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Mono-dispersed Ag nanoparticles decorated graphitic carbon nitride:An excellent lubricating additive as PPESK composite film

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Friction 2022年第5期10卷 717-731页

作者： Beibei CHEN Mengjie zhang Kan zhang Zhe DONg Jiaye LI gai ZHAO School of Materials and Science Engineering Institute for Advanced MaterialsJiangsu UniversityZhenjiang 212013China State Key Laboratory of Mechanics and Control of Mechanical Structures Nanjing University of Aeronautics and AstronauticsNanjing 210016China

Studies show that two dimensional(2D)nanomaterial and its hybrid have a great promise in tribology for the special laminar ***,the majority of performed investigations about 2D graphitic carbon nitride(g-C_(3)N_(4))nanosheets are most focused on energy storage,catalysis,adsorption,rarely *** the present study,g-C_(3)N_(4) supporting mono-dispersed Ag nanoparticle hybrid(g-C_(3)N_(4)/Ag)is prepared,and its microstructure and chemical composition are *** specifically,the tribological performance as the lubricating additive of poly phthalazinone ether sulfone ketone(PPESK)composite is investigated using the ball-on-disc friction ***,the corresponding enhancement mechanism is well proposed based on the experimental analysis and theoretical *** results show that Ag nanoparticles with a size of about 10-20 nm are homogeneously anchored on g-C_(3)N_(4) nanosheets,favoring for good compatibility between g-C_(3)N_(4)/Ag and *** is found that when 0.3 wt%of g-C_(3)N_(4)/Ag is added to PPESK,the friction coefficient and wear rate of PPESK decrease by 68.9%and 97.1%,*** reductions are mainly attributed to the synergistic self-lubricating effect of Ag nanoparticles and g-C_(3)N_(4) nanosheet,the formation of transfer film,as well as the limited effect of g-C_(3)N_(4)/Ag on the shear deformation of PPESK composite ***,it is found that the proposed g-C_(3)N_(4)/Ag-PPESK composite still keeps reasonable friction-reducing and wear-resistant properties under heavy loads and high rotating *** present study demonstrates that the proposed g-C_(3)N_(4)/Ag hybrid is an excellent lubricating additive for polymer composites.

关键词： g-C_(3)N_(4)/Ag hybrid poly phthalazine ether sulfone ketone(PPESK)composite film friction wear theoretical simulation

Long‐life lithium batteries enabled by a pseudo‐oversaturated electrolyte

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Carbon Energy 2024年第4期6卷 115-127页

作者： Youchun Yu Simeng wang Juyan zhang weiwei Qian Nana zhang guangjie Shao Haiyan Bian Yuwen Liu Lan zhang Hebei Key Laboratory of Applied Chemistry College of Environmental and Chemical EngineeringYanshan UniversityQinhuangdaoChina Beijing Key Laboratory of Ionic Liquids Clean Process CAS Key Laboratory of Green Process and EngineeringInstitute of Process EngineeringChinese Academy of SciencesBeijingChina Haike group Research Institute of Innovation&Technology DongyingChina Langfang green Industrial Technology Center LangfangChina

The specific energy of Li metal batteries(LMBs)can be improved by using high‐voltage cathode materials;however,achieving long‐term stable cycling performance in the corresponding system is particularly challenging for the liquid ***,a novel pseudo‐oversaturated electrolyte(POSE)is prepared by introducing 1,1,2,2‐tetrafluoroethyl‐2,2,3,3‐tetrafluoropropyl ether(TTE)to adjust the coordination structure between diglyme(g2)and lithium bis(trifluoromethanesulfonyl)imide(LiTFSI).Surprisingly,although TTE shows little solubility to LiTFSI,the molar ratio between LiTFSI and g2 in the POSE can be increased to 1:1,which is much higher than that of the saturation state,1:*** and experimental results prove that TTE promotes closer contact of the g2 molecular with Li^(+)in the ***,it also participates in the formation of electrolyte/electrode *** electrolyte shows outstanding compatibility with both the Li metal anode and typical high‐voltage ***||Li symmetric cells show a long life of more than 2000 h at 1 mA cm^(−2),1 mAh cm^(−2).In the meantime,Li||LiNi_(0.8)Co_(0.1)Mn_(0.1)O_(2)(NCM811)cell with the POSE shows a high reversible capacity of 134.8 mAh g^(−1 )after 900 cycles at 4.5 V,1 C *** concept of POSE can provide new insight into the Li^(+)solvation structure and in the design of advanced electrolytes for LMBs.

关键词： high voltage lithium metal batteries pseudo‐oversaturated electrolyte solid electrolyte interphases(SEI) solvation structure

Enrichment and reconfiguration of titanium-bearing phase in vortex smelting reduction process of vanadium-titanium magnetite

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Journal of Iron and Steel Research International 2024年第7期31卷 1582-1589页

作者： Yong-chao Han Zhi-he Dou Rui zhang Ting-an zhang Shuai Fang Key Laboratory for Ecological Metallurgy of Multimetallic Ores(Ministry of Education) Shenyang 110819LiaoningChina School of Metallurgy Northeastern UniversityShenyang 110819LiaoningChina

To comprehensively utilize the low-iron high-vanadium-titanium magnetite,a new method of vortex smelting reduction of vanadium-titanium magnetite was proposed,and the enrichment and reconstitution regularity of Ti-bearing phases in the slag was investigated through X-ray fluorescence spectrometry,X-ray photoelectron spectroscopy,X-ray diffraction analysis,and optical *** phase diagram revealed that the preferential crystallization of MgTi_(2)O_(5) can be achieved by adjusting the CaO,MgO,and TiO_(2) contents of *** predominant Ti-bearing phases in the slag obtained from the reduction process are MgxTi_(3_x)O_(5)(0≤x≤1)and CaTiO_(3).FeTiO_(3) is present at carbon-iron ratio(CR)=1.3,while MgTi_(2)O4 and TiC are formed at CR=*** enrichment of TiO_(2) in the slag increases first and then decreases as the CR increases,and at CR=1.1,the enrichment of TiO_(2) in the slag reaches 51.3 wt.%.Additionally,the concentrations of MgxTi_(3_x)O_(5)(0≤x≤1)and CaTiO_(3) in the slag,along with the grain width of MgxTi_(3_x)O_(5)(0≤x≤1),decrease with the increase in CR.

关键词： Vanadium-titanium magnetite Vortex smelting reduction Phase reconfiguration TiO_(2)enrichment

Construction and properties of venlafaxine hydrochloride sustained release system based on hollow mesoporous silica microspheres

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Particuology 2024年第3期86卷 205-210页

作者： Chenjing Liang Lingling Shi Zhengguo Chen Lan Zhou Zhaoxia zhang guoqing zhang School of Materials Science and Engineering Zhejiang Sci-tech UniversityHangzhouChina College of Textile Science and Engineering Zhejiang Sci-tech UniversityHangzhouChina Zhejiang Provincial Innovation Center of Advanced Textile Technology ShaoxingChina

The aim of this work is to develop a venlafaxine hydrochloride sustained release system based on hollow mesoporous silica microspheres(HMSMs).HMSMs were innovatively prepared with tetraethyl silicate(TEOS)as the precursor and volatile n-heptane as a soft *** obtained HMSMs show a well-defined hollow structure with an average size of 967 nm and pore volume of 0.85 cm^(3)/g,implying it is a potential drug ***,venlafaxine hydrochloride(VF)was absorbed in the HMSMs with a content of 37.67% or *** sustained release effect is further measured by the dissolution in-strument at 37℃ and 50 rpm in ultrapure *** results showed that the HMSMs/VF system shows good sustained release properties compared with sustained release tablets with hydroxypropyl meth-ylcellulose as the main *** HMSMs sustained release system appears to be a promising candidate for a sustained drug release.

关键词： Hollowmesoporous silica microspheres(HMSMs) Venlafaxine hydrochloride Drug loading Sustained release

wAEAS:An Optimization Scheme of EAS Scheduler for wearable Applications

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Tsinghua Science and Technology 2021年第1期26卷 72-84页

作者： Zhan zhang Xiang Cong wei Feng Haipeng zhang guodong Fu Jianyun Chen the School of Computer Science and Technology Harbin Institute of TechnologyHarbin 150001China Beijing Information Technology Institute Beijing 100192China

The rapid development of wearable computing technologies has led to an increased involvement of wearable devices in the daily lives of *** main power sources of wearable devices are batteries;so,researchers must ensure high performance while reducing power consumption and improving the battery life of wearable *** purpose of this study is to analyze the new features of an Energy-Aware Scheduler(EAS)in the Android 7.1.2 operating system and the scarcity of EAS schedulers in wearable application ***,the paper proposed an optimization scheme of EAS scheduler for wearable applications(wearable-Application-optimized Energy-Aware Scheduler(wAEAS)).This scheme improves the accuracy of task workload prediction,the energy efficiency of central processing unit core selection,and the load *** experimental results presented in this paper have verified the effectiveness of a wAEAS scheduler.

关键词： wearable devices heterogeneous multicore system big.LITTLE architecture task scheduling

Molecular diffusion in ternary poly(vinyl alcohol)solutions

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Frontiers of Chemical Science and Engineering 2022年第6期16卷 1003-1016页

作者： Katarzyna Majerczak Ophelie Squillace Zhiwei Shi Zhanping zhang Zhenyu J.zhang School of Chemical Engineering University of BirminghamBirmingham B152TTUK The Procter and gamble Company CincinnatiOH 45040USA

The diffusion kinetics of a molecular probe-rhodamine B-in ternary aqueous solutions containing poly(vinyl alcohol),glycerol,and surfactants was investigated using fluorescence correlation spectroscopy and dynamic light *** show that the diffusion characteristics of rhodamine B in such complex systems is determined by a synergistic effect of molecular crowding and intermolecular interactions between chemical *** presence of glycerol has no noticeable impact on rhodamine B diffusion at low concentration,but significantly slows down the diffiision of rhodamine B above 3.9%(w/v)due to a dominating steric inhibition ***,introducing surfactants(cationic/nonionic/anionic)to the system results in a decreased diffusion coefficient of the molecular *** solutions containing nonionic surfactant,this can be explained by an increased crowding *** ternary poly(vinyl alcohol)solutions containing cationic or anionic surfactant,surfactant-polymer and surfactant-rhodamine B interactions alongside the crowding effect of the molecules slow down the overall diffiisivity of rhodamine *** results advance our insight of molecular migration in a broad range of industrial complex formulations that incorporate multiple compounds,and highlight the importance of selecting the appropriate additives and surfactants in formulated products.

关键词： fluorescence correlation spectroscopy poly(vinyl alcohol) anomalous diffusion crowding effects dynamic light scattering binding effects rhodamine B

Preparation and Spectral Characterization of 3-Benzyl-6-aryl-1,2,4-triazolothiadiazoles

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Chemical Research in Chinese Universities 2002年第3期18卷 280-283页

作者： zhang Li xue zhang An jiang CHEN guang CHEN Fei yu JIANg Yi ping zhang Zi yi Department of Chemistry Wenzhou TeachersCollegeWenzhou 325003P.R.China Department of Chemistry Lanzhou UniversityLanzhou 730000P.R.China

Benzyl 4 amino 5 mercapto 1,2,4 triazole reacted with aromatic acids in the presence of phosphorus oxychloride, yielding a series of new compounds, i.e. , 3 benzyl 6 aryl 1,2,4 triazolothiadiazoles, each of which has an active methylene at 3 position. The structures of all the title compounds were confirmed by elementary analysis, IR, 1H NMR and 13 C NMR spectra.

关键词： 3-Benzyl-6-aryl-1,2,4-triazolo[3,4-b]thiadiazoles Preparation Spectral characterization

Frequency-constrained Co-planning of generation and Energy Storage with High-penetration Renewable Energy

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Journal of Modern Power Systems and Clean Energy 2021年第4期9卷 760-775页

作者： Chengming zhang Lu Liu Haozhong Cheng Dundun Liu Jianping zhang gang Li Key Laboratory of Control of Power Transmission and Conversion Shanghai Jiao Tong UniversityShanghaiChina East China Branch of State grid Corporation ShanghaiChina

Large-scale renewable energy integration decreases the system inertia and restricts frequency regulation. To maintain the frequency stability, allocating adequate frequency-support sources poses a critical challenge to planners. In this context, we propose a frequency-constrained coordination planning model of thermal units, wind farms, and battery energy storage systems (BESSs) to provide satisfactory frequency supports. Firstly, a modified multi-machine system frequency response (MSFR) model that accounts for the dynamic responses from both synchronous generators and grid-connected inverters is constructed with preset power-headroom. Secondly, the rate-of-change-of-frequency (ROCOF) and frequency response power are deduced to construct frequency constraints. A data-driven piecewise linearization (DDPwL) method based on hyperplane fitting and data classification is applied to linearize the highly nonlinear frequency response power. Thirdly, frequency constraints are inserted into our planning model, while the unit commitment based on the coordinated operation of the thermal-hydro-wind-BESS hybrid system is implemented. At last, the proposed model is applied to the IEEE RTS-79 test system. The results demonstrate the effectiveness of our co-planning model to keep the frequency stability.

关键词： Battery energy storage system(BESS) data-driven piecewise linearization generation planning multi-machine system frequency response unit commitment wind farm

Extracting embedded messages using adaptive steganography based on optimal syndrome-trellis decoding paths

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Digital Communications and Networks 2022年第4期8卷 455-465页

作者： Jialin Li Xiangyang Luo Yi zhang Pei zhang Chunfang Yang Fenlin Liu State Key Laboratory of Mathematical Engineering and Advanced Computing Zhengzhou450000China

Privacy protection is the key to maintaining the Internet of Things(IoT)communication *** is an important way to achieve covert communication that protects user data *** technology is the key to checking steganography security,and its ultimate goal is to extract embedded *** methods cannot extract under known cover *** this end,this paper proposes a method of extracting embedded messages under known cover ***,the syndrome-trellis encoding process is ***,a decoding path in the syndrome trellis is obtained by using the stego sequence and a certain parity-check matrix,while the embedding process is simulated using the cover sequence and parity-check *** the decoding path obtained by the stego sequence and the correct parity-check matrix is optimal and has the least distortion,comparing the path consistency can quickly filter the coding parameters to determine the correct matrices,and embedded messages can be extracted *** proposed method does not need to embed all possible messages for the second time,improving coding parameter recognition *** experimental results show that the proposed method can identify syndrome-trellis coding parameters in stego images embedded by adaptive steganography quickly to realize embedded message extraction.

关键词： Information security Image steganography STC coding Parameter recognition