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Superhydrophilic nickel hydroxide ultrathin nanosheets enable high-performance asymmetric supercapacitors

Rare Metals 2024年第1期43卷 138-147页

作者： Yi-Ran Wang Fei Zhang Jian-Min Gu Xiao-Yu Zhao Ran Zhao Xing Wang tian-hui wu Jing Wang Ji-Dong Wang De-Song Wang State Key Laboratory of Metastable Materials Science and Technology(MMST) Hebei Key Laboratory of Applied ChemistryYanshan UniversityQinhuangdao 066004China Department of Food and Pharmaceutical Engineering Suihua UniversitySuihua 152000China School of Chemical Science and Engineering Tongji UniversityShanghai 200092China School of Sciences Hebei University of Science and TechnologyShijiazhuang 050018China

Superhydrophilic surfaces have been applied for supercapacitor;however,during energy storage reaction,how the wettability affects the process of electrochemical reaction specifically is still ***,we demonstrate superhydrophilic surface for promotion of electrochemical reactions by liquid affinity and further explain the mechanism,where the transition of the wettability state caused by the change in surface free energy is the main reason for the obvious increase in specific *** citric acid assistance strategy,an intrinsically hydrophobic Ni(OH)_(2)thick nanosheets(HNHTNs,16 nm)can be transitioned into superhydrophilic Ni(OH)_(2)ultrathin nanosheets(SNHUNs,6.8 nm),where the water contact angle was 0°and the surface free energy increased from 8.6to 65.8 mN·m^(-1),implying *** with HNHTNs,the specific capacitance of SNHUNs is doubled:from 1230 F·g^(-1)(HNHTNs)to 2350 F·g^(-1)(2A·g^(-1))and,even at 20 A·g^(-1),from 833 F·g^(-1)(HNHTNs)to 1670 F·g^(-1).The asymmetric capacitors assembled by SNHUNs and activated carbon show 52.44 Wh·kg^(-1)at 160W·kg^(-1)and excellent stability with~90%retention after5000 cycles(~80%retention after 9500 cycles).The promotion of electrochemical performances is ascribed to the change of surface wettability caused by surface free energy,which greatly increase affinity of electrode to the surrounding liquid environment to reduce the interface resistance and optimize the electron transport path.

关键词： Asymmetric supercapacitor Superhydrophilic interface Transition metal hydroxides Ultrathin nanosheets High specific capacitance

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长江上游保护区干流江安-重庆段禁渔初期鱼类时空分布特点

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水生生物学报 2024年第4期48卷 558-567页

作者：田盼盼李祥艳邓华堂王导群刘绍平陈大庆段辛斌王珂田辉伍中国水产科学研究院长江水产研究所/国家农业科学重庆观测实验站武汉430223 西南大学生命科学学院重庆400715

为掌握“长江十年禁渔”初期长江上游保护区干流江安-重庆江段鱼类资源时空分布特征,研究在开展鱼类资源调查的同时,利用SIMRADEK80分裂波束科研回声探测仪于2020年12月和2021年5月在江安-重庆江段开展水声探测。水声学探测结果表明,江... 详细信息

为掌握“长江十年禁渔”初期长江上游保护区干流江安-重庆江段鱼类资源时空分布特征,研究在开展鱼类资源调查的同时,利用SIMRADEK80分裂波束科研回声探测仪于2020年12月和2021年5月在江安-重庆江段开展水声探测。水声学探测结果表明,江安-重庆江段2020年12月和2021年5月鱼类平均密度分别为25.31和41.23 ind./1000 m^(3),鱼类目标强度均值分别为–55.81和–52.79 dB,无显著差异,估算鱼类平均体长分别为17.97和24.36 cm。在水平方向上,两次调查鱼类都主要分布在重庆-江津江段,两次水声学探测的鱼类密度在垂直方向上呈现出一定差异,2020年12月表现为下层>中层>上层,2021年5月表现为上层>中层>下层。此次鱼类资源调查共发现了鱼类12科62种,其中瓦氏黄颡鱼、光泽黄颡鱼、蒙古鲌和贝氏䱗等小型鱼类的数量占比达到50.21%,与水声学结果一致。研究初步探究了保护区内鱼类在不同时段的空间分布规律,评估了禁捕初期长江上游鱼类分布特征,为长江“十年禁渔”生态效果评估提供基础数据参考。

关键词：鱼类资源水声学时空分布禁渔长江上游保护区

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金沙江下游向家坝库区鱼类群落结构空间格局

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水生态学杂志 2024年第4期45卷 82-91页

作者：熊飞郭祺张伟刘红艳翟东东段辛斌田辉伍陈大庆江汉大学生命科学学院湖北省汉江流域特色生物资源保护开发与利用工程技术研究中心湖北武汉430056 江汉大学持久性有毒污染物环境与健康危害湖北省重点实验室湖北武汉430056 中国水产科学研究院长江水产研究所湖北武汉430223

探究鱼类群落结构空间分布特征及其对梯级水电开发的响应,为水电开发生态环境影响评价及鱼类保护提供依据,为长江“十年禁渔”效果评估提供本底资料。2016-2018年采用复合刺网和地笼对向家坝库区库首邵女坪、库中绥江和库尾桧溪的鱼类... 详细信息

探究鱼类群落结构空间分布特征及其对梯级水电开发的响应,为水电开发生态环境影响评价及鱼类保护提供依据,为长江“十年禁渔”效果评估提供本底资料。2016-2018年采用复合刺网和地笼对向家坝库区库首邵女坪、库中绥江和库尾桧溪的鱼类群落进行了7次调查,探究了建坝后的鱼类种类组成、个体大小、生态类群及其空间分布特征。调查共采集到鱼类59种,隶属于6目16科49属,其中长江上游特有鱼类5种,外来鱼类12种。在邵女坪、绥江和桧溪江段分别采集到鱼类39、40和39种,Jaccard相似性指数分析表明,3个江段鱼类群落物种组成为中等相似。相对重要性指数(IRI)分析显示,邵女坪江段鱼类群落的优势种为中华倒刺鲃(Spinibarbus sinensis)和䱗(Hemiculter leucisclus),绥江江段优势种为䱗、鲢(Hypophthalmichthys molitrix)、瓦氏黄颡鱼(Pseudobagrus vachelli)和鳙(Aristichthys nobilis),桧溪江段优势种为瓦氏黄颡鱼、镜鲤(Cyprinus carpio ***)、鲤(Cyprinus carpio)、䱗、草鱼(Ctenopharyngodon idellus)和鲫(Carassius auratus)。NMDS分析显示,库首邵女坪和库尾桧溪江段鱼类群落差异相对较大,Bray-Curtis相异指数为0.59;库中绥江与库首邵女坪鱼类群落更为相似,Bray-Curtis相异指数为0.41;库中绥江和库尾桧溪的Bray-Curtis相异指数为0.46。广适性鱼类是向家坝库区各江段的优势类群,分别占鱼类种类、数量和重量的57.7%±5.9%、65.2%±20.7%和47.7%±16.1%;从库首至库尾江段其数量比分别为43.3%、67.8%和84.5%,呈现逐渐增加趋势。向家坝库区渔获群体体长为29~655 mm,平均体长为(128±65)mm,体重为0.1~5408 g,平均体重为(70±218)g,主要种类(鲤和镜鲤除外)在不同江段间个体大小差异显著(P<0.05)。与蓄水前(2011年)相比,金沙江下游鱼类群落发生了显著变化,流水性的特有鱼类减少,外来鱼类增多。

关键词：优势种特有鱼类外来鱼类向家坝库区金沙江下游

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Small intestinal submucosa improves islet survival and function during in vitro culture

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World Journal of Gastroenterology 2005年第46期11卷 7378-7383页

作者： Xiao-hui tian wu-Jun Xue Xiao-Ming Ding Xin-Lu Pang Yan Teng Pu-Xun tian Xin-Shun Feng Center of Renal Transplantation The First Hospital of Xi'an Jiaotong UniversityXi'an 710061 Shaanxi Province China

AIM： To evaluate the recovery and function of isolated rat pancreatic islets during in vitro culture with small intestinal submucosa （SIS）. METHODS： Pancreatic islets were isolated from Wistar rats by standard surgical procurement followed by intraductal collagenase distension, mechanical dissociation and Euroficoll purification. Purified islets were cultured in plates coated with multilayer SIS （SIS-treated group） or without multilayer SIS （standard cultured group） for 7 and 14 d in standard islet culture media of RPMI 1640. After isolation and culture, islets from both experimental groups were stained with dithizone and counted. Recovery of islets was determined by the ratio of counts after the culture to the yield of islets immediately following islet isolation. Viability of islets after the culture was assessed by the glucose challenge best with low （2.7 mmol/L） and high glucose （16.7 mmol/L） solution supplemented with 50 mmol/L 3-isobutyl-1- methylxanthine （IBMX） solution. Apoptosis of islet cells after the culture was measured by relative quantification of histone-complexed DNA fragments using ELISA. RESULTS： After 7 or 14 d of in vitro tissue culture, the recovery of islets in SIS-treated group was significantly higher than that cultured in plates without SIS coating. The recovery of islets in SIS-treated group was about twice more than that of in the control group. In SIS treated group, there was no significant difference in the recovery of islets between short- and long-term periods of culture （95.8±1.0% vs 90.8±1.5%, P〉0.05）. When incubated with high glucose （16.7 mmol/L） solution, insulin secretion in SIS-treated group showed a higher increase than that in control group after 14 d of culture （20.7±1.1 mU/L vs 11.8±1.1 mU/L, P〈0.05）. When islets were placed in high glucose solution containing IBMX, stimulated insulin secretion was higher in SlS-treated group than in control group. Calculated stimulation index of SlS-treated group was about 23 times of

关键词： Islet culture Islet survival Islet function Small intestinal submucosa

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应用鱼类生物完整性指数评价黑水河河流健康状况

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水生态学杂志 2024年第2期45卷 73-83页

作者：李文滕航田辉伍邓华堂成必新杨少荣刘绍平陈大庆段辛斌中国水产科学研究院长江水产研究所农业农村部长江中上游渔业资源环境科学观测实验站湖北武汉430223 华中农业大学水产学院湖北武汉430070 西南大学生命科学学院重庆400715 上海勘测设计研究院有限公司上海200434 中国三峡建工(集团)有限公司四川成都610041

黑水河为金沙江下游一级支流,是白鹤滩库区干流鱼类的重要替代生境和优先保护支流,评价黑水河河流健康状况,可为黑水河鱼类栖息地生态修复提供数据支撑。2018年11月至2019年9月在黑水河23个采样点开展了4次鱼类资源调查,共采集到鱼类45(... 详细信息

黑水河为金沙江下游一级支流,是白鹤滩库区干流鱼类的重要替代生境和优先保护支流,评价黑水河河流健康状况,可为黑水河鱼类栖息地生态修复提供数据支撑。2018年11月至2019年9月在黑水河23个采样点开展了4次鱼类资源调查,共采集到鱼类45(亚)种,隶属于4目10科33属。以黑水河河口、水文站上游和825回水点作为参照点,经过分布范围、判别能力及Pearson相关性分析等指标构建黑水河鱼类生物完整性指数(F-IBI)评价体系。使用1、3、5赋值法和比值法计算各采样点的IBI分值以评价各采样点健康状况,结果显示,1、3、5赋值法和比值法的结果虽不完全相同,但趋势是一致的。黑水河大部分采样点的健康状况处于“较差”和“一般”水平。相关性分析结果显示,F-IBI分值与海拔呈显著负相关(P<0.01)。丰度生物量比较曲线显示,黑水河鱼类群落结构整体上受到中度干扰。

关键词：鱼类生物完整性指数河流健康黑水河

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An Experimental Study on the Effect of a Nanofluid on Oil-Water Relative Permeability

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Fluid Dynamics & Materials Processing 2024年第6期20卷 1265-1277页

作者： hui tian Dandan Zhao Yannan wu Xingyu Yi Jun Ma Xiang Zhou Baikouquan Oil Production Plant PetroChina Xinjiang Oilfield CompanyKaramay834000China Research Institute of Petroleum Exploration Development PetroChina Liaohe OilfieldPanjin124010China Petroleum Engineering School Southwest Petroleum UniversityChengdu610500China Oil and Gas Development Haosheng Xincheng Energy TechnologyLtd.of SicuanChengdu610213China

The low porosity and low permeability of tight oil reservoirs call for improvements in the current technologies for oil *** chemical solutions with large molecular size cannot effectively flow through the nanopores of the *** this study,the feasibility of Nanofluids has been investigated using a high pressure high temperature core-holder and nuclear magnetic resonance(NMR).The results of the experiments indicate that the specified Nanofluids can enhance the tight oil recovery *** water and oil relative permeability curve shifts to the high water saturation side after Nanofluid flooding,thereby demonstrating an increase in the water wettability of the *** the Nanofluid flooding process the oil recovery was enhanced by 15.1%,compared to waterflooding *** T2 spectra using the NMR show that after Nanofluid flooding,a 7.18%increment in oil recovery factor was gained in the small pores,a 4.9%increase in the middle pores,and a 0.29%increase in the large *** results confirm that the Nanofluids can improve the flow state in micro-sized pores inside the core and increase the ultimate oil recovery factor.

关键词： Tight oil reservoir nanofluid relative permeability nuclear magnetic resonance T2 spectrum

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Multifunctional carbon materials from rugose rose for energy storage and water purification

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FRONTIERS OF CHEMICAL SCIENCE AND ENGINEERING 2024年第9期18卷 97-0页

作者： Li, Peng-hui Zhou, hui wu, Wen-Juan Nanjing Forestry Univ Jiangsu Coinnovat Ctr Efficient Proc & Utilizat Fo Nanjing 210037 Peoples R China Nanjing Forestry Univ Coll Light Ind & Food Engn Nanjing 210037 Peoples R China East China Univ Sci & Technol Coll Chem Engn Shanghai 200237 Peoples R China State Key Lab Chem Engn Shanghai 200237 Peoples R China

With the advancement of social process, the resource problem is becoming more prominent, biomass materials come into being, and it is becoming more and more important to explore and prepare efficient and multifunctional biomass materials to alleviate the problems of energy storage and water pollution. In this paper, nitrogen-doped hierarchical porous carbon materials (NRRC) were produced by one-step carbonization of withered rose as raw material and melamine as nitrogen source with KOH-activated porosification. The resulting nitrogen-doped porous carbon material had the most abundant pores and the best microspherical graded pore structure, with a specific surface area of up to 1393 m2g-1, a pore volume of 0.68 cm3g-1, and a nitrogen-doped content of 5.52%. Electrochemical tests showed that the maximum specific capacitance of NRRC in the three-electrode system was 346.4 Fg-1 (0.5 Ag-1), which was combined with favorable capacitance retention performance and cycling stability. The NRRC//NRRC symmetric supercapacitors were further assembled, and the maximum energy density of a single device was 23.88 Whkg-1, which still maintains excellent capacitance retention and cyclic charging/discharging stability. For example, the capacitance retention rate was always close to 96.27% with almost negligible capacitance loss after 10000 consecutive charge/discharge cycles (current density: 10 Ag-1). Regardless of the three-electrode or two-electrode system, the super capacitive performance of NRRC porous carbon materials was comparable to the electrochemical performance of many reported biomass porous carbon materials, which showed better energy storage advantages and practical application potential. In addition, NRRC porous carbon materials had excellent water purification ability. The dye adsorption test confirmed that NRRC had a high adsorption capacity (491.47 mgg-1) for methylene blue. This und

关键词： rose carbon adsorption electrode material electrochemical performance POROUS CARBON SUPERIOR PERFORMANCE ACTIVATED CARBON SURFACE-AREA SUPERCAPACITOR BIOMASS ADSORPTION ELECTRODE NITROGEN

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Tuning the membrane rejection behavior by surface wettability engineering for an effective water-in-oil emulsion separation

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Chinese Chemical Letters 2024年第6期35卷 480-485页

作者： Yan Zou Yin-Shuang Hu Deng-hui tian Hong wu Xiaoshu Lv Guangming Jiang Yu-Xi Huang Engineering Research Center for Waste Oil Recovery Technology and Equipment Ministry of EducationChongqing Technology and Business UniversityChongqing 400067China School of Environmental Science and Engineering Sun Yat-sen UniversityGuangzhou 510275China Guangdong Provincial Key Laboratory of Environmental Pollution Control and Remediation Technology(Sun Yat-sen University) Guangzhou 510275China

Membrane-based separation is a promising technology to eliminate water impurities from the oil ***,it remains a great challenge to separate water from highly emulsified viscous oil owing to the high stability of the water droplets in *** we report a surface wettability engineering on an alumina ceramic membrane to achieve an efficient separation of a water-in-oil(W/O)*** with different carbon chain lengths and fluorinated status were introduced to endow the alumina membrane with different surface *** all the modified membranes exhibited excellent separation of the W/O without Span 80(surfactant),the one with amphiphobic wettability and lowest surface energy failed to separate the Span 80 stabilized W/*** presence of Span 80 reduced the interfacial tension of water droplets,making them easier to deform and penetrate the modified membrane with the lowest surface *** reveals that engineering proper surface wettability is the key to separating the oil and water ***,the modified membranes maintained decent separation performance and stability under long-term run separation of the emulsified W/O.

关键词： Water-in-oil emulsion Ceramic membrane Membrane separation Surface wettability

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Preparation of Self-limiting Heating Cables with Excellent Processability, Mechanical Properties and PTC Effect via Thermal and Electrical Treatments

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Chinese Journal of Polymer Science 2024年第4期42卷 511-520页

作者： tian-Hao Yang Tong wu Qiang Fu State Key Laboratory of Polymer Materials Engineering College of Polymer Science and EngineeringSichuan UniversityChengdu610065China State Key Laboratory of Polymer Materials Engineering Polymer Research Institute of Sichuan UniversityChengdu610065China

Polymer/conductive filler composites have been widely used for the preparation of self-limiting heating cables with the positive temperature coefficient (PTC) effect. The control of conductive filler distribution and network in polymer matrix is the most critical for performance of PTC materials. In order to compensate for the destruction of the filler network structure caused by strong shearing during processing, an excessive conductive filler content is usually added into the polymer matrix, which in turn sacrifices its processability and mechanical properties. In this work, a facile post-treatment of the as-extruded cable, including thermal and electrical treatment to produce high-density polyethylene (HDPE)/carbon black (CB) cable with excellent PTC effect, is developed. It is found for the as-extruded sample, the strong shearing makes the CB particles disperse uniformly in HDPE matrix, and 25 wt% CB is needed for the formation of conductive paths. For the thermal-treated sample, a gradually aggregated CB filler structure is observed, which leads to the improvement of PTC effect and the notable reduction of CB content to 20 wt%. It is very interesting to see that for the sample with combined thermal and electrical treatment, CB particles are agglomerated and oriented along the electric field direction to create substantial conductive paths, which leads to a further decrease of CB content down to 15 wt%. In this way, self-limiting heating cables with excellent processability, mechanical properties and PTC effect have simultaneously been achieved.

关键词： Self-limiting heating cables Positive temperature coefficient Thermal treatment Electrical treatment

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Principal components of nuclear mass models

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Science China(Physics,Mechanics & Astronomy) 2024年第7期67卷 65-71页

作者： Xin-hui wu Pengwei Zhao Department of Physics Fuzhou UniversityFuzhou 350108China State Key Laboratory of Nuclear Physics and Technology School of PhysicsPeking UniversityBeijing 100871China

Principal component analysis(PCA)is employed to extract the principal components(PCs)present in nuclear mass models for the first *** effects from different nuclear mass models are reintegrated and reorganized in the extracted *** PCs are recombined to build new mass models,which achieve better accuracy than the original theoretical mass *** comparison indicates that using the PCA approach,the effects contained in different mass models can be collaborated to improve nuclear mass predictions.

关键词： nuclear mass principal component analysis nuclear models statistical methods

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