be ***,we report a nitric oxide(NO)-triggered slow hydrolysis strategy for the controlled construction of biomimetic supramolecular toroids(STs),thus realizing their visualization of intermediate structures and regulation of geometry *** presented protocol harnesses hydrolysis reactions to control of non-equilibrium self-assembly processes for the construction of self-assemblies with complex topologies successfully,w.ich sheds light on how the hydrolysis reaction rate can modulate the kinetic pathway of assembly,thus realizing the artificial establishment of bio-inspired hierarchical structures.

关键词： supramolecular toroids controlled self-assembly nitic oxide-triggered hydrolysis pathway regulation

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Artificial intelligence Meets Flexible Sensors:Emerging Smart Flexible Sensing Systems Driven by Machine Learning and Artificial Synapses

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Nano-Micro Letters 2024年第1期16卷 235-273页

作者： Tianming Sun Bin Feng Jinpeng huo Yu Xiao wengan wang Jin Peng Zehua Li Chengjie Du wenxian wang Guisheng Zou Lei Liu Department of Mechanical Engineering State Key Laboratory of Tribology in Advanced EquipmentKey Laboratory for Advanced Manufacturing by Materials Processing TechnologyMinistry of Education of PR ChinaTsinghua UniversityBeijing 100084People’s Republic of China College of Materials Science and Engineering Shanxi ProvinceTaiyuan University of TechnologyTaiyuan 030024People’s Republic of China

The recent wave of the artificial intelligence(Ai)revolution has aroused unprecedented interest in the intelligentialize of human *** an essential component that bridges the physical world and digital signals,flexible sensors are evolving from a single sensing element to a smarter system,w.ich is capable of highly efficient acquisition,analysis,and even perception of vast,multifaceted *** challenging from a manual perspective,the development of intelligent flexible sensing has been remarkably facilitated owing to the rapid advances of brain-inspired Ai innovations from both the algorithm(machine learning)and the framework(artificial synapses)*** review presents the recent progress of the emerging Ai-driven,intelligent flexible sensing *** basic concept of machine learning and artificial synapses are *** new enabling features induced by the fusion of Ai and flexible sensing are comprehensively reviewed,w.ich significantly advances the applications such as flexible sensory systems,soft/humanoid robotics,and human activity *** two of the most profound innovations in the twenty-first century,the deep incorporation of flexible sensing and Ai technology holds tremendous potential for creating a smarter world for human beings.

关键词： Flexible electronics wearable electronics Neuromorphic Memristor Deep learning

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Effects of ulinastatin combined with dexmedetomidine on cognitive dysfunction and emergence agitation in elderly patients who underwent total hip arthroplasty

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world Journal of Psychiatry 2024年第1期14卷 26-35页

作者： Qi-Fan huo Li-Juan Zhu Jian-w.i Guo Yan-An Jiang Jing Zhao Department of Anesthesiology Shaanxi Provincial People’s HospitalXi’an 710068Shaanxi ProvinceChina

BACKGROUND with the continuous growth of the modern elderly population,the risk of fracture *** fracture is a common type of fracture in older *** hip arthroplasty(THA)has significant advantages in relieving chronic pain and promoting the recovery of hip joint *** To investigate the effect of ulinastatin combined with dexmedetomidine(Dex)on the incidences of postoperative cognitive dysfunction(POCD)and emergence agitation in elderly patients who underwent *** A total of 397 patients who underwent THA from February 2019 to August *** conducted a three-year retrospective cohort study in Shaanxi Provincial People’s *** demographic data were obtained from the electronic medical record *** collected preoperative,intraoperative,and postoperative *** hundred twenty-nine patients who were administered Dex during the operation were included in the Dex *** hundred fifty patients who were intravenously injected with ulinastatin 15 min before anesthesia induction were included in the ulinastatin *** hundred eighteen patients who were administered ulinastatin combined with Dex during the operation were included in the Dex+ulinastatin *** patients’perioperative conditions,hemodynamic indexes,postoperative Mini-Mental State Examination(MMSE)scores,Ramsay score,incidence of POCD,and serum inflammatory cytokines were *** There was a significant difference in the 24 h visual analogue scale score among the three groups,and the score in the Dex+ulinastatin group was the lowest(Pwith the Dex and ulinastatin group,the MMSE scores of the Dex+ulinastatin group were significantly increased at 1 and 7 d after the operation(all Pwith those in the Dex and ulinastatin groups,incidence of POCD,levels of serum inflammatory cytokines in the Dex+ulinastatin group were significantly decreased at 1 and 7 d after the operation(all P<0.05).The observer’s assessment of th

关键词： Ulinastatin Dexmedetomidine Postoperative cognitive dysfunction inflammatory cytokines Total hip arthroplasty

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insights from TARGET-seq:inflammation drives TP53-mediated clonal evolution

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The innovation 2024年第2期5卷 7-8页

作者： Yeqian Zhao wenxuan huo Yue Liang Xiaodong Mo Shanshan Pei Yanmin Zhao Bone Marrow Transplantation Center the First Affiliated HospitalZhejiang University School of MedicineHangzhou 310009China Liangzhu Laboratory Zhejiang University Medical CenterHangzhou 311121China institute of Hematology Zhejiang UniversityHangzhou 311121China Peking University People’s Hospital Peking University Institute of HematologyNational Clinical Research Center for Hematologic DiseaseBeijing 100044China

Approximately 10%–20%myeloproliferative neoplasms(MPNs)can progress into blast-phase MPNs,also termed secondary acute myeloid leukemias(sAMLs),presenting dismal *** exhibits a distinctive clinical and pathological profile compared to de novo AML,marked by a higher incidence of erythroid leukemias and reduced responsive to conventional chemotherapies,resulting in a median survival of approximately 6 ***53 alterations are prevalent adverse events in leukemic transformation(LT),occurring in around one-third of sAML subjects.

关键词： TP53 neoplasms alterations

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Elastic three-dimensional phononic topological insulators with Dirac hierarchy

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Science China(Physics,Mechanics & Astronomy) 2024年第5期67卷 54-62页

作者： Shao-Yong huo Qiu-Shuang Yang Jiu-Jiu Chen Hong-Kang Li Long-Chao Yao Fu-Chun He Chun-Ming Fu College of Mechanical Engineering University of South ChinaHengyang 421001China State Key Laboratory of Advanced Design and Manufacturing for Vehicle Body College of Mechanical and Vehicle EngineeringHunan UniversityChangsha 410082China

Three-dimensional(3D)phononic topological insulators(Tis)featuring two-dimensional(2D)surface states and one-dimensional(1D)hinge states have opened up a new route for multi-dimensional robust wave transport,providing unprecedented methods for integrated acoustic sensors and energy harvesting ***,aiming at the elastic 3D phononic Ti with gapless surface states and hinge states,the realization of elastic 3D phononic Tis with gapless surface states and hinge states is a significant challenge due to the complicated multi-mode polarization of elastic waves in 3D *** this study,we demonstrate an elastic 3D phononic Ti with a Dirac hierarchy by elaborately operating the corresponding spatial symmetries of the chiral honeycomb ***,a 3D double Dirac cone of elastic wave can be achieved by doubling the lattice along the outof-plane direction to fold two iso-frequency weyl *** topological phase transitions and 2D gapless two-fold Dirac surface states of elastic wave are realized by breaking the half-lattice spatial translation ***,based on the Brillouin zone folding along the in-plane direction,the 2D gapless two-fold surface Dirac cones are folded into four-fold surface Dirac ***,by inducing the relative radius of adjacent holes to break the in-plane spatial inversion symmetry,the fourfold surface Dirac cones are gapped and associated with a surface state inversion,in w.ich the gapless 1D hinge Dirac dispersion is *** research offers a route for engineering the hierarchies of Tis in 3D elastic wave systems and provides new possibilities for designing 3D ultrasonic devices with unconventional functions.

关键词： Dirac topological hierarchy

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Ascending phase of solar cycle 25 tilts the current El Ni?o-Southern oscillation transition

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Atmospheric and Oceanic Science Letters 2024年第1期 36-40页

作者： wenjuan huo Ziniu Xiao Liang Zhao Fei Liu GEOMAR Helmholtz Centre for Ocean Research State Key Laboratory of Numerical Modeling for Atmospheric Sciences and Geophysical Fluid Dynamics Institute of Atmospheric PhysicsChinese Academy of Sciences School of Atmospheric Sciences Sun Yat-Sen UniversityKey Laboratory of Tropical Atmosphere-Ocean SystemMinistry of Educationand Southern Marine Science and Engineering Guangdong Laboratory

自2020年初夏,赤道太平洋地区出现拉尼娜现象并持续两年半多(以下简称2020拉尼娜),对其未来演变的预测引起了很多关注,考虑到11年太阳周期活动对热带太平洋SST异常可能存在锁相影响,本研究分析了当前太阳活动周(即第25太阳周(SC25))对... 详细信息

自2020年初夏,赤道太平洋地区出现拉尼娜现象并持续两年半多(以下简称2020拉尼娜),对其未来演变的预测引起了很多关注,考虑到11年太阳周期活动对热带太平洋SST异常可能存在锁相影响,本研究分析了当前太阳活动周(即第25太阳周(SC25))对目前热带太平洋ENSO现象未来演变的调节作用,基于历史太阳周的统计特征,作者对第25太阳周达到其最大值的时间提出三种可能的情景,并讨论了不同情景下的太阳活动对未来两年ENSO演变的可能影响,第25太阳周的持续上升阶段在一定程度上抑制了当前2023厄尔尼诺现象发展为超级事件.

关键词：厄尔尼诺-南方涛动太阳活动热带太平洋位相转变预测三重拉尼娜现象

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institutional inclusiveness

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China weekly 2024年第9期 37-39页

作者： huo Siyi 不详

More institutional reform and openness are required in achieving high-quality economic development,says Tsinghua expert On July 18,the 20th Central Committeeof the Communist Party of China(CPC)concluded its third plenary session in Beijing,issuing a Communiquéthat describes opening up as"a defining feature of Chinese modernization."The resolution adopted at the session focuses on further deepening reform comprehensively to advance Chinese modernization and renewing the country's plan for opening up.

关键词： deepening modernization session

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