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Tertiary montane origin of the Central Asian flora,evidence inferred from cpDNA sequences of Atraphaxis(Polygonaceae)

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Journal of Integrative Plant Biology 2014年第12期56卷 1125-1135页

作者： Ming-Li Zhang Stewart C.Sanderson Yan-Xia Sun vyacheslav v.byalt Xiao-Li Hao Key Laboratory of Biogeography and Bioresource in Arid Land Xinjiang Institute of Ecology and Geography the Chinese Academy of Sciences Institute of Botany the Chinese Academy of Sciences Shrub Sciences Laboratory Intermountain Research Station Forest Service US Department of Agriculture Provo UT 84601 USA Wuhan Botanical Garden the Chinese Academy of Sciences Komarov Botanical Institute Russian Academy of Sciences St Petersburg RU‐197376 Russia School of Life Science Shihezi University

Atraphaxis has approximately 25 species and a distribution center in Central Asia. It has been previously used to hypothesize an origin from montane forest. We sampled 18 species covering three sections within the genus and sequenced five cpDNA spacers, atpB -rbcL, psbK -psbI, psbA -trnH, rbcL, and trnL -trnF. BEAST was used to reconstruct phylogenetic relationship and time divergences, and S-DIvA and Lagrange were used, based on distribution area and ecotype data, for reconstruction of ancestral areas and events. Our results appear compatible with designation of three taxonomic sections within the genus. The generic stem and crown ages were Eocene, approximately 47 Ma, and Oligocene 27 Ma,respectively. The origin of Atraphaxis is confirmed as montane,with an ancestral area consisting of the Junggar Basin and uplands of the Pamir-Tianshan-Alatau-Altai mountain chains,and ancestral ecotype of montane forest. Two remarkable paleogeographic events, shrinkage of the inland Paratethys Sea at the boundary of the late Oligocene and early Miocene, and the time intervals of cooling and drying of global climate from24（22） Ma onward likely facilitated early diversification of Atraphaxis, while rapid uplift of the Tianshan Mountains during the late Miocene may have promoted later diversification.

关键词： Allopatric diversification Atraphaxis biogeography Central Asia flora molecular clock montane origin phylogeny Polygonaceae

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Olefin Polymerization Behavior of Titanium(Iv) Complexes with Fluorinated and Non-fluorinated Aliphatic Phenoxyimine Ligands

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Chinese Journal of Polymer Science 2024年第1期42卷 52-62,I0007页

作者： vladislav A.Tuskaev Kasim F.Magomedov Svetlana Ch.Gagieva Dmitry A.Kurmaev Yulia v.Nelyubina Evgenii K.Golubev Maria D.Evseeva viktor G.vasil'ev Galina G.Nikiforova Mikhail I.Buzin vyacheslav S.Bogdanov Boris M.Bulychev Department of Chemistry M.V.Lomonosov Moscow State UniversityMoscow 119992Russian Federation A.N.Nesmeyanov Institute of Organoelement Compounds Russian Academy of SciencesMoscow119991Russian Federation Enikolopov Institute of Synthetic Polymer Materials Russian Academy of SciencesMoscow 117393Russian Federation

A series of Ti(Ⅳ) dichloride and dialkoxide com plexes with phenoxyimine ligands containing fluorinated and nonfluorinated aliphatic imine fragments have been *** molecular structures of complexes 1 and 4 were established by single-crystal X-ray diffraction *** complexes adopt a distorted octahedral coordination structure around the titanium atom and two oxygen atoms are situated in trans position while two nitrogen atoms and two outgoing ligands(Cl or iPrO) are situated in cis *** of activators(MMAO-12 and combinations Et_nAICl_(3-n)+Bu_(2)Mg) and outgoing ligand(Cl or iPrO) nature on the catalytic activity and properties of the resulting polymers was *** Ti complexes,despite the nature of the outgoing ligands(Cl or iPrO) in the presence of Al/Mg activators,was found to display a high ethylene polymerization activity in the range 1600-3830 kg_(polymer)·mol_(Ti)^(-1)·h^(-1)·atm^(-1) with a viscosity average molecular weight(M_v) value in the range 1.1×10~6-7.1×10~6 Dalton(Da).The resulting UHMWPE can be processed by a solventless method into high-strength and high-modulus oriented *** rheological characteristics of a polymer melt have been *** absence of a cross-over point did not allow to compare the values of the molecular weight distribution of polymers obtained on fluorinated and non-fluorinated pre-catalysts,however,the estimation of the entanglement density is in good agreement with the mechanical characteristics of oriented film *** activation with methylalumoxane,the activity of the com plexes decreased very significantly;however,a polymer with a molecular weight of about 12 million Da was *** the process of ethylene/octene-1 copolymerization,fluorine-containing precatalysts showed a clear advantage over non-fluorinated analogues both in activity and in comonomer content.

关键词： FI catalysts Titanium(Iv) (Co)polymerization Al/Mg co-catalyst Ultra-high molecular weight polyethylene

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Gut Microbiota and Cytokine Profile in Cirrhosis

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Journal of Clinical and Translational Hepatology 2024年第8期12卷 689-700页

作者： Irina Efremova Roman Maslennikov Anna Kudryavtseva Anastasia Avdeeva George Krasnov Mikhail Diatroptov vyacheslav Bakhitov Salekh Aliev Natalia Sedova Maria Fedorova Elena Poluektova Oxana Zolnikova Nariman Aliev Anna Levshina vladimir Ivashkin Department of Internal Medicine Gastroenterology and HepatologySechenov UniversityMoscowRussia Post-Genomic Research Laboratory Engelhardt Institute of Molecular BiologyRussian Academy of SciencesMoscowRussia v.A.Nasonova Research Institute of Rheumatology MoscowRussia Consultative and Diagnostic Center 2 of the Moscow Health Department MoscowRussia First Hospital Surgery Department Pirogov Russian National Research Medical UniversityMoscowRussia Department of Clinical Laboratory Diagnostics FGBOU DPO“Russian Medical Academy of Continuing Professional Education of the Ministry of Health of the Russian Federation”MoscowRussia The Interregional Public Organization“Scientific Community for the Promotion of the Clinical Study” MoscowRussia

Background and Aims:Gut dysbiosis and abnormal cytokine profiles are common in *** study aimed to evaluate the correlations between ***:In the blood plasma of cirrhosis patients and controls,27 cytokines were examined using a multiplex *** plasma levels of nitrites(stable metabolites of the endothelial dysfunction biomarker nitric oxide)and lipopolysaccharide(LPS)were *** fecal microbiota was assessed by 16S rRNA gene ***:Levels of IL-1b,IL-2,IL-6,IL-13,IP-10,IFN-g,TNF-a,LPS,and nitrites were higher in cirrhosis patients than in controls,while levels of IL-4,IL-7,and PDGF-BB were *** LPS level was directly correlated with the levels of IL-1b,IL1-Ra,IL-9,IL-17,PDGF-BB,IL-6,TNF-a,and *** nitrite level was significantly directly correlated with the levels of TNF-a,GM-CSF,IL-17,and IL-12,and inversely correlated with the IL-7 ***-a levels were directly correlated with ascites severity and the abundance of Negativicutes,Enterobacteriaceae,veillonellaceae,and Klebsiella,while inversely correlated with the abundance of Firmicutes,Clostridia,and ***-g levels were directly correlated with the abundance of Bacteroidaceae,Lactobacillaceae,Bacteroides,and Megasphaera,and inversely correlated with the abundance of verrucomicrobiota,Akkermansiaceae,Coriobacteriaceae,Akkermansia,Collinsella,and ***-1b levels were directly correlated with the abundance of Comamonadaceae and Enterobacteriaceae and inversely correlated with the abundance of Marinifilaceae and ***-6 levels were directly correlated with the abundance of Enterobacteriaceae,hepatic encephalopathy,and ascites severity,and inversely correlated with the abundance of Peptostreptococcaceae,Streptococcaceae,and ***:The abundance of harmful gut microbiota taxa and endotoxinemia directly correlates with the levels of proinflammatory cytokines.

关键词： Endotoxin Leaky gut Gut microbiome Systemic inflammation Gut-liver axis Endotoxemia

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Change of photosensitizer fluorescence at its diffusion in viscous liquid flow

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Journal of Innovative Optical Health Sciences 2016年第2期9卷 25-30页

作者： valeriya S.Maryakhina vyacheslav v.Gun'kov Orenburg State University 13 Pobedy st. Orenburg 460018Russia

In this paper,the mathematical model of distribution of the injected compound in biological liquid flow has been *** is considered that biological liquid contains a few phases such as water,peptides and *** injected compound(for example,photosensitizer)can interact with peptides and *** the time,viscosity of the biological liquid depends on pathology present in *** obtained distribution of the compound connects on changes of its fluorescence spectra which are registered during fluorescent diagnostics of *** is obtained that the curves do not have monotonic *** is a sharp curves decline in the first few seconds after *** of curves rises after *** is especially pronounced for wavelength 590 nm and 580 nm(near the"transparency window"of biological tissues).Time of inflection point shifts from 8.4 s to 6.9 s for longer ***,difference between curves is little for di®erent viscosity means of the biological ***,additional pathology present in organism does not impact to the results of in vivo biomedical investigations.

关键词： Fluorescence diffusion biomedical diagnostics photosensitizer viscosity

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Risk factors and urinary biomarkers of non-albuminuric and albuminuric chronic kidney disease in patients with type 2 diabetes

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World Journal of Diabetes 2019年第11期10卷 517-533页

作者： Anton I Korbut vadim v Klimontov Ilya v vinogradov vyacheslav v Romanov Laboratory of Endocrinology Research Institute of Clinical and Experimental Lymphology-Branch of the Institute of Cytology and GeneticsSiberian Branch of Russian Academy of Sciences(RICEL-Branch of IC&G SB RAS)Novosibirsk 630060Russia Clinical Laboratory “MBU-Technology”ltd.Novosibirsk 630090Russia

BACKGROUND A number of recent studies indicate a transformation in the natural course of chronic kidney disease(CKD)in type 2 diabetes(T2D)patients:an increasing prevalence of declined renal function without proceeding to the accompanying elevation of *** has been suggested that albuminuric and nonalbuminuric CKD patterns could be different in their phenotypes and pathogenic *** To identify the risk factors and biomarkers of albuminuric and non-albuminuric patterns of CKD in patients with *** Three hundred sixty patients with T2D duration≥10 years were included in this observational cross-sectional *** associations of a panel of demographic and clinical characteristics,complications,comorbidities,and metabolic and hematology parameters with albuminuric and non-albuminuric CKD patterns were *** urinary excretion of nephrin and podocin,two podocytespecific markers,and WAP-four-disulfide core domain protein 2(WFDC-2),a marker of tubulointerstitial fibrosis,was determined by ELISA in comparison with healthy *** Non-albuminuric CKD was associated with age≥65 years(P=0.0001),female sex(P=0.04),diabetes duration≥15 years(P=0.0009),and the use of diuretics(P=0.0005).Male sex(P=0.01),smoking(P=0.01),waist-to-hip ratio>1.0(P=0.01)and hemoglobin A1c(HbA1c)>8.0%(P=0.005)were risk factors for elevated albuminuria not accompanied by a decrease in estimated glomerular filtration rate(eGFR).Duration of diabetes≥15 years and the use of calcium channel blockers were risk factors for albuminuria with decreased eGFR(both P=0.01).In multivariate logistic regression analysis,age,HbA1c,female sex and diuretics were significant predictors for reduced eGFR,while waist-to-hip ratio,HbA1c and male sex were associated with elevated urinary albumin-to-creatinine ratio(UACR).Excretion of nephrin and podocin was increased in patients with albuminuria,regardless of decline in renal function(Pvely with *** urin

关键词： Diabetes mellitus Chronic kidney disease Albuminuria Glomerular filtration rate Podocytes Risk factors Biomarkers

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Decomposition of carbon dioxide hydrate in the samples of natural coal with different degrees of metamorphism

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Chinese Journal of Chemical Engineering 2020年第2期28卷 492-501页

作者： vyacheslav G. Smirnov valeriy v. Dyrdin Andrey Yu. Manakov Zinfer R. Ismagilov Kuzbass State Technical University Vesennaya str.28Kemerovo 650000Russian Federation Nikolaev Institute of Inorganic Chemistry SB RAS Ac.Lavrentiev ave.3Novosibirsk 630090Russian Federation Novosibirsk State University Pirogov Str.2Novosibirsk 630090Russian Federation Institute of Coal Chemistry and Material Science SB RAS Sovetsky ave.18Kemerovo 650000Russian Federation

Methane and carbon dioxide hydrates are one of the possible forms in which these gases exist in natural coal(for more detailed discussion see Refs [1,2]). In this work, the decomposition of carbon dioxide hydrate in five samples of natural coal differing from each other in metamorphism degree was investigated experimentally. Carbon dioxide hydrate dispersed in coals was synthesized from water adsorbed in these coals. During a linear temperature rise in an autoclave with the coal + hydrate sample the hydrate decomposition manifests itself as a step of increase in gas pressure, accompanied by a decrease/stabilization of the temperature of coal sample. The dependencies of the amount of hydrate formed on initial coal humidity and on gas pressure during hydrate formation were studied. It was demonstrated that each coal sample is characterized by its own humidity threshold below which hydrate formation in natural coal is impossible. With an increase in gas pressure, the amount of water transformed into hydrate increases. For the studied coal samples, the decomposition of carbon dioxide hydrates proceeds within a definite temperature and pressure range, and this range is close to the curve of phase equilibrium for bulk hydrate.

关键词： Gas hydrate Carbon dioxide Coal Coal rank Phase transformation Coal bed gas

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Incubation of PbSe Thin Films in a Tin(Ⅱ) Salt Aqueous Solution:Modification and Ion-Exchange Reactions

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Journal of Materials Science & Technology 2015年第8期31卷 790-797页

作者： Zinaida I.Smirnova Larisa N.Maskaeva vyacheslav F.Markov vladimir I.voronin Mikhail v.Kuznetsov Ural Federal University(named after the First President of Russia B.N.Yeltsin) ul.Mira 19Yekaterinburg620002Russia Ural Institute of State Fire Service of EMERCOM of Russia Yekaterinburgul.Mira 22620062Russia Institute of Metal Physics Ural BranchRussian Academy of Sciencesul.S.Kovalevskoy 18Yekaterinburg620041Russia Institute of Solid State Chemistry Ural BranchRussian Academy of Sciencesul.Pervomaiskaya 91Yekaterinburg620990Russia

Topochemical ion-exchange reactions between solid micro- and nanostructured metal chalcogenides and aqueous salt solutions are generally used for formation of composite structures based on initial metal chalcogenides and products of their ion-exchange transformation. However, ion exchange has promises as a route to obtaining both composites and solid solutions based on the initial and the end chalcogenide phases. With the help of the ion-exchange technique, single-phase films of Phi xSnxSe substitutional solid solutions with a tin content up to -2 at.%, which are promising for mid- and long-wavelength infrared radiation （IR） optoelectronics, have been obtained at the interface between PbSe poly- crystalline thin films and SnCl2 aqueous solutions containing sodium citrate. It has been shown that the pH value and temperature of the reaction system play an important role in the ion-exchange process. Incubation of lead selenide （PbSe） films in a tin（II） salt aqueous solution also leads to their modification with oxygen-containing tin compounds to a depth of-3 nm. Differences in the film structure, such as changes in the coherent scattering region sizes and orientation of crystallites along the [220] direction, which arise during the contact with citrate-containing SnCl2 solutions, have also been revealed. For the first time, an idea of the existence of a relatively wide reaction zone of an intragranular topochemical ion-exchange reaction in an aqueous solution, within which substitutional solid solutions can form in micro- and nanostructured systems, has been set forth.

关键词： Ion-exchange synthesis Thin films Lead selenide Tin selenide Substitutional solid solutions Topochemical reaction

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Sediments from cryoconite holes and dirt cones on the surface of Svalbard glaciers:main chemical and physicochemical properties

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Acta Geochimica 2023年第2期42卷 346-359页

作者： Timur Nizamutdinov Bulat Mavlyudov vyacheslav Polyakov Evgeny Abakumov Department of Applied Ecology Faculty of BiologySt.Petersburg State University16th Liniya V.O.29St.PetersburgRussia 199178 Russian Academy of Sciences Institute of GeographyMoscowRussia 119017

The paper discussed the influence of the forms of sediment accumulation on the surface of glaciers on their chemical and physicochemical *** materials sampled from the surface of five glaciers of the Svalbard Archipelago was *** studied such forms of sediment accumulation as dirt cones-the ice core covered with sediments and cryoconite holes-hollows on the glacier surface containing cryoconite *** such as total organic carbon content,microbiological activity,pH,the content of mobile forms of potassium and phosphorus,and concentrations of heavy and trace metals were ***,mesomorphological studies were carried out and the polydisperse composition of the sediments was *** to the results of this work,it was found that the content of organic carbon in the material selected from dirt cones and cryoconite holes can be up to 2.5%,but the content of clay particles in it is mainly at the 10–15%*** concentrations are up to 250 mg/kg,and phosphorus is up to 800 mg/*** content of metals is typical or lower than in the previously published *** main influence on the chemical composition of materials has a geographical factor of the sampling site,rather than the form of material accumulation.

关键词： Arctic Soil-like bodies Glacier sediments Accumulation

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Comprehensive semen examination in patients with pancreatic-sufficient and pancreatic-insufficient cystic fibrosis

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Asian Journal of Andrology 2023年第5期25卷 591-597页

作者： Anna O Sedova Maria I Shtaut Elizaveta E Bragina Tatyana M Sorokina Galina v Shmarina Marina v Andreeva Lyubov E Kurilo Stanislav A Krasovskiy Aleksander v Polyakov vyacheslav B Chernykh Research Centre for Medical Genetics Russia Moscow 115522

We examined a cohort of 93 cystic fibrosis(CF)male patients who were pancreatic-sufficient(PS-CF;n=40)or pancreatic-insufficient(PI-CF;n=53).Complex semen examination was performed,including standard semen analysis,quantitative karyological analysis(QKA)of immature germ cells(IGCs),transmission electronic microscopy(TEM),biochemical analysis,and sperm DNA fragmentation by terminal deoxynucleotidyl transferase-mediated dUTP nickend labeling(TUNEL)*** was diagnosed in 83(89.2%)*** other 10(10.8%)patients were found to be nonazoospermic and showed various spermatological diagnoses(asthenozoospermia,n=2;asthenoteratozoospermia,n=3;oligoasthenozoospermia,n=1;oligoasthenoteratozoospermia,n=3;and normozoospermia,n=1)with no specific morphological *** was detected in 89.2%azoospermic and 30.0%nonazoospermic *** seminal pH(vealed in 2.4%azoospermic and 40.0%nonazoospermic semen *** signs of partial meiotic arrest at prophase I were found in 4 of 6 nonazoospermic patients examined by QKA of *** content of fructose and citrate was low in oligospermic and normal in nonoligospermic semen *** increased percentage(>30%)of spermatozoa with noncondensed(“immature”)chromatin was revealed in 2 of 6 nonazoospermic semen samples analyzed by TEM.

关键词： congenital bilateral agenesia/aplasia of vas deferens cystic fibrosis cystic fibrosis transmembrane conductance regulator gene semen spermatozoa

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Submonolayer Eu superstructures—A class of 2D magnets

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Nano Research 2023年第1期16卷 1500-1506页

作者： Dmitry v.Averyanov Ivan S.Sokolov Alexander N.Taldenkov Oleg E.Parfenov Andrey M.Tokmachev vyacheslav G.Storchak National Research Center“Kurchatov Institute” Kurchatov Sq.1Moscow 123182Russia

Two-dimensional(2D)magnetic materials promise unconventional properties and quantum phases as well as advances in ultracompact *** of 2D magnets often reaches a single monolayer but in general can go beyond this limit,as demonstrated by 2D magnetism of submonolayer Eu superstructures coupled with *** question is whether the submonolayer magnetism constitutes a general ***,we demonstrate that regular Eu lattices form a class of 2D magnets displaying various structures,stoichiometries,and chemical *** synthesized and studied a set of Eu superstructures on Ge(001).Their magnetic properties are consistent with the emergence of a magnetic order such as ferro-or *** particular,control over the magnetic transition temperature by weak magnetic fields indicates the 2D nature of the *** together,Eu/Ge and Eu/Si superstructures seed a nucleus of the research area addressing the emergence of magnetism in submonolayer chemical species.

关键词： two-dimensional(2D)magnetism submonolayer superstructure surface reconstruction germanium

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